We experimentally study a fiber-based three-stage nonlinear interferometer and demonstrate its application in generating heralded single photons with high efficiency and purity by spectral engineering. We obtain a heralding efficiency of 90% at a brightness of 0.039 photons/pulse. The purity of the source is checked by two-photon Hong-Ou-Mandel interference with a visibility of 95%+-6% (after correcting Raman scattering and multi-pair events). Our investigation indicates that the heralded source of single photons produced by the three-stage nonlinear interferometer has the advantages of high purity, high heralding efficiency, high brightness, and flexibility in wavelength and bandwidth selection.
Although heralding signals in quantum optics experiments are typically based on the detection of exactly one photon, it has recently been theoretically shown that heralding based on the detection of zero photons can be useful in a number of quantum information applications. Here we describe an experimental technique for "heralding on zero photons" using conventional single-photon detectors and time-tagging methods. We find that detector efficiency and dark count rates play a counterintuitive role in the ability to accurately detect zero photons, and demonstrate these effects in an experiment t…
We investigate the possibility of generating pure heralded single photons through spontaneous parametric down-conversion comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. We estimate the Schmidt number associated to the temporal modes as a function of the pump pulse duration for three particular configurations, showing how the different phase-matching conditions influences the degree of separability that can be achieved.
We investigate different strategies suitable to generate pure heralded single photons through spontaneous parametric down-conversion, comparing the counter-propagating geometry studied in [1] with more conventional co-propagating configurations which enhance the purity of the heralded photon state through the technique of group-velocity matching. Our analysis is based on the correlation of twin photons in the temporal domain,a non-standard approach that provides a physical view of the mechanisms that permit to eliminate the temporal entanglement of the state and to generate high-purity heralde…
Multi-photon interference is central to photonic quantum information processing and quantum simulation, usually requiring multiple sources of non-classical light followed by a unitary transformation on their modes. Here, we observe interference in the four-photon events generated by a single silicon waveguide, where the different modes are six frequency channels. Rather than requiring a unitary transformation, the frequency correlations of the source are configured such that photons are generated in superposition states across multiple channels, and interference effects can be seen without fur…
Photon pairs produced by parametric down-conversion or four-wave mixing can interfere with each other in multiport interferometers, or carry entanglement between distant nodes for use in entanglement swapping. This requires the photons be spectrally pure to ensure good interference, and have high heralding efficiency to know accurately the number of photons involved and to maintain high rates as the number of photons grows. Spectral filtering is often used to remove noise and define spectral properties. For heralded single photons high purity and heralding efficiency is possible by filtering t…
Evolving photonic quantum technologies and applications require higher and higher rates of single photon generation. In parallel, it is required that these generated photons are kept spectrally pure for multi-photon experiments and that multi-photon noise be kept to a minimum. In spontaneous parametric down-conversion sources, these requirements are conflicting, because spectral filtering to increase spectral purity always means lowering the rate at which photons are generated, and increasing the pump power means increasing the multi-photon noise. In this paper, we present a scheme, called ext…
The ideal photon-pair source for building up multi-qubit states needs to produce indistinguishable photons with high efficiency. Indistinguishability is crucial for minimising errors in two-photon interference, central to building larger states, while high heralding rates will be needed to overcome unfavourable loss scaling. Domain engineering in parametric down-conversion sources negates the need for lossy spectral filtering allowing one to satisfy these conditions inherently within the source design. Here, we present a telecom-wavelength parametric down-conversion photon source that operates…
We present a detailed study on the properties of single photons generated by spontaneous parametric down conversion (SPDC) when both the spectral and spatial degrees of freedom are controlled by means of filters. Our results show that it is possible to obtain pure heralded single photons with high heralding efficiency despite the use of filters. Moreover, we report an asymmetry on the single photon properties exhibited in type-II SPDC sources that depends on choosing the signal or the idler photon as the heralding one.
Simplified scheme for continuous-variable entanglement distillation: multicopy distillation of Gaussian entanglement without heralding Gaussian measurements
Optical quantum protocols are reliant on the production of highly pure single photons. However, most parametric heralded single photon sources possess spectral correlations, limiting the purity of the produced photon. The most common method for restoring the purity is with narrowband spectral filtering, which comes at the cost of reducing the rate of heralding detection. Here, we characterize this trade-off analytically for a large class of parametric sources. It is possible to achieve up to 20% heralding success probabilities with 90% heralded photon purities.
Efficient, high rate photon sources with high single photon purity are essential ingredients for quantum technologies. Single photon sources based on solid state emitters such as quantum dots are very advantageous for integrated photonic circuits, but they can suffer from a high two-photon emission probability, which in cases of non-cryogenic environment cannot be spectrally filtered. Here we propose two temporal purification-by-heralding methods for using a two photon emission process to yield highly pure and efficient single photon emission, bypassing the inherent problem of spectrally overl…
Photon indistinguishability plays a fundamental role in information processing, with applications such as linear-optical quantum computation and metrology. It is then necessary to develop appropriate tools to quantify the amount of this resource in a multiparticle scenario. Here we report a four-photon experiment in a linear-optical interferometer designed to simultaneously estimate the degree of indistinguishability between three pairs of photons. The interferometer design dispenses with the need of heralding for parametric down-conversion sources, resulting in an efficient and reliable optic…
Mode-selective nonlinear interference for high-brightness and high-purity fiber-coupled SPDC sources
Fraunhofer Institute for Applied Optics and Precision Engineering（弗劳恩霍夫应用光学和精密工程研究所）；Friedrich Schiller University Jena, Institute of Applied Physics, Abbe Center of Photonics（耶拿弗里德里希·席勒大学应用物理学院阿贝光子学中心）
We provide a compact full description of multiboson correlation measurements of arbitrary order N in passive linear interferometers with arbitrary input single-photon pure states. This allows us to physically analyze the novel problem of multiboson correlation sampling at the output of random linear interferometers. Our results also describe general multiboson correlation landscapes for an arbitrary number of input single photons and arbitrary interferometers. In particular, we use two different schemes to demonstrate, respectively, arbitrary-order quantum beat interference and 100% visibility…
Entangled photon pair sources based on bulk optics are approaching optimal design and implementation, with high state fidelities, spectral purities and heralding efficiencies, but generally low brightness. Integrated entanglement sources, while providing higher brightness and low-power operation, often sacrifice performance in output state quality and coupling efficiency. Here we present a polarization-entangled pair source based on a hybrid approach of waveguiding and bulk optics, addressing every metric simultaneously. We show 96% fidelity to the singlet state, 82% Hong-Ou-Mandel interferenc…
Parametric down-conversion (PDC) is one of the most widely used methods to create pure single-photon states for quantum information applications. However little attention has been paid to higher-order photon components in the PDC process, yet these ultimately limit the prospects of generating single-photons of high quality. In this paper we investigate the impacts of higher-order photon components and multiple frequency modes on the heralding rates and single-photon fidelities. This enables us to determine the limits of PDC sources for single-photon generation. Our results show that a perfectl…
Telecommunication wavelength with well-developed optical communication technologies and low losses in the waveguide are advantageous for quantum applications. However, an experimental generation of non-classical states called non-Gaussian states at the telecommunication wavelength is still underdeveloped. Here, we generate highly-pure-single-photon states, one of the most primitive non-Gaussian states, by using a heralding scheme with an optical parametric oscillator and a superconducting nano-strip photon detector. The Wigner negativity, the indicator of non-classicality, of the generated sin…
We report a bright and tunable source of spectrally pure heralded single photons in the telecom O-Band, based on cross-polarized four wave mixing in a commercial birefringent optical fiber. The source can achieve a purity of 85%, heralding efficiency of 30% and high coincidences to accidentals ratio of 108. Furthermore, the possibility of building multiple identical sources is explored. Through the measurements of joint spectral intensities, we find that the fiber is homogeneous over atleast 45 centimeters and can potentially realize 4 identical sources. This paves the way for a cost-effective…
Conditional detection is an important tool to extract weak signals from a noisy background and is closely linked to heralding, which is an essential component of protocols for long distance quantum communication and distributed quantum information processing in quantum networks. Here we demonstrate the conditional detection of time-bin qubits after storage in and retrieval from a photon-echo based waveguide quantum memory. Each qubit is encoded into one member of a photon-pair produced via spontaneous parametric down conversion, and the conditioning is achieved by the detection of the other me…
Current sources of heralded single photons based on nonlinear optics operate in a probabilistic manner. In order to build quantum-enhanced devices based around the use of single photons, compact, turn-key and deterministic sources are required. A possible solution is to multiplex a number of sources to increase the single-photon generation probability and in so doing reducing the waiting time to deliver large numbers of photons simultaneously, from independent sources. Previously it has been shown that, in the ideal case, 17 multiplexed sources allow deterministic generation of heralded single…
We experimentally control the spectral structure of photon pairs created via spontaneous four-wave mixing in microstructured fibers. By fabricating fibers with designed dispersion, one can manipulate the photons' wavelengths, joint spectrum, and, thus, entanglement. As an example, we produce photon-pairs with no spectral correlations, allowing direct heralding of single photons in pure-state wave packets without filtering. We achieve an experimental purity of $85.9\pm1.6%$, while theoretical analysis and preliminary tests suggest 94.5% purity is possible with a much longer fiber.
Entangled photon sources with simultaneously near-unity heralding efficiency and indistinguishability are the fundamental elements for scalable photonic quantum technologies. We design and realize a degenerate entangled-photon source from an ultrafast pulsed laser pumped spontaneous parametric down-conversion (SPDC), which show simultaneously ~97% heralding efficiency and ~96% indistinguishability between independent single photons. Such a high-efficiency and frequency-uncorrelated SPDC source allows generation of the first 12-photon genuine entanglement with a state fidelity of 0.572(24). We …
We present a source of polarization entangled photon pairs based on spontaneous parametric downconversion engineered for frequency uncorrelated telecom photon generation. Our source provides photon pairs that display, simultaneously, the key properties for high-performance quantum information and fundamental quantum science tasks. Specifically, the source provides for high heralding efficiency, high quantum state purity and high entangled state fidelity at the same time. Among different tests we apply to our source we observe almost perfect non-classical interference between photons from indep…
A quantum random access memory (qRAM) is considered an essential computing unit to enable polynomial speedups in quantum information processing. Proposed implementations include using neutral atoms and superconducting circuits to construct a binary tree, but these systems still require demonstrations of the elementary components. Here, we propose a photonic integrated circuit (PIC) architecture integrated with solid-state memories as a viable platform for constructing a qRAM. We also present an alternative scheme based on quantum teleportation and extend it to the context of quantum networks. …
Entanglement distillation is the process of concentrating entanglement from a given quantum state. We present a technique for distillation of bi-partite polarization entanglement using interferometry. This technique can be optimized to extract maximal entanglement from any pure or mixed entangled state. A model for this method is presented and in particular we present experimental results for pure states when using polarizing Mach-Zehnder interferometers. These experimentally distilled states always demonstrate an increased violation of Bell's inequality.
Heralded entangled state generation enhanced by photon addition and subtraction
University of Science and Technology of China（中国科学技术大学）；Laboratory of Quantum Information, University of Science and Technology of China（中国科学技术大学量子信息实验室）；Anhui Province Key Laboratory of Quantum Network, University of Science and Technology of China（中国科学技术大学安徽省量子网络重点实验室）；CAS Center for Excellence in Quantum Information and Quantum Physics, University of Science and Technology of China（中国科学技术大学中科院量子信息与量子物理卓越创新中心）；Hefei National Laboratory, University of Science and Technology of China（中国科学技术大学合肥国家实验室）
本文提出了一种基于高斯源的 heralded 熵生成方案，通过结合单模压缩、线性干涉仪和辅助模式的条件光子数测量，实现双轨编码的 Bell、GHZ 和 W 状态生成，并优化参数以提高生成效率和保真度。
Multi-photon quantum interference is the underlying principle for optical quantum information processing protocols. Indistinguishability is the key to quantum interference. Therefore, the success of many protocols in optical quantum information processing relies on the availability of photon states with a well-defined spatial and temporal mode. Photons in single spatial mode can be obtained from nonlinear processes in single-mode waveguides. For the temporal mode, the common approach is to engineer the nonlinear processes. But it is complicated because the spectral properties and the nonlinear…
A key obstacle to the experimental realization of many photonic quantum-enhanced technologies is the lack of low-loss sources of single photons in pure quantum states. We demonstrate a promising solution: generation of heralded single photons in a silica photonic chip by spontaneous four-wave mixing. A heralding efficiency of 40%, corresponding to a preparation efficiency of 80% accounting for detector performance, is achieved due to efficient coupling of the low-loss source to optical fibers. A single photon purity of 0.86 is measured from the source number statistics without filtering, and c…
We investigate the connection between the shot-noise limit in linear interferometers and particle entanglement. In particular, we ask whether or not sub shot-noise sensitivity can be reached with all pure entangled input states of $N$ particles if they can be optimized with local operations. Results on the optimal local transformations allow us to show that for $N=2$ all pure entangled states can be made useful for sub shot-noise interferometry while for $N>2$ this is not the case. We completely classify the useful entangled states available in a bosonic two-mode interferometer. We apply our r…
We give a full description of the problem of Multi-Boson Correlation Sampling (MBCS) at the output of a random interferometer for single input photons in arbitrary multimode pure states. The MBCS prob- lem is the task of sampling at the interferometer output from the probability distribution associated with polarization- and time-resolved detections. We discuss the richness of the physics and the complexity of the MBCS problem for nonidentical input photons. We also compare the MBCS problem with the standard bo- son sampling problem, where the input photons are assumed to be identical and the …
We implement an ultrafast pulsed type-II parametric down conversion source in a periodically poled KTP waveguide at telecommunication wavelengths with almost identical properties between signal and idler. As such, our source resembles closely a pure, genuine single mode photon pair source with indistinguishable modes. We measure the joint spectral intensity distribution and second order correlation functions of the marginal beams and find with both methods very low effective mode numbers corresponding to a Schmidt number below 1.16. We further demonstrate the indistinguishability as well as th…
While integrated photonics is a robust platform for quantum information processing, architectures for photonic quantum computing place stringent demands on high quality information carriers. Sources of single photons that are highly indistinguishable and pure, that are either near-deterministic or heralded with high efficiency, and that are suitable for mass-manufacture, have been elusive. Here, we demonstrate on-chip photon sources that simultaneously meet each of these requirements. Our photon sources are fabricated in silicon using mature processes, and exploit a novel dual-mode pump-delaye…
Quantum memories are key components in quantum information networks. Their ability to store and retrieve information on demand makes repeat-until-success strategies scalable. Warm alkali-metal vapours are interesting candidates for the implementation of such memories, thanks to their long storage times and experimental simplicity. Operation with the Raman protocol enables high time-bandwidth products, which allows for multiple synchronisation trials of probabilistically operating quantum gates via memory-based temporal multiplexing. This makes the Raman memory a promising tool, whose broad spe…
Realistic single-photon sources do not generate single photons with certainty. Instead they produce statistical mixtures of photons in Fock states $\ket{1}$ and vacuum (noise). We describe how to eliminate the noise in the output of the sources by means of another noisy source or a coherent state and cross phase modulation (XPM). We present a scheme which announces the production of pure single photons and thus eliminates the vacuum contribution. This is done by verifying a XPM related phase shift with a Mach-Zehnder interferometer.
Using ultra-bright sources of pure-state entangled photons from parametric down conversion, an eight-photon interferometer and post-selection detection, we demonstrate the ability to experimentally manipulate eight individual photons and report the creation of an eight-photon Schrödinger cat state with an observed fidelity of $0.708 \pm 0.016$.
Entanglement swapping and heralding are at the heart of many protocols for distributed quantum information. For photons, this typically involves Bell state measurements based on two-photon interference effects. In this context, hybrid systems that combine high rate, ultra-stable and pure quantum sources with long-lived quantum memories are particularly interesting. Here, we develop a theoretical description of pulsed two-photon interference of photons from dissimilar sources to predict the outcomes of second-order cross-correlation measurements. These are directly related to, and hence used to…
In this article we propose a method to estimate with high accuracy pure quantum states of a single qudit. Our method is based on the minimization of the squared error between the complex probability amplitudes of the unknown state and its estimate. We show by means of numerical experiments that the estimation accuracy of the present method, which is given by the expectation of the squared error on the sample space of estimates, is state independent. Furthermore, the estimation accuracy delivered by our method is close to twice the Gill-Massar lower bound, which represents the best achievable a…
Characterizing Photonic Partial Distinguishability Through Gram Matrix Tomography
Center for Quantum Enabled-Computing, Center for Theoretical Physics of the Polish Academy of Sciences（波兰科学院理论物理中心量子使能计算中心）；International Iberian Nanotechnology Laboratory (INL)（伊比利亚纳米技术国际实验室）；Centre for Quantum Information and Communication, École polytechnique de Bruxelles, CP 165/59, Université libre de Bruxelles（布鲁塞尔自由大学布鲁塞尔理工学院量子信息与通信中心）；Instituto de Física, Universidade Federal Fluminense（弗鲁米嫩塞联邦大学物理研究所）
Silicon ring resonators are used as photon pair sources by taking advantage of silicon's large third order nonlinearity with a process known as spontaneous four wave mixing. These sources are capable of producing pairs of indistinguishable photons but typically suffer from an effective $50\%$ loss. By slightly decoupling the input waveguide from the ring, the drop port coincidence ratio can be significantly increased with the trade-off being that the pump is less efficiently coupled into the ring. Ring resonators with this design have been demonstrated having coincidence ratios of $\sim 96\%$ …
Single photon sources based on spontaneous photon-pair generation have enabled pioneering experiments in quantum optics. However, their non-determinism presents a bottleneck to scaling up photonic and hybrid quantum-enhanced technologies. Furthermore, photon pairs are typically emitted into many correlated frequency modes, producing an undesirable mixed state on heralding. Here we present a complete fibre-integrated heralded single photon source that addresses both these difficulties simultaneously. We use active switching to provide a path to deterministic operation by multiplexing separate s…
Quantum computing experiments are moving into a new realm of increasing size and complexity, with the short-term goal of demonstrating an advantage over classical computers. Boson sampling is a promising platform for such a goal, however, the number of involved single photons was up to five so far, limiting these small-scale implementations to a proof-of-principle stage. Here, we develop solid-state sources of highly efficient, pure and indistinguishable single photons, and 3D integration of ultra-low-loss optical circuits. We perform an experiment with 20 single photons fed into a 60-mode int…
We demonstrate pulsed polarization-entangled photons generated from a periodically poled $\mathrm{KTiOPO_4}$ (PPKTP) crystal in a Sagnac interferometer configuration at telecom wavelength. Since the group-velocity-matching (GVM) condition is satisfied, the intrinsic spectral purity of the photons is much higher than in the previous scheme at around 800 nm wavelength. The combination of a Sagnac interferometer and the GVM-PPKTP crystal makes our entangled source compact, stable, highly entangled, spectrally pure and ultra-bright. The photons were detected by two superconducting nanowire single …
