Takashi Yamamoto, Kiyoshi Tamaki, Masato Koashi, Nobuyuki Imoto
An experimental scheme for preparing a polarization entangled W states from four photons emitted by parametric down-conversion is proposed. We consider two different configurations and a method of improving the yield by using single photon sources. In the proposed scheme, one uses only linear optical elements and photon detectors, so that this scheme is feasible by current technologies.
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We propose a simple scheme to produce the polarization entangled photon pairs without the type II phase match. The same scheme can also be used to produce the macroscopic entangled photon states in both photon number space and the polarization space(A. Lamas-Linares, J.C. Howell and D. Bouwmeester, Nature, 412887(2001)). Advantages and applications of our scheme in quantum key distribution are discussed.
We consider six-photon entangled state emitted from a single third-order parametric down-conversion process. In the regime of weak nonlinearities, we present a symmetry detector which is capable of analyzing the twin-beam six-photon symmetric states. By cascading the symmetry detectors, as an application, it is shown that one can purify the desired six-photon entangled state from an arbitrary twin-beam six-photon symmetric state. With linear optics we propose a fruitful scheme for exploring a class of multimode-photon entangled states from third-order parametric down-conversion process. Furthe…
Starting from the standard Hamiltonian describing the optical non-linear process of spontaneous parametric down-conversion, we theoretically show that the generated entangled photon-pairs carry non-negligible orbital angular momentum in the degrees of freedom of relative movement in the type-II cases due to spatial symmetry breaking. We also show that the orbital angular momentum carried by photon-pairs in these degrees of freedom escapes detection in the traditional measurement scheme, which demands development of new techniques for further experimental investigations.
We have generated a new type of biphoton state by cavity-enhanced down-conversion in a type-II phase-matched, periodically-poled KTiOPO_4 (PPKTP) crystal. By introducing a weak intracavity birefringence, the polarization-entangled output was modulated between the singlet and triplet states according to the arrival-time difference of the signal and idler photons. This cavity-enhanced biphoton source is spectrally bright, yielding a single-mode fiber-coupled coincidence rate of 0.7 pairs/s per mW of pump power per MHz of down-conversion bandwidth. Its novel biphoton behavior may be utilized in s…
The quantum characteristics of sum-frequency process in an optical cavity with an input signal optical beam, which is a half of entangled optical beams, are analyzed. The calculated results show that the quantum properties of the signal beam can be maintained after its frequency is conversed during the intracavity nonlinear optical interaction. The frequency-conversed output signal beam is still in an entangled state with the retained other half of initial entangled beams. The resultant quantum correlation spectra and the parametric dependences of the correlations on the initial squeezing fact…
We describe the full characterization of the biaxial nonlinear crystal BiB3O6 (BiBO) as a polarization entangled photon source using non-collinear type-II parametric down-conversion. We consider the relevant parameters for crystal design, such as cutting angles, polarization of the photons, effective nonlinearity, spatial and temporal walk-offs, crystal thickness and the effect of the pump laser bandwidth. Experimental results showing entanglement generation with high rates and a comparison to the well investigated beta-BaB2O4 (BBO) crystal are presented as well. Changing the down-conversion c…
We address the process of generation of the photon-number entangled states of light in the stimulated nonlinear parametric down conversion process and build the simple model describing the generation, not involving the traditional parametric approximation. The motion equations for the system of pumping and two-mode outgoing field are solved for the case of the strong correlation between two modes, the evolution of the state parameters of the generated modes is obtained. The solution is briefly analyzed for particular types of photon-number entangled states.
The theory of parametric down conversion of the vacuum, based on a real zeropoint, or "vacuum" electromagnetic field, has been treated in earlier articles. The same theory predicts a hitherto unsuspected phenomenon - parametric up conversion of the vacuum. This article describes how the phenomenon may be demonstrated experimentally.
We present a first experimental test of the existence of Spontaneus Parametric Up Conversion, predicted by a specific local realistic model based on Wigner function formalism. The measurement has been made using a ccd camera on the emission of a LiIO3 crystal pumped by a 351 nm and/or a 789 (1064) nm lasers. We obtain an upper limit of 160 times on the ratio between intensity of Spontaneus Parametric Up Conversion and Spontaneous Parametric Down conversion.
We introduce a novel time-frequency quantum key distribution (TFQKD) scheme based on photon pairs entangled in these two conjugate degrees of freedom. The scheme uses spectral detection and phase modulation to enable measurements in the temporal basis by means of time-to-frequency conversion. This allows large-alphabet encoding to be implemented with realistic components. A general security analysis for TFQKD with binned measurements reveals a close connection with finite-dimensional QKD protocols and enables analysis of the effects of dark counts on the secure key size.
We use photon counters to obtain the joint photon counting statistics from twin-beam non-degenerate parametric down conversion, and we demonstrate directly, and with no auxiliary assumptions, that these twin beams are nonclassical.
We report on a method for optimizing the collection of entangled photon pairs in type-II parametric fluorescence. With this technique, we detected 360000 polarization-entangled photon pairs per second in the near-IR region in single-mode optical fibers. The entanglement of the photon pairs was verified by measuring polarization correlations in different bases of at least 96%.
Coincidence-structures in the transverse plane of Type-II spontaneous parametric down-conversion carrying orbital angular momentum are obtained. Azimuthal symmetry breaking around the pump beam direction reveals itself on these quantum images. Analytical expressions for the amplitude probability of the down conversion process are shown including the nonlinear polarizability components.
We present an experiment of preparing Werner state via spontaneous parametric down-conversion and controlled decoherence of photons in this paper. In this experiment two independent BBO (beta-barium borate) crystals are used to produce down-conversion light beams, which are mixed to prepare Werner state.
We derive lower limits on the inefficiency and classical communication costs of dilution between two-term bipartite pure states that are partially entangled. We first calculate explicit relations between the allowable error and classical communication costs of entanglement dilution using the protocol of Lo-Popescu and then consider a two-stage dilution from singlets with this protocol followed by some unknown protocol for conversion between partially entangled states. Applying the lower bounds on classical communication and inefficiency of Harrow-Lo and Hayden-Winter to this two-stage protocol…
We experimentally demonstrate that paired photons generated in different sections of a down-conversion cone, when some of the interacting waves show Poynting vector walk-off, carry different spatial correlations, and therefore a different degree of spatial entanglement. This is shown to be in agreement with theoretical results. We also discuss how this azimuthal distinguishing information of the down-conversion cone is relevant for the implementation of quantum sources aimed at the generation of entanglement in other degrees of freedom, such as polarization.
Recent work using spontaneous parametric down-conversion (SPDC) has made possible investigations of the Einstein-Podolsky-Rosen paradox in its original (position-momentum) form. We propose an experiment that uses SPDC photon pairs to measure through which slit a photon passes while simultaneously observing double-slit interference.
Surface spontaneous parametric down-conversion is predicted as a consequence of continuity requirements for electric- and magnetic-field amplitudes at a discontinuity of chi2 nonlinearity. A generalization of the usual two-photon spectral amplitude is suggested to describe this effect. Examples of nonlinear layered structures and periodically-poled nonlinear crystals show that surface contributions to spontaneous down-conversion can be important.
We propose a novel scheme to generate polarization entanglement from spatially-correlated photon pairs. We experimentally realized a scheme by means of a spatial correlation effect in a spontaneous parametric down-conversion and a modified Michelson interferometer. The scheme we propose in this paper can be interpreted as a conversion process from spatial correlation to polarization entanglement.
We implement experimentally a method to generate photon-number$-$path and polarization entangled photon pairs using ``beamlike'' type-II spontaneous parametric down-conversion (SPDC), in which the signal-idler photon pairs are emitted as two separate circular beams with small emission angles rather than as two diverging cones.
In most configurations aimed at generating entangled photons based on spontaneous parametric down conversion (SPDC), the generated pairs of photons are required to be entangled in only one degree of freedom. Any distinguishing information coming from the other degrees of freedom that characterize the photon should be suppressed to avoid correlations with the degree of freedom of interest. However, this suppression is not always possible. Here, we show how the frequency information available affects the purity of the two-photon state in space, revealing a correlation between the frequency and t…
We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t_c is much shorter than the duration of the pump pulse Delta t, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter chi, which is a function of t_c/Delta t. We present a direct measurement of chi through a simple experimental setup. The full theoretical analysis is also p…
High-gain parametric down-conversion (PDC) is a source of bright squeezed vacuum, which is a macroscopic nonclassical state of light and a promising candidate for quantum information applications. Here we study its properties, such as the intensity spectral width and the spectral width of pairwise correlations.
We propose efficient schemes for converting three-photon, four-photon and five-photon GHZ state to a $W$ state or Dicke state, respectively with the nitrogen-vacancy (N-V) centers via single-photon input-output process and cross-Kerr nonlinearities. The total success probability can be improved by iterating the conversion process for the case of three-photon and five-photon while it does not require iteration for converting four-photon GHZ state to a $W$ state. The analysis of feasibility shows that our scheme is feasible for current experimental technology.
High-dimensional maximally entangled photon pairs in parametric down-conversion
针对无限OAM基矢高维子空间中难以直接生成最大纠缠态的问题，提出同时利用泵浦光束空间分布和晶体非线性轮廓的方法，无需额外空间滤波即可生成最大纠缠态，并以d=3和d=5为例进行了演示。
Photon-added coherent states have been realized in optical parametric down-conversion by Zavatta {\em et al} [Science 306 (2004) 660-662]. In this report, it is established that the states generated in the process are {\em ideal} photon-added coherent states. It is shown that the scheme can generate higher order photon-added coherent states. A comparative study of the down-conversion process and atom-cavity interaction in generating the photon-added coherent states is presented.
Spontaneous parametric down-conversion (SPDC) sources are an important technology for quantum sensing and imaging. We demonstrate a general simulation method, based on modeling from first principles, reproducing the spectrally and spatially resolved absolute counts of a SPDC experiment. By simulating additional processes and effects we accomplish good agreement with the experimental results. This method is broadly applicable and allows for the separation of contributing processes, virtual characterization of SPDC sources, and enables the simulation of many quantum based applications.
We analyze the long-time quantum dynamics of degenerate parametric down-conversion from an initial sub-harmonic vacuum (spontaenous down-conversion). Standard linearization of the Heisenberg equations of motions fails in this case, since it is based on an expansion around an unstable classical solution and neglects pump depletion. Introducing a mean-field approximation we find a periodic exchange of energy between the pump and subharmonic mode goverened by an anharmonic pendulum equation. From this equation the optimum interaction time or crystal length for maximum conversion can be determined…
In this paper we report our systematic study of a promising absolute calibration technique of analog photo-detectors, based on the properties of parametric down conversion. Our formal results and a preliminary uncertainty analysis show that the proposed method can be effectively developed with interesting applications to metrology.
The phenomenon of parametric down conversion from the vacuum may be understood as a process in classical electrodynamics, in which a nonlinear crystal couples the modes of the pumping field with those of the zeropoint, or "vacuum" field. This is an entirely local theory of the phenomenon, in contrast with the presently accepted nonlocal theory. The new theory predicts a hitherto unsuspected phenomenon - parametric up conversion from the vacuum.
We study the two-photon detection amplitude of the down-converted beams in spontaneous parametric down-conversion when the physical variable of orbital angular momentum is involved, taking into account both conservation and non-conservation of angular momentum. Agreeing with experimental observations, our theoretical calculation shows that spatial structure of the two-photon detection amplitude of the down-converted beams carries important information about conservation or non-conservation of orbital angular momentum in spontaneous parametric down-conversion.
We introduce an effective numerical method of density matrix determination of fiber coupled single photon generated in process of spontaneous parametric down conversion in type I non-collinear configuration. The presented theory has been successfully applied in case of source exploited in Phys. Rev. Lett. 99, 123601 (2007) to demonstrate the experimental characterization of spectral state of single photon.
We solve analytically master equations that describe a cavity filled with a kerr medium, taking into account the dissipation induced by the environment, and parametric down conversion processes. We use superoperator techniques.
We investigate the quantum state generated by optical parametric down-conversion in a $χ^{(2) } $ medium driven by two noncollinear light modes. The analysis shows the emergence of multipartite, namely 3- or 4-partite, entangled states in a subset of the spatio-temporal modes generated by the process. These appear as bright spots against the background fluorescence, providing an interesting analogy with the phenomenology recently observed in two-dimensional nonlinear photonic crystals. We study two realistic setups: i) Non-critical phase-matching in a periodically poled Lithium Tantalate slab,…
We show how stimulated parametric processes can be employed in experiments on beyond the diffraction limit to overcome the problem of low visibility obtained by using spontaneous down conversion operating in the high gain regime. We further show enhancement of the count rate by several orders when stimulated parametric processes are used. Both the two photon counts and the visibility can be controlled by the phase of the stimulating coherent beam.
A novel method for preparation of a single photon in temporally-delocalized entangled modes is proposed and analyzed. We show that two single-photon pulses propagating in a driven nonabsorbing medium with different group velocities are temporally split under parametric interaction into well-separated pulses. In consequence, the single-photon "time-bin-entangled" states are generated with a programmable entanglement easily controlled by driving field intensity. The experimental study of nonclassical features and nonlocality of generated states by means of balanced homodyne tomography is discuss…
A theory of spontaneous parametric down-conversion, which gives rise to a quantum state that is entangled in multiple parameters, such as three-dimensional wavevector and polarization, allows us to understand the unusual characteristics of fourth-order quantum interference in many experiments, including ultrafast type-II parametric down-conversion, the specific example illustrated in this paper. The comprehensive approach provided here permits the engineering of quantum states suitable for quantum information schemes and new quantum technologies.
We describe parametric down conversion process in a two-level atomic gas, where the atoms are in a superposition state of relevant energy levels. This superposition results in splitting of the phase matching condition into three different conditions. Another, more important, peculiarity of the system under discussion is the nonsaturability of amplification coefficients with increasing pump wave intensity, under "sideband" generation conditions.
Tripartite entangled states, such as GHZ and W states, are typically generated by manipulating two pairs of polarization-entangled photons in bulk optics. Here we propose a scheme to generate W states that are entangled in the energy degree of freedom in an integrated optical circuit. Our approach employs photon pairs generated by spontaneous four-wave mixing (SFWM) in a micro- ring resonator. We also present a feasible procedure for demonstrating the generation of such a state, and we compare polarization-entangled and energy-entangled schemes for the preparation of W states.
Using a basic Mach-Zehnder interferometer, we demonstrate experimentally the measurement of the photonic de Broglie wavelength of an entangled photon pair (a biphoton) generated by spontaneous parametric down-conversion. The observed interference manifests the concept of the photonic de Broglie wavelength. The result also provides a proof-of-principle of the quantum lithography that utilizes the reduced interferometric wavelength.
There is a serious flaw in the proposal [arXiv:1603.06857] for the achievement of unity efficiency in SPDC. This is a replacement due to mistakes in the table of probabilities. Numbers have been corrected.
A study of "high temperature" entangled states in a system of two parametrically coupled quantum oscillators placed into independent thermal baths is performed taking into account partially coherent parametric pump. Processes in an open system are considered based on the Heisenberg-Langevin formalism. We obtain a closed system of equations for the averaged quadratic correlation functions in quantum stochastic problem as a result of Markov processes approximation. On the basis of numerical calculations the dynamics of the logarithmic negativity, which is the measure of entanglement in the syste…
We report the efficient generation of high-gain parametric down-conversion, including pump depletion, with pump powers as low as 100 $μ$W (energies $0.1$~$μ$J/pulse) and conversion efficiencies up to 33\%. In our simple configuration, the pump beam is tightly focused into a bulk periodically poled lithium niobate crystal placed in free space. We also observe a change in the photon number statistics for both the pump and down-converted beams as the pump power increases to reach the depleted pump regime. The experimental results are a clear signature of the interplay between the pump and the dow…
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
Spontaneous parametric down conversion has been largely exploited as a tool for absolute calibration of photon counting detectors, photomultiplier tubes or avalanche photodiodes working in Geiger regime. In this work we investigate the extension of this technique from very low photon flux of photon counting regime to the absolute calibration of analog photodetectors at higher photon flux. Moving toward higher photon rate, i.e. at high gain regime, with the spontaneous parametric down conversion shows intrinsic limitations of the method, while the stimulated parametric down conversion process, …
We study the quantum properties of the polarization of the light produced in type II spontaneous parametric down-conversion in the framework of a multi-mode model valid in any gain regime. We show that the the microscopic polarization entanglement of photon pairs survives in the high gain regime (multi-photon regime), in the form of nonclassical correlation of all the Stokes operators describing polarization degrees of freedom.
We suggest a variant of the recently proposed experiment for the generation of a new kind of Schroedinger-cat states, using two coupled parametric down-converter nonlinear crystals [F. De Martini, Phys. Rev. Lett. 81, 2842 (1998)]. We study the parametric oscillator case and find that an entangled Schroedinger-cat type state of two cavities, whose mirrors are placed along the output beams of the nonlinear crystals, can be realized under suitable conditions.
By utilizing the nondegenerate optical parametric amplifier, the quantum state transfer from a pump state with high frequency to a signal state of lower frequency is studied theoretically. The noiseless state transfer is characterized by frequency conversion efficiency and noise figure. It is shown that the quantum state can be well preserved during the frequency conversion as long as the optical parametric amplifier is operated far below the threshold, and meanwhile injected with an input idler field with a power density about ten times greater than that of the pump. The dependence of the noi…
We show that the transfer of the angular spectrum of the pump beam to the two-photon state in spontaneous parametric down-conversion enables the generation of entangled Hermite-Gaussian modes. We derive an analytical expression for the two-photon state in terms of these modes and show that there are restrictions on both the parity and order of the down-converted Hermite-Gaussian fields. Using these results, we show that the two-photon state is indeed entangled in Hermite-Gaussian modes. We propose experimental methods of creating maximally-entangled Bell states and non-maximally entangled pure…
What are the orbital angular momentum correlations between spatially entangled photon pairs generated in spontaneous parametric down-conversion? We show that the answer to this question can be given in two alternative, although complementary, ways. The answer posed in this letter explains satisfactorily the seemingly contradictory results obtained in different experiments, and theoretical approaches.
We derive the steady state solution of the Fokker-Planck equation that describes the dynamics of the nondegenerate optical parametric oscillator in the truncated Wigner representation of the density operator. The adiabatic limit of strong pump damping is assumed. This phase space image provides a clear view of the intracavity two-mode entangled state valid in all operating regimes of the OPO. A nongaussian distribution is obtained for the above threshold solution.
We propose a method for generation of a single-cycle squeezed light by parametric down-conversion in a chirped quasi-phase-matched nonlinear crystal. We find an exact quantum solution for this process valid for an arbitrary parametric gain, and discover an ultrabroadband squeezing in the down-converted light with flat squeezing spectrum comprising the full optical octave. We describe a scheme for observation of this kind of squeezing using second-harmonic generation as an ultrafast correlator.
Type-II parametric down conversion in the Wigner-function formalism. Entanglement and Bell's inequalities
本文将I型参量下转换的Wigner函数分析扩展至II型，揭示纠缠是信号与真空涨落的关联，并通过探测分析支持以纯Maxwell电磁波描述该过程。
We describe an experiment in which photon pairs from a pulsed parametric down-conversion source were coupled into single-mode fibers. Detecting one of the photons heralded the presence of the other photon in its fiber with a probability of 83%. The heralded photons were then used in a simple multi-photon interference experiment to illustrate their potential for quantum information applications.
We propose and design a high-brightness, ultra-compact electrically pumped GaSb-based laser source of entangled photons generated by mode-matched intracavity parametric down-conversion of lasing modes. To describe the nonlinear mixing in highly dispersive and dissipative waveguides, we develop a nonperturbative quantum theory of parametric down-conversion of waveguide modes which takes into account the effects of modal dispersion, group and phase mismatch, propagation, dissipation, and coupling to noisy reservoirs. We extend our theory to the regime of quantized pump fields with a new approach…
We theoretically discuss one-photon and two-photon double-slit interferences for spontaneous and stimulated parametric down-conversions. We show that the two-photon sub-wavelength interference can exist in a general spontaneous parametric down-conversion (SPDC) for both type I and type II crystals. We propose an alternative way to observe sub-wavelength interference by a joint-intensity measurement which occurs for only type I crystal in a higher gain of SPDC. When a signal beam injects into the crystal, it may create two interference patterns by two stimulated down-converted beams, showing no…
We present a novel yet simple approach to produced multiple entangled photon pairs through spontaneous parametric downconversion. We have developed Gaussian masks to subdivide the pump beam before passing it through a nonlinear medium. In this way, we are able to observe simultaneous separate down-converted emission cones with spatial overlap. The technique we employ can be used to greatly increase the dimensionality of entangled photonic systems generated from spontaneous parametric down conversion, affording greater scalability to optical quantum computing than previously explored.
Preparation of Schrödinger cat quantum state using parametric down-conversion interaction
本研究针对量子光学中薛定谔猫态的制备需求，提出一种基于简并参量下转换与泵浦模式光子数预示测量的亮多光子薛定谔猫态条件生成新方法，且该方法原则上可通过现有高Q光学微谐振器实现。
Quantum networks require interfacing stationary and flying qubits. These flying qubits are usually nonclassical states of light. Here we consider two of the leading source technologies for nonclassical light, spontaneous parametric down-conversion and single semiconductor quantum dots. Down-conversion delivers high-grade entangled photon pairs, whereas quantum dots excel at producing single photons. We report on an experiment that joins these two technologies and investigates the conditions under which optimal interference between these dissimilar light sources may be achieved.
We investigate the third order spontaneous parametric down-conversion process in a nonlinear media with inversion centers. Specifically, we analyze in details the three-photon differential count rate in unit frequency and angular regions, total count rate and measurement time for rutile and calcite crystals which have comparatively large cubic susceptibilities. Special attention is given to consideration of limited frequency and angular detection ranges in order to calculate experimentally available detection rate values.
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