Zero-Temperature Casimir Fluctuations and the Limits of Force Microscope Sensitivity
John A. Sidles
备注：
Revised as submitted to PRL: (a) the predicted fluctuations are 8% larger, due to the correction of a minor algebraic error, (b) additional physical motivation is provided at each step of the calculation, (c) the figure is nicer. RevTeX, four pages, one embedded figure, uses epsf.sty
It is predicted that in force microscopy the quantum fluctuations responsible for the Casimir force can be directly observed as temperature-independent force fluctuations having spectral density $9π/(40\ln(4/e)) \hbar δk$, where $\hbar$ is Planck's constant and $δk$ is the observed change in spring constant as the microscope tip approaches a sample. For typical operating parameters the predicted force noise is of order $10^{-18}$ Newton in one Hertz of bandwidth. The Second Law is respected via the fluctuation-dissipation theorem. For small tip-sample separations the cantilever damping is predicted to increase as temperature is reduced, a behavior that is reminiscent of the Kondo effect.
Experimental methods and procedures required for precision measurements of the Casimir force are presented. In particular, the best practices for obtaining stable cantilevers, calibration of the cantilever, correction of thermal and mechanical drift, measuring the contact separation, sphere radius and the roughness are discussed.
We calculate the additional force due to two-axion exchange acting in a sphere-disc geometry, used in experiments on measuring the gradient of the Casimir force. With this result, stronger constraints on the pseudoscalar coupling constants of an axion and axion-like particles to a proton and a neutron are obtained over the wide range of axion masses from 0.03mV to 1eV. Among the three experiments with Au-Au, Au-Ni and Ni-Ni boundary surfaces performed by means of dynamic atomic force microscope, major improving is achieved for the experiment with Au-Au test bodies. Here, the constraints obtain…
We consider detailed roughness and conductivity corrections to the Casimir force in the recent Casimir force measurement employing an Atomic Force Microscope. The roughness of the test bodies-a metal plate and a sphere- was investigated with the Atomic Force Microscope and the Scanning Electron Microscope respectively. It consists of separate crystals of different heights and a stochastic background. The amplitude of roughness relative to the zero roughness level was determined and the corrections to the Casimir force were calculated up to the fourth order in a small parameter (which is this a…
We present measurement results for the gradient of the Casimir force between an Au-coated sphere and an Au-coated plate obtained by means of an atomic force microscope operated in a frequency shift technique. This experiment was performed at a pressure of 3x10^{-8} Torr with hollow glass sphere of 41.3 mcm radius. Special attention is paid to electrostatic calibrations including the problem of electrostatic patches. All calibration parameters are shown to be separation-independent after the corrections for mechanical drift are included. The gradient of the Casimir force was measured in two way…
We present a Casimir force setup based on an all-optical ferrule-top sensor. We demonstrate that the instrument can be used to measure the gradient of the Casimir force between a gold coated sphere and a gold coated plate with results that are comparable to those achieved by similar atomic force microscope experiments. Thanks to the monolithic design of the force sensor (which does not require any optical triangulation readout) and to the absence of electronics on the sensing head, the instrument represents a significant step ahead for future studies of the Casimir effect under engineered cond…
We report an improved precision measurement of the Casimir force. The force is measured between a large Al coated sphere and flat plate using an Atomic Force Microscope. The primary experimental improvements include the use of smoother metal coatings, reduced noise, lower systematic errors and independent measurement of surface separations. Also the complete dielectric spectrum of the metal is used in the theory. The average statistical precision remains at the same 1% of the forces measured at the closest separation.
We compare theoretical expectations for the Casimir force with the results of precise measurements. The force is calculated at finite temperature for multilayered covering of the bodies using the Lifshitz theory. We argue that the dielectric function of the metallization has to be directly measured to reach the necessary precision in the force calculation. Without knowledge of this function one can establish a well defined upper limit on the force using parameters of perfect single-crystal materials. The force measured in the torsion pendulum experiment does not contradict to the upper limit. …
Quantum electrodynamic fluctuations cause an attractive force between metallic surfaces. At separations where the finite speed of light affects the interaction, it is called the Casimir force. Thermal motion determines the fundamental sensitivity limits of its measurement at room temperature, but several other systematic errors contribute uncertainty as well and become more significant in air relative to vacuum. Here we discuss the viability of several measurement techniques in air (force modulation, frequency modulation, and quasi-static deflection), characterize their sensitivity and accurac…
We discuss a proposal to measure the Casimir force in the parallel plate configuration in the $1-10μ$m range via a high-sensitivity torsional balance. This will allow to measure the thermal contribution to the Casimir force therefore discriminating between the various approaches discussed so far. The accurate control of the Casimir force in this range of distances is also required to improve the limits to the existence of non-Newtonian forces in the micrometer range predicted by unification models of fundamental interactions.
The Casimir effect in graphene systems is reviewed with emphasis made on the large thermal correction to the Casimir force predicted at short separations between the test bodies. The computational results for the Casimir pressure and for the thermal correction are presented for both pristine graphene and real graphene sheets, which possess nonzero energy gap and chemical potential, obtained by means of exact polarization tensor. Two experiments on measuring the gradient of the Casimir force between an Au-coated sphere and graphene- coated substrates performed by using a modified atomic force m…
The measurement of the Casimir force between a large gold coated sphere and single crystal silicon plate is performed with an atomic force microscope. A rigorous statistical comparison of data with theory is done, without use of the concept of root-mean-square deviation, and excellent agreement is obtained. The Casimir force between metal and semiconductor is demonstrated to be significantly different than between two similar or dissimilar metals.
The experimentally demonstration of Casimir force transition from attraction to repulsion is still challenging. Herein, the Casimir forces for a sphere above a plate immersed in different liquids were precisely measured using Atomic force microscope, and the long-range repulsive Casimir force in the gold-cyclohexane-PTFE system is observed for the first time. The experimental data are consistent with the calculation by Lifshitz theory, which offers the direct evidence for the system of ε1<ε3<ε2. It further verifies the reasonability of van Zwol et al. dielectric model to describe the interveni…
We report an improved precision measurement of the Casimir force using metallic gold surfaces. The force is measured between a large gold coated sphere and flat plate using an Atomic Force Microscope. The use of gold surfaces removes some theoretical uncertainties in the interpretation of the measurement. The forces are also measured at smaller surface separations. The complete dielectric spectrum of the metal is used in the comparison of theory to the experiment. The average statistical precision remains at the same 1% of the forces measured at the closest separation. These results should lea…
A measurement of the Casimir force between a gold coated sphere and two Si plates of different carrier densities is performed using a high vacuum based atomic force microscope. The results are compared with the Lifshitz theory and good agreement is found. Our experiment demonstrates that by changing the carrier density of the semiconductor plate by several orders of magnitude it is possible to modify the Casimir interaction. This result may find applications in nanotechnology.
An upper limit on the Casimir force is found using the dielectric functions of perfect crystalline materials which depend only on well defined material constants. The force measured with the atomic force microscope is larger than this limit at small separations between bodies and the discrepancy is significant. The simplest modification of the experiment is proposed allowing to make its results more reliable and answer the question if the discrepancy has any relation with the existence of a new force.
The lateral Casimir force between a sinusoidally corrugated gold coated plate and large sphere was measured for surface separations between 0.2 $μ$m to 0.3 $μ$m using an atomic force microscope. The measured force shows the required periodicity corresponding to the corrugations. It also exhibits the necessary inverse fourth power distance dependence. The obtained results are shown to be in good agreement with a complete theory taking into account the imperfectness of the boundary metal. This demonstration opens new opportunities for the use of the Casimir effect for lateral translation in micr…
The normal Casimir force between a sinusoidally corrugated gold coated plate and a sphere was measured at various angles between the corrugations using an atomic force microscope. A strong dependence on the orientation angle of the corrugation is found. The measured forces were found to deviate from the proximity force approximation and are in agreement with the theory based on the gradient expansion including correlation effects of geometry and material properties. We analyze the role of temperature. The obtained results open new opportunities for control of the Casimir effect in micromechani…
A significant decrease in the magnitude of the Casimir force (from 21% to 35%) was observed after an indium tin oxide (ITO) sample interacting with an Au sphere was subjected to the UV treatment. Measurements were performed by using an atomic force microscope (AFM) in high vacuum. The experimental results are compared with theory, and a hypothetical explanation for the observed phenomenon is proposed.
We report on measurements of the Casimir force in a sphere-plane geometry using a cryogenic force microscope to move the force probe in situ over different materials. We show how the electrostatic environment of the interacting surfaces plays an important role in weak force measurements and can overcome the Casimir force at large distance. After minimizing these parasitic forces, we measure the Casimir force between a gold-coated sphere and either a gold-coated or a heavily doped silicon surface in the 100-400 nm distance range. We compare the experimental data with theoretical predictions and…
We have used an atomic force microscope to make precision measurements of the Casimir force between a metallized sphere of diameter 196 microns and flat plate. The force was measured for plate-sphere separations from 0.1 to 0.9 microns. The experimental results are consistent with present theoretical calculations including the finite conductivity, roughness, and temperature corrections. The root mean square average deviation of 1.6 pN between theory and experiment corresponds to a 1% deviation at the smallest separation.
We report development of a high-sensitivity torsion balance to measure the thermal Casimir force. Special emphasis is placed on experimental investigations of a possible surface electric force originating from surface patch potentials that have been recently noticed by several experimental groups. By gaining a proper understanding of the actual contribution of the surface electric force in real materials, we aim to undertake precision force measurements to resolve the Casimir force at finite temperature in real metals, as well as in other semiconducting materials, such as graphene.
We demonstrate the Casimir interaction between two ferromagnetic boundary surfaces using the dynamic atomic force microscope. The experimental data are found to be in excellent agreement with the predictions of the Lifshitz theory for magnetic boundary surfaces combined with the plasma model approach. It is shown that for magnetic materials the role of hypothetical patch potentials is opposite to that required for reconciliation of the data with the Drude model.
The gradient of the Casimir force between a Si-SiO${}_2$-graphene substrate and an Au-coated sphere is measured by means of a dynamic atomic force microscope operated in the frequency shift technique. It is shown that the presence of graphene leads to up to 9% increase in the force gradient at the shortest separation considered. This is in qualitative agreement with the predictions of an additive theory using the Dirac model of graphene.
We have measured the normalized gradient of the Casimir force between Au-coated surfaces of the sphere and the plate and equivalent Casimir pressure between two parallel Au plates at T=77K. These measurements have been performed by means of dynamic force microscope adapted for operating at low temperatures in the frequency shift technique. It was shown that the measurement results at T=77K are in a very good agreement with those at T=300K and with computations at T=77K using both theoretical approaches to the thermal Casimir force proposed in the literature. No thermal effect in the Casimir pr…
We propose a theory of the thermal Casimir interaction for multilayered test bodies coated with a graphene sheet. The reflection coefficients on such structures are expressed in terms of the components of the polarization tensor and the dielectric permittivities of material layers. The developed theory is applied to calculate the gradient of the Casimir force between an Au-coated sphere and a graphene sheet deposited on a SiO${}_2$ film covering a Si plate, which is the configuration of a recent experiment performed by means of a dynamic atomic force microscope. The theoretical results are fou…
The experimental investigation of the Casimir force between a large metallized sphere and semiconductor plate is performed using an atomic force microscope. Improved calibration and measurement procedures permitted reduction in the role of different uncertainties. Rigorous statistical procedures are applied for the analysis of random, systematic and total experimental errors at 95% confidence. The theoretical Casimir force is computed for semiconductor plates with different conductivity properties taking into account all theoretical uncertainties discussed in literature. The comparison between…
Casimir effect is the attractive force which acts between two plane parallel, closely spaced, uncharged, metallic plates in vacuum. This phenomenon was predicted theoretically in 1948 and reliably investigated experimentally only in recent years. In fact, the Casimir force is similar to the familiar van der Waals force in the case of relatively large separations when the relativistic effects come into play. We review the most important experiments on measuring the Casimir force by means of torsion pendulum, atomic force microscope and micromechanical torsional oscillator. Special attention is …
We performed measurements of the gradient of the Casimir force between Au-coated surfaces of a sphere and a plate by means of significantly upgraded dynamic atomic force microscope (AFM) based technique. By introducing combined cleaning procedure of interior surfaces of the vacuum chamber and the test bodies by means of UV light and Ar ions, we reached higher vacuum and eliminated the role of electrostatic patches. Furthermore, the use of much softer cantilever allowed a sixfold decrease of the systematic error in measuring the force gradient. The experimental data are compared with theoretica…
It is well known that residual electrostatic forces create significant difficulties to precise measurements of the Casimir force and to wide use of Casimir-operated microdevices. We experimentally demonstrate that with the help of Ar-ion cleaning of the surfaces it is possible to make electrostatic effects negligibly small as compared to the Casimir interaction. Our experimental setup consists of the dynamic atomic force microscope supplemented with an Ar-ion gun and argon reservoir. The residual potential difference between the Au-coated surfaces of a sphere and a plate was measured both befo…
We review modern achievements and problems in physics of the van der Waals and Casimir forces which arise due to zero-point and thermal fluctuations of the electromagnetic field between closely spaced material surfaces. This subject attracted great experimental and theoretical attention during the last few years because the fluctuation-induced forces find a lot of applications in both fundamental physics and nanotechnology. After a short introduction to the subject, we describe main experimental and theoretical results obtained in the field during the last fifteen years. In the following prese…
The Casimir Force, a quantum mechanical effect, has been observed in several microelectromechanical systems (MEMS) platforms. Due to its extreme sensitivity to the separation of two objects, the Casimir Force has been proposed as an excellent avenue for quantum metrology. Practical application, however, is challenging due to attractive forces leading to stiction and failure of the device, called Casimir pull-in. In this work, we design and simulate a Casimir-driven metrology platform, where a time-delay based parametric amplification technique is developed to achieve a steady state and avoid p…
In the current work we present the complete results for the measurement of normal Casimir force between shallow and smooth sinusoidally corrugated gold coated sphere and a plate at various angles between the corrugations using an atomic force microscope. All measured data were compared with the theoretical approach using the proximity force approximation and theory based on derivative expansion. In both cases real material properties of the surfaces and non-zero temperature were taken into account. Special attention is paid to the description of electrostatic interactions between corrugated su…
Casimir forces between charge-neutral bodies originate from quantum vacuum fluctuations of electromagnetic fields, which exhibit a critical dependence on material's electromagnetic properties. Over the years, in-situ modulation of material's optical properties has been enabled through various means and has been widely exploited in a plethora of applications such as electro-optical modulation, transient color generation, bio- or chemical sensing, etc. Yet Casimir force modulation has been hindered by difficulty in achieving high modulation signals due to the broadband nature of the Casimir inte…
The lateral Casimir force acting between a sinusoidally corrugated gold plate and sphere was calculated and measured. The experimental setup was based on the atomic force microscope specially adapted for the measurement of the lateral Casimir force. The measured force oscillates sinusoidally as a function of the phase difference between the two corrugations. Both systematic and random errors are analysed and a lateral force amplitude of $3.2\times 10^{-13} $N was measured at a separation distance of 221 nm with a resulting relative error 24% at a 95% confidence probability. The dependence of t…
We present the results of an experiment on measuring the gradient of the Casimir force between an Au-coated hollow glass microsphere and graphene-coated fused silica plate by means of a modified atomic force microscope cantilever based technique operated in the dynamic regime. These measurements were performed in high vacuum at room temperature. The energy gap and the concentration of impurities in the graphene sample used have been measured utilizing scanning tunnelling spectroscopy and Raman spectroscopy, respectively. The measurement results for the gradients of the Casimir force are found …
We report precision measurements of the Casimir interaction at larger separation distances between the Au-coated surfaces of a sphere and a plate in ultrahigh vacuum using a much softer cantilever of the dynamic atomic force microscope-based setup and two-step cleaning procedure of the vacuum chamber and test body surfaces by means of UV light and Ar-ion bombardment. Compared to the previously performed experiment, two more measurement sets for the gradient of the Casimir force are provided which confirmed and slightly improved the results. Next, additional measurements have been performed wit…
We present Casimir force measurements in a sphere-plate configuration that consists of a high quality nanomembrane resonator and a millimeter sized gold coated sphere. The nanomembrane is fabricated from stoichiometric silicon nitride metallized with gold. A Kelvin probe method is used in situ to image the surface potentials to minimize the distance-dependent residual force. Resonance-enhanced frequency-domain measurements of the nanomembrane motion allow for very high resolution measurements of the Casimir force gradient (down to a force gradient sensitivity of 3 uN/m). Using this technique, …
We formulate a method allowing to confirm or exclude the alternative models of material properties at some definite confidence level in experiments on measuring the Casimir force. The method is based on the consideration of differences between the theoretical and mean measured quantities and the confidence intervals for these differences found at sufficiently high or low confidence probabilities. The developed method is applied to the data of four recent experiments on measuring the gradient of the Casimir force by means of a dynamic atomic force microscope. It is shown that in experiments wit…
We report stronger constraints on the parameters of Yukawa-type corrections to Newtonian gravity from measurements of the lateral Casimir force between sinusoidally corrugated surfaces of a sphere and a plate. In the interaction range from 1.6 to 14 nm the strengthening of previously known high confidence constraints up to a factor of $2.4\times 10^7$ is achieved using these measurements. It is shown that the replacement of a plane plate with a corrugated one in the measurements of the normal Casimir force by means of an atomic force microscope would result in the strengthening of respective h…
The Lifshitz theory provides a method to calculate the Casimir force between two flat plates if the frequency dependent dielectric function of the plates is known. In reality any plate is rough and its optical properties are known only to some degree. For high precision experiments the plates must be carefully characterized otherwise the experimental result cannot be compared with the theory or with other experiments. In this chapter we explain why optical properties of interacting materials are important for the Casimir force, how they can be measured, and how one can calculate the force usin…
Microscopic imaging of local magnetic fields provides a window into the organizing principles of complex and technologically relevant condensed matter materials. However, a wide variety of intriguing strongly correlated and topologically nontrivial materials exhibit poorly understood phenomena outside the detection capability of state-of-the-art high-sensitivity, high-resolution scanning probe magnetometers. We introduce a quantum-noise-limited scanning probe magnetometer that can operate from room to cryogenic temperatures with unprecedented DC-field sensitivity and micron-scale resolution. T…
The Casimir force between two metallic plates is affected by their roughness state. This effect is usually calculated through the so-called `proximity force approximation' which is only valid for small enough wavevectors in the spectrum of the roughness profile. We introduce here a more general description with a wavevector-dependent roughness sensitivity of the Casimir effect. Since the proximity force approximation underestimates the effect, a measurement of the roughness spectrum is needed to achieve the desired level of accuracy in the theory-experiment comparison.
We propose a method of achieving large temperature sensitivity in the Casimir force that involves measuring the stable separation between dielectric objects immersed in fluid. We study the Casimir force between slabs and spheres using realistic material models, and find large > 2nm/K variations in their stable separations (hundreds of nanometers) near room temperature. In addition, we analyze the effects of Brownian motion on suspended objects, and show that the average separation is also sensitive to changes in temperature . Finally, this approach also leads to rich qualitative phenomena, suc…
We compare theory and experiment in the Casimir force measurement between gold surfaces performed with the atomic force microscope. Both random and systematic experimental errors are found leading to a total absolute error equal to 8.5 pN at 95% confidence. In terms of the relative errors, experimental precision of 1.75% is obtained at the shortest separation of 62 nm at 95% confidence level (at 60% confidence the experimental precision of 1% is confirmed at the shortest separation). An independent determination of the accuracy of the theoretical calculations of the Casimir force and its appli…
We show that the detection sensitivity of a linear detector is lower bounded by some quantum limits. For the force detection, relevant for atomic force microscopes, the lower bound is given by the so-called ultimate quantum limit. For the displacement detection, relevant for detecting gravitational waves, a generalized lower bound is obtained.
We present complete results of the experiment on measuring the Casimir force between an Au-coated sphere and an untreated or, alternatively, UV-treated indium tin oxide film deposited on a quartz substrate. Measurements were performed using an atomic force microscope in a high vacuum chamber. The measurement system was calibrated electrostatically. Special analysis of the systematic deviations is performed, and respective corrections in the calibration parameters are introduced. The corrected parameters are free from anomalies discussed in the literature. The experimental data for the Casimir …
The experimental demonstration of the modification of the Casimir force between a gold coated sphere and a single-crystal Si membrane by light pulses is performed. The specially designed and fabricated Si membrane was irradiated with 514 nm laser pulses of 5 ms width in high vacuum leading to a change of the charge-carrier density. The difference in the Casimir force in the presence and in the absence of laser radiation was measured by means of an atomic force microscope as a function of separation at different powers of the absorbed light. The total experimental error of the measured force di…
We show that Rabi oscillations of a degenerate fermionic or bosonic gas trapped in a double-well potential can be exploited for the interferometric measurement of external forces at micrometer length scales. The Rabi interferometer is less sensitive, but easier to implement, than the Mach-Zehnder since it does not require dynamical beam-splitting/recombination processes. As an application we propose a measurement of the Casimir-Polder force acting between the atoms and a dielectric surface. We find that even if the interferometer is fed with a coherent state of relatively small number of atoms…
We present the status of an experimental test for gravitational strength forces below 1 mm. Our experiment uses small 1 kilohertz oscillators as test masses, with a stiff counducting shield between them to suppress backgrounds. At the present sensitivity of approximately 1000 times gravitational strength, we see no evidence for new forces with interaction ranges between 75 microns and 1 mm. While the Casimir background is not expected to be significant at this range, an extension of the shielding technique we employ may be useful for reducing this background in experiments below a few microns.…
We propose two novel experiments on the measurement of the Casimir force acting between a gold coated sphere and semiconductor plates with markedly different charge carrier densities. In the first of these experiments a patterned Si plate is used which consists of two sections of different dopant densities and oscillates in the horizontal direction below a sphere. The measurement scheme in this experiment is differential, i.e., allows the direct high-precision measurement of the difference of the Casimir forces between the sphere and sections of the patterned plate or the difference of the equ…
Squeezing is a resource that enables precision enhancements in quantum metrology and can be used as a basis for the generation of entanglement by linear optics. While strong squeezing is challenging to generate in optical fields, here we present simple periodic modulation protocols in optomechanical systems that can generate large squeezing of their mechanical degrees of freedom for realistic system parameters. We then proceed to show how such protocols can serve to improve the measurement precision of weak forces and enhance the generation of entanglement between test masses that are subject …
State-of-the-art microscopes use intense lasers that can severely disturb biological processes, function and viability. This introduces hard limits on performance that only quantum photon correlations can overcome. Here we demonstrate this absolute quantum advantage, achieving signal-to-noise beyond the photodamage-free capacity of conventional microscopy. We achieve this in a coherent Raman microscope, which we use to image molecular bonds within a cell with both quantum-enhanced contrast and sub-wavelength resolution. This allows the observation of nanoscale biological structures that would …
The displacement of micro-electro-mechanical-systems (MEMS) cantilevers is used to measure a broad variety of phenomena in devices ranging from force microscopes to biochemical sensors to thermal imaging systems. We demonstrate the first direct measurement of a MEMS cantilever displacement with a noise floor at 40% of the shot noise limit (SNL). By combining multi-spatial-mode quantum light sources with a simple differential measurement, we show that sub-SNL MEMS displacement sensitivity is highly accessible compared to previous efforts that measured the displacement of macroscopic mirrors wit…
