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arXiv 2201.00605physics.flu-dyn
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离子液体在非均匀微流控装置中的电荷相关滑移流动:压降和电粘性效应

Charge-dependent slip flow of ionic liquids through the non-uniform microfluidic device: pressure drop and electroviscous effects

Jitendra Dhakar, Ram Prakash Bharti

摘要:

本文研究了对称(1:1)电解质液体通过均匀带电狭缝收缩-膨胀(4:1:4)微流控装置的稳态压力驱动层流中存在电荷相关滑移时的电粘滞效应。数学模型包括泊松,能斯特-普朗克,纳维尔-斯托克斯,和电流连续性方程数值求解使用有限元法(FEM)。流场(电势,电荷,感应电场强度,压降和电粘性校正因子)已获得,并提出了广泛的参数,如反德拜长度(K=2-20),表面电荷密度(S=4-16)和滑移长度($0\le B_0\le 0.20$)在固定施密特数(Sc=1000)和低雷诺数(Re=0.01)。流场表现出复杂的依赖于控制参数。与无滑移条件相比,电荷依赖滑移进一步增强了依赖性的复杂性。相对于无滑移流动,在条件范围内,总电势($|ΔU|$)最大增加78.68%,并且压降($|ΔP|$)最大减小63.42%。在无滑移($B_0=0$)条件下,电粘性修正因子($Y=$表观粘度与物理粘度之比)增加了33.58%。它($Y$)最大增加72.10%,为电荷相关的滑移比在无滑移流的条件下考虑的范围。基于均匀截面上的Poiffille流动和薄孔板的压力损失,建立了一个简单的电粘性流动压降的分析模型。该模型从数值上高估了2 - 4%的压降。最后,预测关系,描绘的功能依赖于控制参数的数值结果,为他们的实际使用中的微流控器件的设计和工程。

英文摘要:

This work investigates electroviscous effects in presence of charge-dependent slip in steady pressure-driven laminar flow of a symmetric (1:1) electrolyte liquid through a uniformly charged slit contraction - expansion (4:1:4) microfluidic device. The mathematical model comprising Poisson's, Nernst-Planck, Navier-Stokes, and current continuity equations are solved numerically using finite element method (FEM). The flow fields (electrical potential, charge, induced electric field strength, pressure drop, and electroviscous correction factor) have been obtained and presented for a wide range of parameters like inverse Debye length (K=2-20), surface charge density (S=4-16) and slip length ($0\le B_0\le 0.20$) at fixed Schmidt number (Sc=1000) and low Reynolds number (Re=0.01). The flow fields have shown complex dependence on governing parameters. The charge-dependent slip has further enhanced complexity of dependency in comparison to no-slip condition. The total electrical potential ($|ΔU|$) maximally increases by 78.68%, and pressure drop ($|ΔP|$) maximally decreases by 63.42%, relative to no-slip flow, over the ranges of conditions. The electroviscous correction factor ($Y=$ ratio of apparent to physical viscosity) increases by 33.58% under the no-slip ($B_0=0$) condition. It ($Y$) increases maximally by 72.10% for charge-dependent slip than in no-slip flow for considered ranges of the conditions. A simple analytical model to estimate the pressure drop in the electroviscous flow has been developed based on the Poiseuille flow in individual uniform sections and pressure loss due to thin orifice. The model overpredicts pressure drop by 2 - 4% from the numerical values. Finally, the predictive relations, depicting the functional dependence of numerical results on governing parameters, are presented for their practical use in design and engineering of microfluidic devices.

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