本文报道了一种非常干净的空穴掺杂单晶Ba $_{0.68}$ K $_{0.32}$ Fe $_{2}$ As $_{2}$($T_{\rm {c}}=38.5$ K)的核磁共振研究。自旋-晶格弛豫速率$1/T_{1}$示出了从$T \simeq 0.45 T_{\rm c}$到$T \simeq 0.11 T_{\rm c}$的指数下降,这指示完全打开的能隙。从比值$(T_{1})_{c} / (T_{1})_{a}$(其中$a$和$c$表示晶体方向),我们发现反铁磁自旋涨落在$T_{\rm c}$上方的自旋空间中是各向异性的。各向异性在$T_{\rm c}$以下降低,在$T \rightarrow 0$处消失。我们认为,各向异性源于自旋轨道耦合的影响消失时,自旋单重态电子对形成一个无节点的差距。
英文摘要:
We report $^{75}$As nuclear magnetic resonance studies on a very clean hole-doped single-crystal Ba$_{0.68}$K$_{0.32}$Fe$_{2}$As$_{2}$ ($T_{\rm {c}}=38.5$ K). The spin-lattice relaxation rate $1/T_{1}$ shows an exponential decrease below $T \simeq 0.45 T_{\rm c}$ down to $T \simeq 0.11 T_{\rm c}$, which indicates a fully opened energy gap. From the ratio $(T_{1})_{c} / (T_{1})_{a}$, where $a$ and $c$ denote the crystal directions, we find that the antiferromagnetic spin fluctuation is anisotropic in the spin space above $T_{\rm c}$. The anisotropy decreases below $T_{\rm c}$ and disappears at $T \rightarrow 0$. We argue that the anisotropy stems from spin-orbit coupling whose effect vanishes when spin-singlet electron pairs form with a nodeless gap.
Emergent Phases of Nodeless and Nodal Superconductivity Separated by Antiferromagnetic Order in Iron-based Superconductor (Ca4Al2O6)Fe2(As1-xPx)2: 75As- and 31P-NMR Studies
我们报告$^{31}$ P-和$^{75}$ As-NMR研究(Ca $_4$ Al $_2$ O $_{6}$)Fe $_2$(As $_{1-x}$ P $_x$)$_2$与P等价取代As。我们提出了新的演化的紧急阶段,节点无超导(SC)在0 $\le x \le$ 0.4和节点的$x$ =1附近是密切分离的开始相称的条纹型反铁磁(AFM)的顺序在0.5 $\le x \le$ 0.95,作为一个等价的替代P为As降低了氮族元素的高度$h_{Pn}$从Fe平面测量。结果表明,原子力显微镜的有序化发生在1.32 π $\le h_{Pn} \le$ 1.42 π的条件下,这也适用于(Fe $Pn$)$^{-}$层中具有Fe $^{2+}$态的其他铁磷族化合物.这种新的相位演化与$h_{Pn}$的变化点的重要性,电子相关的出现SC以及AFM秩序。
The ThIrSi superconductor, with $T_c = 6.5$ K, is expected to show unusual features in view of its noncentrosymmetric structure and the presence of heavy elements featuring a sizable spin-orbit coupling. Here, we report a comprehensive study of its electronic properties by means of local-probe techniques: muon-spin rotation and relaxation ({\textmu}SR) and nuclear magnetic resonance (NMR). Both the superfluid density $ρ_\mathrm{sc}(T)$ (determined via transverse-field {\textmu}SR) and the spin-lattice relaxation rate $T_1^{-1}(T)$ (determined via NMR) suggest a nodeless superconductivity. Furt…
NMR evidence for an intimate relationship between antiferromagnetic spin fluctuations and extended s-wave superconductivity in mono-crystalline SrFe2(As_{1-x}P_{x})2
We report a comprehensive study of the noncentrosymmetric NbReSi superconductor by means of muon-spin rotation and relaxation ($μ$SR) and nuclear magnetic resonance (NMR) techniques. NbReSi is a bulk superconductor with $T_c = 6.5$ K, characterized by a large upper critical field, which exceeds the Pauli limit. Both the superfluid density $ρ_\mathrm{sc}(T)$ (determined via transverse-field $μ$SR) and the spin-lattice relaxation rate $T_1^{-1}(T)$ (determined via NMR) suggest a nodeless superconductivity (SC) in NbReSi. We also find signatures of multigap SC, here evidenced by the field-depende…
Identifying the uniqueness of FeP-based superconductors may shed new lights on the mechanism of superconductivity in iron-pnictides. Here, we report nuclear magnetic resonance(NMR) studies on LiFeP and LiFeAs which have the same crystal structure but different pnictogen atoms. The NMR spectrum is sensitive to inhomogeneous magnetic fields in the vortex state and can provide the information on the superconducting pairing symmetry through the temperature dependence of London penetration depth $λ_L$. We find that $λ_L$ saturates below $T \sim 0.2$ $T_c$ in LiFeAs, where $T_c$ is the superconducti…
Concerning the superconducting gap symmetry in YBa2Cu3O7-δ, YBa2Cu4O8, and La2-xSrxCuO4 determined from muon spin rotation in mixed states of crystals and powders
用μ子自旋旋转(μ+SR)方法测量了YBa_2Cu_3 O_7-δ(δ { \approx } 0.05)、YBa_2Cu_4 O_8和La_(2-x)Sr_xCuO_4(x ~ 0.15-0.17)超导混合态的局域磁场σ的平方根二阶矩,并对它们的超导能隙对称性进行了比较分析。对于取向晶体,它示出的σ对温度T和施加的场H的异常依赖性,作为测量和提取的a-和b-轴分量,归因于磁通钉扎和混乱,模糊了超导穿透深度的内在特征。来自定向晶体数据的随机平均值与相应的非定向粉末明显不同,这是由于高质量晶体中钉扎的影响较弱。钉扎扰动的相关指标,如σ的非单调H依赖性,不可重现的数据和表观转变温度的强H依赖性也是显而易见的。强的内禀钉扎抑制了σ的c轴分量的热异常,这反映了YBa 2Cu 3 O 7-δ和YBa 2Cu 4 O 8中的无节点能隙对称性。对于YBa 2Cu 3 O 7-δ,晶体(a-b分量,经脱钉校正)和粉末数据都反映了无节能隙(然而,对于晶体YBa 2Cu 4 O 8和La1.83Sr0.17CuO4,a-b对称性仍未解决)。讨论了晶体数据的多重能隙解释和节点能隙解释中所包含的信息,以及体μ+SR和表面灵敏测量之间观察到的差异。
Antiferromagnetic spin correlations and pseudogap-like behavior in Ca(Fe1-xCox)2As2 studied by 75As nuclear magnetic resonance and anisotropic resistivity
本文报道了在350~ $^{\circ}$ C退火7天的单晶Ca(Fe $_{1-x}$ Co $_x$)$_2$ As $_2$($x$ = 0.023,0.028,0.033和0.059)的$^{75}$ As核磁共振(NMR)测量结果。根据在条纹型反铁磁(AFM)状态下观察$^{75}$ As NMR谱的特征形状,如在$x$ = 0的情况下,($T_{\rm N}$ = 170 K),在$x$ = 0.023中观察到了与伴随的结构相变相称的AFM相变的明确证据($T_{\rm N}$ = 106 K)和$x$ = 0.028($T_{\rm N}$ = 53 K)。通过Knight位移和核自旋晶格弛豫速率的温度依赖性,(1/ $T_1$),尽管在顺磁状态下实现了与其他铁磷属元素化物超导体的情况一样的条纹型AFM自旋波动,但是我们发现AFM自旋波动在低于交叉温度$T^*$的情况下逐渐减小,该交叉温度几乎与Co取代浓度无关,并且归因于这些系统的自旋激发谱中的类赝隙行为。$T^*$特征发现与温度相关的平面间电阻率$ρ_c(T)$中的特征相关,但不与平面内电阻率$ρ_a (T)$相关。通过在平行和垂直于$c$轴的磁场下测量的1/ $T_1$数据,跟踪了各向异性条带型AFM自旋涨落在顺磁和赝能隙相中的温度演化。基于我们的NMR数据,我们在Ca(Fe $_{1-x}$ Co $_x$)$…