Spectrally intrinsically uncorrelated biphoton states generated from nonlinear crystals are very important but rare resources for quantum photonics and quantum information applications. Previously, such biphoton states were generated from several kinds of crystals, however, their wavelength ranges and nonlinear efficiencies were still limited for various applications. In order to explore new crystal for wider wavelength range and higher nonlinear efficiency, here we theoretically study the generation of spectrally uncorrelated biphoton states from 14 crystals in the `BBO family', including BBO, CLBO, KABO, KBBF, RBBF, CBBF, BABF, BiBO, LBO, CBO, LRB4, LCB, YCOB, and GdCOB. They satisfy three kinds of group-velocity matching condition from near-infrared to telecom wavelengths. Furthermore, heralded single photons can be generated with a purity as high as 0.98, which is achieved without any narrow filtering. The indistinguishability of photons from independent sources is examined by the Hong-Ou-Mandel interference, which results in a visibility of 98% also without any further filtering, i.e., photons from different heralded single-photon sources are highly indistinguishable. Our study may provide single-photon sources with good performance for quantum information processing at near-infrared and telecom wavelengths.
We theoretically investigate the spectral property of biphoton state from the cascade emissions from a Doppler-broadened atomic ensemble. This biphoton state is spontaneously created in the four-wave-mixing process. The upper transition of the emissions lies in telecom bandwidth, which prevails in fiber-based quantum communication for low-loss transmission. We obtain the spectral property in terms of superradiant decay rates of the lower transition, excitation pulse durations, and temperature of the medium. We quantify their frequency entanglement by Schmidt decomposition and find that more en…
Spectrally unentangled biphotons with high single-spatiotemporal-mode purity are highly desirable for many quantum information processing tasks. We generate biphotons with an inferred heralded-state spectral purity of 99%, the highest to date without any spectral filtering, by pulsed spontaneous parametric downconversion in a custom-fabricated periodically-poled KTiOPO$_4$ crystal under extended Gaussian phase-matching conditions. To efficiently characterize the joint spectral intensity of the generated biphotons at high spectral resolution, we employ a commercially available dispersion compen…
Spectrally uncorrelated biphoton state generated from the spontaneous nonlinear optical process is an important resource for quantum information. Currently such spectrally uncorrelated biphoton state can only be prepared from limited kinds of nonlinear media, thus limiting their wavelengths. In order to explore wider wavelength range, here we theoretically study the generation of spectrally uncorrelated biphoton state from 14 isomorphs of potassium dihydrogen phosphate (KDP) crystal. We find that 11 crystals from the `KDP family' still maintain similar nonlinear optical properties of KDP, such…
We utilized the all-copropagating scheme, which maintains the phase-match condition, in the spontaneous four-wave mixing (SFWM) process to generate biphotons from a hot atomic vapor. The scheme enables our biphotons not only to surpass those in the previous works of hot-atom SFWM, but also to compete with the biphotons that are generated by either the cold-atom SFWM or the cavity-assisted spontaneous parametric down conversion. The biphoton linewidth in this work is tunable for an order of magnitude. As we tuned the linewidth to 610 kHz, the maximum two-photon correlation function, $g_{s,as}^{…
We theoretically investigated spectrally uncorrelated biphotons generated in a counter-propagating spontaneous parametric downconversion (CP-SPDC) from periodically poled MTiOXO4 (M = K, Rb, Cs; X = P, As) crystals. By numerical calculation, it was found that the five crystals from the KTP family can be used to generate heralded single photons with high spectral purity and wide tunability. Under the type-0 phase-matching condition, the purity at 1550 nm was between 0.91 and 0.92, and the purity can be maintained over 0.90 from 1500 nm to 2000 nm wavelength. Under the type-II phase-matching con…
Multiparticle interference is a fundamental phenomenon in the study of quantum mechanics.It was discovered in a recent experiment [Ra, Y.-S. et al, Proc. Natl Acad. Sci. USA \textbf{110}, 1227(2013)] that spectrally uncorrelated biphotons exhibited a nonmonotonic quantum-to-classical transition in a four-photon Hong-Ou-Mandel (HOM) interference. In this work, we consider the same scheme with spectrally correlated photons.By theoretical calculation and numerical simulation, we found the transition not only can be nonmonotonic with negative-correlated or uncorrelated biphotons, but also can be m…
We theoretically investigate the preparation of mid-infrared (MIR) spectrally-uncorrelated biphotons from a spontaneous parametric down-conversion process using doped LN crystals, including MgO doped LN, ZnO doped LN, and In2O3 doped ZnLN with doping ratio from 0 to 7 mol%. The tilt angle of the phase-matching function and the corresponding poling period are calculated under type-II, type-I, and type-0 phase-matching conditions. We also calculate the thermal properties of the doped LN crystals and their performance in Hong-Ou-Mandel interference. It is found that the doping ratio has a substan…
Indistinguishable single photons are key ingredient for a plethora of quantum information processing applications ranging from quantum communications to photonic quantum computing. A mainstream platform to produce indistinguishable single photons over a wide spectral range is based on biphoton generation through spontaneous parametric down-conversion (SPDC) in nonlinear crystals. The purity of the SPDC biphotons, however, is limited by their spectral correlations. Here, we present a design recipe, based on a machine-learning framework, for the engineering of biphoton joint spectrum amplitudes …
We theoretically investigate the spectral property of a biphoton state from multiplexed thermal atomic ensembles. This biphoton state originates from the cascade emissions, which can be generated by two weak pump fields under four-wave mixing condition. Under this condition, a signal photon from the upper transition, chosen in a telecommunication bandwidth, can be generated along with a correlated idler photon from the lower infrared transition. We can spectrally shape the biphoton state by multiplexing the atomic ensembles with frequency-shifted emissions, where the entropy of entanglement ca…
Analytical expressions are derived for the distribution rates of spatial coincidences in the counting of photons produced by spontaneous parametric down conversion (SPDC). Gaussian profiles are assumed for the wave function of the idler and signal light created in type-I SPDC. The distribution rates describe ellipses on the detection planes that are oriented at different angles according to the photon coincidences in either horizontal-horizontal, vertical-vertical, horizontal-vertical or vertical-horizontal position variables. The predictions are in agreement with the experimental data obtaine…
Generation of two-photon wavepackets, produced by spontaneous parametric down conversion in crystals with linearly chirped quasi-phase matching grating, is analyzed. Although being spectrally broad, two-photon wavepackets produced this way are not Fourier transform limited. In the paper we discuss the temporal compression of the wavepackets, exploiting the insertion of a standard optical fiber in the path of one of the two photons. The effect is analyzed by means of full numerical calculation and the exact dispersion dependencies in both the crystal and the fiber are considered. The study open…
The optimal strategy of two-photon interferometric sensing in diverse noise environments
School of Physics and Information Science, Shaanxi University of Science and Technology（陕西科技大学物理与信息科学学院）；Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control of Ministry of Education, Department of Physics and Synergetic Innovation Center for Quantum Effects and Applications, Hunan Normal University（湖南师范大学物理与协同创新中心量子效应及应用教育部低维量子结构与量子控制重点实验室）；Hubei Key Laboratory of Optical Information and Pattern Recognition, Wuhan Institute of Technology（武汉工程大学湖北省光学信息与模式识别重点实验室）
The frequency correlation (or decorrelation) of photon pairs is of great importance in long-range quantum communications and photonic quantum computing. We experimentally characterize a spontaneous parametric down conversion (SPDC) source, based on a Beta-Barium Borate (BBO) crystal cut for type-II phase matching at 1550 nm which emits photons with the positive or no spectral correlations. Our system employs a carefully designed detection method exploiting two InGaAs detectors.
On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limit…
Near-infrared Hong-Ou-Mandel quantum interference is observed in silicon nanophotonic directional couplers with raw visibilities on-chip at 90.5%. Spectrally-bright 1557-nm two-photon states are generated in a periodically-poled KTiOPO4 waveguide chip, serving as the entangled photon source and pumped with a self-injection locked laser, for the photon statistical measurements. Efficient four-port coupling in the communications C-band and in the high-index-contrast silicon photonics platform is demonstrated, with matching theoretical predictions of the quantum interference visibility. Constitue…
Preservation of photon statistics upon selective molecular modulation in hollow-core fibers
University of the Basque Country (EHU)（巴斯克大学）；University of Limoges（利摩日大学）；CNRS UMR 7252（法国国家科学研究中心）；University of Erlangen-Nürnberg（埃尔朗根-纽伦堡大学）；Max Planck Institute for the Science of Light（马克斯·普朗克光科学研究所）；IKERBASQUE, Basque Foundation for Science（伊克尔巴斯基奎，巴斯克科学基金会）
