Generation, characterization and use of atom-resonant indistinguishable photon pairs
Morgan W. Mitchell
备注：
to appear as a book chapter in a compilation "Engineering the Atom-Photon Interaction" published by Springer in 2015, edited by A. Predojevic and M. W. Mitchell
We describe the generation of atom-resonant indistinguishable photon pairs using nonlinear optical techniques, their spectral purification using atomic filters, characterization using multi-photon interference, and application to quantum-enhanced sensing with atoms. Using either type-I or type-II cavity-enhanced spontaneous parametric down-conversion, we generate pairs of photons in the resonant modes of optical cavities with linewidths comparable to the 6 MHz natural linewidth of the D$_1$ line of atomic rubidium. The cavities and pump lasers are tuned so that emission occurs in a mode or a pair of orthogonally-polarized modes that are resonant to the D$_1$ line, at 794.7 nm. The emission from these frequency-degenerate modes is separated from other cavity emission using ultra-narrow atomic frequency filters, either a Faraday anomalous dispersion optical filter (FADOF) with a 445MHz linewidth and 57 dB of out-of-band rejection or an induced dichroism filter with an 80 MHz linewidth and $\ge$35dB out-of-band rejection. Using the type-I source, we demonstrate interference of photon pair amplitudes against a coherent state and a new method for full characterization of the temporal wave-function of narrow-band photon pairs. With the type-II source we demonstrate high-visibility super-resolving interference, a high-fidelity atom-tuned NooN state, and quantum enhanced sensing of atoms using indistinguishable photon pairs.
Applying high power continuous-wave resonant s-shell excitation to a single self-assembled In- GaAs quantum dot, we demonstrate the generation of post-selected single-indistinguishable photons from the Mollow triplet sidebands. A sophisticated spatial filtering technique based on a double Michelson interferometer enabled us to separate the spectrally close lying individual Mollow components and perform almost background free two-photon interference measurements. Showing high consistency with the results of an independent determination of the emission coherence of 250 +/- 30 ps, our analysis re…
We present a mechanism to produce indistinguishable single-photon pulses on demand from an optical cavity. The sequences of two laser pulses generate, at the two Raman transitions of a four-level atom, the same cavity-mode photons without repumping of the atom between photon generations. Photons are emitted from the cavity with near-unit efficiency in well-defined temporal modes of identical shapes controlled by the laser fields. The second order correlation function reveals the single-photon nature of the proposed source. A realistic setup for the experimental implementation is presented.
Single-photon sources play a key role in photonic quantum technologies. Semiconductor quantum dots can emit indistinguishable single photons under resonant excitation. However, the resonance fluorescence technique typically requires cross-polarization filtering which causes a loss of the unpolarized quantum dot emission by 50%. To solve this problem, we demonstrate a method to generate indistinguishable single photons with optically controlled polarization by two laser pulses off-resonant with neutral exciton states. This scheme is realized by exciting the quantum dot to the biexciton state an…
Hong-Ou-Mandel interference of more than 10 indistinguishable atoms
Leibniz Universität Hannover（汉诺威莱布尼茨大学）；Deutsches Zentrum für Luft- und Raumfahrt e.V. (DLR)（德国航空航天中心）；Instituto Nazionale di Ottica, Consiglio Nazionale delle Ricerche (INO-CNR)（意大利国家光学研究所，国家研究委员会）；University of the Basque Country UPV/EHU（巴斯克大学）
We investigate superradiance and subradiance of indistinguishable atoms with quantized motional states, starting with an initial total state that factorizes over the internal and external degrees of freedom of the atoms. Due to the permutational symmetry of the motional state, the cooperative spontaneous emission, governed by a recently derived master equation [F. Damanet et al., Phys. Rev. A 93, 022124 (2016)], depends only on two decay rates $γ$ and $γ_0$ and a single parameter $Δ_{\mathrm{dd}}$ describing the dipole-dipole shifts. We solve the dynamics exactly for $N=2$ atoms, numerically f…
We demonstrate a straightforward implementation of a push-button like single-photon source which is based on a strongly coupled atom-cavity system. The device operates intermittently for periods of up to 100 microseconds, with single-photon repetition rates of 1.0 MHz and an efficiency of 60 %. Atoms are loaded into the cavity using an atomic fountain, with the upper turning point near the cavity's mode centre. This ensures long interaction times without any disturbances induced by trapping potentials. The latter is the key to reaching deterministic efficiencies as high as obtained in probabal…
Optimization of two-photon excitation by indistinguishable photons in a three-level atom
Institute of Physics, Faculty of Physics, Astronomy and Informatics, Nicolaus Copernicus University（尼古拉·哥白尼大学物理、天文学与信息学院物理研究所）；Institute of Advanced Studies, Nicolaus Copernicus University（尼古拉·哥白尼大学高等研究院）；Institute of Theoretical Physics and Astrophysics, Faculty of Mathematics, Physics and Informatics, University of Gdańsk（格但斯克大学数学、物理与信息学院理论物理与天体物理研究所）
High Purcell-enhancement in quantum-dot hybrid circular Bragg grating cavities for GHz-clockrate generation of indistinguishable photons
Technische Universität Berlin（柏林工业大学）；Institute of Semiconductors, Chinese Academy of Sciences（中国科学院半导体研究所）；University of Chinese Academy of Sciences（中国科学院大学）
We demonstrate a high-brightness source of pairs of indistinguishable photons based on a type-II phase-matched doubly-resonant optical parametric oscillator operated far below threshold. The cavity-enhanced down-conversion output of a PPKTP crystal is coupled into two single-mode fibers with a mode coupling efficiency of 58%. The high degree of indistinguishability between the photons of a pair is demonstrated by a Hong-Ou-Mandel interference visibility of higher than 90% without any filtering at an instantaneous coincidence rate of 450 000 pairs/s per mW of pump power per nm of down-conversio…
A central challenge in developing quantum computers and long-range quantum networks lies in the distribution of entanglement across many individually controllable qubits. Colour centres in diamond have emerged as leading solid-state 'artificial atom' qubits, enabling on-demand remote entanglement, coherent control of over 10 ancillae qubits with minute-long coherence times, and memory-enhanced quantum communication. A critical next step is to integrate large numbers of artificial atoms with photonic architectures to enable large-scale quantum information processing systems. To date, these effo…
Photon-photon interactions are an essential requirement of quantum photonic information processing. One way to generate these interactions is to utilize an atom strongly coupled to an optical cavity. This system exhibits the photon blockade effect which enables single photon switching and creation of non-classical light. But the nonlinear effects enabled by this system suffer from a fundamental time-bandwidth constraint. For the the simple case of splitting an input pulse of two indistinguishable photons, this constraint imposes a limit on the efficiency of routing photons to different output …
We demonstrate purely resonant continuous-wave optical laser excitation to coherently prepare an excitonic state of a single semiconductor quantum dot (QDs) inside a high quality pillar microcavity. As a direct proof of QD resonance fluorescence, the evolution from a single emission line to the characteristic Mollow triplet10 is observed under increasing pump power. By controlled utilization of weak coupling between the emitter and the fundamental cavity mode through Purcell-enhancement of the radiative decay, a strong suppression of pure dephasing is achieved, which reflects in close to Fouri…
Realization of quantum optical circuits is at the heart of quantum photonic information processing. A long-standing obstacle however has been the absence of a platform of single photon sources (SPSs) that simultaneously satisfies the following required characteristics: spatially ordered SPS arrays that produce, on-demand, highly pure, and indistinguishable single photons with sufficiently uniform emission characteristics across the array, needed for controlled interference between photons from distinct sources to enable functional quantum optical networks. Here we report on such a platform of …
The optical interference constitutes a paramount resource in modern physics. At the scale of individual atoms and photons, it is a diverse concept that causes different coherent phenomena. We present the experimental characterization of both coherent and statistical properties of light emitted from ensembles of trapped ions increasing with a number of contributing phase-incoherent independent atomic particles ranging from a single to up to several hundreds. It conclusively demonstrates how super-Poissonian quantum statistics non-trivially arises purely from the finite number of indistinguishab…
The optical scheme is proposed for realization of controlled phase quantum gate based on the off-resonant interaction of photon with three-level atom in single mode QED-cavity. Possible physical implementation of this scheme is discussed.
Trapped atomic ions embedded in optical cavities are a promising platform to enable long-distance quantum networks and their most far-reaching applications. Here we achieve and analyze photon indistinguishability in a telecom-converted ion-cavity system. First, two-photon interference of cavity photons at their ion-resonant wavelength is observed and found to reach the limits set by spontaneous emission. Second, this limit is shown to be preserved after a two-step frequency conversion replicating a distributed scenario, in which the cavity photons are converted to the telecom C band and then b…
When two indistinguishable single photons are fed into the two input ports of a beam splitter, the photons will coalesce and leave together from the same output port. This is a quantum interference effect, which occurs because the two possible paths where the photons leave in different output ports interfere destructively. This effect was first observed in parametric downconversion by Hong, Ou and Mandel, and then with single photons produced one after the other by the same quantum emitter. With the recent development of quantum information, a lot of attention has been devoted to this coalesce…
We demonstrate vacuum squeezing at the D1 line of atomic rubidium (795 nm) with a tunable, doubly-resonant, monolithic sub-threshold optical parametric oscillator in periodically-poled Rb-doped potassium titanyl phosphate. The squeezing appears to be undiminished by a strong dispersive optical nonlinearity recently observed in this material.
A new scheme of photon echo based quantum memory in the optimal optical QED cavity with off-resonant Raman atomic transition is proposed. The scheme employs the atomic ensembles characterized by an optically thin resonant transition and natural inhomogeneous broadening of the resonant line composed of the arbitrary narrow homogeneous spectral components. The scheme provides robust and quite simple coherent control of the light-atoms dynamics that can be implemented by using an existing optical technique and opens a practical way for realization of the efficient long-lived multi-mode optical qu…
The cascade-emitted biphotons generated from the alkali metal atomic ensembles are an excellent entanglement resource which enables long-distance quantum communication. The communication of quantum information between distant locations can be realized by utilizing the low-loss telecom bandwidth in the upper transition of the cascaded photons in a fiber-based quantum network. Meanwhile, the infrared photon from the lower transition of this highly directional and frequency-correlated biphoton can be created under the four-wave mixing process and can be stored locally as a collective spin wave. H…
We demonstrate quantum interference between photons generated by the radiative decay processes of excitons that are bound to isolated fluorine donor impurities in ZnSe/ZnMgSe quantum-well nanostructures. The ability to generate single photons from these devices is confirmed by auto-correlation experiments, and indistinguishability of single photons from two independent devices is confirmed via a Hong-Ou-Mandel dip. These results indicate that donor impurities in appropriately engineered semiconductor structures can portray atom-like homogeneity and coherence properties, potentially enabling sc…
We demonstrate a high-purity source of indistinguishable single photons using a quantum dot embedded in a nanophotonic waveguide. The source features a near-unity internal coupling efficiency and the collected photons are efficiently coupled off-chip by implementing a taper that adiabatically couples the photons to an optical fiber. By quasi-resonant excitation of the quantum dot, we measure a single-photon purity larger than 99.4% and a photon indistinguishability of up to 94+-1% by using p-shell excitation combined with spectral filtering to reduce photon jitter. A temperature-dependent stud…
We propose a scheme to generate arbitrary Fock states |N> in a cavity QED using N resonant Rydberg atoms. The atom-field interaction times are controlled via Stark-shifts adjusted in a way that each atom transfers a photon to the cavity, turning atomic detections useless. Fluctuations affecting the control of the atom-field interactions are also considered.
We study the optimal focusing of two-level atoms with a near resonant standing wave light, using both classical and quantum treatments of the problem. Operation of the focusing setup is considered as a nonlinear spatial squeezing of atoms in the thin- and thick-lens regimes. It is found that the near-resonant standing wave focuses the atoms with a reduced background in comparison with far-detuned light fields. For some parameters, the quantum atomic distribution shows even better localization than the classical one. Spontaneous emission effects are included via the technique of quantum Monte C…
Quantum systems combining indistinguishable photon generation and spin-based quantum information processing are essential for remote quantum applications and networking. However, identification of suitable systems in scalable platforms remains a challenge. Here, we investigate the silicon vacancy centre in silicon carbide and demonstrate controlled emission of indistinguishable and distinguishable photons via coherent spin manipulation. Using strong off-resonant excitation and collecting photons from the ultra-stable zero-phonon line optical transitions, we show a two-photon interference contr…
In this paper we show that three cavity fields can be entangled when they are tuned on resonance with an ensemble of dressed three-level atoms. The master equation for the three cavity modes is derived by using atomic dressed states and the inseparability of the three output cavity modes is described by using a sufficient criterion proposed by van Loock and Furusawa. The physical cause is the atomic coherence effects, by which the quantum correlations are created in the field dynamics.
Multiparticle entangled states generated via interaction between narrow-band light and an ensemble of identical two-level atoms are considered. Depending on the initial photon statistics, correlation between atoms and photons can give rise to entangled states of these systems. It is found that the state of any pair of atoms interacting with weak single-mode squeezed light is inseparable and robust against decay. Optical schemes for preparing entangled states of atomic ensembles by projective measurement are described.
We demonstrate the generation of rubidium-resonant heralded single photons for quantum memories. Photon pairs are created by cavity-enhanced down-conversion and narrowed in bandwidth to 7 MHz with a novel atom-based filter operating by "interaction-free measurement" principles. At least 94% of the heralded photons are atom-resonant as demonstrated by a direct absorption measurement with rubidium vapor. A heralded auto-correlation measurement shows $g_c^{(2)}(0)=0.040 \pm 0.012$, i.e., suppression of multi-photon contributions by a factor of 25 relative to a coherent state. The generated herald…
The phenomenological two-level atom is re-analysed using the methods of effective field theory. By presenting the Dicke-Jaynes-Cummings model in real space, an exact diagonalization is accomplished going beyond the rotating wave approximation. The meaning of the symmetries and conserved quantities in the theory is discussed and the model is related to non-equilibrium field theory. The structure of the solution raises a question about the rotating wave approximation in quantum mechanics.
We present a time-dependent quantum calculation of the van der Waals interaction between a pair of dissimilar atoms, one of which is initially excited while the other one is in its ground state. For small detuning, the interaction is predominantly mediated at all distances by the exchange of doubly resonant photons between the two atoms. We find that it presents both temporal and spatial oscillations. Spatially oscillating terms depend on the resonant frequencies of both atoms, while the frequency of the time oscillations is given by their detuning. We analyse the physical content of our findi…
Within the framework of quantization of the macroscopic electromagnetic field, a master equation describing both the resonant dipole-dipole interaction (RDDI) and the resonant atom-field interaction (RAFI) in the presence of dispersing and absorbing macroscopic bodies is derived, with the relevant couplings being expressed in terms of the surroundings-assisted Green tensor. It is shown that under certain conditions the RDDI can be regarded as being governed by an effective Hamiltonian. The theory, which applies to both weak and strong atom-field coupling, is used to study the resonant energy e…
Spin vs. position conjugation in quantum simulations with atoms: application to quantum chemistry
Quantum Technology Centre, M.V. Lomonosov Moscow State University（莫斯科国立大学量子技术中心）；St. Petersburg State University（圣彼得堡国立大学）；Russian Quantum Center（俄罗斯量子中心）；Centre for Interdisciplinary Basic Research, HSE University（高等经济学院跨学科基础研究系）；Department of Optics, Palacký University（帕拉茨基大学光学系）；Department of Physics, Old Dominion University（老道明大学物理系）
Single--photon which is initially uncorrelated with atom, will evolve to be entangled with the atom on their continuous kinetic variables in the process of resonant scattering. We find the relations between the entanglement and their physical control parameters, which indicates that high entanglement can be reached by broadening the scale of the atomic wave or squeezing the linewidth of the incident single--photon pulse.
We observe the interaction of a single trapped calcium ion with single photons produced by a narrow-band, resonant down-conversion source [A. Haase et al., Opt. Lett. 34, 55 (2009)], employing a quantum jump scheme. Using the temperature dependence of the down-conversion spectrum and the tunability of the narrow source, absorption of the down-conversion photons is quantitatively characterized.
We investigate the dynamical Casimir effect and its detection with Rydberg atoms. The photons are created in a resonant cavity with a plasma mirror of a semiconductor slab which is irradiated by periodic laser pulses. The canonical Hamiltonian is derived for the creation and annihilation operators showing the explicit time-variation in the couplings, which originates from the external configuration such as a nonstationary plasma mirror. The number of created photons is evaluated as squeezing from the Heisenberg equations with the Hamiltonian. Then, the detection of the photons as the atomic ex…
With a resonant amplitude-modulation field on two Rydberg atoms, we propose a Rydberg antiblockade (RAB) regime, where the Rabi oscillation between collective ground and excited states is induced. A controlled-Z gate can be yielded through a Rabi cycle. Further, several common issues of the RAB gates are solved by modifying the parameter relation. The gate fidelity and the gate robustness against the control error are enhanced with a shaped pulse. The requirement of control precision of the Rydberg-Rydberg interaction strength is relaxed. In addition, the atomic excitation is restrained and th…
Within the framework of quantization of the macroscopic electromagnetic field, equations of motion and an effective Hamiltonian for treating both the resonant dipole-dipole interaction between two-level atoms and the resonant atom-field interaction are derived, which can suitably be used for studying the influence of arbitrary dispersing and absorbing material surroundings on these interactions. The theory is applied to the study of the transient behavior of two atoms that initially share a single excitation, with special emphasis on the role of the two competing processes of virtual and real …
We consider the resonant interaction energy and force between two identical atoms, one in an excited state and the other in the ground state, placed inside a photonic crystal. The atoms, having the same orientation of their dipole moment, are supposed prepared in their symmetrical state and interact with the quantum electromagnetic field. We consider two specific models of photonic crystals: a one-dimensional model and an isotropic model. We show that in both cases the resonant interatomic force can be strongly enhanced by the presence of the photonic crystal, as a consequence of the modified …
In this paper we address the analytical solution of the non-resonant interaction between two identical V-type three-level atoms passing consecutively through a single-mode cavity field in the presence of intensity-dependent coupling. By considering an identical initial condition for both atoms and an initial coherent field, we find the analytical solution of the state vector of the entire atom-field system. Accordingly, we could carefully investigate the influence of various parameters in the circumstances of the interacting system on different physical quantities such as the atomic population…
We present a complete set of analytical and invariant expressions for the steady-state density matrix of atoms in a resonant radiation field with arbitrary intensity and polarization. The field drives the closed dipole transition with arbitrary values of the angular momenta $J_{g}$ and $J_{e}$ of the ground and excited state. The steady-state density matrix is expressed in terms of spherical harmonics of a complex direction given by the field polarization vector. The generalization to the case of broad-band radiation is given. We indicate various applications of these results.
We present an analytical treatment of coherent excitation of a Two-Level Atom driven by a far-off resonant classical field. A class of pulse envelope is obtained for which this problem is exactly solvable. The solutions are given in terms of Heun function which is a generalization of the Hypergeometric function. The degeneracy of Heun to Hypergeometric equation can give all the exactly solvable pulse shapes of Gauss Hypergeometric form, from the generalized pulse shape obtained here. We discuss the application of the results obtained to the generation of XUV.
This paper describes a novel atom-cavity interaction induced by periodically poled atom-cavity coupling constant which leads to multiple narrow photoemission bands for an initially inverted two-level atom under the strong coupling condition. The emission bandpass narrowing has a close analogy with the folded Solc filter in the context of quasi-phase matching by periodic poling. We present a closed form solution of the emission probability at the end of interaction and deduce the multiple phase matching condition for this system which is programmable by the interaction time. The Bloch sphere an…
The electromagnetically induced transparency (EIT) in an $N$ configuration is studied under both resonant and off-resonant conditions. In a certain off-resonant condition the dark state of the four level system, which is almost the same as the resonant dark state in $Λ$ configuration, is rebuilt. The actual system with damping is examined using optical Bloch equation, both numerically and analytically. Based on this detuned dark state, some new applications with frequency shifts can be realized.
We derive a cross-Kerr type effective Hamiltonian for the four-level atom interacting with three electromagnetic fields in the N-configuration. When the atom has relaxed into the ground state a cross-Kerr nonlinearity arises between two weak probe fields. As a development on earlier work we show in general that the atom will also display a linear and self-Kerr response. However, if certain resonance conditions are satisfied then the linear and self-Kerr interactions will vanish. The electrical susceptibilities of the probe transitions are also explored and it is shown that a large, pure cross-…
The development of scalable sources of non-classical light is fundamental to unlock the technological potential of quantum photonics\cite{Kimble:Nat2008}. Among the systems under investigation, semiconductor quantum dots are currently emerging as near-optimal sources of indistinguishable single photons. However, their performances as sources of entangled-photon pairs are in comparison still modest. Experiments on conventional Stranski-Krastanow InGaAs quantum dots have reported non-optimal levels of entanglement and indistinguishability of the emitted photons. For applications such as entangle…
We describe how a coherent optical drive that is near-resonant with the upper rungs of a three-level ladder system, in conjunction with a short pulse excitation, can be used to provide a frequency-tunable source of on-demand single photons. Using an intuitive master equation model, we identify two distinct regimes of device operation: (i) for a resonant drive, the source operates using the Autler-Townes effect, and (ii) for an off-resonant drive, the source exploits the ac Stark effect. The former regime allows for a large frequency tuning range but coherence suffers from timing jitter effects…
An on-demand source of indistinguishable and entangled photon pairs is a fundamental component for different quantum information applications such as optical quantum computing, quantum repeaters, quantum teleportation and quantum communication. Parametric down-conversion and four-wave mixing sources of entangled photons have shown high degrees of entanglement and indistinguishability but the probabilistic nature of their generation process also creates zero or multiple photon pairs following a Poissonian distribution. This limits their use in complex algorithms where many qubits and gate opera…
Resonance fluorescence of two-level quantum systems has emerged as a powerful tool in quantum information processing. Extension of this approach to higher-level systems provides new opportunities for quantum optics applications. Here we introduce a coherent driving scheme of a three-level ladder system utilizing Autler-Townes and ac Stark effects by resonant excitation with two laser fields. We propose theoretically and demonstrate experimentally the feasibility of this approach towards all-optical spectral tuning of quantum dot-based single-photon sources and investigate photon indistinguisha…
In this chapter we will discuss the technology and experimental techniques to realize quantum dot (QD) single photon sources combining high outcoupling efficiencies and highest degrees of non-postselected photon indistinguishability. The system, which is based on ultra low density InAs QDs embedded in a quasi planar single sided microcavity with natural photonic traps is an ideal testbed to study quantum light emission from single QDs. We will discuss the influence of the excitation conditions on the purity of the single photon emission, and in particular on the degree of indistinguishability …
We propose a scheme for the generation of highly indistinguishable single photons using semiconductor quantum dots and demonstrate its performance and potential. The scheme is based on the resonant two-photon excitation of the biexciton followed by stimulation of the biexciton to selectively prepare an exciton. Quantum-optical simulations and experiments are in good agreement and show that the scheme provides significant advantages over previously demonstrated excitation methods. The two-photon excitation of the biexciton suppresses re-excitation and enables ultra-low multi-photon errors, whil…
Single photons coupled to atomic systems have shown to be a promising platform for developing quantum technologies. Yet a bright on-demand, highly pure and highly indistinguishable single-photon source compatible with atomic platforms is lacking. In this work, we demonstrate such a source based on a strongly interacting Rydberg system. The large optical nonlinearities in a blockaded Rydberg ensemble convert coherent light into a single-collective excitation that can be coherently retrieved as a quantum field. We observe a single-transverse-mode efficiency up to 0.18(2), $g^{(2)}=2.0(1.5)\times…
A key ingredient for quantum photonic technologies is an on-demand source of indistinguishable single photons. State-of-the-art indistinguishable single-photon sources typically employ resonant excitation pulses with fixed repetition rates, creating a string of single photons with predetermined arrival times. However, in future applications, an independent electronic signal from a larger quantum circuit or network will trigger the generation of an indistinguishable photon. Further, operating the photon source up to the limit imposed by its lifetime is desirable. Here, we report on the applicat…
Photoionization of an atom via interatomic correlations to N neighboring atoms may be strongly enhanced due to constructive interference of quantum pathways. The ionization proceeds via resonant photoexcitation of a neighbor atom and subsequent interatomic Coulombic decay. The enhancement can scale with N^2, leading to "super-enhanced photoionization".
