Photon correlations are investigated for a single laser-excited ion trapped in front of a mirror. Varying the relative distance between the ion and the mirror, photon correlation statistics can be tuned smoothly from an antibunching minimum to a bunching-like maximum. Our analysis concerns the non-Markovian regime of the ion-mirror interaction and reveals the field establishment in a half-cavity interferometer.
A cavity-modified master equation is derived for a coherently driven, V-type three-level atom coupled to a single-mode cavity in the bad cavity limit. We show that population inversion in both the bare and dressed-state bases may be achieved, originating from the enhancement of the atom-cavity interaction when the cavity is resonant with an atomic dressed-state transition. The atomic populations in the dressed state representation are analysed in terms of the cavity-modified transition rates. The atomic fluorescence spectrum and probe absorption spectrum also investigated, and it is found that…
We theoretically demonstrate the enhanced and dephasing immune squeezing in the resonance fluorescence of a single quantum dot (QD) confined to a pillar-microcavity and driven by a continuous wave laser. We employ a formalism based on Polaron master equation theory for incorporating the influence of exciton-phonon coupling quite accurately in the dot-cavity system. We show a significant enhancement of squeezing due to cavity coupling of the QD as compared to that of an ideal single two-level system in free space. Particularly, we show a four-fold enhancement in squeezing as compared to that of…
We present a supervised learning model to calibrate the photon collection rate during the fluorescence imaging of cold atoms. The linear regression model finds the collection rate at each location on the sensor such that the atomic population difference equals that of a highly precise optical cavity measurement. This 192 variable regression results in a measurement variance 27% smaller than our previous single variable regression calibration. The measurement variance is now in agreement with the theoretical limit due to other known noise sources. This model efficiently trains in less than a mi…
The fluorescence light emitted by a 4-level system in $J=1/2$ to $J=1/2$ configuration driven by a monochromatic laser field and in an external magnetic field is studied. We show that the spectrum of resonance fluorescence emitted on the $π$ transitions shows a signature of spontaneously generated interference effects. The degree of interference in the fluorescence spectrum can be controlled by means of the external magnetic field, provided that the Landé g-factors of the excited and the ground state doublet are different. For a suitably chosen magnetic field strength, the relative weight of t…
The squeezing spectrum of the resonance fluorescence is studied for a coherently driven four-level atom in the Y-type configuration. It is found that the squeezing properties of the fluorescence radiation are modified significantly when quantum interference of the spontaneous decays channels is included. We show a considerable enhancement of steady-state squeezing in spectral components for strong and off-resonant driving fields. The squeezing may be increased in both the inner and outer sidebands of the spectrum depending upon the choice of parameters. We also show that the interference can d…
In this paper we derive a general expression for the emission rate of an emitter which is placed at the center of a real cavity drilled in a generic random medium. We apply our formalism to the computation of the decay rate of a single atom which seats within a small molecule embedded in a continuous medium.
Squeezing of atomic resonance fluorescence is shown to be optimized by a properly designed environment, which can be realized by a quasi-resonant cavity. Optimal squeezing is achieved if the atomic coherence is maximized, corresponding to a pure atomic quantum state. The atomic-state purification is achieved by the backaction of the cavity field on the atom, which increases the atomic coherence and decreases the atomic excitation. For realistic cavities, the coupling of the atom to the cavity field yields a purity of the atomic state of more than 99%. The fragility of squeezing against dephasi…
We discuss the spontaneous emission from a coherently prepared and microwave driven doublet of potentially closely spaced excited states to a common ground level. Multiple interference mechanisms are identified which may lead to fluorescence inhibition in well-separated regions of the spectrum or act jointly in cancelling the spontaneous emission. In addition to phase independent quantum interferences due to combined absorptions and emissions of driving field photons, we distinguish two competing phase dependent interference mechanisms as means of controlling the fluorescence. The indistinguis…
We report the implementation of projective measurement on a single 1/2 nuclear spin of the 171Yb atom by measuring the polarization of cavity-enhanced fluorescence. To obtain cavity-enhanced fluorescence having a nuclear-spin-dependent polarization, we construct a two-mode cavity QED system, in which two cyclic transitions are independently coupled to each of the orthogonally polarized cavity modes, by manipulating the energy level of 171Yb. This system can associate the nuclear spin degrees of freedom with the polarization of photons, which will facilitate the development of hybrid quantum sy…
We study the resonance fluorescence from a coherently driven four-level atom in the Y-type configuration. The effects of quantum interference induced by spontaneous emission on the fluorescence properties of the atom are investigated. It is found that the quantum interference resulting from cascade emission decays of the atom leads to a splitting of resonances in the excited level populations calculated as a function of light detuning. For some parameters, interference assisted enhancement of inner sidebands and narrowing of central peaks may also occur in the fluorescence spectrum. We present…
We calculate the fluorescence spectra of a driven lattice of coupled cavities. To do this, we extend methods of evaluating two-time correlations in infinite lattices to open quantum systems; this allows access to momentum resolved fluorescence spectrum. We illustrate this for a driven-dissipative transverse field anisotropic XY model. By studying the fluctuation dissipation theorem, we find the emergence of a quasi-thermalized steady state with a temperature dependent on system parameters; for blue detuned driving, we show this effective temperature is negative. In the low excitation density l…
In quantum physics, measurement results are random but their statistics can be predicted assuming some knowledge about the system in the past. Additional knowledge from a future measurement deeply changes the statistics in the present and leads to purely quantum features. In particular conditioned average outcomes of a weak measurement, so-called weak values, were shown to go beyond the conventional range, give a way to directly measure complex quantities, and can be used to enhance the sensitivity of quantum meters. Recently, these concepts have been considered in the general case of open qua…
It has been observed experimentally [H.R. Xia, C.Y. Ye, and S.Y. Zhu, Phys. Rev. Lett. {\bf 77}, 1032 (1996)] that quantum interference between two molecular transitions can lead to a suppression or enhancement of spontaneous emission. This is manifested in the fluorescent intensity as a function of the detuning of the driving field from the two-photon resonance condition. Here we present a theory which explains the observed variation of the number of peaks with the mutual polarization of the molecular transition dipole moments. Using master equation techniques we calculate analytically as wel…
A scheme for engineering quantum interference in a $Λ$-type atom coupled to a frequency-tunable, single-mode cavity field with a pre-selected polarization at finite temperature is proposed. Interference-assisted population trapping, population inversions and probe gain at one sideband of the Autler-Townes spectrum are predicted for certain cavity resonant frequencies.
We show that cavity-induced interference may result in spectral line narrowing in the absorption spectrum of a $Ξ$-type atom coupled to a single-mode, frequency-tunable cavity field with a pre-selected polarization at finite temperature.
We propose a scheme for generating entangled states for two superconducting quantum interference devices in a thermal cavity with the assistance of a microwave pulse.
We report the phase control of spatial interference of resonance fluorescence from two duplicated two-level atoms, driving by two orthogonally polarized fields. In this closed-loop system, the relative phase is of crucial importance to the recovery of the interference patten in the fluorescence light even with strong driving.In order to improve the experimental realizability, we propose a scheme to recover the visibility with fixed relative phase by adjusting the relative intensities between the two driving fields or alternatively by using a standing-wave field.
We study the Autler-Townes spectrum of a V-type atom coupled to a single-mode, frequency-tunable cavity field at finite termperature, with a pre-selected polarization in the bad cavity limit, and show that, when the mean number of thermal photons $N\gg 1$ and the excited sublevel splitting is very large (the same order as the cavity linewidth), the probe gain may occur at either sideband of the doublet, depending on the cavity frequency, due to the cavity-induced interference.
We show how interference effects are responsible for manipulating the output electromagnetic field of an optical micro-resonator in the good-cavity limit. The system of interest consists in a moderately strongly pumped two-level emitter embedded in the optical cavity. When an additional weaker laser of the same frequency is pumping the combined system through one of the resonator's mirrors then the output cavity electromagnetic field can be almost completely suppressed or enhanced. This is due to the interference among the scattered light by the strongly pumped atom into the cavity mode and th…
We discuss quantum interference phenomena in a system consisting from a laser driven three-level ladder-type emitter possessing orthogonal transition dipoles and embedded in a leaking optical resonator. The cavity mean-photon number vanishes due to the destructive nature of the interference phenomena. The effect occurs for some particular parameter regimes which were identified. Furthermore, upper bare-state population inversion occurs as well.
Stochastic perturbation of two-level atoms strongly driven by a coherent light field is analyzed by the quantum trajectory method. A new method is developed for calculating the resonance fluorescence spectra from numerical simulations. It is shown that in the case of dominant incoherent perturbation, the stochastic noise can unexpectedly create phase correlation between the neighboring atomic dressed states. This phase correlation is responsible for quantum interference between the related transitions resulting in anomalous modifications of the resonance fluorescence spectra.
Resonance fluorescence from a quantum emitter is an ideal source to extract indistinguishable photons. By using the cross polarization to suppress the laser scattering, we observed resonance fluorescence from GeV color centers in diamond at cryogenic temperature. The Fourier-transform-limited linewidth emission with $T_2/2T_1\sim0.86$ allows for two-photon interference based on single GeV color center. Under pulsed excitation, the 24 ns separated photons exhibit a Hong-Ou-Mandel visibility of $0.604\pm0.022$, while the continuous-wave excitation leads to a coalescence time window of 1.05 radia…
We present a scheme to achieve maximally entangled states, controlled phase-shift gate, and SWAP gate for two superconducting-quantum-interference-device (SQUID) qubits, by placing SQUIDs in a microwave cavity. We also show how to transfer quantum information from one SQUID qubit to another. In this scheme, no transfer of quantum information between the SQUIDs and the cavity is required, the cavity field is only virtually excited and thus the requirement on the quality factor of the cavity is greatly relaxed.
We study in detail the dynamics of a non-stationary system composed of a Quantum Well confined in an optomechanical cavity. This system is investigated with classical and quantized motion of the cavity movable mirror. In both the cases, the cavity frequency is rapidly modulated in time. The resultant periodically modulated spectra is presented. In particular, we study the effect of two-photon process on the number of intracavity photons. The intensity of fluorescent light emitted by excitons in the quantum well is also examined for these non-stationary systems. It is observed that the initial …
We investigate the fluorescence spectrum of a two-level atom in a cavity when the atom is driven by a classical field. We show that forbidden dipole transitions in the Jaynes-Cummings Ladder structure are induced in the presence of the cavity damping, which deteriorates the degree of otherwise perfect destructive interference among the transition channels. With the larger cavity decay, these transitions are more enhanced.
We propose schemes to create cluster states and W states by many superconducting-quantum-interference-device (SQUID) qubits in cavities under the influence of the cavity decay. Our schemes do not require auxiliary qubits, and the excited levels are only virtually coupled throughout the scheme, which could much reduce the experimental challenge. We consider the cavity decay in our model and analytically demonstrate its detrimental influence on the prepared entangled states.
We demonstrate purely resonant continuous-wave optical laser excitation to coherently prepare an excitonic state of a single semiconductor quantum dot (QDs) inside a high quality pillar microcavity. As a direct proof of QD resonance fluorescence, the evolution from a single emission line to the characteristic Mollow triplet10 is observed under increasing pump power. By controlled utilization of weak coupling between the emitter and the fundamental cavity mode through Purcell-enhancement of the radiative decay, a strong suppression of pure dephasing is achieved, which reflects in close to Fouri…
A scheme for implementing 2-qubit quantum controlled phase gate (QCPG) is proposed with two superconducting quantum interference devices (SQUIDs) in a cavity. The gate operations are realized within the two lower flux states of the SQUIDs by using a quantized cavity field and classical microwave pulses. Our scheme is achieved without any type of measurement, does not use the cavity mode as the data bus and only requires a very short resonant interaction of the SQUID-cavity system. As an application of the QCPG operation, we also propose a scheme for generating the cluster states of many SQUIDs…
We study the spectra of emission of a system composed by an atom, tightly confined inside a high-finesse resonator, when the atom is driven by a laser and is at steady state of the cooling dynamics induced by laser and cavity field. In general, the spectrum of resonance fluorescence and the spectrum at the cavity output contain complementary information about the dynamics undergone by the system. In certain parameter regimes, quantum interference effects between the scattering processes induced by cavity and laser field lead to the selective suppression of features of the resonance fluorescenc…
Annual Review of Astronomy and Astrophysics, Volume 51, page 511e studied for coherently driven single photon sources, such as atoms and quantum dots. Maximal squeezing is realized, if the electronic subsystem of the emitter is in a pure quantum state. The purification is achieved by using a cavity as a second decay channel, besides the incoherent coupling to the electromagnetic vacuum. For realistic cavities this yields a purity of the electronic state of more than 99%. Aside from numerical calculations, we also derive approximate analytical results. Based on the approximations, effects are s…
Crossovers between Time-Bin and Energy-Time Entanglement in Homodyned Resonance Fluorescence
Beijing Academy of Quantum Information Sciences（北京量子信息科学研究院）；Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences（中国科学院物理研究所凝聚态物理国家实验室）；University of Chinese Academy of Sciences（中国科学院大学）
We study the optical properties of coupled quantum dot-microcavity systems with elliptical cross section. First, we develop an analytic model that describes the spectrum of the cavity modes that are split due to the reduced symmetry of the resonator. By coupling the QD emission to the polarized fundamental cavity modes, we observe the vectorial nature of the Purcell enhancement, which depends on the intrinsic polarization of the quantum dot and its relative alignment with respect to the cavity axis. The variable interaction strength of the QD with the polarized cavity modes leads to the observ…
Semiconductor quantum dots embedded in micro-pillar cavities are excellent emitters of single photons when pumped resonantly. Often, the same spatial mode is used to both resonantly excite a quantum dot and to collect the emitted single photons, requiring cross-polarization to reduce the uncoupled scattered laser light. This inherently reduces the source brightness to 50 %. Critically, for some quantum applications the total efficiency from generation to detection must be over 50 %. Here, we demonstrate a resonant-excitation approach to creating single photons that is free of any cross-polariz…
We propose an approach to realize an $n$-qubit controlled-$U$ gate with superconducting quantum interference devices (SQUIDs) in cavity QED. In this approach, the two lowest levels of a SQUID represent the two logical states of a qubit while a higher-energy intermediate level serves the gate manipulation. Our method operates essentially by creating a single photon through one of the control SQUIDs and then performing an arbitrary unitrary transformation on the target SQUID with the assistance of the cavity photon. In addition, we show that the method can be applied to implement an $n $% -qubit…
In electromagnetically-induced transparency (EIT), the absorption of a probe beam is greatly reduced due to destructive interference between two dressed atomic states produced by a strong laser beam. Here we show that a similar reduction in the single-photon absorption rate can be achieved by tuning a probe beam to be halfway between the resonant frequencies of two modes of a cavity. This technique is expected to be useful in enhancing two-photon absorption while reducing losses due to single-photon scattering.
We theoretically study the quantum interference induced photon blockade phenomenon in atom cavity QED system, where the destructive interference between two different transition pathways prohibits the two-photon excitation. Here, we first explore the single atom cavity QED system via an atom or cavity drive. We show that the cavity-driven case will lead to the quantum interference induced photon blockade under a specific condition, but the atom driven case can't result in such interference induced photon blockade. Then, we investigate the two atoms case, and find that an additional transition …
We propose a quantum interference cooling scheme for a nano-mechanical resonator (NAMR) in a hybrid optomechanical system, where the atoms are trapped in an optomechanical cavity, coupling to an additional optical cavity. The absorption of the optomechanical resonator can be modified by quantum interference effects induced by the atom-cavity and cavity-cavity couplings independently. With the employment of the quantum interference, the desired transition for cooling is enhanced, along with the heating suppression due to the undesired transition. As a result, the NAMR vibration can be cooled do…
The phase dependence of the cavity quantum dynamics in a driven equidistant three-level ladder-type system found in a quantum well structure with perpendicular transition dipoles is investigated in the good cavity limit. The pumping laser phases are directly transferred to the superposed amplitudes of the cavity-quantum-well interaction. Their phase difference may be tuned in order to obtain destructive quantum interferences. Therefore, the cavity field vanishes although the emitter continues to be pumped.
High-bandwidth, fiber-based optical cavities are a promising building block for future quantum networks. They are used to resonantly couple stationary qubits such as single or multiple atoms with photons routing quantum information into a fiber network at high rates. In high-bandwidth cavities, standard fluorescence imaging on the atom-cavity resonance line for controlling atom positions is impaired since the Purcell effect strongly suppresses all-directional fluorescence. Here, we restore imaging of $^{87}$Rb atoms strongly coupled to such a fiber Fabry-Pérot cavity by detecting the repumper …
We theoretically study a quantum destructive interference (QDI) induced photon blockade in a two-qubit driven cavity QED system with dipole-dipole interaction (DDI). In the absence of dipole-dipole interaction, we show that a QDI-induced photon blockade can be achieved only when the qubit resonance frequency is different from the cavity mode frequency. When DDI is introduced the condition for this photon blockade is strongly dependent upon the pump field frequency, and yet is insensitive to the qubit-cavity coupling strength. Using this tunability feature we show that the conventional energy-l…
When N driven atoms emit in phase into a high-Q cavity mode, the intracavity field generated by collective scattering interferes destructively with the pump driving the atoms. Hence atomic fluorescence is suppressed and cavity loss becomes the dominant decay channel for the whole ensemble. Microscopically 3D light-intensity minima are formed in the vicinity of the atoms that prevent atomic excitation and form a regular lattice. The effect gets more pronounced for large atom numbers, when the sum of the atomic decay rates exceeds the rate of cavity losses and one would expect the opposite behav…
We examine the competition among one- and two-photon processes in an ultra-cold, three-level atom undergoing cascade transitions as a result of its interaction with a bimodal cavity. We show parameter domains where two-photon transitions are dominant and also study the effect of two-photon emission on the mazer action in the cavity. The two-photon emission leads to the loss of detailed balance and therefore we obtain the photon statistics of the cavity field by the numerical integration of the master equation. The photon distribution in each cavity mode exhibits sub- and super- Poissonian beha…
Recently we predicted a random blinking, i.e. macroscopic quantum jumps, in the fluorescence of a laser-driven atom-cavity system [Metz et al., Phys. Rev. Lett. 97, 040503 (2006)]. Here we analyse the dynamics underlying this effect in detail and show its robustness against parameter fluctuations. Whenever the fluorescence of the system stops, a macroscopic dark period occurs and the atoms are shelved in a maximally entangled ground state. The described setup can therefore be used for the controlled generation of entanglement. Finite photon detector efficiencies do not affect the success rate …
We benchmark a selection of semiclassical and perturbative dynamics techniques by investigating the correlated evolution of a cavity-bound atomic system to assess their applicability to study problems involving strong light-matter interactions in quantum cavities. The model system of interest features spontaneous emission, interference, and strong coupling behaviour, and necessitates the consideration of vacuum fluctuations and correlated light-matter dynamics. We compare a selection of approximate dynamics approaches including fewest switches surface hopping, multi-trajectory Ehrenfest dynami…
The ability to detect single photons with high efficiency is a crucial requirement for various quantum information applications. By combining the storage process of a quantum memory for photons with fluorescence-based quantum state measurement, it is in principle possible to achieve high efficiency photon counting in large ensembles of atoms. The large number of atoms can, however, pose significant problems in terms of noise stemming from imperfect initial state preparation and off-resonant fluorescence. We propose a concrete implementation of a photon number resolving detector based on an ion…
