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arXiv 2406.01075quant-ph
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通过温度控制的SPDC增强尼罗红(Nile Red)的纠缠双光子吸收

Enhancing entangled two-photon absorption of Nile Red via temperature-controlled SPDC

Aleksa Krstić, Tobias Bernd Gäbler, Nitish Jain, Patrick Then, Valerio Flavio Gili, Sina Saravi, Frank Setzpfandt, Christian Eggeling, Markus Gräfe

AI总结:

针对纠缠双光子吸收实验证据不足、现有模型难预测复杂染料行为的问题,提出考虑染料化学性质的模拟方法,发现吸收概率与非线性材料相位匹配温度显著相关,并以尼罗红实验数据验证了模型有效性。

摘要:

纠缠双光子吸收可使荧光发射与激发功率呈线性标度关系。与呈二次标度关系的经典双光子吸收相比,这种特性能够以最低曝光强度实现具有高轴向分辨率的荧光成像或光刻技术。然而,大多数关于双光子吸收的实验研究都无法给出纠缠光子对驱动荧光发射的明确证据。另一方面,现有理论模型难以准确预测化学结构复杂的染料的纠缠双光子吸收行为。在本文中,我们提出了一种考虑常见荧光染料化学性质的纠缠双光子吸收模拟方法。我们的理论模型能够让人们更深入地理解实验结果,进而理解纠缠双光子吸收的发生机制。特别地,我们发现吸收概率与非线性材料的相位匹配温度存在显著的依赖关系。此外,我们将该理论方法的计算结果与尼罗红(Nile Red)的实验数据进行了对比。

英文摘要:

Entangled two-photon absorption can enable a linear scaling of fluorescence emission with the excitation power. In comparison to classical two-photon absorption with a quadratic scaling, this can allow fluorescence imaging or photolithography with high axial resolution at minimal exposure intensities. However, most experimental studies on two-photon absorption were not able to show an unambiguous proof of fluorescence emission driven by entangled photon pairs. On the other hand, existing theoretical models struggle to accurately predict the entangled two-photon absorption behavior of chemically complex dyes. In this paper, we introduce an approach to simulate entangled two-photon absorption in common fluorescence dyes considering their chemical properties. Our theoretical model allows a deeper understanding of experimental results and thus the occurrence of entangled two-photon absorption. In particular, we found a remarkable dependency of the absorption probability on the phase-matching temperature of the nonlinear material. Further, we compared results of our theoretical approach to experimental data for Nile Red.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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