We propose a new method for generating photon pairs from coherent light using polarization-dependent two-photon absorption. We study the photon statistics of two orthogonally polarized modes by solving a master equation, and show that when we prepare a coherent state in one polarization mode, photon pairs are created in the other mode. The photon pairs have the same frequency as that of the incident light.
For dissipation-free photon-photon interaction at the single photon level, we analyze one-photon transition and two-photon transition induced by photon pairs in three-level atoms using two-photon wavefunctions. We show that the two-photon absorption can be substantially enhanced by adjusting the time correlation of photon pairs. We study two typical cases: Gaussian wavefunction and rectangular wavefunction. In the latter, we find that under special conditions one-photon transition is completely suppressed while the high probability of two-photon transition is maintained.
We consider polarization states of three photons, each in the same given spectral-angular mode. A general form of such states is a superposition of four basic three-photon polarization modes, to be referred to as three-photon polarization ququarts. All such states can be considered as consisting of one- and two-photon parts, which can be entangled with each other. The degrees of entanglement and polarization as well as the Schmidt decomposition and Stokes vectors of three-photon polarization ququarts are found and discussed.
A solid state device to discriminate all the four Bell states is proposed. The device is composed of controlled absorption crystals, rotators, and retarders. The controlled absorption, where the state of one photon affects the absorption of the other photon, is realized by two photon absorption in a cubic crystal. The controlled absorption crystal detects a particular Bell state and is transparent for the other Bell states. The rotators and retarders transform a Bell state to another. This device may solve the problems in the early quantum teleportation experiments in photon polarization state…
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
Together with photon emission, the absorption of a single photon by a single atom is a fundamental process in matter-light interaction that manifests its quantum mechanical nature. As an experimentally controlled process, it is a key tool for the realization of quantum technologies. In particular, in an atom/photon based quantum network scenario, in which localized atomic particles are used as quantum information processing nodes while photons are used as carriers of quantum information between distant nodes, controlling both emission and absorption of single photons by single atoms is require…
We have investigated the excitation-power dependence of polarization-entangled photon-pairs generated from a CuCl single crystal using biexciton resonant hyper-parametric scattering. The measured two-photon polarization density matrix which corresponds to the two-photon polarization state changes with increasing the excitation power. The evaluation of the tangle and the linear entropy obtained from the measured density matrix indicates that the two-photon polarization density matrix can be expressed as the mixed state of an ideal state and a totally mixed state, and the mixture ratio of the to…
We provide a compendium of the quantum mechanical equations for photon emission rates, photon absorption cross sections, and photon scattering cross sections. For each case, the different equations that apply for discrete or continuous electron states of the emitting, absorbing, or scattering material are given.
A scheme to distinguish entangled two-photon-polarization states (ETP) from two independent entangled one-photon-polarization states (EOP) is proposed. Using this scheme, the experimental generation of ETP by parametric down-conversion is confirmed through the anti-correlations between three orthogonal two-photon-polarization states. The estimated fraction of ETP among the correlated photon pairs is 37% in the present experimental setup.
We report on a single-photon-to-single-atom interface, where a single photon generated by Spontaneous Parametric Down Conversion (SPDC) is absorbed by a single trapped ion. The photon is heralded by its time-correlated partner generated in the SPDC process, while the absorption event is heralded by a single photon emitted in its course. Coincidence detection marks doubly-heralded absorption, enabling photon-to-atom quantum state transfer [1, 2]. Background in the coincidence measurement is strongly suppressed by a new method that discriminates real absorption events from dark count-induced coi…
We propose a method for producing on-demand single-photon states based on collision-induced exchanges of photons and unbalanced linear absorption between two single-mode light fields. These two effects result in an effective nonlinear absorption of photons in one of the modes, which can lead to single photon states. A quantum nonlinear attenuator based on such a mechanism can absorb photons in a normal input light pulse and terminate the absorption at a single-photon state. Because the output light pulses containing single photons preserve the properties of the input pulses, we expect this met…
We present a theoretical analysis of two-photon absorption of classical and squeezed light valid when one-photon absorption to an intermediate state is either resonant or far-detuned from resonance, and in both the low and high intensity regimes. In this paper we concentrate on continuous-wave excitation, although the approach we develop is more general. We calculate the energy removed from an incident field for typical experimental parameters and consider the limiting cases when the photon pairs are narrowband or broadband compared to the molecular linewidths. We find an enhancement of the tw…
We analyze the rate of two-photon absorption in tapered optical fibers with diameters less than the wavelength of the incident light. The rate of two-photon absorption is shown to be enhanced due to the small mode volume of the tapered fiber and the relatively large overlap of the evanescent field with an atomic vapor that surrounds the tapered region. The two-photon absorption rate is optimized as a function of the diameter of the tapered region.
We calculate the rate of two-photon absorption for frequency entangled photons in a tapered optical fiber whose diameter is comparable to the wavelength of the light. The confinement of the electric field in the transverse direction increases the intensity associated with a single photon, while the two-photon absorption rate is further enhanced by the fact that the sum of the frequencies of the two photons is on resonance with the upper atomic state, even though each photon has a relatively broad linewidth. As a result, the photons are effectively confined in all three dimensions and the two-p…
In this paper we examine the N-photon absorption properties of "N00N" states, a subclass of path entangled number states. We consider two cases. The first involves the N-photon absorption properties of the ideal N00N state, one that does not include spectral information. We study how the N-photon absorption probability of this state scales with N. We compare this to the absorption probability of various other states. The second case is that of two-photon absorption for an N = 2 N00N state generated from a type II spontaneous down conversion event. In this situation we find that the absorption …
We have previously shown that two-photon absorption (TPA) and the quantum Zeno effect can be used to make deterministic quantum logic devices from an otherwise linear optical system. Here we show that this type of quantum Zeno gate can be used with additional two-photon absorbing media and weak laser pulses to make a heralded single photon source. A source of this kind is expected to have a number of practical advantages that make it well suited for large scale quantum information processing applications.
We present two-photon interference experiments with polarization-entangled photon pairs in a polarization-based Franson-type interferometer. Although the two photons do not meet at a common beamsplitter, a phase-insensitive Hong-Ou-Mandel type two-photon interference peak and dip fringes are observed, resulting from the two-photon interference effect between two indistinguishable two-photon probability amplitudes leading to a coincidence detection. A spatial quantum beating fringe is also measured for nondegenerate photon pairs in the same interferometer, although the two-photon states have no…
It is shown that a highly phase sensitive polarization squeezed (2n-1)-photon state can be generated by subtracting a diagonally polarized photon from the 2n photon component generated in collinear type II downconversion. This polarization wedge state has the interesting property that its photon number distribution in the horizontal and vertical polarizations remains sharply defined for phase shifts of up to 1/n between the circularly polarized components. Phase shifts at the Heisenberg limit are therefore observed as nearly deterministic transfers of a single photon between the horizontal and…
We propose a new type of attack on Ekert protocol in which, rather surprisingly, Eve drives a violation of Bell inequalities in Alice's and Bob's detectors with a mixture of separable states. She does so by sending correlated pulses containing several photons at frequencies where only multiple-photon absorptions are possible in their detectors. Whenever the photons stemming from a same pulse are dispatched in such a way that the number of photons is insufficient to trigger a multiple-photon absorption in either channel, the pulse remains undetected. We show that this simple feature leads to vi…
Recently, the photon absorption attracts lots of interest and plays an important role in a variety of applications. Here, we propose a valuable scheme to investigate the perfect photon absorption in a hybrid atom-optomechanical system both under and beyond the low-excitation limit. The perfect photon absorption persists both in the linear atomic excitation regime and nonlinear atomic excitation regime, below the threshold of the optical bistability/multistability, respectively. We also show that the optical nonlinearity raised by the nonlinear optomechanical interaction and nonlinear atomic ex…
We demonstrate negative polarization created by light-hole exciton excitation in g-factor engineered GaAs quantum wells measured by time-resolved Kerr rotation and polarization-resolved photoluminescence. This negative polarization is a result of polarization transfer from a photon to an electron spin mediated by a light hole. This demonstration is an important step towards achieving quantum media conversion from a photonic qubit to an electron spin qubit required for building a quantum repeater.
The influence of the center of mass motion of a trapped two level system on efficient resonant single photon absorption is investigated. It is shown that this absorption process depends strongly on the ratio between the characteristic time scales of spontaneous photon emission and of the two level system's center of mass motion. In particular, if the spontaneous photon emission process occurs almost instantaneously on the time scale of the center of mass motion coherent control of the center of mass motion offers interesting perspectives for optimizing single photon absorption. It is demonstra…
We discuss how two-photon absorption (TPA) of squeezed and coherent states of light can be detected in measurements of the transmitted light fields. Such measurements typically suffer from competing loss mechanisms such as experimental imperfections and linear scattering losses inside the sample itself, which can lead to incorrect assessments of the two-photon absorption cross section. We evaluate the sensitivity with which TPA can be detected and find that TPA sensitivity of squeezed vacua or squeezed coherent states can become independent of linear losses at sufficiently large photon numbers…
We investigate the quantum decoherence of frequency and polarization variables of photons via polarization mode dispersion in optical fibers. By observing the analogy between the propagation equation of the field and the Schrödinger equation, we develop a master equation under Markovian approximation and analytically solve for the field density matrix. We identify distinct decay behaviors for the polarization and frequency variables for single-photon and two-photon states. For the single photon case, purity functions indicate that complete decoherence for each variable is possible only for inf…
It is shown that the degree of polarization of light, generated by superposition in a single-photon interference experiment, may depend on the indistinguishability of the photon-paths.
We propose an integrated photonics device for mapping qubits encoded in the polarization of a photon onto the spin state of a solid-state defect coupled to a photonic crystal cavity: a `Polarization-Encoded Photon-to-Spin Interface' (PEPSI). We perform a theoretical analysis of the state fidelity's dependence on the device's polarization extinction ratio and atom-cavity cooperativity. Furthermore, we explore the rate-fidelity trade-off through analytical and numerical models. In simulation, we show that our design enables efficient, high fidelity photon-to-spin mapping.
The deterministic single-photon emission by means of STIRAP through the atoms with degenerate levels is studied. The expression for the polarization matrix of the emitted photon is obtained and its dependence on the polarization of the driving laser field and on the initial atomic state is examined.
Nonlinear optical effects can be enhanced in tapered optical fibers with diameters less than the wavelength of the propagating light. Here we report on the observation of two-photon absorption using tapered fibers in rubidium vapor at power levels of less than 150 nW. Transit-time broadening produces two-photon absorption spectra with sharp peaks that are very different from conventional line shapes.
We show that polarization entangled photons at x-ray energies can be generated via spontaneous parametric down conversion. Each of the four Bell states can be generated by choosing the angle of incidence and polarization of the pumping beam.
In this paper, the generation of polarization entangled photon pairs at 1.5 μm is experimentally demonstrated utilizing a polarization maintaining all-fiber loop, consisting of a piece of commercial polarization maintaining fiber and a polarization beam splitter/combiner with polarization maintaining fiber pigtails. A quantum state tomography measurement is performed to analyze the entanglement characteristic of the generated quantum state. In the experiment, a polarization entangled Bell state is generated with a entanglement fidelity of 0.97+/-0.03 and a purity of 0.94+/-0.03 demonstrating t…
Based on quantum mechanical approach the polarization transport of photons which propagate in a medium with slow varying refractive index is studied. The photon polarizations are separated in opposite directions normal to the ray which is called "Spin Hall effect" of photons, and also the rotation of polarization plane, a manifestation of the Berry phase, occurs. This approach can be generalized to other spinning particles in inhomogeneous media as a universal approach.
We experimentally investigate various quantum polarization features of three-photon quantum states, including product and entangled states with varying purity. The three-photon quantum states are categorized into six classes based on the rotation symmetry of mean, variance, and skewness of the polarization distribution. The representative three-photon quantum states in each category is prepared from double-pair emission from pulsed spontaneous parametric down-conversion and quantum interferometry. We demonstrate that the three-photon quantum states show interesting quantum polarization propert…
We propose a simple scheme for expanding a polarization-entangled W state. By mixing a single photon and one of the photons in an n-photon W state at a polarization-dependent beam splitter (PDBS), we can obtain an (n+1)-photon W state after post-selection. Our scheme also opens the door for generating n-photon W states using single photons and linear optics.
We demonstrate a simple, robust, and ultrabright parametric down-conversion source of polarization-entangled photons based on a polarization Sagnac interferometer. Bidirectional pumping in type-II phase-matched periodically poled KTiOPO4 yields a measured flux of 5 000 polarization-entangled pairs/s per mW of pump power in a 1-nm bandwidth at 96.8% quantum-interference visibility. The common-path arrangement of the Sagnac interferometer eliminates the need for phase stabilization for the biphoton output state.
We demonstrate a heralded quantum memory based on mapping of a photon polarization state onto a single collective-spin excitation (magnon) shared between two spatially overlapped atomic ensembles. The polarization fidelity is measured by quantum state tomography to be above 90(2)% for any input polarization, which far exceeds the classical limit of 2/3. The process also constitutes a quantum non-destructive probe that detects and regenerates a photon without touching its - potentially undetermined - polarization.
The generation of pulsed polarization entangled photon pair has been realized using type-I phase matching in the spontaneous parametirc downconversion process in a space cascaded two-crystal geometry. The optical axes of the crystal are aligned in such a way that the horizontal polarization photon pair is produced from up crystal, and the vertical polarization photon pair is produced from down crystal. These two processes are simultaneous, but are separable in space. We get the high entangled polarization photon pair by using the single mode fiber to erase the spatial information between these…
In elaborating on the multiple-photon absorption attack on Ekert protocol proposed in arXiv:1011.4740, we show that it can be used in other entanglement-based protocols, in particular the BBM92 protocol. In this attack, the eavesdropper (Eve) is assumed to be in control of the source, and she sends pulses correlated in polarization (but not entangled) containing several photons at frequencies for which only multiple-photon absorptions are possible in Alice's and Bob's detectors. Whenever the photons stemming from one pulse are dispatched in such a way that the number of photons is insufficient…
We demonstrate a fiber-based source of polarization-entangled photon pairs at visible wavelengths suitable for integration with local quantum processing schemes. The photons are created through birefringent phase-matching in spontaneous four-wave mixing inside a Sagnac interferometer. We address entanglement degradation due to temporal distinguishability of the photons to enable the generation of a spectrally unfiltered polarization-entangled photon-pair state with $95.86\pm0.10%$ fidelity to a maximally entangled Bell state, evaluated with a tomographic state reconstruction without applying a…
The Tavis-Cummings model of N two-level atoms interacting with a single resonant mode is extended to various cases of off-resonance, initial photon densities, and atom number N. For stimulated absorption and small numbers of mean photon number a very unexpected results showing well defined rise and fall of oscillation is found.
We propose a scheme to produce the maximally two photon polarization entangled state(EPR state) with single photon sources and the linear optics devices. In particular, our scheme requires the photon detectors only to distinguish the vacuum and non-vacuum Fock number states. A sophisticated photon detector distinguishing one or two photon states is unnecessary.
We study the quantum properties of the polarization of the light produced in type II spontaneous parametric down-conversion in the framework of a multi-mode model valid in any gain regime. We show that the the microscopic polarization entanglement of photon pairs survives in the high gain regime (multi-photon regime), in the form of nonclassical correlation of all the Stokes operators describing polarization degrees of freedom.
Comparison of Spatial Entanglement between dissociated atom and ion : molecular ion photo-dissociated by sequential two-photon absorption and correlated two-photon absorption
Indian Association for the Cultivation of Science（印度科学培养印度协会）
In the fluorescence light of a single atom, the probability for emission of a photon with certain polarization depends on the polarization of the photon emitted immediately before it. Here correlations of such kind are investigated with a single trapped calcium ion by means of second order correlation functions. A theoretical model is developed and fitted to the experimental data, which show 91% probability for the emission of polarization-correlated photon pairs within 24 ns.
We investigate conditions under which multiatom absorption of a single photon leads to cooperative decay. Our analysis reveals the symmetry properties of the multiatom Dicke states underlying the cooperative decay dynamics and their spatio-temporal manifestations, particularly, the forward-directed spontaneous emission investigated by Scully et al.
We present, characterize, and apply a photonic quantum interface between the near infrared and telecom spectral regions. A singly resonant optical parametric oscillator (OPO) operated below threshold, in combination with external filters, generates high-rate ($>2.5\cdot10^6~{\rm s}^{-1}$) narrowband photon pairs ($\sim 7$ MHz bandwidth); the signal photons are tuned to resonance with an atomic transition in Ca$^+$, while the idler photons are at telecom wavelength. Quantum interface operation is demonstrated through high-rate absorption of single photons by a single trapped ion ($\sim 670~{\rm…
Joint probability distributions of photon polarization correlations are computed, as well as those corresponding to the cases when only one of the photon's polarization is measured in $e^{+}e^{-}$ annihilation, in flight, in QED. This provides a dynamical, rather than a kinematical, description of photon polarization correlations as stemming from the ever precise and realistic QED theory. Such computations may be relevant to recent and future experiments involved in testing Bell-like inequalities as described.
We investigate how entanglement can enhance two-photon absorption in a three-level system. First, we employ the Schmidt decomposition to determine the entanglement properties of the optimal two-photon state to drive such a transition, and the maximum enhancement which can be achieved in comparison to the optimal classical pulse. We then adapt the optimization problem to realistic experimental constraints, where photon pairs from a down-conversion source are manipulated by local operations such as spatial light modulators. We derive optimal pulse shaping functions to enhance the absorption effi…
Two-photon absorption is theoretically analyzed within the semiclassical formalism of radiation-matter interaction. We consider an ensemble of inhomogeneously broadened three-level atoms subjected to the action of two counterpropagating fields of the same frequency. By concentrating in the limit of large detuning in one-photon transitions, we solve perturbatively the Bloch equations in a non-usual way. In this way we derive an analytical expression for the width of the two-photon resonance that makes evident sub-Doppler two--photon spectroscopy. We also derive an analytical expression for the …
Excitation with entangled photon pairs may lead to an increase in the efficiency of two-photon absorption at low photon flux. The corresponding process, entangled two-photon absorption (E2PA), has been investigated in numerous theoretical and experimental studies. However, significant ambiguity and inconsistency remain in the literature about the absolute values of E2PA cross-sections. Here, we use a fluorescence-based registration scheme to experimentally determine upper bounds on the cross-sections for six fluorophores. These bounds are up to four orders of magnitude lower than the smallest …
In this paper, we briefly show how the quantum key distribution with blind polarization bases [Kye et al., Phys. Rev. Lett. 95, 040501 (2005)] can be made secure against the invisible photon attack.
Using the process of cavity-enhanced spontaneous parametric down-conversion (SPDC), we generate a narrow-band polarization-entangled photon pair resonant on the rubidium (Rb) D1 line (795 nm). The degenerate single-mode photon pair is selected by multiple temperature controlled etalons. The linewidth of generated polarization-entangled photon pairs is 15 MHz which matches the typical atomic memory bandwidth. The measured Bell parameter for the polarization-entangled photons S=2.73+-0.04 which violates the Bell-CHSH inequality by ~18 standard deviations. The presented entangled photon pair sour…
We experimentally demonstrate polarization entanglement for squeezed vacuum pulses containing more than 10^5 photons. We also study photon-number entanglement by calculating the Schmidt number and measuring its operational counterpart. Theoretically, our pulses are the more entangled the brighter they are. This promises important applications in quantum technologies, especially photonic quantum gates and quantum memories.
We present an optical filter that transmits photon pairs only if they share the same horizontal or vertical polarization, without decreasing the quantum coherence between these two possibilities. Various applications for entanglement manipulations and multi-photon qubits are discussed.
We present a concentration and purification scheme for nonmaximally entangled pure and mixed porization entangled state. We firstly show that two distant parties Alice and Bob first start with two shared but less entangled photon pure states to produce a four photon GHZ state, and then perform a 45 polarization measurement onto one of the two photons at each location such that the remaining two photon are projected onto a maximally entangled state. We further show the scheme also can be used to purify a class of mixed polarization-entangled state.
We propose a simple probabilistic optical gate to expand polarization entangled W states. The gate uses one polarization-dependent beamsplitter and a horizontally polarized single photon as an ancilla. The gate post-selectively expands $N$-photon W states to $(N+1)$-photon W states. A feasibility analysis considering the realistic experimental conditions show that the scheme is within the reach of the current quantum optical technologies.
