Emergent Phases of Nodeless and Nodal Superconductivity Separated by Antiferromagnetic Order in Iron-based Superconductor (Ca4Al2O6)Fe2(As1-xPx)2: 75As- and 31P-NMR Studies
H. Kinouchi, H. Mukuda, Y. Kitaoka, P. M. Shirage, H. Fujikura, Y. Gotoh, H. Eisaki, A. Iyo
备注:
5pages, 4figures; accepted for publication as a Rapid Communication in Phys. Rev. B
我们报告$^{31}$ P-和$^{75}$ As-NMR研究(Ca $_4$ Al $_2$ O $_{6}$)Fe $_2$(As $_{1-x}$ P $_x$)$_2$与P等价取代As。我们提出了新的演化的紧急阶段,节点无超导(SC)在0 $\le x \le$ 0.4和节点的$x$ =1附近是密切分离的开始相称的条纹型反铁磁(AFM)的顺序在0.5 $\le x \le$ 0.95,作为一个等价的替代P为As降低了氮族元素的高度$h_{Pn}$从Fe平面测量。结果表明,原子力显微镜的有序化发生在1.32 π $\le h_{Pn} \le$ 1.42 π的条件下,这也适用于(Fe $Pn$)$^{-}$层中具有Fe $^{2+}$态的其他铁磷族化合物.这种新的相位演化与$h_{Pn}$的变化点的重要性,电子相关的出现SC以及AFM秩序。
英文摘要:
We report $^{31}$P- and $^{75}$As-NMR studies on (Ca$_4$Al$_2$O$_{6}$)Fe$_2$(As$_{1-x}$P$_x$)$_2$ with an isovalent substitution of P for As. We present the novel evolution of emergent phases that the nodeless superconductivity (SC) in 0$\le x \le$0.4 and the nodal one around $x$=1 are intimately separated by the onset of a commensurate stripe-type antiferromagnetic (AFM) order in 0.5$\le x \le$ 0.95, as an isovalent substitution of P for As decreases a pnictogen height $h_{Pn}$ measured from the Fe plane. It is demonstrated that the AFM order takes place under a condition of 1.32Å$\le h_{Pn} \le$1.42Å, which is also the case for other Fe-pnictides with the Fe$^{2+}$ state in (Fe$Pn$)$^{-}$ layers. This novel phase evolution with the variation in $h_{Pn}$ points to the importance of electron correlation for the emergence of SC as well as AFM order.
Unconventional superconductivity and antiferromagnetic quantum critical behavior in the isovalent-doped BaFe2(As1-xPx)2
用$^{31}$ P NMR研究了BaFe $_2$(As $_{1-x}$ P $_x$)$_2$的自旋动力学随P浓度的变化.我们的核磁共振研究表明,二维反铁磁(AF)的波动显着增强与静态磁化率的变化不大接近AF阶段从超导圆顶。此外,磁有序温度$θ$推导出的弛豫速率在最佳掺杂消失。这些结果为量子临界点(QCP)提供了明确的证据,表明与QCP相关的AF涨落在高- $T_c$超导性中发挥着核心作用。