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arXiv 2301.03061quant-ph
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J=1/2-J'=1/2原子系统共振荧光中的量子干涉:量子拍、非经典性与非高斯性

Quantum interference in the resonance fluorescence of a $J=1/2$-$J'=1/2$ atomic system: Quantum beats, nonclassicality, and non-Gaussianity

H. M. Castro-Beltrán, O. de los Santos-Sánchez, L. Gutiérrez, A. D. Alcantar-Vidal

AI总结:

本文研究J=1/2-J'=1/2原子系统在激光驱动下由π跃迁量子干涉产生的共振荧光,揭示量子拍、非经典性与非高斯性,并分析其光谱和关联特征。

摘要:

我们从理论上研究了一个角动量为 J=1/2 - J'=1/2 的单原子或系统在单色线偏振激光场驱动下共振荧光的量子统计和光谱性质,这种性质源于其两个反平行的 π 跃迁之间的量子干涉。施加一个平行于激光偏振方向的磁场以解除简并(Zeeman 效应)。在非简并情况下,π 跃迁以不同的广义 Rabi 频率演化,在强度以及偶极-偶极、强度-强度和正交分量-强度关联中产生量子拍。对于强激光和大的 Zeeman 分裂,拍的平均频率和调制频率分别由 Rabi 频率的平均值和差值给出,这与许多光谱系统中所研究的拍不同,后者表现为调制指数式衰减。此外,这些 Rabi 频率正是该系统 Mollow 型光谱中各对边带的频率。在双时关联中,交叉贡献,即两个 π 跃迁概率幅乘积的项,其作用小于来自概率密度干涉的项。相比之下,总强度中没有交叉项。我们还考虑了相位依赖荧光在弱至中等激发以及拍区情况下的非经典和非高斯性质。拍区中的荧光是非经典的,主要来自三阶偶极涨落,这些涨落表明其也具有很强的非高斯性,并且它们的正交分量光谱在 Rabi 频率附近显示出复杂特征。对于小的激光和 Zeeman 失谐,弱至中等激光场将系统部分泵浦到其中一个基态,在双时关联中表现出缓慢衰减,并在正交分量光谱中出现窄峰。

英文摘要:

We study theoretically quantum statistical and spectral properties of the resonance fluorescence of a single atom or system with angular momentum $J=1/2 - J'=1/2$ driven by a monochromatic linearly polarized laser field, due to quantum interference among its two antiparallel, $π$ transitions. A magnetic field parallel to the laser polarization is applied to break the degeneracy (Zeeman effect). In the nondegenerate case, the $π$ transitions evolve at different generalized Rabi frequencies, producing quantum beats in the intensity and the dipole-dipole, intensity-intensity, and quadrature-intensity correlations. For a strong laser and large Zeeman splitting the beats have mean and modulation frequencies given by the average and difference, respectively, of the Rabi frequencies, unlike thebeats studied in many spectroscopic systems, characterized by a modulated exponential-like decay. Further, the Rabi frequencies are those of the pairs of sidebands of the Mollow-like spectrum of the system. In the two-time correlations, the cross contributions, i.e., those with products of probability amplitudes of the two $π$ transitions, have a lesser role than those from the interference of the probability densities. In contrast, there are no cross terms in the total intensity. We also consider nonclassical and non-Gaussian properties of the phase-dependent fluorescence for the cases of weak to moderate excitation and in the regime of beats. The fluorescence in the beats regime is nonclassical, mainly from third-order dipole fluctuations, which reveal them to be also strongly non-Gaussian, and their quadrature spectra show complex features around the Rabi frequencies. For small laser and Zeeman detunings, a weak to moderate laser field pumps the system partially to one of the ground states, showing slow decay in the two time correlations and a narrow peak in the quadrature spectra.

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