We show that the transfer of the angular spectrum of the pump beam to the two-photon state in spontaneous parametric down-conversion enables the generation of entangled Hermite-Gaussian modes. We derive an analytical expression for the two-photon state in terms of these modes and show that there are restrictions on both the parity and order of the down-converted Hermite-Gaussian fields. Using these results, we show that the two-photon state is indeed entangled in Hermite-Gaussian modes. We propose experimental methods of creating maximally-entangled Bell states and non-maximally entangled pure states of first order Hermite-Gaussian modes.
We provide a general decomposition of the two-photon state produced by spontaneous parametric down-conversion in Hermite-Gaussian modes, in the case that the pump beam is described by a Hermite-Gaussian beam of any order. We show that the spatial correlations depend explicitly on the order of the pump beam, as well as other experimental parameters. We use the decomposition to demonstrate a few interesting cases. Our results are applicable to the engineering of two-photon spatial entanglement, in particular for non-Gaussian states.
We report on an experiment demonstrating the conservation of orbital angular momentum in stimulated down-conversion. The orbital angular momentum is not transferred to the individual beams of the spontaneous down-conversion, but it is conserved when twin photons are taken individually. We observe the conservation law for an individual beam of the down-conversion through cavity-free stimulated emission.
We study the two-photon detection amplitude of the down-converted beams in spontaneous parametric down-conversion when the physical variable of orbital angular momentum is involved, taking into account both conservation and non-conservation of angular momentum. Agreeing with experimental observations, our theoretical calculation shows that spatial structure of the two-photon detection amplitude of the down-converted beams carries important information about conservation or non-conservation of orbital angular momentum in spontaneous parametric down-conversion.
We found that the Hermit-Gaussian(HG) modes of the down converted beams from the spontaneous parametric down conversion are quasi-conserved and the generated photon pairs are HG modes entangled for some special cases. This is valuable for either the investigation of fundament properties of multi-dimensional entanglement or quantum information applications.
We show that the transfer of the plane wave spectrum of the pump beam to the fourth-order transverse spatial correlation function of the two-photon field generated by spontaneous parametric down-conversion leads to the conservation and entanglement of orbital angular momentum of light. By means of a simple experimental setup based on fourth-order (or two-photon) interferometry, we show that our theoretical model provides a good description for down-converted fields carrying orbital angular momentum.
We report a proof-of-principle experiment demonstrating that appropriately chosen set of Hermite-Gaussian modes constitutes a Schmidt decomposition for transverse momentum states of biphotons generated in the process of spontaneous parametric down conversion. We experimentally realize projective measurements in Schmidt basis and observe correlations between appropriate pairs of modes. We perform tomographical state reconstruction in the Schmidt basis, by direct measurement of single-photon density matrix eigenvalues.
Nonlinear optical frequency conversion, observed more than half a century ago, is a corner stone in modern applications of nonlinear and quantum optics. It is well known that frequency conversion processes are constrained by conservation laws, such as momentum conservation that requires phase matching conditions for efficient conversion. However, conservation laws alone could not fully capture the features of nonlinear frequency conversion. Here it is shown that topology can provide additional constraints in nonlinear multi-frequency conversion processes. Unlike conservation laws, a topologica…
Quantum entanglement associated with transverse wave vectors of down conversion photons is investigated based on the Schmidt decomposition method. We show that transverse entanglement involves two variables: orbital angular momentum and transverse frequency. We show that in the monochromatic limit high values of entanglement are closely controlled by a single parameter resulting from the competition between (transverse) momentum conservation and longitudinal phase matching. We examine the features of the Schmidt eigenmodes, and indicate how entanglement can be enhanced by suitable mode selecti…
Parametric down-conversion (PDC) offers the possibility to control the fabrication of non-Gaussian states such as Fock states. However, in conventional PDC sources energy and momentum conservation introduce strict frequency and photon number correlations, which impact the fidelity of the prepared state. In our work we optimize the preparation of single-photon Fock states from the emission of waveguided PDC via spectral filtering. We study the effect of correlations via photon number resolving detection and quantum interference. Our measurements show how the reduction of mixedness due to filter…
Many quantum information protocols require a Bell-state measurement of entangled systems. Most optical Bell-state measurements utilize two-photon interference at a beam splitter. By creating polarization-entangled photons with spontaneous parametric down-conversion using a first-order Hermite-Gaussian pump beam, we invert the usual interference behavior and perform an incomplete Bell-state measurement in the coincidence basis. We discuss the possibility of a complete Bell-state measurement in the coincidence basis using hyperentangled states [Phys. Rev. A, \textbf{58}, R2623 (1998)].
Strong correlations in two conjugate variables are the signature of quantum entanglement and have played a key role in the development of modern physics. Entangled photons have become a standard tool in quantum information and foundations. An impressive example is position-momentum entanglement of photon pairs, explained heuristically through the correlations implied by a common birth zone and momentum conservation. However, these arguments entirely neglect the importance of the `quantumness', i.e. coherence, of the driving force behind the generation mechanism. We study theoretically and expe…
Light beams with orbital angular momentum (OAM) are convenient carriers of quantum information. They can be also used for imparting rotational motion to particles and provide high resolution in imaging. Due to the conservation of OAM in parametric down-conversion (PDC), signal and idler photons generated at low gain have perfectly anti-correlated OAM values. It is interesting to study the OAM properties of high-gain PDC, where the same OAM modes can be populated with large, but correlated, numbers of photons. Here we investigate the OAM spectrum of high-gain PDC and show that the OAM mode cont…
We experimentally demonstrate a programmable parametric mode sorter of high-dimensional signals in a composite spatiotemporal Hilbert space through mode-selective quantum frequency up-conversion. As a concrete example and with quantum communication applications in mind, we consider the Laguerre-Gaussian and Hermite-Gaussian modes as the spatial and temporal state basis for the signals, respectively. By modulating the spatiotemporal profiles of the up-conversion pump, we demonstrate the faithful selection of single photons in those modes and their superposition modes. Our results show an improv…
We consider multimode two-photon interference at a beam splitter by photons created by spontaneous parametric down-conversion. The resulting interference pattern is shown to depend upon the transverse spatial symmetry of the pump beam. In an experiment, we employ the first-order Hermite-Gaussian modes in order to show that, by manipulating the pump beam, one can control the resulting two-photon interference behavior. We expect these results to play an important role in the engineering of quantum states of light for use in quantum information processing and quantum imaging.
We report, for the first time, the generation of entangled photon pairs via type-0 spontaneous parametric down conversion in an ultra-thin wafer of lithium niobate in which momentum between the pump photon and daughter photons is not conserved. The characteristics of the emission are investigated using several techniques. We find that non-phase matched SPDC is a promising source of ultra-broadband two photon radiation that exhibits remarkably tight correlation widths in both the spatial and temporal domains.
Coherent control of the spatial properties of light is central to a wide variety of applications from high bandwidth quantum and classical communication to high power fiber lasers. Low-loss conversion amongst a complete and orthogonal set of modes is particularly important for robust mode-multiplexed communication. Here, we introduce tunable impedance mismatch between coupled Fabry-Pérot resonators as a powerful tool for manipulation of the spatial and temporal properties of optical fields. In the single-mode regime, frequency dependent impedance matching enables tunable finesse optical resona…
We study quantum frequency translation and two-color photon interference enabled by the Bragg scattering four-wave mixing process in optical fiber. Using realistic model parameters, we computationally and analytically determine the Green function and Schmidt modes for cases with various pump-pulse lengths. These cases can be categorized as either "non-discriminatory" or "discriminatory" in regards to their propensity to exhibit high-efficiency translation or high-visibility two-photon interference for many different shapes of input wave packets or for only a few input wave packets, respectivel…
Quantum state engineering, the cornerstone of quantum photonic technologies, mainly relies on spontaneous parametric down-conversion and four-wave mixing, where one or two pump photons decay into a photon pair. Both these nonlinear effects require momentum conservation (i.e., phase-matching) for the participating photons, which strongly limits the versatility of the resulting quantum states. Nonlinear metasurfaces, due to their subwavelength thickness, relax this constraint and extend the boundaries of quantum state engineering. Here, we generate entangled photons via spontaneous parametric do…
Decay of a particle into more particles is a ubiquitous phenomenon to interacting quantum systems, taking place in colliders, nuclear reactors, or solids. In a non-linear medium, even a single photon would decay by down-converting (splitting) into lower frequency photons with the same total energy, at a rate given by Fermi's Golden Rule. However, the energy conservation condition cannot be matched precisely if the medium is finite and only supports quantized modes. In this case, the photon's fate becomes the long-standing question of many-body localization (MBL), originally formulated as a ged…
Stimulated Parametric Down-Conversion: From Foundational Coherence to Structured Light Applications
Instituto Federal de Mato Grosso（马托格罗索联邦学院）；Departamento de Física, Universidade Federal de Santa Catarina（圣卡塔琳娜联邦大学物理系）；Universidad de Concepción（孔塞普西翁大学）；Millennium Institute for Research in Optics, Universidad de Concepción（孔塞普西翁大学光学研究千年研究所）
Due to the transfer of the angular spectrum of the pump beam to the two-photon state in spontaneous parametric down-conversion the generated twin photons are entangled in Hermite-Gaussian (HG) modes. This enables one using HG modes as an alphabet for quantum communication. For global quantum communication purposes, we derive an analytic expression for two-photon detection probability in terms of HG modes taking into account the effects of the turbulent atmosphere. Our result is more general as it accounts for the propagation of both, signal and idler photons through the atmosphere, as opposed …
We discuss the problem of the information transfer (exchange of states configuration) between two interacting quantum systems along their evolution in time. We consider the specific case of two modes of the electromagnetic field with rotating wave coupling interaction (up-conversion in a nonlinear crystal). We verify that for certain initial states of the fields the swapping of state configuration occurs with conservation of the mean energy of each mode (without energy transfer), characterising thus pure information flow.
High-order harmonic generation stands as a unique nonlinear optical up-conversion process, mediated by a laser-driven electron recollision mechanism, which has been shown to conserve energy, momentum, and spin and orbital angular momentum. Here we present theoretical simulations which demonstrate that this process also conserves a mixture of the latter, the torus-knot angular momentum $J_γ$, by producing high-order harmonics with driving pulses that are invariant under coordinated rotations. We demonstrate that the charge $J_γ$ of the emitted harmonics scales linearly with the harmonic order, …
We propose the effective simulation of light-matter ultrastrong-coupling phenomena with strong-coupling systems. Recent theory and experiments have shown that the quantum Rabi Hamiltonian can be simulated by a Jaynes--Cummings system with the addition of two classical drives. This allows to implement nonlinear processes that do not conserve the total number of excitations. However, parity is still a conserved quantity in the quantum Rabi Hamiltonian, which forbids a wide family of processes involving virtual transitions that break this conservation. Here, we show that these parity-non-conservi…
We consider the question of whether it is possible to use the entanglement between spatially separated modes of massive particles to observe nonlocal quantum correlations. Mode entanglement can be obtained using a single particle, indicating that it requires careful consideration before concluding whether experimental observation, e.g. violation of Bell inequalities, is possible or not. In the simplest setups analogous to optics experiments, that observation is prohibited by fundamental conservation laws. However, we show that using auxiliary particles, mode entanglement can be converted into …
Imaging systems measuring intensity in the far field succumb to Rayleigh's curse, a resolution limitation dictated by the finite aperture of the optical system. Many proof-of-principle and some two-dimensional imaging experiments have shown that, by using spatial mode demultiplexing (SPADE), the field information collected is maximal, and thus, the resolution increases beyond the Rayleigh criterion. Hitherto, the SPADE approaches are based on resolving the lateral splitting of a Gaussian wavefunction. Here, we consider the case in which the light field originates from a bi-photon source, i.e. …
In this paper we extend the investigation of Adami and Ver Steeg [Class. Quantum Grav. \textbf{31}, 075015 (2014)] to treat the process of black hole particle emission effectively as the analogous quantum optical process of parametric down conversion (PDC) with a dynamical (depleted vs. non-depleted) `pump' source mode which models the evaporating black hole (BH) energy degree of freedom. We investigate both the short time (non-depleted pump) and long time (depleted pump) regimes of the quantum state and its impact on the Holevo channel capacity for communicating information from the far past …
