We demonstrate a high-brightness source of pairs of indistinguishable photons based on a type-II phase-matched doubly-resonant optical parametric oscillator operated far below threshold. The cavity-enhanced down-conversion output of a PPKTP crystal is coupled into two single-mode fibers with a mode coupling efficiency of 58%. The high degree of indistinguishability between the photons of a pair is demonstrated by a Hong-Ou-Mandel interference visibility of higher than 90% without any filtering at an instantaneous coincidence rate of 450 000 pairs/s per mW of pump power per nm of down-conversion bandwidth. For the degenerate spectral mode with a linewidth of 7 MHz at 795 nm a rate of 70 pairs/(s mW MHz) is estimated, increasing the spectral brightness for indistinguishable photons by two orders of magnitude compared to similar previous sources.
We demonstrate two-photon interference using two remote single molecules as bright solid-state sources of indistinguishable photons. By varying the transition frequency and spectral width of one molecule, we tune and explore the effect of photon distinguishability. We discuss future improvements on the brightness of single-photon beams, their integration by large numbers on chips, and the extension of our experimental scheme to coupling and entanglement of distant molecules.
We describe the generation of atom-resonant indistinguishable photon pairs using nonlinear optical techniques, their spectral purification using atomic filters, characterization using multi-photon interference, and application to quantum-enhanced sensing with atoms. Using either type-I or type-II cavity-enhanced spontaneous parametric down-conversion, we generate pairs of photons in the resonant modes of optical cavities with linewidths comparable to the 6 MHz natural linewidth of the D$_1$ line of atomic rubidium. The cavities and pump lasers are tuned so that emission occurs in a mode or a p…
Single-photon sources play a key role in photonic quantum technologies. Semiconductor quantum dots can emit indistinguishable single photons under resonant excitation. However, the resonance fluorescence technique typically requires cross-polarization filtering which causes a loss of the unpolarized quantum dot emission by 50%. To solve this problem, we demonstrate a method to generate indistinguishable single photons with optically controlled polarization by two laser pulses off-resonant with neutral exciton states. This scheme is realized by exciting the quantum dot to the biexciton state an…
Narrowband single photons that couple well to atomic ensembles could prove essential for future quantum networks, but the efficient generation of such photons remains an outstanding challenge. We realize a spatially-multiplexed heralded source of single photons that are inherently compatible with the commonly employed D2 line of rubidium. Our source is based on four-wave mixing in hot rubidium vapor, requiring no laser cooling or optical cavities, and generates single photons with high rate and low noise. We use Hong-Ou-Mandel interference to verify the indistinguishability of the photons gene…
Long-distance quantum communication relies on the ability to efficiently generate and prepare single photons at telecom wavelengths. In many applications these photons must also be indistinguishable such that they exhibit interference on a beamsplitter, which implements effective photon-photon interactions. However, deterministic generation of indistinguishable single photons with high brightness remains a challenging problem. We demonstrate two-photon interference at telecom wavelengths using an InAs/InP quantum dot in a nanophotonic cavity. The cavity enhances the quantum dot emission, resul…
Parametric downconversion (PDC) in semiconductor Bragg-reflection waveguides (BRW) is routinely exploited for photon-pair generation in the telecommunication range. Contrary to many conventional PDC sources, BRWs offer possibilities to create spectrally broadband but nevertheless indistinguishable photon pairs in orthogonal polarizations that simultaneously incorporate high frequency entanglement. We explore the characteristics of co-propagating twin beams created in a type-II ridge BRW. Our PDC source is bright and efficient, which serves as a benchmark of its performance and justifies its ex…
We report on the generation of indistinguishable photon pairs at telecom wavelengths based on a type-II parametric down conversion process in a periodically poled potassium titanyl phosphate (PPKTP) crystal. The phase matching, pump laser characteristics and coupling geometry are optimised to obtain spectrally uncorrelated photons with high coupling efficiencies. Four photons are generated by a counter- propagating pump in the same crystal and anlysed via two photon interference experiments between photons from each pair source as well as joint spectral and g^(2) measurements. We obtain a spec…
We generate indistinguishable photons from a semiconductor diode containing a InAs/GaAs quantum dot. Using an all-electrical technique to populate and control a single-photon emitting state we filter-out dephasing by Stark-shifting the emission energy on timescales below the dephasing time of the state. Mixing consecutive photons on a beam-splitter we observe two-photon interference with a visibility of 64%.
The implementation and engineering of bright and coherent solid state quantum light sources is key for the realization of both on chip and remote quantum networks. Despite tremendous efforts for more than 15 years, the combination of these two key prerequisites in a single, potentially scalable device is a major challenge. Here, we report on the observation of bright and coherent single photon emission generated via pulsed, resonance fluorescence conditions from a single quantum dot (QD) deterministically centered in a micropillar cavity device via cryogenic optical lithography. The brightness…
We report on the triggered generation of indistinguishable photons by solid-state single-photon sources in two separate cryogenic laser scanning microscopes. Organic fluorescent molecules were used as emitters and investigated by means of high resolution laser spectroscopy. Continuous-wave photon correlation measurements on individual molecules proved the isolation of single quantum systems. By using frequency selective pulsed excitation of the molecule and efficient spectral filtering of its emission, we produced triggered Fourier-limited single photons. In a further step, local electric fiel…
In this chapter we will discuss the technology and experimental techniques to realize quantum dot (QD) single photon sources combining high outcoupling efficiencies and highest degrees of non-postselected photon indistinguishability. The system, which is based on ultra low density InAs QDs embedded in a quasi planar single sided microcavity with natural photonic traps is an ideal testbed to study quantum light emission from single QDs. We will discuss the influence of the excitation conditions on the purity of the single photon emission, and in particular on the degree of indistinguishability …
Filter-Free Indistinguishable Photon Generation from Continuous-Wave-Driven Integrated Microresonators
University of Science and Technology of China（中国科学技术大学）；Hefei National Laboratory（合肥国家实验室）；International Quantum Academy（国际量子科学院）；Shenzhen Futian SUSTech Institute for Quantum Technology and Engineering（深圳福田南方科技大学量子技术与工程研究所）；Southern University of Science and Technology（南方科技大学）
Indistinguishable photons play a key role in quantum optical information technologies. We characterize the output of an ultra-bright photon-pair source using multi-particle tomography [R. B. A. Adamson et al., Phys. Rev. Lett. 98, 043601 (2007)] and separately identify coherent errors, decoherence, and distinguishability. We demonstrate generation of high-quality indistinguishable pairs and polarization NOON states with 99% fidelity to an ideal NOON state. Using a NOON state we perform a super-resolving angular measurement with 90% visibility.
Applying high power continuous-wave resonant s-shell excitation to a single self-assembled In- GaAs quantum dot, we demonstrate the generation of post-selected single-indistinguishable photons from the Mollow triplet sidebands. A sophisticated spatial filtering technique based on a double Michelson interferometer enabled us to separate the spectrally close lying individual Mollow components and perform almost background free two-photon interference measurements. Showing high consistency with the results of an independent determination of the emission coherence of 250 +/- 30 ps, our analysis re…
Single molecules in solid-state matrices have been proposed as sources of single-photon Fock states back 20 years ago. Their success in quantum optics and in many other research fields stems from the simple recipes used in the preparation of samples, with hundreds of nominally identical and isolated molecules. Main challenges as of today for their application in photonic quantum technologies are the optimization of light extraction and the on-demand emission of indistinguishable photons. We here present Hong-Ou-Mandel experiments with photons emitted by a single molecule of dibenzoterrylene in…
The generation of nonclassical states of light in miniature chips is a crucial step towards practical implementations of future quantum technologies. Semiconductor materials are ideal to achieve extremely compact and massively parallel systems and several platforms are currently under development. In this context, spontaneous parametric down conversion in AlGaAs devices combines the advantages of room temperature operation, possibility of electrical injection and emission in the telecom band. Here we report on a chip-based AlGaAs source, producing indistinguishable and energy-time entangled ph…
We demonstrate unambiguous entangling operation of a photonic quantum-logic gate driven by an ultrabright solid-state single-photon source. Indistinguishable single photons emitted by a single semiconductor quantum dot in a micropillar optical cavity are used as target and control qubits. For a source brightness of 0.56 collected photons-per-pulse, the measured truth table has an overlap with the ideal case of 68.4%, increasing to 73.0% for a source brightness of 0.17 photons- per-pulse. The gate is entangling: at a source brightness of 0.48, the Bell-state fidelity is above the entangling thr…
The development of scalable sources of non-classical light is fundamental to unlock the technological potential of quantum photonics\cite{Kimble:Nat2008}. Among the systems under investigation, semiconductor quantum dots are currently emerging as near-optimal sources of indistinguishable single photons. However, their performances as sources of entangled-photon pairs are in comparison still modest. Experiments on conventional Stranski-Krastanow InGaAs quantum dots have reported non-optimal levels of entanglement and indistinguishability of the emitted photons. For applications such as entangle…
We investigate theoretically the generation of indistinguishable single photons from a strongly dissipative quantum system placed inside an optical cavity. The degree of indistinguishability of photons emitted by the cavity is calculated as a function of the emitter-cavity coupling strength and the cavity linewidth. For a quantum emitter subject to strong pure dephasing, our calculations reveal that an unconventional regime of high indistinguishability can be reached for moderate emittercavity coupling strengths and high quality factor cavities. In this regime, the broad spectrum of a dissipat…
Single photons produced by fundamentally dissimilar physical processes will in general not be indistinguishable. We show how photons produced from a quantum dot and by parametric down-conversion in a nonlinear crystal can be manipulated to be indistinguishable. The measured two-photon coalescence probability is 16%, and is limited by quantum-dot decoherence. Temporal filtering to the quantum dot coherence time and accounting for detector time response increases this to 61% while retaining 25% of the events. This technique can connect different elements in a scalable quantum network.
We propose a scheme for the generation of highly indistinguishable single photons using semiconductor quantum dots and demonstrate its performance and potential. The scheme is based on the resonant two-photon excitation of the biexciton followed by stimulation of the biexciton to selectively prepare an exciton. Quantum-optical simulations and experiments are in good agreement and show that the scheme provides significant advantages over previously demonstrated excitation methods. The two-photon excitation of the biexciton suppresses re-excitation and enables ultra-low multi-photon errors, whil…
Single photons coupled to atomic systems have shown to be a promising platform for developing quantum technologies. Yet a bright on-demand, highly pure and highly indistinguishable single-photon source compatible with atomic platforms is lacking. In this work, we demonstrate such a source based on a strongly interacting Rydberg system. The large optical nonlinearities in a blockaded Rydberg ensemble convert coherent light into a single-collective excitation that can be coherently retrieved as a quantum field. We observe a single-transverse-mode efficiency up to 0.18(2), $g^{(2)}=2.0(1.5)\times…
Lossless filtering of a single coherent (Schmidt) mode from spatially multimode radiation is a problem crucial for optics in general and for quantum optics in particular. It becomes especially important in the case of nonclassical light that is fragile to optical losses. An example is bright squeezed vacuum generated via high-gain parametric down conversion or four-wave mixing. Its highly multiphoton and multimode structure offers a huge increase in the information capacity provided that each mode can be addressed separately. However, the nonclassical signature of bright squeezed vacuum, photo…
A strong limitation of linear optical quantum computing is the probabilistic operation of two-quantum bit gates based on the coalescence of indistinguishable photons. A route to deterministic operation is to exploit the single-photon nonlinearity of an atomic transition. Through engineering of the atom-photon interaction, phase shifters, photon filters and photon- photon gates have been demonstrated with natural atoms. Proofs of concept have been reported with semiconductor quantum dots, yet limited by inefficient atom-photon interfaces and dephasing. Here we report on a highly efficient singl…
Quantum dots in cavities have been shown to be very bright sources of indistinguishable single photons. Yet the quantum interference between two bright quantum dot sources, a critical step for photon based quantum computation, has never been investigated. Here we report on such a measurement, taking advantage of a deterministic fabrication of the devices. We show that cavity quantum electrodynamics can efficiently improve the quantum interference between remote quantum dot sources: poorly indistinguishable photons can still interfere with good contrast with high quality photons emitted by a so…
We present an experimental demonstration of heralded single photons prepared in pure quantum states from a parametric downconversion source. It is shown that, through controlling the modal structure of the photon pair emission, one can generate pairs in factorable states and thence eliminate the need for spectral filters in multiple-source interference schemes. Indistinguishable heralded photons were generated in two independent spectrally engineered sources, and, by performing a Hong-Ou-Mandel interference between them without spectral filters at a raw visibility of 94.4%, their purity was me…
Coherent temporal filtering of multimode parametric down-conversion using a quantum pulse gate
Integrated Quantum Optics Group, Institute for Photonic Quantum Systems (PhoQS), Paderborn University（帕德博恩大学光子量子系统研究所）；School of Mathematics and Physics, University of Queensland（昆士兰大学数学与物理学院）
A BosonSampling device is a quantum machine expected to perform tasks intractable for a classical computer, yet requiring minimal non-classical resources as compared to full-scale quantum computers. Photonic implementations to date employed sources based on inefficient processes that only simulate heralded single-photon statistics when strongly reducing emission probabilities. BosonSampling with only single-photon input has thus never been realised. Here, we report on a BosonSampling device operated with a bright solid-state source of single-photon Fock states with high photon-number purity: t…
We demonstrate a high-purity source of indistinguishable single photons using a quantum dot embedded in a nanophotonic waveguide. The source features a near-unity internal coupling efficiency and the collected photons are efficiently coupled off-chip by implementing a taper that adiabatically couples the photons to an optical fiber. By quasi-resonant excitation of the quantum dot, we measure a single-photon purity larger than 99.4% and a photon indistinguishability of up to 94+-1% by using p-shell excitation combined with spectral filtering to reduce photon jitter. A temperature-dependent stud…
Resonance fluorescence in the Heitler regime provides access to single photons with coherence well beyond the Fourier transform limit of the transition, and holds the promise to circumvent environment-induced dephasing common to all solid-state systems. Here we demonstrate that the coherently generated single photons from a single self-assembled InAs quantum dot display mutual coherence with the excitation laser on a timescale exceeding 3 seconds. Exploiting this degree of mutual coherence we synthesize near-arbitrary coherent photon waveforms by shaping the excitation laser field. In contrast…
Parametric down-conversion (PDC) offers the possibility to control the fabrication of non-Gaussian states such as Fock states. However, in conventional PDC sources energy and momentum conservation introduce strict frequency and photon number correlations, which impact the fidelity of the prepared state. In our work we optimize the preparation of single-photon Fock states from the emission of waveguided PDC via spectral filtering. We study the effect of correlations via photon number resolving detection and quantum interference. Our measurements show how the reduction of mixedness due to filter…
We report the development of a fiber-based single spatial mode source of photon-pairs where the efficiency of extracting photon-pairs is improved over a previous source [18] through the use of fiber-end expansion and Bragg filters. This improvement in efficiency enabled a spectrally bright and pure photon-pair source having a small second-order correlation function (0.03) and a raw spectral brightness of 44,700 pairs/(s nm mW). The source can be configured to generate entangled photon-pairs,characterized via optimal and minimal quantum state tomography, to have a fidelity of 97% and tangle of …
High visibility on-chip quantum interference among indistinguishable single-photons from multiples sources is a key prerequisite for integrated linear optical quantum computing. Resonant enhancement in micro-ring resonators naturally enables brighter, purer and more indistinguishable single-photon production without any tight spectral filtering. The indistinguishability of heralded single-photons from multiple micro-ring resonators has not been measured in any photonic platform. Here, we report on-chip indistinguishability measurements of heralded single-photons generated from independent micr…
Solid state atom-like systems have great promise for linear optic quantum computing and quantum communication but are burdened by phonon sidebands and broadening due to surface charges. Nevertheless, coupling to a small mode volume cavity would allow high rates of extraction from even highly dephased emitters. We consider the nitrogen vacancy centre in diamond, a system understood to have a poor quantum optics interface with highly distinguishable photons, and design a silicon nitride cavity that allows 99 % efficient extraction of photons at 200 K with an indistinguishability of > 50%, improv…
We report on the experimental generation of an entangled state with a spectrally pure heralded single-photon state and a weak coherent state. By choosing group-velocity matching in the nonlinear crystal, our system for producing entangled photons was 60 times brighter than that in the earlier experiment [Phys. Rev. Lett. 90, 240401 (2003)], with no need of bandpass filters. This entanglement system is useful for quantum information protocols that require indistinguishable photons from independent sources.
The key challenge to scalable optical quantum computing, boson sampling, and quantum metrology is sources of single photons with near-unity system efficiency and simultaneously near-perfect indistinguishability in all degrees of freedom (including spectral, temporal, spatial, and polarization). However, previous high-indistinguishability solid-state single-photon sources had to rely on polarization filtering that reduced the system efficiency by at least 50%. Here, we overcome this challenge by developing a new single-photon source based on a coherently driven quantum dot embedded in an ellipt…
We introduce a filter using a noise-free quantum buffer with large optical bandwidth that can both filter temporal-spectral modes, as well as inter-convert them and change their frequency. We show that such quantum buffers optimally filter out temporal-spectral noise; producing identical single-photons from many distinguishable noisy single-photon sources with the minimum required reduction in brightness. We then experimentally demonstrate a noise-free quantum buffer in a warm atomic system that is well matched to quantum dots and can outperform all intensity (incoherent) filtering schemes for…
Indistinguishable single photons are key ingredient for a plethora of quantum information processing applications ranging from quantum communications to photonic quantum computing. A mainstream platform to produce indistinguishable single photons over a wide spectral range is based on biphoton generation through spontaneous parametric down-conversion (SPDC) in nonlinear crystals. The purity of the SPDC biphotons, however, is limited by their spectral correlations. Here, we present a design recipe, based on a machine-learning framework, for the engineering of biphoton joint spectrum amplitudes …
The ideal photon-pair source for building up multi-qubit states needs to produce indistinguishable photons with high efficiency. Indistinguishability is crucial for minimising errors in two-photon interference, central to building larger states, while high heralding rates will be needed to overcome unfavourable loss scaling. Domain engineering in parametric down-conversion sources negates the need for lossy spectral filtering allowing one to satisfy these conditions inherently within the source design. Here, we present a telecom-wavelength parametric down-conversion photon source that operates…
On-demand indistinguishable single photon sources are essential for quantum networking and communication. Semiconductor quantum dots are among the most promising candidates, but their typical emission wavelength renders them unsuitable for use in fibre networks. Here, we present quantum frequency conversion of near-infrared photons from a bright quantum dot to the telecommunication C-band, allowing integration with existing fibre architectures. We use a custom-built, tunable 2400 nm seed laser to convert single photons from 942 nm to 1550 nm in a difference frequency generation process. We ach…
Integrated photonics is becoming an ideal platform for generating two-photon entangled states with high brightness, high stability and scalability. This high brightness and high quality of photon pair sources encourages researchers further to study and manipulate multi-photon entangled states. Here, we experimentally demonstrate frequency-degenerate four-photon entangled state generation based on a single silicon nanowire 1 cm in length. The polarization encoded entangled states are generated with the help of a Sagnac loop using additional optical elements. The states are analyzed using quantu…
Using the approach of coupled wave equations, we consider spontaneous parametric down-conversion (SPDC) in the narrow-band regime and its relationship to classical nonlinear processes such as sum-frequency generation. We find simple expressions in terms of mode overlap integrals for the absolute pair production rate into single spatial modes, and simple relationships between the efficiencies of the classical and quantum processes. The results, obtained with Green function techniques, are not specific to any geometry or nonlinear crystal. The theory is applied to both degenerate and non-degener…
Single-photons are key elements of many future quantum technologies, be it for the realisation of large-scale quantum communication networks for quantum simulation of chemical and physical processes or for connecting quantum memories in a quantum computer. Scaling quantum technologies will thus require efficient, on-demand, sources of highly indistinguishable single-photons. Semiconductor quantum dots inserted in photonic structures are ultrabright single photon sources, but the photon indistinguishability is limited by charge noise induced by nearby surfaces. The current state of the art for …
Advanced photonic quantum technology relies on multi-photon interference which requires bright sources of high-purity single photons. Here, we implement a novel domain-engineering technique for tailoring the nonlinearity of a parametric down-conversion crystal. We create pairs of independently-heralded telecom-wavelength photons and achieve high heralding, brightness and spectral purities without filtering.
Sources of entanglement are an enabling resource in quantum technology, and pushing the limits of generation rate and quality of entanglement is a necessary pre-requisite towards practical applications. Here, we present an ultra-bright source of polarization-entangled photon pairs based on time-reversed Hong-Ou-Mandel interference. By superimposing four pair-creation possibilities on a polarization beam splitter, pairs of identical photons are separated into two spatial modes without the usual requirement for wavelength distinguishability or non-collinear emission angles. Our source yields hig…
We present an experimental demonstration of a bright and high fidelity polarization entangled photon pair source. The source is constructed using two critically phase matched $β$-Barium Borate crystals with parallel optical axes and photon pairs are collected after filtering with a circular field-stop. Near unity fidelities are obtained with detected pair rates exceeding \SI{100000}{pairs/\s/\mW} approaching the brightness of practical quasi-phase matched entangled photon sources. We find that the brightness scales linearly with the crystal length. We present models supporting the experimental…
We study theoretically how the brightness of pumps, with fixed profiles, affects the temporal mode structure of squeezed states generated by fixed parametric waveguided sources. We find that the temporal modes of these squeezed states can be partially mismatched and thus distinguishable, which is undesirable when using these states as resources for quantum computing or heralded state generation. By studying common frequency filtering techniques used experimentally, we find that although one can regain indistinguishability it comes at the price of potentially greatly reducing the purity of the …
Single epitaxially-grown semiconductor quantum dots have great potential as single photon sources for photonic quantum technologies, though in practice devices often exhibit non-ideal behavior. Here, we demonstrate that amplitude modulation can improve the performance of quantum-dot-based sources. Starting with a bright source consisting of a single quantum dot in a fiber-coupled microdisk cavity, we use synchronized amplitude modulation to temporally filter the emitted light. We observe that the single photon purity, temporal overlap between successive emission events, and indistinguishabilit…
