We propose a method for producing on-demand single-photon states based on collision-induced exchanges of photons and unbalanced linear absorption between two single-mode light fields. These two effects result in an effective nonlinear absorption of photons in one of the modes, which can lead to single photon states. A quantum nonlinear attenuator based on such a mechanism can absorb photons in a normal input light pulse and terminate the absorption at a single-photon state. Because the output light pulses containing single photons preserve the properties of the input pulses, we expect this method to be a means for building a highly controllable single photon source.
For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon absorption can be substantially enhanced by adjusting the time correlation of photon pairs. We study two typical cases: Gaussian wavefunction and rectangular wavefunction. In the latter, we find that under special conditions one-photon transition is completely suppressed while the high probability of two-photon transition is maintained.
A solid state device to discriminate all the four Bell states is proposed. The device is composed of controlled absorption crystals, rotators, and retarders. The controlled absorption, where the state of one photon affects the absorption of the other photon, is realized by two photon absorption in a cubic crystal. The controlled absorption crystal detects a particular Bell state and is transparent for the other Bell states. The rotators and retarders transform a Bell state to another. This device may solve the problems in the early quantum teleportation experiments in photon polarization state…
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
We provide a compendium of the quantum mechanical equations for photon emission rates, photon absorption cross sections, and photon scattering cross sections. For each case, the different equations that apply for discrete or continuous electron states of the emitting, absorbing, or scattering material are given.
We propose a new method for generating photon pairs from coherent light using polarization-dependent two-photon absorption. We study the photon statistics of two orthogonally polarized modes by solving a master equation, and show that when we prepare a coherent state in one polarization mode, photon pairs are created in the other mode. The photon pairs have the same frequency as that of the incident light.
We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coi…
We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity regimes. In this paper we concentrate on continuous-wave excitation, although the approach we develop is more general. We calculate the energy removed from an incident field for typical experimental parameters and consider the limiting cases when the photon pairs are narrowband or broadband compared to the molecular linewidths. We find an enhancement of the tw…
We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered fiber and the relatively large overlap of the evanescent field with an atomic vapor that surrounds the tapered region. The two-photon absorption rate is optimized as a function of the diameter of the tapered region.
We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction increases the intensity associated with a single photon, while the two-photon absorption rate is further enhanced by the fact that the sum of the frequencies of the two photons is on resonance with the upper atomic state, even though each photon has a relatively broad linewidth. As a result, the photons are effectively confined in all three dimensions and the two-p…
In this paper we examine the N-photon absorption properties of "N00N" states, a subclass of path entangled number states. We consider two cases. The first involves the N-photon absorption properties of the ideal N00N state, one that does not include spectral information. We study how the N-photon absorption probability of this state scales with N. We compare this to the absorption probability of various other states. The second case is that of two-photon absorption for an N = 2 N00N state generated from a type II spontaneous down conversion event. In this situation we find that the absorption …
We have previously shown that two-photon absorption (TPA) and the quantum Zeno effect can be used to make deterministic quantum logic devices from an otherwise linear optical system. Here we show that this type of quantum Zeno gate can be used with additional two-photon absorbing media and weak laser pulses to make a heralded single photon source. A source of this kind is expected to have a number of practical advantages that make it well suited for large scale quantum information processing applications.
We propose a new type of attack on Ekert protocol in which, rather surprisingly, Eve drives a violation of Bell inequalities in Alice's and Bob's detectors with a mixture of separable states. She does so by sending correlated pulses containing several photons at frequencies where only multiple-photon absorptions are possible in their detectors. Whenever the photons stemming from a same pulse are dispatched in such a way that the number of photons is insufficient to trigger a multiple-photon absorption in either channel, the pulse remains undetected. We show that this simple feature leads to vi…
Recently, the photon absorption attracts lots of interest and plays an important role in a variety of applications. Here, we propose a valuable scheme to investigate the perfect photon absorption in a hybrid atom-optomechanical system both under and beyond the low-excitation limit. The perfect photon absorption persists both in the linear atomic excitation regime and nonlinear atomic excitation regime, below the threshold of the optical bistability/multistability, respectively. We also show that the optical nonlinearity raised by the nonlinear optomechanical interaction and nonlinear atomic ex…
Together with photon emission, the absorption of a single photon by a single atom is a fundamental process in matter-light interaction that manifests its quantum mechanical nature. As an experimentally controlled process, it is a key tool for the realization of quantum technologies. In particular, in an atom/photon based quantum network scenario, in which localized atomic particles are used as quantum information processing nodes while photons are used as carriers of quantum information between distant nodes, controlling both emission and absorption of single photons by single atoms is require…
The influence of the center of mass motion of a trapped two level system on efficient resonant single photon absorption is investigated. It is shown that this absorption process depends strongly on the ratio between the characteristic time scales of spontaneous photon emission and of the two level system's center of mass motion. In particular, if the spontaneous photon emission process occurs almost instantaneously on the time scale of the center of mass motion coherent control of the center of mass motion offers interesting perspectives for optimizing single photon absorption. It is demonstra…
We discuss how two-photon absorption (TPA) of squeezed and coherent states of light can be detected in measurements of the transmitted light fields. Such measurements typically suffer from competing loss mechanisms such as experimental imperfections and linear scattering losses inside the sample itself, which can lead to incorrect assessments of the two-photon absorption cross section. We evaluate the sensitivity with which TPA can be detected and find that TPA sensitivity of squeezed vacua or squeezed coherent states can become independent of linear losses at sufficiently large photon numbers…
Nonlinear optical effects can be enhanced in tapered optical fibers with diameters less than the wavelength of the propagating light. Here we report on the observation of two-photon absorption using tapered fibers in rubidium vapor at power levels of less than 150 nW. Transit-time broadening produces two-photon absorption spectra with sharp peaks that are very different from conventional line shapes.
As typically implemented, single photon sources cannot be made to produce single photons with high probability, while simultaneously suppressing the probability of yielding two or more photons. Because of this, single photon sources cannot really produce single photons on demand. We describe a multiplexed system that allows the probabilities of producing one and more photons to be adjusted independently, enabling a much better approximation of a source of single photons on demand.
In elaborating on the multiple-photon absorption attack on Ekert protocol proposed in arXiv:1011.4740, we show that it can be used in other entanglement-based protocols, in particular the BBM92 protocol. In this attack, the eavesdropper (Eve) is assumed to be in control of the source, and she sends pulses correlated in polarization (but not entangled) containing several photons at frequencies for which only multiple-photon absorptions are possible in Alice's and Bob's detectors. Whenever the photons stemming from one pulse are dispatched in such a way that the number of photons is insufficient…
The Tavis-Cummings model of N two-level atoms interacting with a single resonant mode is extended to various cases of off-resonance, initial photon densities, and atom number N. For stimulated absorption and small numbers of mean photon number a very unexpected results showing well defined rise and fall of oscillation is found.
Comparison of Spatial Entanglement between dissociated atom and ion : molecular ion photo-dissociated by sequential two-photon absorption and correlated two-photon absorption
Indian Association for the Cultivation of Science（印度科学培养印度协会）
We investigate conditions under which multiatom absorption of a single photon leads to cooperative decay. Our analysis reveals the symmetry properties of the multiatom Dicke states underlying the cooperative decay dynamics and their spatio-temporal manifestations, particularly, the forward-directed spontaneous emission investigated by Scully et al.
We present, characterize, and apply a photonic quantum interface between the near infrared and telecom spectral regions. A singly resonant optical parametric oscillator (OPO) operated below threshold, in combination with external filters, generates high-rate ($>2.5\cdot10^6~{\rm s}^{-1}$) narrowband photon pairs ($\sim 7$ MHz bandwidth); the signal photons are tuned to resonance with an atomic transition in Ca$^+$, while the idler photons are at telecom wavelength. Quantum interface operation is demonstrated through high-rate absorption of single photons by a single trapped ion ($\sim 670~{\rm…
We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and the maximum enhancement which can be achieved in comparison to the optimal classical pulse. We then adapt the optimization problem to realistic experimental constraints, where photon pairs from a down-conversion source are manipulated by local operations such as spatial light modulators. We derive optimal pulse shaping functions to enhance the absorption effi…
Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating fields of the same frequency. By concentrating in the limit of large detuning in one-photon transitions, we solve perturbatively the Bloch equations in a non-usual way. In this way we derive an analytical expression for the width of the two-photon resonance that makes evident sub-Doppler two--photon spectroscopy. We also derive an analytical expression for the …
Excitation with entangled photon pairs may lead to an increase in the efficiency of two-photon absorption at low photon flux. The corresponding process, entangled two-photon absorption (E2PA), has been investigated in numerous theoretical and experimental studies. However, significant ambiguity and inconsistency remain in the literature about the absolute values of E2PA cross-sections. Here, we use a fluorescence-based registration scheme to experimentally determine upper bounds on the cross-sections for six fluorophores. These bounds are up to four orders of magnitude lower than the smallest …
We describe a scheme that allows for the generation of any desired N-photon state on demand. Under ideal conditions, this requires only N single photon sources, laser pulses and linear optics elements. First, the sources should be initialised with the help of single-qubit rotations and repeat-until-success two-qubit quantum gates [Lim et al., Phys. Rev. Lett. 95, 030305 (2005)]. Afterwards, the state of the sources can be mapped onto the state of N newly generated photons whenever needed.
Spontaneous parametric down-conversion (SPDC) in a laser pumped optical nonlinear medium can produce heralded single photons with a high purity but a very low yield. Improving the yield by increasing the pump power in SPDC inevitably reduces the purity due to excitation of multi-photon events. We propose a scheme to overcome this purity-yield trade-off by suppressing multi-photon events in a cavity-enhanced SPDC via the photon blockade effect. By introducing a strong photon-photon interaction into the intracavity medium and increasing the pump power, we can improve the available single-photon …
In a recent work [Mod. Phys. Lett A13, p-1265 (1998)] we expounded a non-local Quantum Electrodynamics (QED) which predicted a linear two-photon absorption by an atom placed in a laser field of appropriate intensity and frequency. In this paper we extend our earlier work to show that the theory allows for linear 2n-photon absorption by gaseous matter where, under suitable conditions, n may literally run upto thousands. The consequences of this extension of the theory are outlined and predictions are made which may be verified in laboratories.
A pulsed laser scenario, designed to prepare an appropriately chosen self-assembled quantum dot with 100% population in a biexciton state, is proposed. The ensuing radiative emission would provide a near perfect (99.5%) high rate, on-demand, source of entangled photons.
When a low flux of time-frequency-entangled photon pairs (EPP) illuminates a two-photon transition, the rate of two-photon absorption (TPA) can be enhanced considerably by the quantum nature of photon number correlations and frequency correlations. We present a quantum-theoretic derivation of entangled TPA (ETPA) and calculate an upper bound on the amount of quantum enhancement that is possible in such systems. The derived bounds indicate that in order to observe ETPA the experiments would need to operate at a combination of significantly higher rates of EPP illumination, molecular concentrati…
We present a method to remove, using only linear optics, exactly one photon from a field-mode. This is achieved by putting the system in contact with an absorbing environment which is under continuous monitoring. A feedback mechanism then decouples the system from the environment as soon as the first photon is absorbed. We propose a possible scheme to implement this process and provide the theoretical tools to describe it.
While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can incr…
Semiconductor quantum dots embedded in optical cavities are promising on-demand sources of single photons. Here, we theoretically study single photon emission from an optically driven two-photon Raman transition between the biexciton and the ground state of a quantum dot. The advantage of this process is that it allows all-optical control of the properties of the emitted single photon with a laser pulse. However, with the presence of other decay channels and excitation-induced quantum interference, on-demand emission of the single Raman photon is generally difficult to achieve. Here we show th…
We theoretically investigate the dynamic interaction of a quantum dot in a nanocavity with timesymmetric single photon pulses. The simulations, based on a wavefunction approach, reveal that almost perfect single photon absorption occurs for quantum dot-cavity systems operating on the edge between strong and weak coupling regime. The computed maximum absorptions probability is close to unity for pulses with a typical length comparable to the half of the Rabi period. Furthermore, the dynamic control of the quantum dot energy via electric fields allows the freezing of the light-matter interaction…
We show how to capture a single photon of arbitrary temporal shape with one atom coupled to an optical cavity. Our model applies to Raman transitions in three-level atoms with one branch of the transition controlled by a (classical) laser pulse, and the other coupled to the cavity. Photons impinging on the cavity normally exhibit partial reflection, transmission, and/or absorption by the atom. Only a control pulse of suitable temporal shape ensures impedance matching throughout the pulse, which is necessary for complete state mapping from photon to atom. For most possible photon shapes, we der…
We study the dynamics of a system composed of two coupled cavities, each containing a single Rydberg atom. The interplay between Rydberg-Rydberg interaction and photon hopping enables the transition of the atoms from the collective ground state to the double Rydberg excitation state by individually interacting with the hybrid cavity modes and suppressing the up conversion process between them. The atomic transition is accompanied by the two-photon absorption and emission of the hybrid modes. Since the energy level structure of the atom-cavity system is photon number dependent, there is only a …
The emission and absorption of single photons by single atomic particles is a fundamental limit of matter-light interaction, manifesting its quantum mechanical nature. At the same time, as a controlled process it is a key enabling tool for quantum technologies, such as quantum optical information technology [1, 2] and quantum metrology [3, 4, 5, 6]. Controlling both emission and absorption will allow implementing quantum networking scenarios [1, 7, 8, 9], where photonic communication of quantum information is interfaced with its local processing in atoms. In studies of single-photon emission, …
Nonlinear spectroscopy and microscopy techniques are ubiquitous in a wide range of applications across physics and biology. However, these usually rely on high-powered pulsed laser systems. A promising alternative is to exploit entangled two-photon absorption (ETPA), which can lead to tens of orders of magnitude lower incident flux rates than in conventional two-photon absorption (TPA) schemes. However, the role of different entangled degrees of freedom in ETPA was unclear following recent experimental studies, when compared to earlier theoretical works. Here, we first demonstrate a linear dep…
By harnessing the quantum states of light for illumination, precise phase and absorption estimations can be achieved with precision beyond the standard quantum limit. Despite their significance for precision measurements, quantum states are fragile in noisy environments which leads to difficulties in revealing the quantum advantage. In this work, we propose a scheme to improve optical absorption estimation precision by using the correlated photon pairs from spontaneous parametric down-conversion as the illumination. This scheme performs better than clasical illumination when the loss is below …
Single photons from solid-state quantum emitters are playing a crucial role in the development of photonic quantum technologies. Higher order states, such as N-photon Fock-states allow for applications e.g. in quantum-enhanced sensing. In this study, we utilize the dispersion of a hot cesium vapor at the D1 lines to realize a temporal delay for one and two-photon Fock-states as a result of the slow-light effect. Single photons are generated on-demand from an InGaAs quantum dot, while their quantum interference at a beam splitter is used to generate a two-photon Fockstate. We verify the success…
Photonics offers a route to fast and distributed quantum computing in ambient conditions, provided that photon sources and logic gates can be operated deterministically. Quantum memories, capable of storing and re-emitting photons on demand, enable quasi-deterministic operations by synchronising stochastic events. We recently interfaced a Raman-type quantum memory with a travelling-wave heralded photon source. Here we discuss the trade-space for the spectral characteristics of such sources, and we present measurements of our source, which represents a practical compromise enabling passive stab…
We have previously shown that the quantum Zeno effect can be used to implement quantum logic gates for quantum computing applications, where the Zeno effect was produced using a strong two-photon absorbing medium. Here we show that the Zeno effect can also be used to implement classical logic gates whose inputs and outputs are high-intensity fields (coherent states). The operation of the devices can be understood using a quasi-static analysis, and their switching times are calculated using a dynamic approach. The two-photon absorption coefficient of rubidium vapor is shown to allow operation o…
We show that a three-level lambda quantum emitter with equal spontaneous emission rates on both optically active transitions can absorb an incident light field with a probability approaching unity, provided that the focused light profile matches that of the emitter dipole emission pattern. Even with realistic focusing geometries, our results could find applications in long-distance entanglement of spin qubits.
Using on-demand coherence conversion via optical locking in conventional stimulated (three-pulse) photon echoes, ultralong, ultraefficient photon storage has been observed in a rare-earth Pr3+ doped Y2SiO5, where storage time is several orders of magnitude longer and retrieval efficiency is enhanced by fifty times. Compared with the same method applied to two-pulse photon echoes for a rephasing halt, use of spectral grating in the stimulated photon echoes offers a phase-independent coherence conversion between optical and spin states. Eventually an ultralong spin population decay-dependent pho…
We consider a system consisting of a $Λ$-type atom and a V-type atom, which are individually trapped in two spatially separated cavities that are connected by an optical fibre. We show that an extremely entangled state of the two atoms can be deterministically generated through both photon emission of the $Λ$-type atom and photon absorption of the V-type atom in an ideal situation. The influence of various decoherence processes such as spontaneous emission and photon loss on the fidelity of the entangled state is also investigated. We find that the effect of photon leakage out of the fibre on …
We describe a practical implementation of a (semi-deterministic) photon gun based on stimulated Raman adiabatic passage pumping and the strong enhancement of the photonic density of states in a photonic band-gap material. We show that this device allows {\em deterministic} and {\em unidirectional} production of single photons with a high repetition rate of the order of 100kHz. We also discuss specific 3D photonic microstructure architectures in which our model can be realized and the feasibility of implementing such a device using ${Er}^{3+}$ ions that produce single photons at the telecommuni…
We propose two different setups to generate single photons on demand using an atom in front of a mirror, along with either a beam-splitter or a tunable coupling. We show that photon generation efficiency ~99% is straightforward to achieve. The proposed schemes are simple and easily tunable in frequency. The operation is relatively insensitive to dephasing and can be easily extended to generate correlated pairs of photons. They can also in principle be used to generate any photonic qubit of the form $μ|0 \rangle + ν|1\rangle$ in arbitrary wave-packets, making them very attractive for quantum co…
We measure the temperature dependence of the two-photon absorption and optical Kerr nonlinearity of a silicon waveguide over a range of temperatures from 5.5 to 300 K at a wavelength of 1.55 μm. The two-photon absorption coefficient is calculated from the power dependent transmission of a 4.9 ps pulse. We observed a nearly two-fold decrease in the two-photon absorption coefficient from 0.76 cm/GW at 300K to 0.42 cm/GW at 5.5 K. The Kerr nonlinearity is inferred from the self-phase modulation induced spectral broadening of the transmitted pulse. A smaller reduction in Kerr nonlinearity from 5.2…
We perform full time resolved tomographic measurements of the polarization state of pairs of photons emitted during the radiative cascade of the confined biexciton in a semiconductor quantum dot. The biexciton was deterministically initiated using a $π$-area pulse into the biexciton two-photon absorption resonance. Our measurements demonstrate that the polarization states of the emitted photon pair are maximally entangled. We show that the measured degree of entanglement depends solely on the temporal resolution by which the time difference between the emissions of the photon pair is determine…
Over the last several decades, quantum entanglement has been intensively studied for potential applications in quantum information science. Although intensive studies have progressed for nonlocal correlation, fundamental understanding of entanglement itself is still limited. Here, the quantum feature of anticorrelation, the so-called HOM dip, based on probabilistic entangled photon pairs is analyzed for its fundamental physics and compared with a new method of on-demand entangled photon pair generations using coherent light. The fundamental physics why there is no g^((1)) correlation in HOM di…
We present a theory for the diffraction of large molecules or nanoparticles at a standing light wave. Such particles can act as a genuine photon absorbers due to their numerous internal degrees of freedom effecting fast internal energy conversion. Our theory incorporates the interplay of three light-induced properties: the coherent phase modulation due to the dipole interaction, a non-unitary absorption-induced amplitude modulation described as a generalized measurement, and a coherent recoil splitting that resembles a quantum random walk in steps of the photon momentum. We discuss how these e…
We measured photon absorption in dielectric media and proposed the photon-version Beer-Lambert's law to quantify the absorption. We used a Hong-Ou-Mandel interferometer and 810 nm twin-photons. We found that the depth ratio of the null point in the interference patterns of the interferometer agreed with the classical transmittance of the samples. We established a statistical model of the photon absorption process and proposed an information entropy interpretation to understand the meaning of the Beer-Lambert law. Comparisons of the results of the photon absorption experiments with classical ex…
