We report on the controlled transport of drops of magnetic liquid, which are swimming on top of a non-magnetic liquid layer. A magnetic field which is rotating in a vertical plane creates a torque on the drop. Due to surface stresses within the immiscible liquid beneath, the drop is propelled forward. We measure the drop speed for different field amplitudes, field frequencies and drop volumes. Simplifying theoretical models describe the drop either as a solid sphere with a Navier slip boundary condition, or as a liquid half-sphere. An analytical expression for the drop speed is obtained which is free of any fitting parameters and is well in accordance with the experimental measurements. Possible microfluidic applications of the rolling drop are also discussed.
Vertical drop impacts of ferrofluids onto glass slides in a non-uniform magnetic field have been studied using high-speed photography. Outcomes have been classified based on the motion of the fluid-surface contact lines, and formation of peaks (Rosensweig instabilities) which affect the height of the spreading drop. The largest peaks are nucleated at the edge of a spreading drop, similarly to crown-rim instabilities in drop impacts with conventional fluids, and remain there for an extended time. Impact Weber numbers ranged from 18.0 to 489, and the vertical component of the B-field was varied …
In this article, we propose, with the aid of detailed experiments and scaling analysis, the existence of magneto-elastic effects in the impact hydrodynamics of non-Newtonian ferrofluid droplets on superhydrophobic (SH) surfaces in presence of a magnetic field. The effects of magnetic Bond number (Bom), Weber number (We), polymer concentration and magnetic nanoparticle (Fe3O4) concentration in the ferrofluids were investigated. In comparison to Newtonian ferrofluid droplets, addition of polymers caused rebound suppression of the droplets relatively at lower Bom for a fixed magnetic nanoparticle…
We report the experimental investigations on the mixing of a ferrofluid droplet with a non-magnetic fluid in the presence of a time-dependent magnetic field on an open surface microfluidic platform. The bright field visualization technique, in combination with the micro-PIV analysis, is carried out to explore the internal hydrodynamics of the ferrofluid droplet. Also, using the Laser-induced fluorescence (micro-LIF) technique, we quantify the mass transfer occurring between the two droplets, which in effect, determines the underlying mixing performance under the modulation of the frequency of …
We investigate how ferrofluid droplets suspended in a wall-bounded shear flow can organise when subjected to an external magnetic field. By tuning the magnitude of the external magnetic field, we find that the ferrofluid droplets form chain-like structures in the flow direction when the magnetic field is weak, while forming a crystal-like pattern in a strong magnetic field. We provide the phase diagram and the critical conditions for this chain-to-crystal transition, by applying both numerical simulations and analytic calculations. We also examine how the organised patterns of the ferrofluid d…
The spontaneous motion of liquid droplets on solid surfaces is the result of an unbalanced surface tension force, which is sometimes called the "Marangoni effect". This can be triggered by either a difference in surface temperature or a heterogeneity in the topography or chemistry of the surface passively or actively. The imbibition of liquid within capillary tubes, horizontal ice wicking on either hydrophilic or hydrophobic substrates, and inkjet printing for example are just some classic illustrations of where the Lucas-Washburn equation can predict droplet behavior characteristics fairly we…
Deformation and breakup of a ferrofluid compound droplet migrating in a microchannel under a magnetic field: A phase-field-based multiple-relaxation time lattice Boltzmann study
The present article discusses the physics and mechanics of evaporation of pendent, aqueous ferrofluid droplets and modulation of the same by external magnetic field. We show experimentally and by mathematical analysis that the presence of magnetic field improves the evaporation rates of ferrofluid droplets. First we tackle the question of improved evaporation of the colloidal droplets compared to water, and propose physical mechanisms to explain the same. Experiments show that the changes in evaporation rates aided by the magnetic field cannot be explained on the basis of changes in surface te…
Two dimensional free surface flows in Hele-Shaw configurations are a fertile ground for exploring nonlinear physics. Since Saffman and Taylor's work on linear instability of fluid--fluid interfaces, significant effort has been expended to determining the physics and forcing that set the linear growth rate. However, linear stability does not always imply nonlinear stability. We demonstrate how the combination of a radial and an azimuthal external magnetic field can manipulate the interfacial shape of a linearly unstable ferrofluid droplet in a Hele-Shaw configuration. We show that weakly nonlin…
The effect of a spatially uniform magnetic field on the shear rheology of a dilute emulsion of monodispersed ferrofluid droplets, immersed in a non-magnetizable immiscible fluid, is investigated using direct numerical simulations. The direction of the applied magnetic field is normal to the shear flow direction. The droplets extra stress tensor arising from the presence of interfacial forces of magnetic nature is modeled on the basis of the seminal work of G. K. Batchelor, J. Fluid Mech., 41.3 (1970) under the assumptions of a linearly magnetizable ferrofluid phase and negligible inertia. The …
Hydrodynamics and Thermal Multiphysics Lab (HTML), Department of Mechanical Engineering, Indian Institute of Technology Kharagpur（印度理工学院卡拉格普尔分校机械工程系水动力学与热多物理实验室）
The impact and splash of liquid drops on solid substrates are ubiquitous in many important fields. However, previous studies have mainly focused on spherical drops while the non-spherical situations, such as raindrops, charged drops, oscillating drops, and drops affected by electromagnetic field, remain largely unexplored. Using ferrofluid, we realize various drop shapes and illustrate the fundamental role of shape in impact and splash. Experiments show that different drop shapes produce large variations in spreading dynamics, splash onset, and splash amount. However, underlying all these vari…
We present a new system based on alginate gels for the encapsulation of a ferrofluid drop, which allows us to create millimeter-sized elastic capsules that are highly deformable by inhomogeneous magnetic fields. We use a combination of experimental and theoretical work in order to characterize and quantify the deformation behavior of these ferrofluid-filled capsules. We introduce a novel method for the direct encapsulation of unpolar liquids by sodium alginate. The addition of polar alcohol molecules allows us to encapsulate a ferrofluid as a single phase. This encapsulation method increases t…
We report the breakup dynamics of a magnetically active droplet (ferrofluid droplet) in a T-shaped LOC device under the modulation of a non-uniform magnetic field. We adhere to high-speed imaging modalities for the experimental quantification of the droplet splitting phenomena in the presence of a non-uniform force field gradient, while the underlying phenomena is supported by the numerical results in a qualitative manner as well. On reaching the T-junction divergence, the droplet engulfs the intersection fully and eventually deforms into the dumbbell-shaped form making its bulges to move towa…
Recent experiments have shown that liquid Leidenfrost drops levitated by their vapor above a flat hot surface can exhibit symmetry-breaking spontaneous dynamics (A. Bouillant et al., Nature Physics, 14 1188-1192, 2018). Motivated by these observations, we theoretically investigate the translational and rotational dynamics of Leidenfrost drops on the basis of a simplified two-dimensional model, focusing on near-circular drops small relative to the capillary length. The model couples the equations of motion of the drop, which flows as a rigid wheel, and thin-film equations governing the vapor fl…
The study reports the aspects of postimpact hydrodynamics of ferrofluid droplets on superhydrophobic SH surfaces in the presence of a horizontal magnetic field. A wide gamut of dynamics was observed by varying the impact Weber number We, the Hartmann number Ha and the magnetic field strength manifested through the magnetic Bond number Bom. For a fixed We 60, we observed that at moderately low Bom 300, droplet rebound off the SH surface is suppressed. The noted We is chosen to observe various impact outcomes and to reveal the consequent ferrohydrodynamic mechanisms. We also show that ferrohydro…
Angular momentum of spinning bodies leads to their remarkable interactions with fields, waves, fluids, and solids. Orbiting celestial bodies, balls in sports, liquid droplets above a hot plate, nanoparticles in optical fields, and spinning quantum particles exhibit nontrivial rotational dynamics. Here, we report self-guided propulsion of magnetic fast-spinning particles on a liquid surface in the presence of a solid boundary. Above some critical spinning frequency (higher rotational Reynolds numbers), such particles generate localized 3D vortices and form composite 'spinner-vortex' quasi-parti…
