The ability to detect single photons with high efficiency is a crucial requirement for various quantum information applications. By combining the storage process of a quantum memory for photons with fluorescence-based quantum state measurement, it is in principle possible to achieve high efficiency photon counting in large ensembles of atoms. The large number of atoms can, however, pose significant problems in terms of noise stemming from imperfect initial state preparation and off-resonant fluorescence. We propose a concrete implementation of a photon number resolving detector based on an ion Coulomb crystal inside a moderately high-finesse optical cavity. The cavity enhancement leads to an effective optical depth of 15 for a finesse of 3000 with only about 1500 ions interacting with the light field. We show that these values allow for essentially noiseless detection with an efficiency larger than 90%. Moderate experimental parameters allow for repetition rates of about 5 kHz, limited by the time needed for fluorescence collection. Potential applications are discussed.
We experimentally investigate the transient dynamics of an optical cavity field interacting with large ion Coulomb crystals in a situation of electromagnetically induced transparency (EIT). EIT is achieved by injecting a probe field at the single photon level and a more intense control field with opposite circular polarization into the same mode of an optical cavity to couple Zeeman substates of a metastable level in 40Ca+ ions. The EIT interaction dynamics are investigated both in the frequency-domain - by measuring the probe field steady state reflectivity spectrum - and in the time-domain -…
We report on the loading of large ion Coulomb crystals into a linear Paul trap incorporating a high-Finesse optical cavity (F~3200). We show that, even though the 3-mm diameter dielectric cavity mirrors are placed between the trap electrodes and separated by only 12 mm, it is possible to produce in situ ion Coulomb crystals containing more than 100.000 calcium ions of various isotopes and with lengths of up to several millimeters along the cavity axis. We show that the number of ions inside the cavity mode is in principle high enough to achieve strong collective coupling between the ion Coulom…
Quantum storage and retrieval of light in ion Coulomb crystals using cavity electromagnetically induced transparency is investigated theoretically. It is found that, when both the control and probe fields are coupled to the same cavity mode, their transverse mode profile affects the quantum memory efficiency in a non-trivial way. Under such conditions the control field parameters and crystal dimensions that maximize the memory efficiency are calculated.
We present an investigation of the coherent coupling of various transverse field modes of an optical cavity to ion Coulomb crystals. The obtained experimental results, which include the demonstration of identical collective coupling rates for different transverse modes of a cavity field to ions in the same large Coulomb crystal, are in excellent agreement with theoretical predictions. The results furthermore suggest that Coulomb crystals in the future may serve as near-ideal media for highfidelity multi-mode quantum information processing and communication purposes, including the generation an…
A detailed description and theoretical analysis of experiments achieving coherent coupling between an ion Coulomb crystal and an optical cavity field are presented. The various methods used to measure the coherent coupling rate between large ion Coulomb crystals in a linear quadrupole radiofrequency ion trap and a single field mode of a moderately high-finesse cavity are described in detail. Theoretical models based on a semiclassical approach are applied in assessment of the experimental results of [P. F. Herskind et al., Nature Phys. 5, 494 (2009)] and of complementary new measurements. Gene…
We demonstrate light-induced localization of Coulomb-interacting particles in multi-dimensional structures. Subwavelength localization of ions within small multi-dimensional Coulomb crystals by an intracavity optical standing wave field is evidenced by measuring the difference in scattering inside symmetrically red- and blue-detuned optical lattices and is observed even for ions undergoing substantial radial micromotion. These results are promising steps towards the structural control of ion Coulomb crystals by optical fields as well as for complex many-body simulations with ion crystals or fo…
Recent experiments have demonstrated that for a quantum dot in an optical resonator off-resonant cavity mode emission can occur even for detunings of the order of 10 meV. We show that Coulomb mediated Auger processes based on additional carriers in delocalized states can facilitate this far off-resonant emission. Using a novel theoretical approach for a non-perturbative treatment of the Auger-assisted quantum-dot carrier recombination, we present numerical calculations of the far off-resonant cavity feeding rate and cavity mean photon number confirming efficient coupling at higher densities of…
We resolve phonon number states in the spectrum of a superconducting qubit coupled to a multimode acoustic cavity. Crucial to this resolution is the sharp frequency dependence in the qubit-phonon interaction engineered by coupling the qubit to surface acoustic waves in two locations separated by $\sim40$ acoustic wavelengths. In analogy to double-slit diffraction, the resulting self-interference generates high-contrast frequency structure in the qubit-phonon interaction. We observe this frequency structure both in the coupling rate to multiple cavity modes and in the qubit spontaneous emission…
We report on a novel non-invasive method to determine the normal mode frequencies of ion Coulomb crystals in traps based on the resonance enhanced collective coupling between the electronic states of the ions and an optical cavity field at the single photon level. Excitations of the normal modes are observed through a Doppler broadening of the resonance. An excellent agreement with the predictions of a zero-temperature uniformly charged liquid plasma model is found. The technique opens up for investigations of the heating and damping of cold plasma modes, as well as the coupling between them.
The control of one light field by another, ultimately at the single photon level, is a challenging task which has numerous interesting applications within nonlinear optics and quantum information science. Due to the extremely weak direct interactions between optical photons in vacuum, this type of control can in practice only be achieved through highly nonlinear interactions within a medium. Electromagnetic induced transparency (EIT) constitutes one such means to obtain the extremely strong nonlinear coupling needed to facilitate interactions between two faint light fields. Here, we demonstrat…
We determine the optimal parameters for a simple and efficient scheme of dispersive readout of a qubit. Depending on the qubit state (ground or excited), the resonance of a cavity is shifted either to the red or to the blue side. Qubit state is inferred by detecting the photon number transmitted through the cavity. It turns out that this kind of detection provides better measurement fidelity than the detection of the presence or absence of photons only. We show that radiating the cavity on either of the frequencies it shifts to results in a suboptimal measurement. The optimal frequency of the …
The generalized pseudospectral method is employed to study spherical confinement in two simple Coulombic systems: (i) well celebrated and heavily studied H atom (ii) relatively less explored Hulthén potential. In both instances, arbitrary cavity size, as well as low and higher states are considered. Apart from bound state eigenvalues, eigenfunctions, expectation values, quite accurate estimates of the critical cage radius for H atom for all the 55 states corresponding to $n \leq 10$, are also examined. Some of the latter are better than previously reported values. Degeneracy and energy orderin…
We experimentally investigate the formation of subradiant atomic momentum states in Bose-Einstein condensates inside a recoil resolving optical ring resonator according to the theoretical proposal of Cola, Bigerni, and Piovella. The atoms are pumped from the side with laser light that contains two frequency components. They resonantly drive cavity assisted Raman transitions between three discreet atomic momentum states. Within a few hundred microseconds, the system evolves into a stationary subradiant state. In this state, the condensate develops two density gratings suitable to diffract the t…
We demonstrate phase and frequency stabilization of a diode laser at the thermal noise limit of a passive optical cavity. The system is compact and exploits a cavity design that reduces vibration sensitivity. The sub-Hz laser is characterized by comparison to a second independent system with similar fractional frequency stability (1 x 10-15 at 1 s). The laser is further characterized by resolving a 2 Hz wide, ultranarrow optical clock transition in ultracold strontium.
Our goal is to provide a new approach to the construction of geometry-induced entanglement between a pair of $Λ$ type atoms in a system consists of $N$ identical atoms by means of nonadiabatic quantum holonomies. By employing the quantum Zeno effect, we introduce a tripod type interaction Hamiltonian between two selected atoms trapped in an optical cavity, which allows arbitrary geometric entangling power. This would be a substantial step toward resolving the feasibility of realizing universal nonadiabatic holonomic entangling two-qubit gates.
We propose a scheme to modulate the entanglement between two oscillators separated in space via the squeezing cavity field generated by the optical parametric amplifier instead of injecting the squeezing field directly with the assistance of Coulomb interaction. We show that the Coulomb interaction between the oscillators is the essential reason for the existence of entanglement. Due to the gain of the optical parametric amplifier and the phase of the pump driving the optical parametric amplifier can simultaneously modulate the squeezing cavity field, the radiation pressure interaction between…
This work provides the fundamental theoretical framework for the molecular cavity Quantum Electrodynamics by resolving the gauge ambiguities between the Coulomb gauge and the dipole gauge Hamiltonian under the electronic state truncation. Our conjecture for the arising of such gauge ambiguity is that not all operators are properly constrained in the truncated electronic subspace. Based upon this conjecture, we construct a unitary transformation that properly constrains all operators in the subspace, and derive an equivalent and yet convenient expression for the Coulomb gauge Hamiltonian under …
Indistinguishable photons play a key role in quantum optical information technologies. We characterize the output of an ultra-bright photon-pair source using multi-particle tomography [R. B. A. Adamson et al., Phys. Rev. Lett. 98, 043601 (2007)] and separately identify coherent errors, decoherence, and distinguishability. We demonstrate generation of high-quality indistinguishable pairs and polarization NOON states with 99% fidelity to an ideal NOON state. Using a NOON state we perform a super-resolving angular measurement with 90% visibility.
We propose to build a bad cavity laser using forbidden transitions in large ensembles of cold ions that form a Coulomb crystal in a linear Paul trap. This laser might realize an active optical frequency standard able to serve as a local oscillator in next-generation optical clock schemes. In passive optical clocks, large ensembles of ions appear less promising, as they suffer from inhomogeneous broadening due to quadrupole interactions and micromotion-relates shifts. In bad cavity lasers however, the radiating dipoles can synchronize and generate stable and narrow-linewidth radiation. Furtherm…
The dynamics of cold trapped ions in a high-finesse resonator results from the interplay between the long-range Coulomb repulsion and the cavity-induced interactions. The latter are due to multiple scatterings of laser photons inside the cavity and become relevant when the laser pump is sufficiently strong to overcome photon decay. We study the stationary states of ions coupled with a mode of a standing-wave cavity as a function of the cavity and laser parameters, when the typical length scales of the two self-organizing processes, Coulomb crystallization and photon-mediated interactions, are …
We study the dynamics of a driven optomechanical cavity coupled to a charged nanomechanical resonator via Coulomb interaction, in which the tunable double optomechanically induced transparency (OMIT) can be observed from the output field at the probe frequency by controlling the strength of the Coulomb interaction. We calculate the splitting of the two transparency windows, which varies near linearly with the Coulomb coupling strength in a robust way against the cavity decay. Our double-OMIT is much different from previously mentioned double-EIT and can be applied to measure Coulomb coupling s…
We present a unified framework for studying Coulomb interactions in arbitrary environments using macroscopic quantum electrodynamics on the basis of the electromagnetic Green's function. Our theory can be used to derive the Coulomb potential of a single charged particle as well as that between two charges in the presence of media, bodies and interfaces of arbitrary shapes. To demonstrate this, we reproduce the well-known screened Coulomb force, account for local-field effects and consider new cases such as a dielectric cavity and a conducting plate with a hole.
We generalize the Power-Zineau-Woolley transformation to obtain a canonical Hamiltonian of cavity quantum electrodynamics for arbitrary geometry of boundaries. This Hamiltonian is free from the A-square term and the instantaneous Coulomb interaction between distinct atoms. The single-mode models of cavity QED (Dicke, Tavis-Cummings, Jaynes-Cummings) are justified by a term by term mapping to the proposed microscopic Hamiltonian. As one straightforward consequence, the basis of no-go argumentations concerning the Dicke phase transition with atoms in electromagnetic fields dissolves.
The transmission of a probe field experiencing electromagnetically induced transparency and optical switching in an atomic medium enclosed in an optical cavity is investigated. Using a semiclassical input-output theory for the interaction between an ensemble of four-level atoms and three optical cavity fields coupled to the same spatial cavity mode, we derive the steady-state transmission spectra of the probe field and discuss the dynamics of the intracavity field buildup. The analytical and numerical results are in good agreement with recent experiments with ion Coulomb crystals [M. Albert et…
Microscopic simulations of the coupled dynamics of cavity photons, excitons, and biexcitons
Institute for Photonic Quantum Systems (PhoQS), Paderborn University（帕德博恩大学光子量子系统研究所）；Department of Physics and Center for Optoelectronics and Photonics Paderborn (CeOPP), Paderborn University（帕德博恩大学物理系与光电光子学中心）；Wyant College of Optical Sciences, University of Arizona（亚利桑那大学怀特光学学院）
We study the dynamics of a driven optomechanical cavity coupled to a charged nanomechanical resonator via Coulomb interaction. We find the tunable switch between slow-and fast- light in double-mode can be observed from the output field by adjusting the laser-cavity detuning in this coupled system. Moreover, the requencies of signal light can be tuned by Coulomb coupling strength. The proposal may have potential application in optical communcation and nonlinear optics.
An excited two-atom system can decay via different competing relaxation processes. If the excess energy is sufficiently high the system may not only relax via spontaneous emission but can also undergo interatomic Coulombic decay (ICD) or even Auger decay. We provide analytical expressions for the rates by including them into the same quantum optical framework on the basis of macroscopic quantum electrodynamics. By comparing the rates in free space we derive the atomic properties determining which decay channel dominates the relaxation. We show that by modifying the excitation propagation of th…
Realizing quantum mechanical behavior in micro- and nanomechanical resonators has attracted continuous research effort. One of the ways for observing quantum nature of mechanical objects is via the mechanism of phonon blockade. Here, we show that phonon blockade could be achieved in a system of two weakly nonlinear mechanical resonators coupled by a Coulomb interaction. The optimal blockade arises as a result of the destructive quantum interference between paths leading to two-phonon excitation. It is observed that, in comparison to a single drive applied on one mechanical resonator, driving b…
Dissipative generation of spin squeezing in the resolved vacuum Rabi splitting limit
JILA, University of Colorado and National Institute of Standards and Technology（科罗拉多大学与美国国家标准与技术研究院联合JILA研究所）；Department of Physics, University of Colorado（科罗拉多大学物理系）；Center for Theory of Quantum Matter, University of Colorado（科罗拉多大学量子物质理论中心）；T.C.M. Group, Cavendish Laboratory, University of Cambridge（剑桥大学卡文迪许实验室TCM小组）；Institute of Physics（物理研究所）
A quantum dipole interacting with an optical cavity is one of the key models in cavity quantum electrodynamics (cavity-QED). To treat this system theoretically, the typical approach is to truncate the dipole to two levels. However, it has been shown that in the ultrastrong-coupling regime, this truncation naively destroys gauge invariance. By truncating in a manner consistent with the gauge principle, we introduce master equations {for open systems} to compute gauge-invariant emission spectra, photon flux rates, and quantum correlation functions which show significant disagreement with previou…
Electromagnetic signals are always composed of photons, though in the circuit domain those signals are carried as voltages and currents on wires, and the discreteness of the photon's energy is usually not evident. However, by coupling a superconducting qubit to signals on a microwave transmission line, it is possible to construct an integrated circuit where the presence or absence of even a single photon can have a dramatic effect. This system is called circuit quantum electrodynamics (QED) because it is the circuit equivalent of the atom-photon interaction in cavity QED. Previously, circuit Q…
We propose an all optical quantum computation scheme, with trapped electron spin qubits, using their Coulomb exchange interaction with optically excited microcavity exciton-polaritons. This paper describes a single qubit rotation, which together with two-qubit controlled-z gate presented in PRB 85, 241403(R) (2012), form a set of universal logic gates. The errors due to finite cavity lifetime and incorrect orientation of the rotation axis are minimized by optimizing pump pulse parameters. With projective homodyne phase measurement and initialization, our scheme is a promising candidate for the…
Resonant excitation of atoms and ions in macroscopic cavities has lead to exceptional control over quanta of light. Translating these advantages into the solid state with emitters in microcavities promises revolutionary quantum technologies in information processing and metrology. Key is resonant optical reading and writing from the emitter-cavity system. However, it has been widely expected that the reflection of a resonant laser from a micro-fabricated wavelength-sized cavity would dominate any quantum signal. Here we demonstrate coherent photon scattering from a quantum dot in a micro-pilla…
We describe a design to implement a two-qubit geometric phase gate, by which a pair of electrons confined in adjacent quantum dots are entangled. The entanglement is a result of the Coulomb exchange interaction between the optically excited exciton-polaritons and the localized spins. This optical coupling, resembling the electron-electron Ruderman-Kittel-Kasuya-Yosida (RKKY) inter- actions, offers high speed, high fidelity two-qubit gate operation with moderate cavity quality factor Q. The errors due to the finite lifetime of the polaritons can be minimized by optimizing the optical pulse para…
Time- and number-resolved photon detection is crucial for photonic quantum information processing. Existing photon-number-resolving (PNR) detectors usually have limited timing and dark-count performance or require complex fabrication and operation. Here we demonstrate a PNR detector at telecommunication wavelengths based on a single superconducting nanowire with an integrated impedance-matching taper. The prototyping device was able to resolve up to five absorbed photons and had 16.1 ps timing jitter, <2 c.p.s. device dark count rate, $\sim$86 ns reset time, and 5.6% system detection efficienc…
We analyze the dynamics of a chain of singly-charged ions confined in a linear Paul trap and which couple with the mode of a high-finesse optical resonator. In these settings the ions interact via the Coulomb repulsion and are subject to the mechanical forces due to scattering of cavity photons. We show that the interplay of these interactions can give rise to bistable equilibrium configurations, into which the chain can be cooled by cavity-enhanced photon scattering. We characterize the resulting equilibrium structures by determining the stationary state in the semiclassical limit for both ca…
Collective excitation modes in solid state systems play a central role in circuit quantum electrodynamics, cavity optomechanics, and quantum magnonics. In the latter, quanta of collective excitation modes in a ferromagnet, called magnons, interact with qubits to provide the nonlinearity necessary to access quantum phenomena in magnonics. A key ingredient for future quantum magnonics systems is the ability to probe magnon states. Here we observe individual magnons in a millimeter-sized ferromagnet coherently coupled to a superconducting qubit. Specifically, we resolve magnon number states in sp…
A complex quantum system can be constructed by coupling simple quantum elements to one another. For example, trapped-ion or superconducting quantum bits may be coupled by Coulomb interactions, mediated by the exchange of virtual photons. Alternatively quantum objects can be coupled by the exchange of real photons, particularly when driven within resonators that amplify interactions with a single electro-magnetic mode. However, in such an open system, the capacity of a coupling channel to convey quantum information or generate entanglement may be compromised. Here, we realize phase-coherent int…
Heisenberg's uncertainty principle results in one of the strangest quantum behaviors: an oscillator can never truly be at rest. Even in its lowest energy state, at a temperature of absolute zero, its position and momentum are still subject to quantum fluctuations. Resolving these fluctuations using linear position measurements is complicated by the fact that classical noise can masquerade as quantum noise. On the other hand, direct energy detection of the oscillator in its ground state makes it appear motionless. So how can we resolve quantum fluctuations? Here, we parametrically couple a micr…
A tunable double optomechanically induced transparency (OMIT) with a squeezed field is investigated in a system consisting of an optomechanical cavity coupled to a charged nanomechanical resonator via Coulomb interaction. Such a double OMIT can be achieved by adjusting the strength of the Coulomb interaction, and observed even with a single-photon squeezed field at finite temperature. Since it is robust against the cavity decay, but very sensitive to some parameters, such as the environmental temperature, the model under our consideration can be applied as a quantum thermometer for precision m…
The structure of solids and their phases is mainly determined by static Coulomb forces while the coupling of charges to the dynamical, i.e., quantized degrees of freedom of the electromagnetic field plays only a secondary role. Recently, it has been speculated that this general rule can be overcome in the context of cavity quantum electrodynamics (QED), where the coupling of dipoles to a single field mode can be dramatically enhanced. Here we present a first exact analysis of the ground states of a dipolar cavity QED system in the non-perturbative coupling regime, where electrostatic and dynam…
We demonstrate a general technique to achieve a precise radial displacement of the nodal line of the radiofrequency (rf) field in a linear Paul trap. The technique relies on selective adjustment of the load capacitance of the trap electrodes, achieved through the addition of capacitors to the basic resonant rf-circuit used to drive the trap. Displacements of up to 100 micrometer with micrometer precision are measured using a combination of fluorescence images of ion Coulomb crystals and coherent coupling of such crystals to a mode of an optical cavity. The displacements are made without measur…
Mediated photon-photon interactions are realized in a superconducting coplanar waveguide cavity coupled to a superconducting charge qubit. These non-resonant interactions blockade the transmission of photons through the cavity. This so-called dispersive photon blockade is characterized by measuring the total transmitted power while varying the energy spectrum of the photons incident on the cavity. A staircase with four distinct steps is observed and can be understood in an analogy with electron transport and the Coulomb blockade in quantum dots. This work differs from previous efforts in that …
The problem of on-demand generation of entanglement between single-atom qubits via a common photonic channel is examined within the framework of optical interferometry. As expected, for a Mach-Zehnder interferometer with coherent laser beam as input, a high-finesse optical cavity is required to overcome sensitivity to spontaneous emission. We show, however, that with a twin-Fock input, useful entanglement can in principle be created without cavity-enhancement. Both approaches require single-photon resolving detectors, and best results would be obtained by combining both cavity-feedback and twi…
The Jaynes-Cummings Hamiltonian is at the core of cavity quantum electrodynamics, and is ubiquitous in a variety of quantum technologies. The ability to implement and control the various aspects of this Hamiltonian is thus of paramount importance. However, conventional implementations relying on bound-electron systems are fundamentally limited by the Coulomb potential that bounds the electron, in addition to suffering from practical limitations such as requiring cryogenic temperatures for operation and fabrication inhomogeneity. In this work, we propose theoretically a new approach to realize …
We propose a scheme to perform single-shot quantum non-demolition (QND) readout of the spin of an electron trapped in a semiconductor quantum dot (QD). Our proposal relies on the interaction of the QD electron spin with optically excited, quantum well (QW) microcavity exciton-polaritons. The spin-dependent Coulomb exchange interaction between the QD electron and cavity polaritons causes the phase and intensity response of left circularly polarized light to be different to that of the right circularly polarized light, in such a way that the QD electron's spin can be inferred from the response t…
We demonstrate that a very recently obtained formula for the force on a slab in a material planar cavity based on the calculation of the vacuum Lorentz force [C. Raabe and D.-G. Welsch, Phys. Rev. A 71, 013814 (2005)] describes a (medium) screened Casimir force and, in addition to it, a medium-assisted force. The latter force also describes the force on the cavity medium. For dilute media, it implies the atom-mirror interaction of the Casimir-Polder type at large and of the Coulomb type at small atom-mirror distances of which the sign is insensitive to the polarizability type (electric or magn…
We apply a microscopic theory of exciton-polaritons in cavity-confined monolayer transition-metal dichalcogenides including both optical polarizations in the monolayer plane, allowing to describe how chiral cavity photons interact with the valley degrees of freedom of the active material. Upon polariton formation, the degenerate excitons inhabiting the two inequivalent valleys are shown to assume bonding and antibonding superpositions as a result of cavity-mediated intravalley interactions combined with intervalley Coulomb interactions. This is representative of a polariton-induced coherent mi…
