The coherent interaction between a two-level system and electromagnetic fields serves as a foundation for fundamental quantum physics and modern photonic quantum technology. A profound example is resonance fluorescence, where the non-classical photon emission appears in the form of a Mollow-triplet when a two-level system is continuously driven by a resonant laser. Pushing resonance fluorescence from a static to dynamic regime by using short optical pulses generates on-demand emissions of highly coherent single photons. Further increasing the driving strength in the dynamical regime enables the pursuit of exotic non-classical light emission in photon number superposition, photon number entanglement, and photon bundle states. However, the long-sought-after spectrum beyond the Mollow-triplet, a characteristic of dynamic resonance fluorescence under strong driving strength, has not been observed yet. Here we report the direct observation and systematic investigations of dynamic resonance fluorescence spectra beyond the Mollow-triplet in a solid-state cavity quantum electrodynamic system. The dynamic resonance fluorescence spectra with up to five pairs of side peaks, excitation detuning induced spectral asymmetry, and cavity filtering effect are observed and quantitatively modeled by a full quantum model with phonon scattering included. Time-resolved measurements further reveal that the multiple side peaks originate from interference of the emission associated with different temporal positions of the excitation pulses. Our work facilitates the generation of a variety of exotic quantum states of light with dynamic driving of two-level systems.
In this paper we derive a general expression for the emission rate of an emitter which is placed at the center of a real cavity drilled in a generic random medium. We apply our formalism to the computation of the decay rate of a single atom which seats within a small molecule embedded in a continuous medium.
Spontaneously generated coherence and enhanced dispersion in a V-type, three-level atomic system interacting with a single mode field can considerably reduce the radiative and cavity decay rates. This may eliminate the use of high finesse, miniaturized cavities in optical cavity quantum electrodynamics experiments under strong atom-field coupling conditions.
Coherent light-matter interaction at the single photon and electronic qubit level promises the remarkable potential for nonclassical information processing. Against the efforts of improving the figure of merit of the cavities, here we demonstrate strong anharmonicity in the polariton dressed states via dark state resonances in a highly dissipative cavity. It is shown that vacuum Rabi oscillation occurs for a single quantum emitter inside a cavity even with bosonic decay-to-interaction rate ratio exceeding $10^{2}$, when the photon field is coupled to an auxiliary high-$Q$ cavity. Moreover, pho…
Optical nonlinearities sensitive to individual photons may be extremely useful as elements in quantum logic circuits for photonic qubits. A much cited example is the work of Turchette et al. [Phys. Rev. Lett. 75, 4710 (1995)], in which a phase shift of about 10 degrees was reported. To improve this result, we propose a single sided cavity geometry with minimal cavity losses. It should then be possible to achieve a nonlinear phase shift of 180 degrees.
A cavity-modified master equation is derived for a coherently driven, V-type three-level atom coupled to a single-mode cavity in the bad cavity limit. We show that population inversion in both the bare and dressed-state bases may be achieved, originating from the enhancement of the atom-cavity interaction when the cavity is resonant with an atomic dressed-state transition. The atomic populations in the dressed state representation are analysed in terms of the cavity-modified transition rates. The atomic fluorescence spectrum and probe absorption spectrum also investigated, and it is found that…
We experimentally realize a Fabry-Perot-type optical microresonator near the cesium D2 line wavelength based on a tapered optical fiber, equipped with two fiber Bragg gratings which enclose a sub-wavelength diameter waist. Owing to the very low taper losses, the finesse of the resonator reaches F = 86 while the on-resonance transmission is T = 11 %. The characteristics of our resonator fulfill the requirements of non-linear optics and cavity quantum electrodynamics in the strong coupling regime. In combination with its demonstrated ease of use and its advantageous mode geometry, it thus opens …
Photon correlations are investigated for a single laser-excited ion trapped in front of a mirror. Varying the relative distance between the ion and the mirror, photon correlation statistics can be tuned smoothly from an antibunching minimum to a bunching-like maximum. Our analysis concerns the non-Markovian regime of the ion-mirror interaction and reveals the field establishment in a half-cavity interferometer.
We demonstrate the fabrication of ultra-low-loss, all-fiber Fabry-Pérot cavities containing a nanofiber section, optimized for cavity quantum electrodynamics. By continuously monitoring the finesse and fiber radius during fabrication of a nanofiber between two fiber Bragg gratings, we are able to precisely evaluate taper transmission as a function of radius. The resulting cavities have an internal round-trip loss of only 0.31% at a nanofiber waist radius of 207 nm, with a total finesse of 1380, and a maximum expected internal cooperativity of $\sim$ 1050 for a cesium atom on the nanofiber surf…
We present an all-fiber emitter-cavity quantum electrodynamics (QED) system which consists of two two-level emitters and a nanofiber cavity. Our scheme makes it possible to observe the higher-order exceptional points based on the coupling between the emitters and the nanofiber cavity. The effective gain of this cavity can be obtained by weakly driven to the nanofiber cavity via two identical laser fields, which will realize coherent perfect absorption (CPA) in the implementation of the experiments. Under the experimental feasible parameters, the Hamiltonian of this system is in the condition o…
We experimentally studied the microwave response of a transmon artificial atom coupled to two closely spaced resonant modes. When the atom is under driven with one of the modes, the atom state and mode photons are superposed, forming the dressed states. Dressed states with 1st, 2nd and 3rd excited states of the atom were prepared and probed via the strong coupling to the other resonant mode from the point of view of cavity quantum electrodynamics. The transmission of the probe tone is modulated by the driving microwave amplitude, displaying multi-photon process associated with the inter-atomic…
The time-resolved physical spectrum of luminescence is theoretically studied for a standard cavity quantum electrodynamics system. In contrast to the power spectrum for the steady state, the correlation functions up to the present time are crucial for the construction of the time-resolved spectrum, while the correlations with future quantities are inaccessible because of the causality, i.e., the future quantities cannot be measured until the future comes. We find that this causality plays a key role to understand the time-resolved spectrum, in which the Rabi doublet can never be seen during th…
Cavity quantum electrodynamics studies light-matter interactions at single quanta level. Chiral photon-emitter coupling in photonic structures is characterized as unidirectional propagation locked by the local polarization of light. However, to realize the strong interaction of photon-emitter with direction-locked propagation, which will bring novel applications in nonreciprocal quantum devices, has not been reported yet. Here, we propose the coupled photonic crystal and metallic nanoparticle structure, where through strong local field with high helicity, the rate of circularly polarized photo…
We present a study of collective multi-photon blockade in coherently driven atoms in a single mode cavity. Considering two atoms strongly coupled to an optical cavity, we show that the two-photon blockade with two-photon anti-bunching, and the three-photon blockade with three-photon anti-bunching can be observed simultaneously. The three-photon blockade probes both dressed states in the two photon and three photon spaces. The two photon and three photon blockades strongly depend on the location of two atoms in the strong coupling regime. The asymmetry in the atom-cavity coupling constants open…
In this article we discuss a scheme of teleportation of atomic states. The experimental realization proposed makes use of cavity Quatum Electrodynamics involving the interaction of Rydberg atoms with a micromaser cavity prepared in a coherent state. We start presenting a scheme to prepare atomic Bell states via the interaction of atoms with a cavity. In our scheme the cavity and some atoms play the role of auxiliary systems used to achieve the teleportation.
We propose an experimentally feasible scheme to realize the nonlocal gate between two different quantum network nodes. With an entanglement-qubit (ebit) acts as a quantum channel, our scheme is resistive to actual environment noise and can get high fidelity in current cavity quantum electrodynamics (C-QED) system.
We study universal quantum computation in the cavity quantum electrodynamics (CQED) framework exploiting two orthonormal two-photon generalized binomial states as qubit and dispersive interactions of Rydberg atoms with high-$Q$ cavities. We show that an arbitrary qubit state may be generated and that controlled-NOT and 1-qubit rotation gates can be realized via standard atom-cavity interactions.
It is shown that a broad class of cavity quantum electrodynamics (QED) problems - which consider the resonant propagation of a single photon interacting with quantum emitters (QEs), such as atoms, quantum dots, or vacancy centers - can be solved directly without application of the second quantization formalism. In the developed approach, the Hamiltonian is expressed through the ket-bra products of collective (photon + cavities + QEs) states. Consequently, the S-matrix of input-output problems is determined exactly by the Mahaux-Weidenmüller formula, which dramatically simplifies the analysis o…
In this letter we present a scheme for the implementation of frequency up- and down-conversion operations in two-mode cavity quantum electrodynamics (QED). This protocol for engineering bilinear two-mode interactions could enlarge perspectives for quantum information manipulation and also be employed for fundamental tests of quantum theory in cavity QED. As an application we show how to generate a two-mode squeezed state in cavity QED (the original entangled state of Einstein-Podolsky-Rosen).
We theoretically demonstrate the enhanced and dephasing immune squeezing in the resonance fluorescence of a single quantum dot (QD) confined to a pillar-microcavity and driven by a continuous wave laser. We employ a formalism based on Polaron master equation theory for incorporating the influence of exciton-phonon coupling quite accurately in the dot-cavity system. We show a significant enhancement of squeezing due to cavity coupling of the QD as compared to that of an ideal single two-level system in free space. Particularly, we show a four-fold enhancement in squeezing as compared to that of…
We present a supervised learning model to calibrate the photon collection rate during the fluorescence imaging of cold atoms. The linear regression model finds the collection rate at each location on the sensor such that the atomic population difference equals that of a highly precise optical cavity measurement. This 192 variable regression results in a measurement variance 27% smaller than our previous single variable regression calibration. The measurement variance is now in agreement with the theoretical limit due to other known noise sources. This model efficiently trains in less than a mi…
This work provides the fundamental theoretical framework for the molecular cavity Quantum Electrodynamics by resolving the gauge ambiguities between the Coulomb gauge and the dipole gauge Hamiltonian under the electronic state truncation. Our conjecture for the arising of such gauge ambiguity is that not all operators are properly constrained in the truncated electronic subspace. Based upon this conjecture, we construct a unitary transformation that properly constrains all operators in the subspace, and derive an equivalent and yet convenient expression for the Coulomb gauge Hamiltonian under …
In this work we show how to engineer bilinear and quadratic Hamiltonians in cavity quantum electrodynamics (QED) through the interaction of a single driven two-level atom with cavity modes. The validity of the engineered Hamiltonians is numerically analyzed even considering the effects of both dissipative mechanisms, the cavity field and the atom. The present scheme can be used, in both optical and microwave regimes, for quantum state preparation, the implementation of quantum logical operations, and fundamental tests of quantum theory.
Semiconductor quantum dots embedded in micro-pillar cavities are excellent emitters of single photons when pumped resonantly. Often, the same spatial mode is used to both resonantly excite a quantum dot and to collect the emitted single photons, requiring cross-polarization to reduce the uncoupled scattered laser light. This inherently reduces the source brightness to 50 %. Critically, for some quantum applications the total efficiency from generation to detection must be over 50 %. Here, we demonstrate a resonant-excitation approach to creating single photons that is free of any cross-polariz…
An Ab initio Framework for Simulating Ultrafast Nonlinear Cavity Quantum Electrodynamics Spectra
School of Science, Hangzhou Dianzi University（杭州电子科技大学理学院）；Graduate School of Computer and Information Sciences, Hosei University（法政大学计算机与信息科学研究生院）；Key laboratory of colloid and interface chemistry, School of Chemistry and Chemical Engineering, Shandong University（山东大学化学与化工学院胶体与界面化学重点实验室）
We demonstrate the remote all-optical control of the spontaneous emission (SE) of quantum dots using coupled photonic crystal cavities. By spectrally tuning a Fabry-Perot cavity in resonance with a target cavity, the quality factor and the local density of states experienced by emitters in the target cavity are modified, leading to a change in the SE rate. From the theoretical analysis of the coupled-cavity quantum electrodynamics system, the SE rate change can be higher than the quality factor change due to a reduction of the vacuum field at the emitter's position when the two cavities are br…
We describe the absorption by the walls of a quantum electrodynamics cavity as a process during which the elementary excitations (photons) of an internal mode of the cavity exit by tunneling through the cavity walls. We estimate by classical methods the survival time of a photon inside the cavity and the quality factor of its mirrors.
We propose a method to perform single-shot optical readout of a quantum bit (qubit) using cavity quantum electrodynamics. We selectively couple the optical transitions associated with different qubit basis states to the cavity, and utilize the change in cavity transmissivity to generate a qubit readout signal composed of many photons. We show that this approach enables single-shot optical readout even when the qubit does not have a good cycling transition required for standard resonance fluorescence measurements. We calculate the probability that the measurement detects the correct spin state …
Cavity quantum electrodynamic schemes for quantum gates are amongst the earliest quantum computing proposals. Despite continued progress, and the dramatic recent demonstration of photon blockade, there are still issues with optimal coupling and gate operation involving high-quality cavities. Here we show dynamic control techniques that allow scalable cavity-QED based quantum gates, that use the full bandwidth of the cavities. When applied to quantum gates, these techniques allow an order of magnitude increase in operating speed, and two orders of magnitude reduction in cavity Q, over passive c…
When ground state atoms are accelerated through a high Q microwave cavity, radiation is produced with an intensity which can exceed the intensity of Unruh acceleration radiation in free space by many orders of magnitude. The cavity field at steady state is described by a thermal density matrix under most conditions. However, under some conditions gain is possible, and when the atoms are injected in a regular fashion, the radiation can be produced in a squeezed state.
We calculate the fluorescence spectra of a driven lattice of coupled cavities. To do this, we extend methods of evaluating two-time correlations in infinite lattices to open quantum systems; this allows access to momentum resolved fluorescence spectrum. We illustrate this for a driven-dissipative transverse field anisotropic XY model. By studying the fluctuation dissipation theorem, we find the emergence of a quasi-thermalized steady state with a temperature dependent on system parameters; for blue detuned driving, we show this effective temperature is negative. In the low excitation density l…
We show that photon coincidence spectroscopy can provide an unambiguous signature of two atoms simultaneously interacting with a quantised cavity field mode. We also show that the single-atom Jaynes-Cummings model can be probed effectively via photon coincidence spectroscopy, even with deleterious contributions to the signal from two-atom events. In addition, we have explicitly solved the eigenvectors and eigenvalues of two two-level atoms coupled to a quantised cavity mode for differing coupling strengths.
Using a single circular Rydberg atom, we have prepared two modes of a superconducting cavity in a maximally entangled state. The two modes share a single photon. This entanglement is revealed by a second atom probing, after a delay, the correlations between the two modes. This experiment opens interesting perspectives for quantum information manipulation and fundamental tests of quantum theory.
We investigate the role of collective effects in the micromaser system as used in various studies of the physics of cavity electrodynamics. We focus our attention on the effect on large-time correlations due to multi-atom interactions. The influence of detection efficiencies and collective effects on the appearance of trapping states at low temperatures is also found to be of particular importance.
A major challenge in quantum optics and quantum information technology is to enhance the interaction between single photons and single quantum emitters. Highly engineered optical cavities are generally implemented requiring nanoscale fabrication precision. We demonstrate a fundamentally different approach in which disorder is used as a resource rather than a nuisance. We generate strongly confined Anderson-localized cavity modes by deliberately adding disorder to photonic crystal waveguides. The emission rate of a semiconductor quantum dot embedded in the waveguide is enhanced by a factor of 1…
A large payload quantum steganography protocol based on cavity quantum electrodynamics (QED) is presented in the paper, which effectively uses the evolution law of atom in cavity QED. The protocol builds up hidden channel to transmit secret messages using entanglement swapping between one GHZ state and one Bell state in cavity QED together with the Hadamard operation. The quantum steganography protocol is insensitive to cavity decay and thermal field. The capacity, imperceptibility and security against eavesdropping are analyzed in detail in the protocol. It turns out that the protocol not onl…
We construct a model which describes a recently performed experiment (Phys. Rev. A 64, 050301(R) (2001)) in which an entangled state between two modes of a single cavity is built. Environmental effects are taken into account and the results agree with the experimental findings. Moreover the model predicts, for different conditions of the same experiment, a decoherence-free subspace. These conditions are analyzed and slightly different experiments suggested in order to test its viability.
We present a new approach to incorporate self-assembled quantum dots into a Fabry-Pérot-like microcavity. Thereby a 3$λ$/4 GaAs layer containing quantum dots is epitaxially removed and attached by van der Waals bonding to one of the microcavity mirrors. We reach a finesse as high as 4,100 with this configuration limited by the reflectivity of the dielectric mirrors and not by scattering at the semiconductor - mirror interface, demonstrating that the epitaxial lift-off procedure is a promising procedure for cavity quantum electrodynamics in the solid state. As a first step in this direction, we…
We demonstrate the effects of cavity quantum electrodynamics for a quantum dot coupled to a photonic molecule, consisting of a pair of coupled photonic crystal cavities. We show anti-crossing between the quantum dot and the two super-modes of the photonic molecule, signifying achievement of the strong coupling regime. From the anti-crossing data, we estimate the contributions of both mode-coupling and intrinsic detuning to the total detuning between the super-modes. Finally, we also show signatures of off-resonant cavity-cavity interaction in the photonic molecule.
We present a general framework for cavity quantum electrodynamics with strongly frequency-dependent mirrors. The method is applicable to a variety of reflectors exhibiting sharp internal resonances as can be realized, for example, with photonic-crystal mirrors or with two-dimensional atomic arrays around subradiant points. Our approach is based on a modification of the standard input--output formalism to explicitly include the dynamics of the mirror's internal resonance. We show how to directly extract the interaction tuning parameters from the comparison with classical transfer matrix theory …
We present coherent reflection spectroscopy on a charge and DC Stark tunable quantum dot embedded in a high-quality and externally mode-matched microcavity. The addition of an exciton to a single-electron charged quantum dot forms a trion that interacts with the microcavity just below strong coupling regime of cavity quantum electrodynamics. Such an integrated, monolithic system is a crucial step towards the implementation of scalable hybrid quantum information schemes that are based on an efficient interaction between a single photon and a confined electron spin.
In this paper we investigate the various aspects of noise and order in the micromaser system. In particular, we study the effect of adding fluctuations to the atom cavity transit time or to the atom-photon frequency detuning. By including such noise-producing mechanisms we study the probability and the joint probability for excited atoms to leave the cavity. The influence of such fluctuations on the phase structure of the micromaser as well as on the long-time atom correlation length is also discussed. We also derive the asymptotic form of micromaser observables.
We show the planned upgrade of a cavity QED experimental apparatus. The system consists of an optical cavity and an ensemble of ultracold $^{85}$Rb atoms coupled to its mode. We propose enhancements to both. First, we document the building process for a new cavity, with a planned finesse of $\sim$20000. We address problems of maintaining mirror integrity during mounting and improving vibration isolation. Second, we propose improvements to the cold atom source in order to achieve better optical pumping and control over the flux of atoms. We consider a 2-D optical molasses for atomic beam deflec…
We introduce a new scalable cavity quantum electrodynamics platform which can be used for quantum computing. This system is composed of coupled photonic crystal (PC) cavities which their modes lie on a Dirac cone in the whole super crystal band structure. Quantum information is stored in quantum dots that are positioned inside the cavities. We show if there is just one quantum dot in the system, energy as photon is exchanged between the quantum dot and the Dirac modes sinusoidally. Meanwhile the quantum dot becomes entangled with Dirac modes. If we insert more quantum dots into the system, the…
Squeezing of atomic resonance fluorescence is shown to be optimized by a properly designed environment, which can be realized by a quasi-resonant cavity. Optimal squeezing is achieved if the atomic coherence is maximized, corresponding to a pure atomic quantum state. The atomic-state purification is achieved by the backaction of the cavity field on the atom, which increases the atomic coherence and decreases the atomic excitation. For realistic cavities, the coupling of the atom to the cavity field yields a purity of the atomic state of more than 99%. The fragility of squeezing against dephasi…
We introduce multiplexed atom-cavity quantum electrodynamics with an atomic ensemble coupled to a single optical cavity mode. Multiple Raman dressing beams establish cavity-coupled spin-wave excitations with distinctive spatial profiles. Experimentally, we demonstrate the concept by observing spin-wave vacuum Rabi splittings, selective superradiance, and interference in the cavity-mediated interactions of two spin waves. We highlight that the current experimental configuration allows rapid, interchangeable cavity-coupling to 4 profiles with an overlap parameter of less than 10%, enough to demo…
We introduce the quantum quincunx, which physically demonstrates the quantum walk and is analogous to Galton's quincunx for demonstrating the random walk. In contradistinction to the theoretical studies of quantum walks over orthogonal lattice states, we introduce quantum walks over nonorthogonal lattice states (specifically, coherent states on a circle) to demonstrate that the key features of a quantum walk are observable albeit for strict parameter ranges. A quantum quincunx may be realized with current cavity quantum electrodynamics capabilities, and precise control over decoherence in such…
We analytically derive the upper bound on the overall efficiency of single-photon generation based on cavity quantum electrodynamics (QED), where cavity internal loss is treated explicitly. The internal loss leads to a tradeoff relation between the internal generation efficiency and the escape efficiency, which results in a fundamental limit on the overall efficiency. The corresponding lower bound on the failure probability is expressed only with an "internal cooperativity," introduced here as the cooperativity parameter with respect to the cavity internal loss rate. The lower bound is obtaine…
We propose a Markovian quantum master equation that can describe the Fano effect directly, by assuming a standard cavity quantum electrodynamics system. The framework allows us to generalize the Fano formula, applicable over the weak and strong coupling regimes with pure dephasing. A formulation of its emission spectrum is also given in a consistent manner. We then find that the interference responsible for the Fano effect is robust against pure dephasing. This is counterintuitive because the impact of interference is, in general, severely reduced by decoherence processes. Our approach thus pr…
