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arXiv 1402.1601cond-mat.supr-con
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PrFe1-xCoxAsO(x = 0.0 ~ 1.0)超导性的演化

Evolution of superconductivity in PrFe1-xCoxAsO with x = 0.0 to 1.0

Poonam Rani, Anand Pal, V. P. S. Awana

摘要:

我们报告的合成和物理性质的表征PrFe 1-xCoxAsO(x = 0.0至1.0)。所研究的样品是通过真空封装法通过固相反应路线合成的。原始的化合物PrFeAsO不表现出超导性,而是表现出一个金属台阶状的过渡,由于自旋密度波有序的Fe力矩低于150 K,其次是另一个向上的步骤,由于在12 K的Pr力矩的异常有序。Fe-SDW和Pr-TN温度均随Co在Fe位的取代而单调降低。超导电性出现在一个狭窄的范围内的x从0.07到0.25与最大Tc在11.12 K x = 0.15。x = 0.25的样品在300 K至2 K的温度范围内表现出金属行为,电阻率没有任何Fe-SDW或Pr-TN阶跃。事实上,尽管Fe-SDW单调减小,但即使x = 0.02,Pr-TN也消失。在14特斯拉以下的超导多晶Co掺杂PrFeAsO的磁输运测量导致上临界场[Hc 2(0)]的外推值高达60特斯拉。

英文摘要:

We report the synthesis and physical property characterization of PrFe1-xCoxAsO with x = 0.0 to 1.0. The studied samples are synthesized by solid state reaction route via vacuum encapsulation method. The pristine compound PrFeAsO does not show superconductivity, but rather exhibits a metallic step like transition due to spin density wave ordering of Fe moments below 150 K, followed by another upward step due to anomalous ordering of Pr moments at 12 K. Both the Fe-SDW and Pr-TN temperatures decrease monotonically with Co substitution at Fe site. Superconductivity appears in a narrow range of x from 0.07 to 0.25 with maximum Tc at 11.12 K for x = 0.15. Samples, with x = 0.25 exhibit metallic behavior right from 300 K down to 2 K, without any Fe-SDW or Pr-TN steps in resistivity. In fact, though Fe-SDW decreases monotonically, the Pr-TN is disappeared even with x = 0.02. The magneto transport measurements below 14 Tesla on superconducting polycrystalline Co doped PrFeAsO lead to extrapolated values of the upper critical fields [Hc2(0)] of up to 60 Tesla.

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