We report on an experiment demonstrating the conservation of orbital angular momentum in stimulated down-conversion. The orbital angular momentum is not transferred to the individual beams of the spontaneous down-conversion, but it is conserved when twin photons are taken individually. We observe the conservation law for an individual beam of the down-conversion through cavity-free stimulated emission.
We observe experimentally the transfer of angular spectrum and image formation in the process of stimulated parametric down-conversion. Images and interference patterns can be transferred either from the pump or the auxiliary laser beams to the stimulated down-converted one. The stimulated field propagates as the complex conjugate of the auxiliary laser. The phase conjugation is observed through intensity pattern measurements.
We show how stimulated parametric processes can be employed in experiments on beyond the diffraction limit to overcome the problem of low visibility obtained by using spontaneous down conversion operating in the high gain regime. We further show enhancement of the count rate by several orders when stimulated parametric processes are used. Both the two photon counts and the visibility can be controlled by the phase of the stimulating coherent beam.
We theoretically discuss one-photon and two-photon double-slit interferences for spontaneous and stimulated parametric down-conversions. We show that the two-photon sub-wavelength interference can exist in a general spontaneous parametric down-conversion (SPDC) for both type I and type II crystals. We propose an alternative way to observe sub-wavelength interference by a joint-intensity measurement which occurs for only type I crystal in a higher gain of SPDC. When a signal beam injects into the crystal, it may create two interference patterns by two stimulated down-converted beams, showing no…
Spontaneous parametric down conversion (SPDC) has been largely exploited as a tool for absolute calibration of photon-counting detectors, i.e detectors registering very small photon fluxes. In [J. Opt. Soc. Am. B 23, 2185 (2006)] we derived a method for absolute calibration of analog detectors using SPDC emission at higher photon fluxes, where the beam is seen as a continuum by the detector. Nevertheless intrinsic limitations appear when high-gain regime of SPDC is required to reach even larger photon fluxes. Here we show that stimulated parametric down conversion allow one to avoid this limit…
Spontaneous parametric down conversion has been largely exploited as a tool for absolute calibration of photon counting detectors, photomultiplier tubes or avalanche photodiodes working in Geiger regime. In this work we investigate the extension of this technique from very low photon flux of photon counting regime to the absolute calibration of analog photodetectors at higher photon flux. Moving toward higher photon rate, i.e. at high gain regime, with the spontaneous parametric down conversion shows intrinsic limitations of the method, while the stimulated parametric down conversion process, …
The intensity transverse profile of the light produced in the process of stimulated down-conversion is derived. A quantum-mechanical treatment is used. We show that the angular spectrum of the pump laser can be transferred to the stimulated down-converted beam, so that images can also be transferred from the pump to the down-converted beam. We also show that the transfer can occur from the stimulating beam to the down-converted one. Finally, we study the process of diffraction through an arbitrarily shaped screen. For the special case of a double-slit, the interference pattern is explicitly ob…
We address the process of generation of the photon-number entangled states of light in the stimulated nonlinear parametric down conversion process and build the simple model describing the generation, not involving the traditional parametric approximation. The motion equations for the system of pumping and two-mode outgoing field are solved for the case of the strong correlation between two modes, the evolution of the state parameters of the generated modes is obtained. The solution is briefly analyzed for particular types of photon-number entangled states.
Three-fold coincidence by stimulated parametric down-conversion
Nexus for Quantum Technologies, University of Ottawa（渥太华大学量子技术联盟）；Department of Physics, University of Naples Federico II（那不勒斯费德里科二世大学物理系）；Faculty of Engineering and Institute of Nanotechnology and Advanced Materials, Bar-Ilan University（巴伊兰大学工程学院与纳米技术及先进材料研究所）；Institute for Quantum Studies, Chapman University（查普曼大学量子研究学院）
A detailed analysis of the stimulated parametric down-conversion (PDC) process is performed to investigate the effects of the spatiotemporal degrees of freedom. The analysis provides information that would be useful for PDC-based metrology applications. Using a Wigner functional approach, we obtain the parametric down-converted state as the Bogoliubov transformed input state, in terms of Bogoliubov kernel functions. The result is used to consider the case for a coherent state seeding stimulated PDC. We also compute the background which is obtained from spontaneous PDC.
We present a quantum optics approach for describing stimulated parametric down conversion in the two type-I crystal "sandwich" configuration, which allows for parametric interaction of vector vortex beams. We analyze the conditions for which phase conjugation of the seed vector beam occurs. We then use two strategies for defining generalized Stokes parameters to describe phase conjugation of vector vortex beams. These allow for geometrical representations, such as higher-order Poincaré spheres. Our results are useful for description and design of stimulated and spontaneous parametric down conv…
We show how to reach high fidelity NOON states with a high count rate inside optical interferometers. Recently it has been shown that by mixing squeezed and coherent light at a beamsplitter it is possible to generate NOON states of arbitrary N with a fidelity as high as 94%. (Afek I. et al. Science 328, 879 (2010)). The scheme is based on higher order interference between "quantum" down-converted light and "classical" coherent light. However, this requires optimizing the amplitude ratio of classical to quantum light thereby limiting the overall count rate for the interferometric super-resoluti…
We investigate the effect of the cumulative phase on the photon statistics of the three-mode state whose evolution is described by the trilinear Hamiltonian $\hat{H}_{I}=i\hbarκ\big(\hat{a}\hat{b}\hat{c}^{\dagger}-\hat{a}^{\dagger}\hat{b}^{\dagger}c\big)$, wherein the pump is taken to be quantized (and prepared in a coherent state) and the signal and idler modes are initially seeded with coherent states. We provide a brief review of the two-mode squeezed coherent states generated by non-degenerate coherently-stimulated parametric down-conversion, whereby the nonlinear crystal is driven by a st…
We present a new method for the spectral characterization of pulsed twin beam sources in the high gain regime, using cascaded stimulated emission. We show an implementation of this method for a ppKTP spontaneous parametric down-conversion source generating up to 60 photon pairs per pulse, and demonstrate excellent agreement between our experiments and our theory. This work enables the complete and accurate experimental characterization of high gain effects in parametric down conversion, including self and cross-phase modulation. Moreover, our theory allows the exploration of designs with the g…
We study the two-photon detection amplitude of the down-converted beams in spontaneous parametric down-conversion when the physical variable of orbital angular momentum is involved, taking into account both conservation and non-conservation of angular momentum. Agreeing with experimental observations, our theoretical calculation shows that spatial structure of the two-photon detection amplitude of the down-converted beams carries important information about conservation or non-conservation of orbital angular momentum in spontaneous parametric down-conversion.
The advanced-wave picture is "... an intuitive treatment of two-photon correlation with the help of the concept of an effective field acting upon one of the two detectors and formed by parametric conversion of the advanced wave emitted by the second detector ..." [A. V. Belinskii and D. N. Klyshko, JETP 78, 259 (1994)]. This quote from Belinskii and Klyshko nicely describes the concept of the advanced-wave picture; an intuitive tool for designing and predicting results from coincidence-based two-photon experiments. Up to now, the advanced-wave picture has been considered primarily for the case…
Coherence can be induced or stimulated in parametric down-conversion using two or three crystals when, for example, the idler modes of the crystals are aligned. Previous experiments with induced coherence [Phys. Rev. Lett. 114, 053601 (2015)] focused on which-path information and the role of vacuum fields in realizing complementarity via reduced visibility in single-photon interference. Here we describe experiments comparing induced and stimulated coherence. Different single-photon interference experiments were performed by blocking one of the pump beams in a three-crystal setup. Each counted …
Third-order parametric down-conversion (TOPDC) describes a class of nonlinear interactions in which a pump photon is converted into a photon triplet. This process can occur spontaneously, or it can be stimulated by seeding fields. In the former case, one typically has the generation of non-Gaussian states of light. In the latter, the situation is more variegated, for stimulated TOPDC (StTOPDC) can be implemented in many ways, depending on the number and properties of the seeding fields. Here we show that StTOPDC can be exploited for the generation of quantum correlated photon pairs. We examine…
Robust stimulated Raman exact passages are requisite for controlling nonlinear quantum systems, with the wide applications ranging from ultracold molecules, non-linear optics to superchemistry. Inspired by shortcuts to adiabaticity, we propose the fast-forward scaling of stimulated Raman adiabatic processes with the nonlinearity involved, describing the transfer from an atomic Bose-Einstein condensate to a molecular one by controllable external fields. The fidelity and robustness of atom-molecule conversion are shown to surpass those of conventional adiabatic passages, assisted by fast-forward…
We show that the transfer of the plane wave spectrum of the pump beam to the fourth-order transverse spatial correlation function of the two-photon field generated by spontaneous parametric down-conversion leads to the conservation and entanglement of orbital angular momentum of light. By means of a simple experimental setup based on fourth-order (or two-photon) interferometry, we show that our theoretical model provides a good description for down-converted fields carrying orbital angular momentum.
Using on-demand coherence conversion via optical locking in conventional stimulated (three-pulse) photon echoes, ultralong, ultraefficient photon storage has been observed in a rare-earth Pr3+ doped Y2SiO5, where storage time is several orders of magnitude longer and retrieval efficiency is enhanced by fifty times. Compared with the same method applied to two-pulse photon echoes for a rephasing halt, use of spectral grating in the stimulated photon echoes offers a phase-independent coherence conversion between optical and spin states. Eventually an ultralong spin population decay-dependent pho…
We show that the transfer of the angular spectrum of the pump beam to the two-photon state in spontaneous parametric down-conversion enables the generation of entangled Hermite-Gaussian modes. We derive an analytical expression for the two-photon state in terms of these modes and show that there are restrictions on both the parity and order of the down-converted Hermite-Gaussian fields. Using these results, we show that the two-photon state is indeed entangled in Hermite-Gaussian modes. We propose experimental methods of creating maximally-entangled Bell states and non-maximally entangled pure…
We consider a quantum memory scheme based on the conversion of a signal pulse into a long-lived spin coherence via stimulated off-resonant Raman process. For a storing medium consisting of alkali atoms, we have calculated the Autler-Townes resonance structure created by a strong control field. By taking into account the upper hyperfine states of the D1 optical transition, we show important deviations from the predictions of the usual three-level Lambda-scheme approximation and we demonstrate an enhancement of the process for particular detunings of the control. We estimate the memory efficienc…
Stimulated Parametric Down-Conversion: From Foundational Coherence to Structured Light Applications
Instituto Federal de Mato Grosso（马托格罗索联邦学院）；Departamento de Física, Universidade Federal de Santa Catarina（圣卡塔琳娜联邦大学物理系）；Universidad de Concepción（孔塞普西翁大学）；Millennium Institute for Research in Optics, Universidad de Concepción（孔塞普西翁大学光学研究千年研究所）
Optical parametric down-conversion (PDC) is a central tool in quantum optics experiments. The number of collected down-converted modes greatly affects the quality of the produced photon state. We use Silicon Photomultiplier (SiPM) number-resolving detectors in order to directly observe the photon-number distribution of a PDC source, and show its dependence on the number of collected modes. Additionally, we show how the stimulated emission of photons and the partition of photons into several modes determine the overall photon number. We present a novel analytical model for the optical crosstalk…
We compute the output of multimode cavity-enhanced spontaneous parametric down-conversion (SPDC) for sub-threshold, but otherwise arbitrary, gain. We find analytic Bogoliubov transformations that allow us to calculate arbitrary field correlation functions, including the second-order intensity correlation function $G^{(2)}(T)$. The results show evidence of increased coherence due to stimulated SPDC. We extend an earlier model [Lu and Ou, Phys. Rev. A, 62, 033804 (2000)] to arbitrary gain and finesse, and show the extension gives accurate results in most scenarios. The results will allow simple,…
Nonlinear optical frequency conversion, observed more than half a century ago, is a corner stone in modern applications of nonlinear and quantum optics. It is well known that frequency conversion processes are constrained by conservation laws, such as momentum conservation that requires phase matching conditions for efficient conversion. However, conservation laws alone could not fully capture the features of nonlinear frequency conversion. Here it is shown that topology can provide additional constraints in nonlinear multi-frequency conversion processes. Unlike conservation laws, a topologica…
Third order parametric down-conversion describes a class of nonlinear processes in which a pump photon can be down-converted into triplets of photons. It has been identified as a source of non-classical light, with capabilities beyond those offered by better-established processes such as spontaneous four-wave mixing. Here we discuss the implementation of TOPDC in integrated photonic systems. We derive equations for the rates of TOPDC in a non-resonant (waveguide) and resonant (microring) platform, such that the scaling with experimental parameters can be plainly seen. We find that generally no…
Entanglement of high dimensional states is becoming increasingly important for quantum communication and computing. The most common source of entangled photons is spontaneous parametric down conversion (SPDC), where the degree of frequency and momentum entanglement is determined by the non-linear interaction volume. Here we show that by reducing the length of a highly non-linear material to the micrometer scale it is possible to relax the longitudinal phase matching condition and reach record levels of transverse wavevector entanglement. From a micro-sized layer of lithium niobate we estimate …
Quantum entanglement associated with transverse wave vectors of down conversion photons is investigated based on the Schmidt decomposition method. We show that transverse entanglement involves two variables: orbital angular momentum and transverse frequency. We show that in the monochromatic limit high values of entanglement are closely controlled by a single parameter resulting from the competition between (transverse) momentum conservation and longitudinal phase matching. We examine the features of the Schmidt eigenmodes, and indicate how entanglement can be enhanced by suitable mode selecti…
Parametric down-conversion (PDC) offers the possibility to control the fabrication of non-Gaussian states such as Fock states. However, in conventional PDC sources energy and momentum conservation introduce strict frequency and photon number correlations, which impact the fidelity of the prepared state. In our work we optimize the preparation of single-photon Fock states from the emission of waveguided PDC via spectral filtering. We study the effect of correlations via photon number resolving detection and quantum interference. Our measurements show how the reduction of mixedness due to filter…
Strong correlations in two conjugate variables are the signature of quantum entanglement and have played a key role in the development of modern physics. Entangled photons have become a standard tool in quantum information and foundations. An impressive example is position-momentum entanglement of photon pairs, explained heuristically through the correlations implied by a common birth zone and momentum conservation. However, these arguments entirely neglect the importance of the `quantumness', i.e. coherence, of the driving force behind the generation mechanism. We study theoretically and expe…
Light beams with orbital angular momentum (OAM) are convenient carriers of quantum information. They can be also used for imparting rotational motion to particles and provide high resolution in imaging. Due to the conservation of OAM in parametric down-conversion (PDC), signal and idler photons generated at low gain have perfectly anti-correlated OAM values. It is interesting to study the OAM properties of high-gain PDC, where the same OAM modes can be populated with large, but correlated, numbers of photons. Here we investigate the OAM spectrum of high-gain PDC and show that the OAM mode cont…
We report, for the first time, the generation of entangled photon pairs via type-0 spontaneous parametric down conversion in an ultra-thin wafer of lithium niobate in which momentum between the pump photon and daughter photons is not conserved. The characteristics of the emission are investigated using several techniques. We find that non-phase matched SPDC is a promising source of ultra-broadband two photon radiation that exhibits remarkably tight correlation widths in both the spatial and temporal domains.
Ultracompact nonlinear optical devices utilizing two-dimensional (2D) materials and nanostructures are emerging as important elements of photonic circuits. Integration of the nonlinear material into a subwavelength cavity or waveguide leads to a strong Purcell enhancement of the nonlinear processes and compensates for a small interaction volume. The generic feature of such devices which makes them especially challenging for analysis is strong dissipation of both the nonlinear polarization and highly confined modes of a subwavelength cavity. Here we solve a quantum-electrodynamic problem of the…
Photonic quantum technologies$^1$, with applications in quantum communication, sensing as well as quantum simulation and computing, are on the verge of becoming commercially available. One crucial building block are tailored nanoscale integratable quantum light sources, matching the specific needs of use-cases. Several different approaches to realize solid-state quantum emitters$^2$ with high performance$^3$ have been pursued. However, the properties of the emitted single photons are always defined by the individual quantum light source and despite numerous quantum emitter tuning techniques$^{…
Decay of a particle into more particles is a ubiquitous phenomenon to interacting quantum systems, taking place in colliders, nuclear reactors, or solids. In a non-linear medium, even a single photon would decay by down-converting (splitting) into lower frequency photons with the same total energy, at a rate given by Fermi's Golden Rule. However, the energy conservation condition cannot be matched precisely if the medium is finite and only supports quantized modes. In this case, the photon's fate becomes the long-standing question of many-body localization (MBL), originally formulated as a ged…
We solve a model that describes a stimulated conversion between ultracold bosonic atoms and molecules. The reaction is triggered by a linearly time-dependent transition throughout the Feshbach resonance. Our solution predicts a nonexponential dependence, with a dynamic phase transition, of the reaction efficiency on the transition rate. We find that the emerging phase can have a thermalized energy distribution with the temperature defined by the rate of the transition. This phase, however, has strong purely quantum correlations.
