We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t_c is much shorter than the duration of the pump pulse Delta t, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter chi, which is a function of t_c/Delta t. We present a direct measurement of chi through a simple experimental setup. The full theoretical analysis is also provided.
An experimental scheme for preparing a polarization entangled W states from four photons emitted by parametric down-conversion is proposed. We consider two different configurations and a method of improving the yield by using single photon sources. In the proposed scheme, one uses only linear optical elements and photon detectors, so that this scheme is feasible by current technologies.
We propose a simple scheme to produce the polarization entangled photon pairs without the type II phase match. The same scheme can also be used to produce the macroscopic entangled photon states in both photon number space and the polarization space(A. Lamas-Linares, J.C. Howell and D. Bouwmeester, Nature, 412887(2001)). Advantages and applications of our scheme in quantum key distribution are discussed.
We consider six-photon entangled state emitted from a single third-order parametric down-conversion process. In the regime of weak nonlinearities, we present a symmetry detector which is capable of analyzing the twin-beam six-photon symmetric states. By cascading the symmetry detectors, as an application, it is shown that one can purify the desired six-photon entangled state from an arbitrary twin-beam six-photon symmetric state. With linear optics we propose a fruitful scheme for exploring a class of multimode-photon entangled states from third-order parametric down-conversion process. Furthe…
Starting from the standard Hamiltonian describing the optical non-linear process of spontaneous parametric down-conversion, we theoretically show that the generated entangled photon-pairs carry non-negligible orbital angular momentum in the degrees of freedom of relative movement in the type-II cases due to spatial symmetry breaking. We also show that the orbital angular momentum carried by photon-pairs in these degrees of freedom escapes detection in the traditional measurement scheme, which demands development of new techniques for further experimental investigations.
We have generated a new type of biphoton state by cavity-enhanced down-conversion in a type-II phase-matched, periodically-poled KTiOPO_4 (PPKTP) crystal. By introducing a weak intracavity birefringence, the polarization-entangled output was modulated between the singlet and triplet states according to the arrival-time difference of the signal and idler photons. This cavity-enhanced biphoton source is spectrally bright, yielding a single-mode fiber-coupled coincidence rate of 0.7 pairs/s per mW of pump power per MHz of down-conversion bandwidth. Its novel biphoton behavior may be utilized in s…
The quantum characteristics of sum-frequency process in an optical cavity with an input signal optical beam, which is a half of entangled optical beams, are analyzed. The calculated results show that the quantum properties of the signal beam can be maintained after its frequency is conversed during the intracavity nonlinear optical interaction. The frequency-conversed output signal beam is still in an entangled state with the retained other half of initial entangled beams. The resultant quantum correlation spectra and the parametric dependences of the correlations on the initial squeezing fact…
We describe the full characterization of the biaxial nonlinear crystal BiB3O6 (BiBO) as a polarization entangled photon source using non-collinear type-II parametric down-conversion. We consider the relevant parameters for crystal design, such as cutting angles, polarization of the photons, effective nonlinearity, spatial and temporal walk-offs, crystal thickness and the effect of the pump laser bandwidth. Experimental results showing entanglement generation with high rates and a comparison to the well investigated beta-BaB2O4 (BBO) crystal are presented as well. Changing the down-conversion c…
We address the process of generation of the photon-number entangled states of light in the stimulated nonlinear parametric down conversion process and build the simple model describing the generation, not involving the traditional parametric approximation. The motion equations for the system of pumping and two-mode outgoing field are solved for the case of the strong correlation between two modes, the evolution of the state parameters of the generated modes is obtained. The solution is briefly analyzed for particular types of photon-number entangled states.
We compare effects of decoherence and detection inefficiency on entangled coherent states (ECSs) and entangled photon pairs (EPPs), both of which are known to be particularly useful for quantum information processing (QIP). When decoherence effects caused by photon losses are heavy, the ECSs outperform the EPPs as quantum channels for teleportation both in fidelities and in success probabilities. On the other hand, when inefficient detectors are used, the teleportation scheme using the ECSs suffers undetected errors that result in the degradation of fidelity, while this is not the case for the…
We introduce a novel time-frequency quantum key distribution (TFQKD) scheme based on photon pairs entangled in these two conjugate degrees of freedom. The scheme uses spectral detection and phase modulation to enable measurements in the temporal basis by means of time-to-frequency conversion. This allows large-alphabet encoding to be implemented with realistic components. A general security analysis for TFQKD with binned measurements reveals a close connection with finite-dimensional QKD protocols and enables analysis of the effects of dark counts on the secure key size.
It is shown that the Greenberger-Horne-Zeilinger theorem can be generalized to the case with only two entangled particles. The reasoning makes use of two photons which are maximally entangled both in polarization and in spatial degrees of freedom. In contrast to Cabello's argument of "all versus nothing" nonlocality with four photons [Phys. Rev. Lett. 87, 010403 (2001)], our proposal to test the theorem can be implemented with linear optics and thus is well within the reach of current experimental technology.
We derive lower limits on the inefficiency and classical communication costs of dilution between two-term bipartite pure states that are partially entangled. We first calculate explicit relations between the allowable error and classical communication costs of entanglement dilution using the protocol of Lo-Popescu and then consider a two-stage dilution from singlets with this protocol followed by some unknown protocol for conversion between partially entangled states. Applying the lower bounds on classical communication and inefficiency of Harrow-Lo and Hayden-Winter to this two-stage protocol…
We experimentally demonstrate that paired photons generated in different sections of a down-conversion cone, when some of the interacting waves show Poynting vector walk-off, carry different spatial correlations, and therefore a different degree of spatial entanglement. This is shown to be in agreement with theoretical results. We also discuss how this azimuthal distinguishing information of the down-conversion cone is relevant for the implementation of quantum sources aimed at the generation of entanglement in other degrees of freedom, such as polarization.
In most configurations aimed at generating entangled photons based on spontaneous parametric down conversion (SPDC), the generated pairs of photons are required to be entangled in only one degree of freedom. Any distinguishing information coming from the other degrees of freedom that characterize the photon should be suppressed to avoid correlations with the degree of freedom of interest. However, this suppression is not always possible. Here, we show how the frequency information available affects the purity of the two-photon state in space, revealing a correlation between the frequency and t…
We present a review of the problem of finding out whether a quantum state of two or more parties is entangled or separable. After a formal definition of entangled states, we present a few criteria for identifying entangled states and introduce some entanglement measures. We also provide a classification of entangled states with respect to their usefulness in quantum dense coding, and present some aspects of multipartite entanglement.
We propose efficient schemes for converting three-photon, four-photon and five-photon GHZ state to a $W$ state or Dicke state, respectively with the nitrogen-vacancy (N-V) centers via single-photon input-output process and cross-Kerr nonlinearities. The total success probability can be improved by iterating the conversion process for the case of three-photon and five-photon while it does not require iteration for converting four-photon GHZ state to a $W$ state. The analysis of feasibility shows that our scheme is feasible for current experimental technology.
We investigate the quantum state generated by optical parametric down-conversion in a $χ^{(2) } $ medium driven by two noncollinear light modes. The analysis shows the emergence of multipartite, namely 3- or 4-partite, entangled states in a subset of the spatio-temporal modes generated by the process. These appear as bright spots against the background fluorescence, providing an interesting analogy with the phenomenology recently observed in two-dimensional nonlinear photonic crystals. We study two realistic setups: i) Non-critical phase-matching in a periodically poled Lithium Tantalate slab,…
We show that the transfer of the angular spectrum of the pump beam to the two-photon state in spontaneous parametric down-conversion enables the generation of entangled Hermite-Gaussian modes. We derive an analytical expression for the two-photon state in terms of these modes and show that there are restrictions on both the parity and order of the down-converted Hermite-Gaussian fields. Using these results, we show that the two-photon state is indeed entangled in Hermite-Gaussian modes. We propose experimental methods of creating maximally-entangled Bell states and non-maximally entangled pure…
We propose and design a high-brightness, ultra-compact electrically pumped GaSb-based laser source of entangled photons generated by mode-matched intracavity parametric down-conversion of lasing modes. To describe the nonlinear mixing in highly dispersive and dissipative waveguides, we develop a nonperturbative quantum theory of parametric down-conversion of waveguide modes which takes into account the effects of modal dispersion, group and phase mismatch, propagation, dissipation, and coupling to noisy reservoirs. We extend our theory to the regime of quantized pump fields with a new approach…
Generation and characterization of entanglement are crucial tasks in quantum information processing. A hypothesis testing scheme for entanglement has been formulated. Three designs were proposed to test the entangled photon states created by the spontaneous parametric down conversion. The time allocations between the measurement vectors were designed to consider the anisotropic deviation of the generated photon states from the maximally entangled states. The designs were evaluated in terms of the p-value based on the observed data. It has been experimentally demonstrated that the optimal time …
We review the problem of discriminating entangled states from separable states for bipartite systems. We formally define what entangled states are, present some important criteria to detect entanglement, and show how they can be classified according to their capability to perform some precisely defined tasks.
We explore the advantages offered by twin light beams produced in parametric down-conversion for precision measurement. The symmetry of these bipartite quantum states, even under losses, suggests that monitoring correlations between the divergent beams permits a high-precision inference of any symmetry-breaking effect, e.g. fiber birefringence. We show that the quantity of entanglement is not the key feature for such an instrument. In a lossless setting, scaling of precision at the ultimate `Heisenberg' limit is possible with photon counting alone. Even as photon losses approach 100% the preci…
Complete complementarity relations, as e.g. $P(ρ_{A})^{2} + C(ρ_{A})^{2} + E(|Ψ\rangle_{AB})^{2}=1$, constrain the local predictability, $P$, and local coherence, $C$, and the entanglement, $E$, of bipartite pure states. For pairs of qubits prepared initially in a particular class of partially entangled pure states with null local coherence, these relations were used in Ref. [Phys. Lett. A, 451, 128414 (2022)] to provide an operational connection between local predictability of the pre-measurement states with the probability of the maximally entangled components of the states after the Bell-ba…
We study the experimental realisation of quantum teleportation as performed by Bouwmeester {\em et al}. [Nature {\bf 390}, 575 (1997)] and the adjustments to it suggested by Braunstein and Kimble [Nature {\bf 394}, 841 (1998)]. These suggestions include the employment of a detector cascade and a relative slow-down of one of the two down-converters. We show that coincidences between photon-pairs from parametric down-conversion automatically probe the non-Poissonian structure of these sources. Furthermore, we find that detector cascading is of limited use, and that modifying the relative strengt…
We consider the problem of obtaining maximally entangled photon states at distance in the presence of loss. We compare the efficiency of two different schemes in establishing $N$ shared ebits: i) $N$ single ebit states with the qubit encoded on polarization; ii) a single continuous variable entangled state (emode) assisted by optimal local operation and classical communication (LOCC) protocol in order to obtain a $2^N$-dimensional maximally entangled state, with qubits encoded on the photon number.
Realising a global quantum network requires combining individual strengths of different quantum systems to perform universal tasks, notably using flying and stationary qubits. However, transferring coherently quantum information between different systems is challenging as they usually feature different properties, notably in terms of operation wavelength and wavepacket. To circumvent this problem for quantum photonics systems, we demonstrate a polarisation-preserving quantum frequency conversion device in which telecom wavelength photons are converted to the near infrared, at which a variety o…
By introducing a quantitative `degree of commutativity' in terms of the angle between spin-observables we present two tight quantitative trade-off relations in the case of two qubits: First, for entangled states, between the degree of commutativity of local observables and the maximal amount of violation of the Bell inequality: if both local angles increase from zero to π/2 (i.e., the degree of local commutativity decreases), the maximum violation of the Bell inequality increases. Secondly, a converse trade-off relation holds for separable states: if both local angles approach π/2 the maximal …
Incomparability of pure bipartite entangled states under deterministic LOCC is a very strange phenomena. We find two possible ways of getting our desired pure entangled state which is incomparable with the given input state, by collective LOCC with certainty. The first one is by providing some pure entanglement through the lower dimensional maximally-entangled states or using further less amount of entanglement and the next one is by collective operation on two pairs which are individually incomparable. It is quite surprising that we are able to achieve maximally entangled states of any Schmid…
Spontaneous down conversion in metal-dielectric interface in case of oblique laser excitation is considered. In this case it is possible to generate pairs of polarization entangled surface plasmon polaritons with high efficiency if to use excitation angle corresponding to the Kretschmann configuration for generated plasmons. The efficiency can be additionally enlarged if to use properly nanostructured metallic film allowing one to directly excite surface plasmon polaritons and to fulfill phase matching condition of them with generated surface plasmon polaritons.
Dynamics of many-qubit systems, that may correspond to computational processing with quantum systems, can be efficiently and generally approximated by a sequence of two- and single-qubit gates. In practical applications, however, a quantum gate prepared as a unitary transformation may appear as a noisy channel and consequently may inhibit quantum advantages. In this work, we apply the scheme of channel discrimination to detect if a quantum gate that is actually realized is unitary or noisy. We show that a two-qubit unitary transformation and its noisy counterpart can be optimally discriminated…
We suggest the generation of photon pairs in a thermally induced nonlinear periodically-poled silica fiber by spontaneous parametric down-conversion. Photons are generated directly in eigenstates of optical angular momentum. Photons in a pair can be entangled in these states as well as in frequencies. We identify suitable spatial and polarization modes giving an efficient nonlinear interaction. By changing the pump field properties both narrow- and broad-band down-converted fields can be obtained.
We develop and experimentally verify a theory of Type-II spontaneous parametric down-conversion (SPDC) in media with inhomogeneous distributions of second-order nonlinearity. As a special case, we explore interference effects from SPDC generated in a cascade of two bulk crystals separated by an air gap. The polarization quantum-interference pattern is found to vary strongly with the spacing between the two crystals. This is found to be a cooperative effect due to two mechanisms: the chromatic dispersion of the medium separating the crystals and spatiotemporal effects which arise from the inclu…
Maximally entangled mixed states are those states that, for a given mixedness, achieve the greatest possible entanglement. For two-qubit systems and for various combinations of entanglement and mixedness measures, the form of the corresponding maximally entangled mixed states is determined primarily analytically. As measures of entanglement, we consider entanglement of formation, relative entropy of entanglement, and negativity; as measures of mixedness, we consider linear and von Neumann entropies. We show that the forms of the maximally entangled mixed states can vary with the combination of…
Quantum mechanics of composite systems, gives rise to certain special states called entangled states. A physical system, that is in an entangled state displays an intricate correlation between its subsystems. There are also some composite quantum states (classically correlated states or separable states) that are not entangled. It is generally claimed, often without a rigorous proof to support, that these intricate correlations of an entangled state cannot occur in a classical system. This expository article, provides an elementary proof that entangled states cannot arise in the setting of cla…
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
The measurement of high-dimensional entangled states of orbital angular momentum prepared by spontaneous parametric down-conversion can be considered in two separate stages: a generation stage and a detection stage. Given a certain number of generated modes, the number of measured modes is determined by the measurement apparatus. We derive a simple relationship between the generation and detection parameters and the number of measured entangled modes.
We present a novel yet simple approach to produced multiple entangled photon pairs through spontaneous parametric downconversion. We have developed Gaussian masks to subdivide the pump beam before passing it through a nonlinear medium. In this way, we are able to observe simultaneous separate down-converted emission cones with spatial overlap. The technique we employ can be used to greatly increase the dimensionality of entangled photonic systems generated from spontaneous parametric down conversion, affording greater scalability to optical quantum computing than previously explored.
We report on the observation of an unusual type of parametric down-conversion. In the regime where collinear degenerate emission is in the anomalous range of group-velocity dispersion, its spectrum is restricted in both angle and wavelength. Detuning from exact collinear-degenerate phasematching leads to a ring shape of the wavelength-angular spectrum, suggesting a new type of spatiotemporal coherence and entanglement of photon pairs. By imposing a phase varying in a specific way in both angle and wavelength, one can obtain an interesting state of an entangled photon pair, with the two photons…
Deterministic sources of high-fidelity entangled qubit pairs encoded in the dual-rail photonic basis, i.e., presence of a single photon in one of two orthogonal modes, are a key enabling technology of many applications of quantum information processing, including high-rate high-fidelity quantum communications over long distances. The most popular and mature sources of such photonic entanglement, e.g., those that leverage spontaneous parametric down-conversion (SPDC) or spontaneous four-wave mixing (sFWM), generate an entangled (so-called, continuous-variable) quantum state that contains contri…
The relation between the violation of the Bell-CHSH inequalities and entanglement properties of quantum states is not clear so one may consider the mixedness of the system to understand the entanglement properties better than the Bell-CHSH inequality. In this respect, we prove that if the mixedness of the state measured by the linear entropy is less than 2/3 but strictly greater than zero then the two qubit states are entangled. But if the linear entropy is greater or equal to 2/3 then the state may or may not be entangled. Further we show that our entanglement criterion detects larger set of …
We discuss the asymptotic behavior of conversions between two independent and identical distributions up to the second-order conversion rate when the conversion is produced by a deterministic function from the input probability space to the output probability space. To derive the second-order conversion rate, we introduce new probability distributions named Rayleigh-normal distributions. The family of Rayleigh-normal distributions includes a Rayleigh distribution and coincides with the standard normal distribution in the limit case. Using this family of probability distributions, we represent …
Entangled photons play a pivotal role in the distribution of quantum information in quantum networks. However, the frequency bands for optimal transmission and storage of photons are not necessarily the same. Here we experimentally demonstrate the coherent frequency conversion of photons entangled in their polarization, a widely used degree of freedom in photonic quantum information processing. We verify the successful entanglement conversion by violating a Clauser-Horne-Shimony-Holt (CHSH) Bell inequality and fully confirm that our characterised fidelity of entanglement transfer is close to u…
In this paper we describe theoretically quantum control of temporal correlations of entangled photons produced by collinear type II spontaneous parametric down-conversion. We examine the effect of spectral phase modulation of the signal or idler photons arriving at a 50/50 beam splitter on the temporal shape of the entangled-photon wave packet . The coincidence count rate is calculated analytically for photon pairs in terms of the modulation depth applied to either the signal or idler beam with a spectral phase filter. It is found that the two-photon coincidence rate can be controlled by varyi…
Entanglement detection in high dimensional systems is a NP-hard problem since it is lacking an efficient way. Given a bipartite quantum state of interest free entanglement can be detected efficiently by the PPT-criterion (Peres-Horodecki criterion), in contrast to detecting bound entanglement, i.e. a curious form of entanglement that can also not be distilled into maximally (free) entangled states. Only a few bound entangled states have been found, typically by constructing dedicated entanglement witnesses, so naturally the question arises how large is the volume of those states. We define a l…
We show that polarization entangled photons at x-ray energies can be generated via spontaneous parametric down conversion. Each of the four Bell states can be generated by choosing the angle of incidence and polarization of the pumping beam.
We propose two schemes to generate four-photon polarization-entangled states from the second-order emission of the spontaneous parametric down-conversion process. By using linear optical elements and the coincidence-detection, the four indistinguishable photons emitted from parametric down-conversion source result in the Greenberger-Horne-Zeilinger (GHZ) state or the superposition of two orthogonal GHZ states. For this superposition state, under particular phase settings we analyze the quantum correlation function and the local hidden variable (LHV) correlation. As a result, the Bell inequalit…
Entangled photons are a crucial resource for quantum communication and linear optical quantum computation. Unfortunately, the applicability of many photon-based schemes is limited due to the stochastic character of the photon sources. Therefore, a worldwide effort has focused in overcoming the limitation of probabilistic emission by generating two-photon entangled states conditioned on the detection of auxiliary photons. Here we present the first heralded generation of photon states that are maximally entangled in polarization with linear optics and standard photon detection from spontaneous p…
In 1999 Raz demonstrated a partial function that had an efficient quantum two-way communication protocol but no efficient classical two-way protocol and asked, whether there existed a function with an efficient quantum one-way protocol, but still no efficient classical two-way protocol. In 2010 Klartag and Regev demonstrated such a function and asked, whether there existed a function with an efficient quantum simultaneous-messages protocol, but still no efficient classical two-way protocol. In this work we answer the latter question affirmatively and present a partial function Shape, which can…
The effect of noise on various protocols of secure quantum communication has been studied. Specifically, we have investigated the effect of amplitude damping, phase damping, squeezed generalized amplitude damping, Pauli type as well as various collective noise models on the protocols of quantum key distribution, quantum key agreement,quantum secure direct quantum communication and quantum dialogue. From each type of protocol of secure quantum communication, we have chosen two protocols for our comparative study; one based on single qubit states and the other one on entangled states. The compar…
A new ultra bright pulsed source of polarization entangled photons has been realized using type-II phase matching in spontaneous parametric down conversion process in two cascaded crystals. The optical axes of the crystals are aligned in such a way that the extraordinarily (ordinarily) polarized cone from one crystal overlaps with the ordinarily (extraordinarily) polarized cone from the second crystal. This spatial overlapping removes the association between the polarization and the output angle of the photons that exist in a single type-II down conversion process. Hence, entanglement of photo…
A scheme to distinguish entangled two-photon-polarization states (ETP) from two independent entangled one-photon-polarization states (EOP) is proposed. Using this scheme, the experimental generation of ETP by parametric down-conversion is confirmed through the anti-correlations between three orthogonal two-photon-polarization states. The estimated fraction of ETP among the correlated photon pairs is 37% in the present experimental setup.
We theoretically investigate up-conversion process of entangled two photons on a dimer molecule, which is coupled by a cavity or nanoscale metallic structure. Within one-dimensional input-output theory, the propagators of the photons are derived analytically and the up-conversion probability is calculated numerically. It is shown that the coupling with the nanostructure clearly enhances the process. We also find that the enhancement becomes further pronounced for some balanced system parameters such as the quantum correlation between photons, radiation decay rates and coupling between the nano…
We experimentally demonstrate a high-fidelity visible-to-telecommunication wavelength conversion of a photon by using a solid-state-based difference frequency generation. In the experiment, one half of a pico-second visible entangled photon pair at 780 nm is converted to a 1522-nm photon, resulting in the entangled photon pair between 780 nm and 1522 nm. Using superconducting single-photon detectors with low dark count rates and small timing jitters, we selectively observed well-defined temporal modes containing the two photons. We achieved a fidelity of $0.93 \pm 0.04$ after the wavelength co…
We present theoretical and experimental study of preparing maximally entangled two-photon polarization states, or Bell states, using femtosecond pulse pumped spontaneous parametric down-conversion (SPDC). First, we show how the inherent distinguishability in femtosecond pulse pumped type-II SPDC can be removed by using an interferometric technique without spectral and amplitude post-selection. We then analyze the recently introduced Bell state preparation scheme using type-I SPDC. Theoretically, both methods offer the same results, however, type-I SPDC provides experimentally superior methods …
Entanglement assistance is known to reduce the quantum communication complexity of evaluating functions with distributed inputs. But does the type of entanglement matter, or are EPR pairs always sufficient? This is a natural question because in several other settings maximally entangled states are known to be less useful as a resource than some partially entangled state. These include non-local games, tasks with quantum communication between players and referee, and simulating bipartite unitaries or communication channels. By contrast, we prove that the bounded-error entanglement-assisted quan…
We implement experimentally a method to generate photon-number$-$path and polarization entangled photon pairs using ``beamlike'' type-II spontaneous parametric down-conversion (SPDC), in which the signal-idler photon pairs are emitted as two separate circular beams with small emission angles rather than as two diverging cones.
