We describe an experiment in which photon pairs from a pulsed parametric down-conversion source were coupled into single-mode fibers. Detecting one of the photons heralded the presence of the other photon in its fiber with a probability of 83%. The heralded photons were then used in a simple multi-photon interference experiment to illustrate their potential for quantum information applications.
We present serial-parallel conversion for a heralded single photon source (heralded SPS). We theoretically show that with the heralding signal, the serial-parallel converter can route a stream of n photons to n different spatial modes more efficiently than is the case without using a heralding signal. We also experimentally demonstrate serial-parallel conversion for two photons generated from a heralded SPS. We achieve a conversion efficiency of 0.533 \pm 0.003, which exceeds the maximum achievable efficiency of 0.5 for serial-parallel conversion using unheralded photons, and is double the eff…
Entanglement is a unique property of quantum systems and an essential resource for many quantum technologies. The ability to transfer or swap entanglement between systems is an important protocol in quantum information science. Entanglement between photons forms the basis of distributed quantum networks and the demonstration of photonic entanglement swapping is essential for their realization. Here an experiment demonstrating entanglement swapping from two independent multimode time-frequency entangled sources is presented, resulting in multiple heralded temporal-mode Bell states. Entanglement…
We report on the realization of a synchronous source of heralded single photons at telecom wavelengths with MHz heralding rates and high heralding efficiency. This source is based on the generation of photon pairs at 810 and 1550 nm via Spontaneous Parametric Down Conversion (SPDC) in a 1 cm periodically poled lithium niobate (PPLN) crystal pumped by a 532 nm pulsed laser. As high rates are fundamental for multi-photon experiments, we show that single telecom photons can be announced at 4.4MHz rate with 45% heralding efficiency. When we focus only on the optimization of the coupling of the her…
We explore the feasibility of using high conversion-efficiency periodically-poled crystals to produce photon pairs for photon-counting detector calibrations at 1550 nm. The goal is the development of an appropriate parametric down-conversion (PDC) source at telecom wavelengths meeting the requirements of high-efficiency pair production and collection in single spectral and spatial modes (single-mode fibers). We propose a protocol to optimize the photon collection, noise levels and the uncertainty evaluation. This study ties together the results of our efforts to model the single-mode heralding…
The nonlinear optical process of spontaneous parametric down-conversion (SPDC) is widely studied for applications in quantum information science due to its ability to produce two photons that can be entangled in many degrees of freedom. For applications in quantum communication, two metrics of this process are particularly important: heralding efficiency and total joint rate. Here, we derive expressions for both quantities for a variety of different beam geometries and frequencies. We pay specific attention to the spectrum of both biphotons and individual photons. We reveal the underlying mech…
Heralding of single photon at 1550 nm from pump pulsed non degenerate spontaneous parametric downconversion is demonstrated. P(1) and P(2) of our source are 0.1871 and 2.4 x 10 ^-3 respectively. Triggering of our source is 2.16 x 10^5 trigger.s^-1. This source may be used in QKD system.
Heralding efficiency and brightness optimization of a micro-ring resonator via tunable coupling
Quantum Engineering Technology Labs, H. H. Wills Physics Laboratory and School of Electrical, Electronic and Mechanical Engineering, University of Bristol（布里斯托大学电气、电子和机械工程学院、H.H.威尔斯物理实验室量子工程技术实验室）；School of Mathematical and Physical Sciences, University of Sheffield（谢菲尔德大学数学与物理科学学院）
Single photons are an important prerequisite for a broad spectrum of quantum optical applications. We experimentally demonstrate a heralded single-photon source based on spontaneous parametric down-conversion in collinear bulk optics, and fiber-coupled bolometric transition-edge sensors. Without correcting for background, losses, or detection inefficiencies, we measure an overall heralding efficiency of 83 %. By violating a Bell inequality, we confirm the single-photon character and high-quality entanglement of our heralded single photons which, in combination with the high heralding efficienc…
We investigate the possibility of generating pure heralded single photons through spontaneous parametric down-conversion comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. We estimate the Schmidt number associated to the temporal modes as a function of the pump pulse duration for three particular configurations, showing how the different phase-matching conditions influences the degree of separability that can be achieved.
Evolving photonic quantum technologies and applications require higher and higher rates of single photon generation. In parallel, it is required that these generated photons are kept spectrally pure for multi-photon experiments and that multi-photon noise be kept to a minimum. In spontaneous parametric down-conversion sources, these requirements are conflicting, because spectral filtering to increase spectral purity always means lowering the rate at which photons are generated, and increasing the pump power means increasing the multi-photon noise. In this paper, we present a scheme, called ext…
Photon pairs produced by parametric down-conversion or four-wave mixing can interfere with each other in multiport interferometers, or carry entanglement between distant nodes for use in entanglement swapping. This requires the photons be spectrally pure to ensure good interference, and have high heralding efficiency to know accurately the number of photons involved and to maintain high rates as the number of photons grows. Spectral filtering is often used to remove noise and define spectral properties. For heralded single photons high purity and heralding efficiency is possible by filtering t…
I investigate the properties of spontaneous parametric down-conversion (SPDC) involving co-linear Gaussian spatial modes for the pump and the photon collection optics. Approximate analytical and numerical results are obtained for the peak spectral density, photon bandwidth, pair collection probability, heralding ratio, and spectral purity, as a function of crystal length and beam focusing parameters. I address the optimization of these properties individually as well as jointly, and find focusing conditions that simultaneously bring the pair collection probability, heralding ratio, and spectra…
We investigate different strategies suitable to generate pure heralded single photons through spontaneous parametric down-conversion, comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. Our analysis is based on the correlation of twin photons in the temporal domain,a non-standard approach that provides a physical view of the mechanisms that permit to eliminate the temporal entanglement of the state and to generate high-purity heralde…
Fast and complete characterization of pulsed spontaneous parametric down conversion (SPDC) sources is important for applications in quantum information processing and communications. We propose a simple method to perform this task, which only requires measuring the counts on the two output channels and the coincidences between them, as well as modeling the filter used to reduce the source bandwidth. The proposed method is experimentally tested and used for a complete evaluation of SPDC sources (pair emission probability, total losses, and fidelity) of different bandwidths. This method can find…
The ideal photon-pair source for building up multi-qubit states needs to produce indistinguishable photons with high efficiency. Indistinguishability is crucial for minimising errors in two-photon interference, central to building larger states, while high heralding rates will be needed to overcome unfavourable loss scaling. Domain engineering in parametric down-conversion sources negates the need for lossy spectral filtering allowing one to satisfy these conditions inherently within the source design. Here, we present a telecom-wavelength parametric down-conversion photon source that operates…
We analyze theoretically performance of four-state quantum key distribution protocols implemented with a realistic heralded single-photon source. The analysis assumes a noisy model for the detector heralding generation of individual photons via spontaneous parametric down-conversion, including dark counts and imperfect photon number resolution. We identify characteristics of the heralding detector that defines the attainable cryptographic key rate and the maximum secure distance. Approximate analytical formulas are applied to multiplexed detection and compared with results of numerical calcula…
We report on a systematic experimental study of heralding efficiency and generation rate of telecom-band infrared photon pairs generated by spontaneous parametric down-conversion and coupled to single mode optical fibers. We define the correlated-mode coupling efficiency--an inherent source efficiency--and explain its relation to heralding efficiency. For our experiment, we developed a reconfigurable computer controlled pump-beam and collection-mode optical apparatus which we used to measure the generation rate and correlated-mode coupling efficiency. The use of low-noise, high-efficiency supe…
Frequency encoding is quickly becoming an attractive prospect for quantum information protocols owing to larger Hilbert spaces and increased resilience to noise compared to other photonic degrees of freedom. To fully make use of frequency encoding as a practical paradigm for QIP, an efficient and simple source of frequency entanglement is required. Here we present a single-pass source of discrete frequency-bin entanglement which does not use filtering or a resonant cavity. We use a domain-engineered nonlinear crystal to generate an eight-mode frequency-bin entangled source at telecommunication…
Heralded spontaneous parametric down-conversion (SPDC) has become the mainstay for single-photon state preparation in present-day photonics experiments. Because they are heralded, in principle one knows when a single photon has been prepared. However, the heralding efficiencies in experimentally realistic SPDC sources are typically very low. To overcome this, multiplexing techniques have been proposed which employ a bank of SPDC sources in parallel, and route successfully heralded photons to the output, thereby effectively boosting the heralding efficiency. However, running a large bank of ind…
We present a simple technique to reduce the emission rate of higher-order photon events from pulsed spontaneous parametric down-conversion. The technique uses extra-cavity control over a mode locked ultrafast laser to simultaneously increase repetition rate and reduce the energy of each pulse from the pump beam. We apply our scheme to a photonic quantum gate, showing improvements in the non-classical interference visibility for 2-photon and 4-photon experiments, and in the quantum-gate fidelity and entangled state production in the 2-photon case.
Gaussian mode coupling of spectrally broadband photons from bulk spontaneous parametric down-conversion: A spatial-spectral mode analysis of fiber coupling
Fraunhofer Institute for Applied Optics and Precision Engineering（弗劳恩霍夫应用光学和精密工程研究所）；Friedrich Schiller University Jena, Institute of Applied Physics, Abbe Center of Photonics（耶拿弗里德里希·席勒大学应用物理学院阿贝光子学中心）
A new ultra bright pulsed source of polarization entangled photons has been realized using type-II phase matching in spontaneous parametric down conversion process in two cascaded crystals. The optical axes of the crystals are aligned in such a way that the extraordinarily (ordinarily) polarized cone from one crystal overlaps with the ordinarily (extraordinarily) polarized cone from the second crystal. This spatial overlapping removes the association between the polarization and the output angle of the photons that exist in a single type-II down conversion process. Hence, entanglement of photo…
Based on the signal and idler photon pairs produced in a piece of high nonlinear fiber by a pulsed pump, we characterize the heralded single photon source from both the theoretical and experimental aspects. In the theory model, started from the derived expression of Bogoliubov transformation for a broadband pulsed pump, the second-order intensity correlation function $g_c^{(2)}(0)$, heralding efficiency $H$, indistinguishability and brightness of the heralded single photons as a function of source parameters are analyzed and discussed. In the experiments, using several kinds of combinations of…
Parametric down-conversion (PDC) is one of the most widely used methods to create pure single-photon states for quantum information applications. However little attention has been paid to higher-order photon components in the PDC process, yet these ultimately limit the prospects of generating single-photons of high quality. In this paper we investigate the impacts of higher-order photon components and multiple frequency modes on the heralding rates and single-photon fidelities. This enables us to determine the limits of PDC sources for single-photon generation. Our results show that a perfectl…
Entangled photon sources with simultaneously near-unity heralding efficiency and indistinguishability are the fundamental elements for scalable photonic quantum technologies. We design and realize a degenerate entangled-photon source from an ultrafast pulsed laser pumped spontaneous parametric down-conversion (SPDC), which show simultaneously ~97% heralding efficiency and ~96% indistinguishability between independent single photons. Such a high-efficiency and frequency-uncorrelated SPDC source allows generation of the first 12-photon genuine entanglement with a state fidelity of 0.572(24). We …
We analyze the generation rates and preparation fidelities of photon triplet states in pulsed cascaded parametric down-conversion (PDC) under realistic experimental circumstances. As a model system, we assume a monolithically integrated device with negligible interface loss between the two consecutive PDC stages. We model the secondary down-conversion process in terms of a lossy channel and provide a detailed analysis of noise contributions. Taking variable pump powers into account, we estimate the impact of higher-order photon contributions and conversion processes on the achievable coinciden…
We describe an experimental demonstration of a novel three-photon NOON state generator using a single source of photons based on spontaneous parametric down-conversion (SPDC). The three-photon number-entangled state is deterministically generated by the detection of a heralding photon. Interference fringes measured with an emulated three-photon absorber reveal the three-photon de Broglie wavelength and exhibit visibility > 70% without background subtraction.
We present a detailed study on the properties of single photons generated by spontaneous parametric down conversion (SPDC) when both the spectral and spatial degrees of freedom are controlled by means of filters. Our results show that it is possible to obtain pure heralded single photons with high heralding efficiency despite the use of filters. Moreover, we report an asymmetry on the single photon properties exhibited in type-II SPDC sources that depends on choosing the signal or the idler photon as the heralding one.
In the development of quantum microwave-to-optical (MO) converters, excessive noise induced by the parametric optical drive remains a major challenge at milli-Kelvin temperatures. Here we study the extraneous noise added to an electro-optic transducer in its quantum ground state under an intense pulsed optical excitation. The integrated electro-optical transducer leverages the inherent Pockels effect of aluminum nitride microrings, flip-chip bonded to a superconducting resonator. Applying a pulsed optical drive with peak power exceeding the cooling power of the dilution refrigerator at its bas…
We report on quantum frequency conversion of memory-compatible narrow-bandwidth photons at 606 nm to the telecom C-band at 1552$\,$nm. The 200$\,$ns long photons, compatible with Praseodymium-based solid-state quantum memories are frequency converted using a single-step difference frequency generation process in a periodically poled Lithium Niobate waveguide. We characterize the noise processes involved in the conversion and by applying strong spectral filtering of the noise, we demonstrate high signal-to-noise ratio conversion at the single photon level (SNR$\,>\,$100 for a mean input photon …
We study the spectral properties of Spontaneous Parametric Down Conversion in a periodically poled waveguided structure of KTP crystal pumped by ultra-short pulses. Our theoretical analysis reveals a strongly multimode and asymmetric structure of the two-photon spectral amplitude for type-II SPDC. Experimental evidence, based on Hong-Ou-Mandel polarization interference with narrowband filtering, confirms this result.
We experimentally investigate a double-pass parametric down-conversion scheme for producing pulsed, polarization-entangled photon pairs with high visibility. The amplitudes for creating photon pairs on each pass interfere to compensate for distinguishing characteristics that normally degrade two-photon visibility. The result is a high-flux source of polarization-entangled photon pulses that does not require spectral filtering. We observe quantum interference visibility of over 95% without the use of spectral filters for 200 femtosecond pulses, and up to 98.1% with 5 nm bandwidth filters.
The dependence of one- and two-photon characteristics of pulsed entangled two-photon fields generated in spontaneous parametric down-conversion on the pump-pulse properties (shape of the pump-pulse spectrum and its internal structure) is examined. It is shown that entangled two-photon fields with defined properties can be generated. A general relation between the spectra of the down-converted fields is established. As a special case interference of two partially overlapping pulsed two-photon fields is studied. Fourth-order interference pattern of entangled two-photon fields is investigated in …
We investigate quantum properties of pulsed light fields point by point in phase space. We probe the negative region of the Wigner function of a single photon generated by the means of waveguided parametric down-conversion. This capability is achieved by employing loss-tolerant photon-number resolving detection, allowing us to directly observe the oscillations of the photon statistics in dependence of applied displacements in phase space. Our scheme is highly mode sensitive and can reveal the single-mode character of the signal state.
We demonstrate a novel scheme for femto-second pulsed spontaneous parametric down-conversion in periodically poled KTP crystals. Our scheme is based on a crossed crystal configuration with collinear quasi-phase-matching. The non-degenerate photon pairs are split in a fiber-based wavelength division multiplexer. The source is easier to align than common pulsed sources based on bulk BBO crystals and exhibits high-quality polarization entanglement as well as non-classical interference capabilities. Hence, we expect this source to be a well-suited candidate for multi-photon state generation e.g. f…
We present the generation of approximated coherent state superpositions - referred to as Schrödinger cat states - by the process of subtracting single photons from picosecond pulsed squeezed states of light at 830 nm. The squeezed vacuum states are produced by spontaneous parametric down-conversion (SPDC) in a periodically poled KTiOPO4 crystal while the single photons are probabilistically subtracted using a beamsplitter and a single photon detector. The resulting states are fully characterized with time-resolved homodyne quantum state tomography. Varying the pump power of the SPDC, we genera…
We report on a source of heralded narrowband (3MHz) single photons compatible with solid-state spin-wave quantum memories based on praseodymium doped crystals. Widely non-degenerate narrow-band photon pairs are generated using cavity enhanced down conversion. One photon from the pair is at telecom wavelengths and serves as heralding signal, while the heralded single photon is at 606nm, resonant with an optical transition in Pr:YSO. The source offers a heralding efficiency of 28% and a generation rate exceeding 2000 pairs/mW in a single-mode. The single photon nature of the heralded field is co…
Frequency conversion (FC) and type-II parametric down-conversion (PDC) processes serve as basic building blocks for the implementation of quantum optical experiments: type-II PDC enables the efficient creation of quantum states such as photon-number states and Einstein-Podolsky-Rosen-states (EPR-states). FC gives rise to technologies enabling efficient atom-photon coupling, ultrafast pulse gates and enhanced detection schemes. However, despite their widespread deployment, their theoretical treatment remains challenging. Especially the multi-photon components in the high-gain regime as well as …
We report a novel Bell state preparation experiment. High-purity Bell states are prepared by using femtosecond pulse pumped \emph{nondegenerate} collinear spontaneous parametric down-conversion. The use of femtosecond pump pulse {\em does not} result in reduction of quantum interference visibility in our scheme in which post-selection of amplitudes and other traditional mechanisms, such as, using thin nonlinear crystals or narrow-band spectral filters are not used. Another distinct feature of this scheme is that the pump, the signal, and the idler wavelengths are all distinguishable, which is …
We present an apparatus that converts every pulse of a pulsed light source to a pulse train in which the intensities of the different pulses are samples of the spatial or temporal frequency spectrum of the original pulse. In this way, the spectrum of the incident light can be measured by following the temporal response of a single detector. The apparatus is based on multiple round-trips inside a 2f- cavity-like mirror arrangement in which the spectrum is spread on the back focal plane, where after each round-trip a small section of the spectrum is allowed to escape. The apparatus is fibre-free…
We study the process of co-polarized spontaneous four-wave mixing in single-mode optical fibers, with an emphasis on an analysis of the conversion efficiency. We consider both the monochromatic-pumps and pulsed-pumps regimes, as well as both the degenerate-pumps and non-degenerate-pumps configurations. We present analytical expressions for the conversion efficiency, which are given in terms of double integrals. In the case of pulsed pumps we take these expressions to closed analytical form with the help of certain approximations. We present results of numerical simulations, and compare them to…
Coherence properties of the down-converted beams generated in spontaneous parametric down-conversion are investigated in detail using an iCCD camera. Experimental results are compared with those from a theoretical model developed for pulsed pumping with a Gaussian transverse profile. The results allow to tailor the shape of correlation area of the signal and idler photons using pump-field and crystal parameters. As an example, splitting of a correlation area caused by a two-peak pump-field spectrum is experimentally studied.
We report a source of polarization-entangled photon pairs in the 1550-nm telecommunication band, which is based on non-collinear spontaneous parametric down-conversion in a periodically poled lithium niobate crystal pumped by picosecond pulses. This source is realized utilizing a polarization-based Sagnac interferometer employing a type-0 non-collinear quasi-phase-matching configuration. Polarization entanglement is verified through measurement of the polarization-correlation interference fringes with visibility >96% and by testing the experimental violation of the Clauser-Horne-Shimony-Holt (…
Various quantum technology applications require high-purity single photons with high generation rate. Although different methods are employed to generate such photons, heralded single photons from spontaneous parametric down-conversion (SPDC) is the most commonly used approach. Photon generation rate from the heralded single-photon sources are limited by the efficiency of the detectors to record coincidence detection of the photon pairs which are lower than the single-photon counts recorded separately on each detector. In this paper we present a revised expression to calculate second-order tem…
We study the spatial correlations of quantum fluctuations that can be observed in multi-mode spontaneous parametric down-conversion in the regime of high gain. A stochastic model has been solved numerically to obtain quantitative results beyond the stationary plane-wave pump approximation. The pulsed shape of the pump beam and other features of the system, such as spatial walk-off and diffraction are taken into account. Their effect on the spatial quantum correlations predicted by the plane-wave pump theory is investigated, both for near field and far field measurements, in a type I and in a t…
The generation of heralded pure Fock states via spontaneous parametric down conversion (PDC) relies on perfect photon-number correlations in the output modes. Correlations in any other degree of freedom, however, degrade the purity of the heralded state. In this paper, we investigate spectral entanglement between the two output modes of a periodically poled waveguide. With the intent of generating heralded 1- and 2-photon Fock states, we expand the output state of the PDC to second order in photon number. We explore the effects of spectral filtering and inefficient detection, of the heralding …
The ability to coherently convert the frequency and temporal waveform of single and entangled photons will be crucial to interconnect the various elements of future quantum information networks. Of particular importance in this context is the quantum frequency conversion of photons emitted by material systems able to store quantum information, so called quantum memories. There have been significant efforts to implement quantum frequency conversion using non linear crystals, with non classical light from broadband photon pair sources and solid state emitters. However, so far, solid state quantu…
We report on the generation of indistinguishable photon pairs at telecom wavelengths based on a type-II parametric down conversion process in a periodically poled potassium titanyl phosphate (PPKTP) crystal. The phase matching, pump laser characteristics and coupling geometry are optimised to obtain spectrally uncorrelated photons with high coupling efficiencies. Four photons are generated by a counter- propagating pump in the same crystal and anlysed via two photon interference experiments between photons from each pair source as well as joint spectral and g^(2) measurements. We obtain a spec…
We describe the results of a parametric down-conversion experiment in which the detection of one photon of a pair causes the other photon to be switched into a storage loop. The stored photon can then be switched out of the loop at a later time chosen by the user, providing a single photon for potential use in a variety of quantum information processing applications. Although the stored single photon is only available at periodic time intervals, those times can be chosen to match the cycle time of a quantum computer by using pulsed down-conversion. The potential use of the storage loop as a ph…
Mode-selective nonlinear interference for high-brightness and high-purity fiber-coupled SPDC sources
Fraunhofer Institute for Applied Optics and Precision Engineering（弗劳恩霍夫应用光学和精密工程研究所）；Friedrich Schiller University Jena, Institute of Applied Physics, Abbe Center of Photonics（耶拿弗里德里希·席勒大学应用物理学院阿贝光子学中心）
We study the physics of four-photon states generated in spontaneous parametric down-conversion with a pulsed pump field. In the limit where the coherence time of the photons t_c is much shorter than the duration of the pump pulse Delta t, the four photons can be described as two independent pairs. In the opposite limit, the four photons are in a four-particle entangled state. Any intermediate case can be characterized by a single parameter chi, which is a function of t_c/Delta t. We present a direct measurement of chi through a simple experimental setup. The full theoretical analysis is also p…
