We describe an experimental demonstration of a novel three-photon NOON state generator using a single source of photons based on spontaneous parametric down-conversion (SPDC). The three-photon number-entangled state is deterministically generated by the detection of a heralding photon. Interference fringes measured with an emulated three-photon absorber reveal the three-photon de Broglie wavelength and exhibit visibility > 70% without background subtraction.
We present an experiment of nonclassical interference between a pure heralded single-photon state and a weak coherent state. Our experiment is the first to demonstrate that spectrally pure single photons can have high interference visibility, 89.4 \pm 0.5%, with weak coherent photons. Our scheme lays the groundwork for future experiments requiring quantum interference between photons in nonclassical states and those in coherent states.
High visibility on-chip quantum interference among indistinguishable single-photons from multiples sources is a key prerequisite for integrated linear optical quantum computing. Resonant enhancement in micro-ring resonators naturally enables brighter, purer and more indistinguishable single-photon production without any tight spectral filtering. The indistinguishability of heralded single-photons from multiple micro-ring resonators has not been measured in any photonic platform. Here, we report on-chip indistinguishability measurements of heralded single-photons generated from independent micr…
We report on the observation of a high visibility Hong-Ou-Mandel interference of two heralded photons emitted from a spontaneous parametric down conversion~(SPDC) pumped by continuous-wave~(cw) light. A non-degenerate photon pair at 1541~nm and 1580~nm is generated by cw-pumped SPDC through a periodically poled lithium niobate waveguide. The heralded single photon at 1541~nm is prepared by the detection of the photon at 1580~nm. We performed the experiment of the Hong-Ou-Mandel interference between heralded single photons in separated time bins and observed a high visibility interference. All …
The challenging requirements of large scale quantum information processing using parametric heralded single photon sources involves maximising the interference visibility whilst maintaining an acceptable photon generation rate. By developing a general theoretical framework that allows us to include large numbers of spatial and spectral modes together with linear and non-linear optical elements, we investigate the combined effects of spectral and photon number impurity on the measured Hong--Ou--Mandel interference visibility of parametric photon sources, considering both threshold and number re…
We study the dynamics of entanglement in continuous variable quantum systems (CVQS). Specifically, we study the phenomena of Entanglement Sudden Death (ESD) in general two-mode-N-photon states undergoing pure dephasing. We show that for these states, ESD never occurs. These states are generalizations of the so-called High NOON states, shown to decrease the Rayleigh limit of lambda to lambda/N, which promises great improvement in resolution of interference patterns if states with large N are physically realized. However, we show that in dephasing NOON states, the time to reach V_crit, critical …
Indistinguishable photons play a key role in quantum optical information technologies. We characterize the output of an ultra-bright photon-pair source using multi-particle tomography [R. B. A. Adamson et al., Phys. Rev. Lett. 98, 043601 (2007)] and separately identify coherent errors, decoherence, and distinguishability. We demonstrate generation of high-quality indistinguishable pairs and polarization NOON states with 99% fidelity to an ideal NOON state. Using a NOON state we perform a super-resolving angular measurement with 90% visibility.
We present an experimental demonstration of heralded single photons prepared in pure quantum states from a parametric downconversion source. It is shown that, through controlling the modal structure of the photon pair emission, one can generate pairs in factorable states and thence eliminate the need for spectral filters in multiple-source interference schemes. Indistinguishable heralded photons were generated in two independent spectrally engineered sources, and, by performing a Hong-Ou-Mandel interference between them without spectral filters at a raw visibility of 94.4%, their purity was me…
NOON state interference (NOON-SI) is a powerful tool to improve the phase sensing precision, and can play an important role in quantum sensing and quantum imaging. However, most of the previous NOON-SI experiments only investigated the center part of the interference pattern, while the full range of the NOON-SI pattern has not yet been well explored.In this Letter, we experimentally and theoretically demonstrate up to six-photon NOON-SI and study the properties of the interference patterns over the full range.The multi-photons were generated at a wavelength of 1584 nm from a PPKTP crystal in a…
We propose an experimental scheme to generate, in a heralded fashion, arbitrary quantum superpositions of two-mode optical states with a fixed total photon number $n$ based on weakly squeezed two-mode squeezed state resources (obtained via weak parametric down conversion), linear optics, and photon detection. Arbitrary $d$-level (qudit) states can be created this way where $d=n+1$. Furthermore, we experimentally demonstrate our scheme for $n=2$. The resulting qutrit states are characterized via optical homodyne tomography. We also discuss possible extensions to more than two modes concluding t…
We present Hong-Ou-Mandel interference of single photons generated via two different physical processes by two independent atomic systems: scattering by a single atom, and parametric generation via four-wave mixing in a cloud of cold atoms. Without any spectral filtering, we observe a visibility of V=62$\pm$4%. After correcting for accidental coincidences, we obtain V=93$\pm$6%. The observed interference demonstrates the compatibility of the two sources, forming the basis for an efficient quantum interface between different physical systems.
Difference-phase (or Hanbury Brown - Twiss type) intensity interference of classical light is considered in higher orders in the intensity. It is shown that, while the visibility of sum-phase (NOON-type) interference for classical sources drops with the order of interference, the visibility of difference-phase interference has opposite behavior. For three-photon and four-photon interference of two coherent sources, the visibility can be as high as 81.8% and 94.4%, respectively. High-visibility three-photon and four-photon interference of space-time and polarization types has been observed in e…
We report on quantum frequency conversion of near-infrared photons from a wavelength of 854nm to the telecommunication O-band at 1310nm with 8% overall conversion efficiency. Entangled photon pairs at 854nm are generated via type-II spontaneous parametric down conversion. One photon is mixed with a strong pump field in a nonlinear ridge waveguide for its conversion to 1310nm. We demonstrate preservation of first and second order coherence of the photons in the conversion process. Based on this we infer the coherence function of the two-photon state and compare it with the actual measured one. …
NOON states are path entangled states which can be exploited to enhance phase resolution in interferometric measurements. In the present paper we analyze the quantum states obtained by optical parametric amplification of polarization NOON states. First we study, theoretically and experimentally, the amplification of a 2-photon state by a collinear Quantum Injected Optical Parametric Amplifier (QIOPA). We compared the stimulated emission regime with the spontaneous one, studied by Sciarrino et al. (PRA 77, 012324), finding comparable visibilities between the two cases but an enhancement of the …
We report measurements of time-frequency entangled photon pairs and heralded single photons at telecommunications wavelengths, generated using a periodically-poled, lithium niobate on insulator (LNOI) waveguide pumped optically by a diode laser. We achieve a high Coincidences-to-Accidentals Ratio (CAR) at high pair brightness, a low value of the conditional self-correlation function [$g^{(2)}$(0)], and high two-photon energy-time Franson interferometric visibility, which demonstrate the high quality of the entangled photon pairs and heralded single photons.
We report measurements of time-frequency entangled photon pairs and heralded single photons at 1550~nm wavelengths generated using a microring resonator pumped optically by a diode laser. Along with a high spectral brightness of pair generation, the conventional metrics used to describe performance, such as Coincidences-to-Accidentals Ratio (CAR), conditional self-correlation [$g^{(2)}(0)$], two-photon energy-time {F}ranson interferometric visibility etc. are shown to reach a high-performance regime not yet achieved by silicon photonics, and attained previously only by crystal, glass and fiber…
It is a fundamental challenge in quantum optics to deterministically generate indistinguishable single photons through non-deterministic nonlinear optical processes, due to the intrinsic coupling of single- and multi-photon generation probabilities in these processes. Actively multiplexing photons generated in many temporal modes can decouple these probabilities, but key issues are to minimize resource requirements to allow scalability, and to ensure indistinguishability of the generated photons. We demonstrate the multiplexing of photons from four temporal modes solely using fiber-integrated …
We demonstrate two key components for optical quantum information processing: a bright source of heralded single photons; and a bright source of entangled photon pairs. A pair of pump photons produces a correlated pair of photons at widely spaced wavelengths (583 nm and 900 nm), via a $χ^{(3)}$ four-wave mixing process. We demonstrate a non-classical interference between heralded photons from independent sources with a visibility of 95%, and an entangled photon pair source, with a fidelity of 89% with a Bell state.
We experimentally study a fiber-based three-stage nonlinear interferometer and demonstrate its application in generating heralded single photons with high efficiency and purity by spectral engineering. We obtain a heralding efficiency of 90% at a brightness of 0.039 photons/pulse. The purity of the source is checked by two-photon Hong-Ou-Mandel interference with a visibility of 95%+-6% (after correcting Raman scattering and multi-pair events). Our investigation indicates that the heralded source of single photons produced by the three-stage nonlinear interferometer has the advantages of high p…
Generating quantum entanglement is not only an important scientific endeavor, but will be essential to realizing quantum-enhanced technologies, in particular, quantum-enhanced measurements with precision beyond classical limits. We investigate the heralded generation of multiphoton entanglement for quantum metrology using a reconfigurable integrated waveguide device in which projective measurement of auxiliary photons heralds the generation of path-entangled states. We use four and six-photon inputs, to analyze the heralding process of two- and four-photon NOON states-a superposition of N phot…
Quantum optics in combination with integrated optical devices shows great promise for efficient manipulation of single photons. New physical concepts, however, can only be found when these fields truly merge and reciprocally enhance each other. Here we work at the merging point and investigate the physical concept behind a two-coupled-waveguide system with an integrated parametric down-conversion process. We use the eigenmode description of the linear system and the resulting modification in momentum conservation to derive the state generation protocol for this type of device. With this new co…
Different degrees of freedom of single photons have been entangled and are used as a resource for various quantum technology applications. We present a simple scheme to perform Bell's test and show the violation of CHSH inequality in a path-entangled single photon state using interferometric and its equivalent non-interferometric approach in beam splitter setting. We demonstrate this experimentally by generating and controlling path-entangled state using both, heralded and un-heralded single photons from spontaneous parametric down-conversion. The experimental results we present show the trans…
Single and two-mode multiphoton states are the cornerstone of many quantum technologies, e.g., metrology. In the optical regime these states are generally obtained combining heralded single-photons with linear optics tools and post-selection, leading to inherent low success probabilities. In a recent paper, we design several protocols that harness the long-range atomic interactions induced in waveguide QED to improve fidelities and protocols of single-mode multiphoton emission. Here, we give full details of these protocols, revisit them to simplify some of their requirements and also extend th…
Precise measurements are the key to advances in all fields of science. Quantum entanglement shows higher sensitivity than achievable by classical methods. Most physical quantities including position, displacement, distance, angle, and optical path length can be obtained by optical phase measurements. Reducing the photon wavelength of the interferometry can further enhance the optical path length sensitivity and imaging resolution. By quantum frequency up conversion, we realized a short wavelength two photon number entangled state. Nearly perfect Hong Ou Mandel interference is achieved after bo…
Quantum networks involve entanglement sharing between multiple users. Ideally, any two users would be able to connect regardless of the type of photon source they employ, provided they fulfill the requirements for two-photon interference. From a theoretical perspective, photons coming from different origins can interfere with a perfect visibility, provided they are made indistinguishable in all degrees of freedom. Previous experimental demonstrations of such a scenario have been limited to photon wavelengths below 900 nm, unsuitable for long distance communication, and suffered from low interf…
Heralded single photons (HSPs) generated by spontaneous parametric down-conversion (SPDC) are useful resource to achieve various photonic quantum information processing. Given a large-scale experiment which needs multiple HSPs, increasing the generation rate with suppressing higher-order pair creation is desirable. One of the promising ways is to use a pump laser with a GHz-order repetition rate. In such a high repetition rate regime, however, single-photon detectors can only partially identify the pulses. Hence, we develop a simple model to consider that effect on the spectral purity, and exp…
We present the first experimental demonstration of the optical Sagnac effect at the single-photon level. Using a high quality guided-wave heralded single- photon source at 1550 nm and a fibre optics setup, we obtain an interference pattern with net visibilities up to (99.2 $\pm$ 0.4%). On the basis of this high visibility and the compactness of the setup, the interest of such a system for fibre optics gyroscope is discussed.
To realize a quantum network based on quantum entanglement swapping, bright and completely autonomous sources are essentially required. Here, we experimentally demonstrate Hong-Ou-Mandel (HOM) quantum interference between two independent bright photon pairs generated via the spontaneous four-wave mixing in Doppler-broadened ladder-type 87Rb atoms. Bright autonomous heralded single photons are operated in a continuous-wave (CW) mode with no synchronization or supplemental filters. The four-fold photon coincidence counts per hour correspond to 5000 events for a temporal range of 10 ns, one order…
An experiment is performed to demonstrate the temporal distinguishability of a four-photon state and a six-photon state, both from parametric down-conversion. The experiment is based on a multi-photon interference scheme in a recent discovered NOON-state projection measurement. By measuring the visibility of the interference dip, we can distinguish the various scenarios in the temporal distribution of the pairs and thus quantitatively determine the degree of temporal (in)distinguishability of a multi-photon state.
We experimentally demonstrated the Hong-Ou-Mandel (HOM) interference between two photons after visible-to-telecommunication wavelength conversion. In the experiment, we prepared a heralded single photon by using spontaneous parametric down-conversion and the other photon from a weak laser source at 780 nm. We converted the wavelength of both photons to the telecommunication wavelength of 1522 nm by using difference-frequency generation in a periodically-poled lithium niobate, and then observed the HOM interference between the photons. The observed visibility is $0.76\pm 0.12$ which clearly sho…
Visibility-Engineered Multiparameter Sensing in Dispersive Quantum Interferometry: Identifiability, Noise Robustness, and Hardware Emulation
Instituto de Física, Universidade Federal de Goiás（戈亚斯联邦大学物理研究所）；Faculty of Civil Engineering and Mechanics, Kunming University of Science and Technology（昆明理工大学土木工程学院）；Instituto de Física de São Carlos, Universidade de São Paulo（圣保罗大学圣卡洛斯物理研究所）
Optical metasurfaces open new avenues for precise wavefront control of light for integrated quantum technology. Here, we demonstrate a hybrid integrated quantum photonic system that is capable to entangle and disentangle two-photon spin states at a dielectric metasurface. By interfering single-photon pairs at a nanostructured dielectric metasurface, a path-entangled two-photon NOON state with circular polarization is generated that exhibits a quantum HOM interference visibility of 86 $\pm$ 4%. Furthermore, we demonstrate nonclassicality and phase sensitivity in a metasurface-based interferomet…
We demonstrate a Hong-Ou-Mandel interference between two independent, intrinsically pure, heralded single photons from spontaneous parametric down conversion (SPDC) at telecom wavelength. A visibility of $85.5\pm8.3%$ was achieved without using any bandpass filter. Thanks to the group-velocity-matched SPDC and superconducting nanowire single photon detectors (SNSPDs), the 4-fold coincidence counts are one order higher than that in the previous experiments. The combination of bright single photon sources and SNSPDs is a crucial step for future practical quantum info-communication systems at tel…
Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family', including BBO…
We show that it is possible to generate a novel single-photon fringe pattern by using two spatially separated identical bi-photon sources. The fringes are similar to the ones observed in a Michelson interferometer and possess certain remarkable properties with potential applications. A striking feature of the fringes is that although the pattern is obtained by detecting only one photon of each photon pair, the fringes shift due to a change in the optical path traversed by the undetected photon. The fringe shift is characterized by a combination of wavelengths of both photons, which implies tha…
Spectrally uncorrelated biphoton state generated from the spontaneous nonlinear optical process is an important resource for quantum information. Currently such spectrally uncorrelated biphoton state can only be prepared from limited kinds of nonlinear media, thus limiting their wavelengths. In order to explore wider wavelength range, here we theoretically study the generation of spectrally uncorrelated biphoton state from 14 isomorphs of potassium dihydrogen phosphate (KDP) crystal. We find that 11 crystals from the `KDP family' still maintain similar nonlinear optical properties of KDP, such…
On-Chip Generation of Co-Polarized and Spectrally Separable Photon Pairs
National University of Singapore（新加坡国立大学）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）；A ∗ STAR Quantum Innovation Centre (Q.InC), Agency for Science, Technology and Research (A ∗ STAR)（新加坡科技研究局A*STAR量子创新中心）；Institute of Materials Research and Engineering (IMRE), Agency for Science, Technology and Research (A ∗ STAR)（新加坡科技研究局A*STAR材料研究与工程学院）
We demonstrate a method to determine the spectral purity of single photons. The technique is based on the Hong-Ou-Mandel (HOM) interference between a single photon state and a suitably prepared coherent field. We show that the temporal width of the HOM dip is not only related to reciprocal of the spectral width but also to the underlying quantum coherence. Therefore, by measuring the width of both the HOM dip and the spectrum one can directly quantify the degree of spectral purity. The distinct advantage of our proposal is that it obviates the need for perfect mode matching, since it does not …
While integrated photonics is a robust platform for quantum information processing, architectures for photonic quantum computing place stringent demands on high quality information carriers. Sources of single photons that are highly indistinguishable and pure, that are either near-deterministic or heralded with high efficiency, and that are suitable for mass-manufacture, have been elusive. Here, we demonstrate on-chip photon sources that simultaneously meet each of these requirements. Our photon sources are fabricated in silicon using mature processes, and exploit a novel dual-mode pump-delaye…
Multi-wavelength quantum light sources, especially at telecom band, are extremely desired in quantum information technology. Despite recent impressive advances, such a quantum light source with high quality remains challenging. Here we demonstrate a multi-wavelength quantum light source using a silicon nitride micro-ring with a free spectral range of 200 GHz. The generation of eight pairs of correlated photons is ensured in a wavelength range of 25.6 nm. With device optimization and noise-rejecting filters, our source enables the generation of heralded single-photons - at a rate of 62 kHz with…
Entangled-photon pairs are an essential resource for quantum information technologies. Chip-scale sources of entangled pairs have been integrated with various photonic platforms, including silicon, nitrides, indium phosphide, and lithium niobate, but each has fundamental limitations that restrict the photon-pair brightness and quality, including weak optical nonlinearity or high waveguide loss. Here, we demonstrate a novel, ultra-low-loss AlGaAs-on-insulator platform capable of generating time-energy entangled photons in a $Q$ $>1$ million microring resonator with nearly 1,000-fold improvement…
We implement an ultrafast pulsed type-II parametric down conversion source in a periodically poled KTP waveguide at telecommunication wavelengths with almost identical properties between signal and idler. As such, our source resembles closely a pure, genuine single mode photon pair source with indistinguishable modes. We measure the joint spectral intensity distribution and second order correlation functions of the marginal beams and find with both methods very low effective mode numbers corresponding to a Schmidt number below 1.16. We further demonstrate the indistinguishability as well as th…
Filter-Free Indistinguishable Photon Generation from Continuous-Wave-Driven Integrated Microresonators
University of Science and Technology of China（中国科学技术大学）；Hefei National Laboratory（合肥国家实验室）；International Quantum Academy（国际量子科学院）；Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering（深圳福田南方科技大学量子技术与工程研究所）；Southern University of Science and Technology（南方科技大学）
We describe the generation of atom-resonant indistinguishable photon pairs using nonlinear optical techniques, their spectral purification using atomic filters, characterization using multi-photon interference, and application to quantum-enhanced sensing with atoms. Using either type-I or type-II cavity-enhanced spontaneous parametric down-conversion, we generate pairs of photons in the resonant modes of optical cavities with linewidths comparable to the 6 MHz natural linewidth of the D$_1$ line of atomic rubidium. The cavities and pump lasers are tuned so that emission occurs in a mode or a p…
We consider the effect of self-phase modulation and cross-phase modulation on the joint spectral amplitude of photon pairs generated by spontaneous four-wave mixing. In particular, the purity of a heralded photon from a pair is considered, in the context of schemes that aim to maximise the purity and minimise correlation in the joint spectral amplitude using birefringent phase-matching and short pump pulses. We find that non-linear phase modulation effects will be detrimental, and will limit the quantum interference visibility that can be achieved at a given generation rate. An approximate exp…
On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limit…
Quantum photonic chips, which integrate quantum light sources alongside active and passive optical elements, as well as single photon detectors, show great potential for photonic quantum information processing and quantum technology. Mature semiconductor nanofabrication processes allow for scaling such photonic integrated circuits to on-chip networks of increasing complexity. Second order nonlinear materials are the method of choice for generating photonic quantum states in the overwhelming part of linear optic experiments using bulk components but integration with waveguide circuitry on a nan…
