A. J. Bennett, R. B. Patel, A. J. Shields, K. Cooper, P. Atkinson, C. A. Nicoll, D. A. Ritchie
We generate indistinguishable photons from a semiconductor diode containing a InAs/GaAs quantum dot. Using an all-electrical technique to populate and control a single-photon emitting state we filter-out dephasing by Stark-shifting the emission energy on timescales below the dephasing time of the state. Mixing consecutive photons on a beam-splitter we observe two-photon interference with a visibility of 64%.
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We have developed a microcavity single-photon source based on a single quantum dot within a planar cavity in which wet-oxidation of a high-aluminium content layer provides lateral confinement of both the photonic mode and the injection current. Lateral confinement of the optical mode in optically pumped structures produces a strong enhancement of the radiative decay rate. Using microcavity structures with doped contact layers, we demonstrate a single-photon emitting diode where current may be injected into a single dot.
We report the observation of a Purcell enhancement in the electroluminescence decay rate of a single quantum dot, embedded in a microcavity light-emitting-diode structure. Lateral confinement of the optical mode was achieved using an annulus of low-refractive-index aluminium oxide, formed by wet oxidation. The same layer acts as a current aperture, reducing the active area of the device without impeding the electrical properties of the p-i-n diode. This allowed single photon electroluminescence to be demonstrated at repetition rates up to 0.5 GHz.
Compact and reliable sources of non-classical light could find many applications in emerging technologies such as quantum cryptography, quantum imaging and also in fundamental tests of quantum physics. Single self-assembled quantum dots have been widely studied for this reason, but the vast majority of reported work has been limited to optically excited sources. Here we discuss the progress made so far, and prospects for, electrically driven single-photon-emitting diodes (SPEDs).
We report a two-photon interference experiment in which the detected photons have very different properties. The interference is observed even when no effort is made to mask the distinguishing features before the photons are detected. The results can only be explained in terms of indistinguishable two-photon amplitudes.
We investigate the single photon scattering by an emitter chirally coupled to a one-dimensional waveguide. The single-photon transport property is essentially different from the symmetrical coupling case. The single photons propagating towards the emitter in opposite directions show different transmission behaviors, which is a manifestation of the single-photon diode. In the ideal chiral coupling case, the transmission probability of the single photon transport in one direction is zero by critical coupling, while in the opposite direction it is unity. The diode works well only when the single-…
Dissipation-assisted few-photon optical diode
该研究通过耗散非线性腔体实现单光子和双光子二极管，揭示了耗散对非 reciprocal 量子设备的潜在应用。
We study the coherent transport of one or two photons in a 1D waveguide chirally coupled to a nonlinear resonator. Analytic solutions of the one-photon and two-photon scattering is derived. Although the resonator acts as a non-reciprocal phase shifter, light transmission is reciprocal at one-photon level. However, the forward and reverse transmitted probabilities for two photons incident from either the left side or the right side of the nonlinear resonator are nonreciprocal due to the energy redistribution of the two-photon bound state. Hence, the nonlinear resonator acts as an optical diode …
By using the zero-phonon line emission of an individual organic molecule, we realized a source of indistinguishable single photons in the near infrared. A Hong-Ou-Mandel interference experiment is performed and a two-photon coalescence probability of higher than 50% at 2 K is obtained. The contribution of the temperature-dependent dephasing processes to the two-photon interference contrast is studied. We show that the molecule delivers nearly ideal indistinguishable single photons at the lowest temperatures when the dephasing is nearly lifetime limited. This source is used to generate post-sel…
We demonstrate two-photon interference using two remote single molecules as bright solid-state sources of indistinguishable photons. By varying the transition frequency and spectral width of one molecule, we tune and explore the effect of photon distinguishability. We discuss future improvements on the brightness of single-photon beams, their integration by large numbers on chips, and the extension of our experimental scheme to coupling and entanglement of distant molecules.
Correlated photon pairs generated through spontaneous parametric down-conversion (SPDC) are a key resource in quantum optics. In many quantum optics applications, such as satellite quantum key distribution (QKD), a compact, high repetition rate pump laser is required. Here we demonstrate the use of a compact, GHz-rate diode-pumped three-element Kerr-lens-modelocked Ti:sapphire laser for the generation of correlated photon pairs at 790 nm. We verify the presence of indistinguishable photons produced via SPDC using Hong-Ou-Mandel (HOM) interferometry and observe a dip in coincidence counts with …
We describe a new scheme to fully control the joint spectrum of paired photons generated in spontaneous parametric down-conversion. We show the capability of this method to generate frequency-uncorrelated photon pairs that are pure and indistinguishable, and whose bandwidth can be readily tuned. Importantly, the scheme we propose here can be implemented in any nonlinear crystal and frequency band of interest.
We report on the generation of indistinguishable photon pairs at telecom wavelengths based on a type-II parametric down conversion process in a periodically poled potassium titanyl phosphate (PPKTP) crystal. The phase matching, pump laser characteristics and coupling geometry are optimised to obtain spectrally uncorrelated photons with high coupling efficiencies. Four photons are generated by a counter- propagating pump in the same crystal and anlysed via two photon interference experiments between photons from each pair source as well as joint spectral and g^(2) measurements. We obtain a spec…
We experimentally demonstrate optical control of negative-feedback avalanche diode (NFAD) detectors using bright light. We deterministically generate fake single-photon detections with a better timing precision than normal operation. This could potentially open a security loophole in quantum cryptography systems. We then show how monitoring the photocurrent through the avalanche photodiode can be used to reveal the detector is being blinded.
We show that a pair of quantized cavity modes interacting with a spectrally broadened ensemble of Lambda-type atoms is analogous to an ensemble of two level systems coupled to a bosonic reservoir. This provides the possibility for an irreversible photon transfer between photon modes. The density of states as well as the quantum state of the reservoir can be engineered allowing the observation of effects such as the quantum Zeno- and anti-Zeno effect, the destructive interference of decay channels and the decay in a squeezed vacuum. As a particular application we discuss a photon diode, i.e. a …
The symmetrization postulate asserts that the state of particular species of particles can only be of one permutation symmetry type: symmetric for bosons and antisymmetric for fermions. We report some experimental results showing that pairs of photons indistinguishable by all degrees of freedom can exhibit not only a bosonic behavior, as expected for photons, but also a surprisingly sharp fermionic behavior under specific conditions.
The semiconductor diode, which acts as an electrical rectifier and allows unidirectional electronic transports, is the key to information processing in integrated circuits. Analogously, an optical rectifier (or diode) working at specific target wavelengths has recently becomes a dreaming device in optical communication and signal processing. In this paper, we propose a scheme to realize an optical diode for photonic transport at the level of few photons. The system consists of two spatially overlapping single-mode semiconductor microcavities coupled via ${χ^{(2)}}$ nonlinearities. The photon b…
We propose a novel scheme of realizing an optical diode at the few-photon level. The system consists of a one-dimensional waveguide coupled asymmetrically to a two-level system. The two or multi-photon transport in this system is strongly correlated. We derive exactly the single and two-photon current and show that the two-photon current is asymmetric for the asymmetric coupling. Thus the system serves as an optical diode which allows transmission of photons in one direction much more efficiently than the opposite.
We propose a semiconductor device that can electrically generate entangled electron spin-photon states, providing a building block for entanglement of distant spins. The device consists of a p-i-n diode structure that incorporates a coupled double quantum dot. We show that electronic control of the diode bias and local gating allow for the generation of single photons that are entangled with a robust quantum memory based on the electron spins. Practical performance of this approach to controlled spin-photon entanglement is analyzed.
We present a mechanism to produce indistinguishable single-photon pulses on demand from an optical cavity. The sequences of two laser pulses generate, at the two Raman transitions of a four-level atom, the same cavity-mode photons without repumping of the atom between photon generations. Photons are emitted from the cavity with near-unit efficiency in well-defined temporal modes of identical shapes controlled by the laser fields. The second order correlation function reveals the single-photon nature of the proposed source. A realistic setup for the experimental implementation is presented.
This paper describes the design, fabrication, and performance of planar-geometry InGaAs-InP devices which were specifically developed for single-photon detection at a wavelength of 1550 nm. General performance issues such as dark count rate, single-photon detection efficiency, afterpulsing, and jitter are described.
Measurement-based quantum communication relies on the availability of highly entangled multi-photon cluster states. The inbuilt redundancy in the cluster allows communication between remote nodes using repeated local measurements, compensating for photon losses and probabilistic Bell-measurements. For feasible applications, the cluster generation should be fast, deterministic, and its photons - indistinguishable. We present a novel source based on a semiconductor quantum-dot device. The dot confines a heavy-hole, precessing in a finely tuned external weak magnetic field while periodically exci…
We demonstrate quantum interference between photons generated by the radiative decay processes of excitons that are bound to isolated fluorine donor impurities in ZnSe/ZnMgSe quantum-well nanostructures. The ability to generate single photons from these devices is confirmed by auto-correlation experiments, and indistinguishability of single photons from two independent devices is confirmed via a Hong-Ou-Mandel dip. These results indicate that donor impurities in appropriately engineered semiconductor structures can portray atom-like homogeneity and coherence properties, potentially enabling sc…
Single-photon sources play a key role in photonic quantum technologies. Semiconductor quantum dots can emit indistinguishable single photons under resonant excitation. However, the resonance fluorescence technique typically requires cross-polarization filtering which causes a loss of the unpolarized quantum dot emission by 50%. To solve this problem, we demonstrate a method to generate indistinguishable single photons with optically controlled polarization by two laser pulses off-resonant with neutral exciton states. This scheme is realized by exciting the quantum dot to the biexciton state an…
Single semiconductor quantum dots have been widely studied within devices that can apply an electric field. In the most common system, the low energy offset between the InGaAs quantum dot and the surrounding GaAs material limits the magnitude of field that can be applied to tens of kVcm^-1, before carriers tunnel out of the dot. The Stark shift experienced by the emission line is typically 1 meV. We report that by embedding the quantum dots in a quantum well heterostructure the vertical field that can be applied is increased by over an order of magnitude whilst preserving the narrow linewidths…
Polarization-orbital angular momentum duality assisted entanglement observation for indistinguishable photons
本研究利用参量下转换产生的不可区分光子的偏振与轨道角动量（OAM）变量，演示了全同粒子纠缠的对偶性，提出了对偶辅助的纠缠观测方法，可验证量子不可区分性在信道中的保持，为分布式量子传感和远程纠缠生成提供研究基础。
Photon-photon interactions are an essential requirement of quantum photonic information processing. One way to generate these interactions is to utilize an atom strongly coupled to an optical cavity. This system exhibits the photon blockade effect which enables single photon switching and creation of non-classical light. But the nonlinear effects enabled by this system suffer from a fundamental time-bandwidth constraint. For the the simple case of splitting an input pulse of two indistinguishable photons, this constraint imposes a limit on the efficiency of routing photons to different output …
Thought experiments involving gases and pistons, such as Maxwell's demon and Gibbs' mixing, are central to our understanding of thermodynamics. Here we present a quantum thermodynamic thought experiment in which the energy transfer from two photonic gases to a piston membrane grows quadratically with the number of photons for indistinguishable gases, while linearly for distinguishable gases. This signature of Bosonic bunching may be observed in optomechanical experiments, highlighting the potential of these systems for the realisation of thermodynamic thought experiments in the quantum realm.
We propose the superfluid to Mott-insulator quantum phase transition in an array of exciton-polariton traps can be utilized for massive parallel generation of indistinguishable single photons. By means of analytical and numerical methods, the device operations and system properties are studied using realistic experimental parameters. Such a deterministic, fault-tolerant, massive parallel generation may open up a new perspective in photonic quantum information processing.
Spatial correlations between two photons are the key resource in realising many quantum imaging schemes. Measurement of the bi-photon correlation map is typically performed using single-point scanning detectors or single-photon cameras based on CCD technology. However, both approaches are limited in speed due to the slow scanning and the low frame-rate of CCD-based cameras, resulting in data acquisition times on the order of many hours. Here we employ a high frame rate, single photon avalanche diode (SPAD) camera, to measure the spatial joint probability distribution of a bi-photon state produ…
We demonstrate a high-brightness source of pairs of indistinguishable photons based on a type-II phase-matched doubly-resonant optical parametric oscillator operated far below threshold. The cavity-enhanced down-conversion output of a PPKTP crystal is coupled into two single-mode fibers with a mode coupling efficiency of 58%. The high degree of indistinguishability between the photons of a pair is demonstrated by a Hong-Ou-Mandel interference visibility of higher than 90% without any filtering at an instantaneous coincidence rate of 450 000 pairs/s per mW of pump power per nm of down-conversio…
We report on the triggered generation of indistinguishable photons by solid-state single-photon sources in two separate cryogenic laser scanning microscopes. Organic fluorescent molecules were used as emitters and investigated by means of high resolution laser spectroscopy. Continuous-wave photon correlation measurements on individual molecules proved the isolation of single quantum systems. By using frequency selective pulsed excitation of the molecule and efficient spectral filtering of its emission, we produced triggered Fourier-limited single photons. In a further step, local electric fiel…
Single-photon emitting devices have been identified as an important building block for applications in quantum information and quantum communication. They allow to transduce and collect quantum information over a long distance via photons as so called flying qubits. In addition, substrates like silicon carbide provides an excellent material platform for electronic devices. In this work we combine these two features and show that one can drive single photon emitters within a silicon carbide p-i-n-diode. To achieve this, we specifically designed a lateral oriented diode. We find a variety of new…
It is a fundamental challenge in quantum optics to deterministically generate indistinguishable single photons through non-deterministic nonlinear optical processes, due to the intrinsic coupling of single- and multi-photon generation probabilities in these processes. Actively multiplexing photons generated in many temporal modes can decouple these probabilities, but key issues are to minimize resource requirements to allow scalability, and to ensure indistinguishability of the generated photons. We demonstrate the multiplexing of photons from four temporal modes solely using fiber-integrated …
We report the results of coincidence counting experiments at the output of a Michelson interferometer using the zero-phonon-line emission of a single molecule at $1.4 K$. Under continuous wave excitation, we observe the absence of coincidence counts as an indication of two-photon interference. This corresponds to the observation of Hong-Ou-Mandel correlations and proves the suitability of the zero-phonon-line emission of single molecules for applications in linear optics quantum computation.
The quantum beam splitter with many partially indistinguishable photons: multiphotonic interference and asymptotic classical correspondence
本文对量子双端口干涉仪中多个部分不可分辨光子的渐近行为进行分析，发现输出分布由围绕特定$j^*$的$O(\sqrt{n})$个通道主导，并呈现半经典双峰包络，对应经典强度分布。
Continuous and deterministic all-photonic cluster state of indistinguishable photons
本研究基于半导体量子点器件，利用束缚空穴自旋连续确定性产生不可区分纠缠光子，首次制备全光子簇态，并通过偏振层析验证了簇纠缠鲁棒性与光子产生确定性。
One of the challenges faced by optical platforms for quantum technologies is the implementation of (ultimately) a transistor. The functionality that is hard to achieve is rectification: having the beam propagating in one direction transmitted, the other reflected. Here we take up a simple model of such a rectifying device, a.k.a.~optical diode, consisting of two atoms with different detuning interacting with light in a one-dimensional waveguide. In previous studies, it was found that high rectifying efficiencies can be achieved with coherent states, while it was claimed that the device cannot …
Room-temperature photonic quantum computing in integrated silicon photonics with germanium-silicon single-photon avalanche diodes
针对光子量子计算依赖低温超导探测器的问题，提出室温波导集成GeSi SPAD及空间复用型PNRAD，结合片上量子光源与可编程干涉回路，有望实现室温高性能光子量子计算。
Single-photon-avalanche diode (SPAD) arrays are essential tools in biophotonics, optical ranging and sensing and quantum optics. However, their small number of pixels, low quantum efficiency and small fill factor have so far hindered their use for practical imaging applications. Here, we demonstrate full-field entangled photon pair correlation imaging using a 100-kpixels SPAD camera. By measuring photon coincidences between more than 500 million pairs of positions, we retrieve the full point spread function of the imaging system and subsequently high-resolution images of target objects illumin…
Entangled Photon Correlations Allow a Continuous-Wave Laser Diode to Measure Single Photon, Time-Resolved Fluorescence
本文提出利用连续波激光二极管产生的纠缠光子对实现时间分辨荧光测量，无需相位调制，具有片上集成、波长可调和飞秒分辨率等优势，为荧光寿命测量提供新途径。
A diode nanocavity for fast, efficient and tunable emission of highly entangled photon pairs and Fourier-transform-limited single photons
研究旨在解决半导体量子点在光子量子技术应用中面临的效率与噪声权衡问题，通过基于量子点嵌入p-i-n二极管圆形布拉格光栅谐振器的可调谐纳米光电器件，实现高效、可调谐的纠缠光子对和单光子发射，为半导体量子光子学提供可行平台。
A key ingredient for quantum photonic technologies is an on-demand source of indistinguishable single photons. State-of-the-art indistinguishable single-photon sources typically employ resonant excitation pulses with fixed repetition rates, creating a string of single photons with predetermined arrival times. However, in future applications, an independent electronic signal from a larger quantum circuit or network will trigger the generation of an indistinguishable photon. Further, operating the photon source up to the limit imposed by its lifetime is desirable. Here, we report on the applicat…
On-demand single-photon sources emitting pure and indistinguishable photons at the telecommunication wavelength are a critical asset towards the deployment of fiber-based quantum networks. Indeed, single photons may serve as flying qubits, allowing communication of quantum information over long distances. Self-assembled InAs quantum dots embedded in GaAs constitute an excellent nearly deterministic source of high quality single photons, but the vast majority of sources operate in the 900-950 nm wavelength range, precluding their adoption in a quantum network. Here, we present a quantum frequen…
Observation of the First-Order Interference Fringes Beyond Coherence Length Employing Commercial Continuous-wave Multi-mode Laser Diode: A Sight of Two-photon Interference
本文利用商用连续波多模激光二极管在远超相干长度的条件下观测到一阶干涉条纹，提出该现象可由时间分辨双光子干涉机制解释，为量子信息科学提供了新方法。
Realization of quantum optical circuits is at the heart of quantum photonic information processing. A long-standing obstacle however has been the absence of a platform of single photon sources (SPSs) that simultaneously satisfies the following required characteristics: spatially ordered SPS arrays that produce, on-demand, highly pure, and indistinguishable single photons with sufficiently uniform emission characteristics across the array, needed for controlled interference between photons from distinct sources to enable functional quantum optical networks. Here we report on such a platform of …
Single-shot high-resolution spectroscopy of single-photon-level optical pulses using a virtually imaged phased-array and single-photon avalanche diode array
本文提出并实验验证了一种结合VIPA频率到空间模式映射与SPAD阵列空间模式检测的单次高分辨率单光子光谱系统，其120 MHz频率模式间隔与掺Pr$^{3+}$离子的Y$_2$SiO$_5$原子频率梳量子存储器相匹配，有望最大化频率复用量子中继器的多路复用能力。
We demonstrate that silicon-vacancy (SiV) centers in diamond can be used to efficiently generate coherent optical photons with excellent spectral properties. We show that these features are due to the inversion symmetry associated with SiV centers, and demonstrate generation of indistinguishable single photons from separate emitters in a Hong-Ou-Mandel (HOM) interference experiment.Prospects for realizing efficient quantum network nodes using SiV centers are discussed.
Transition metal dichalcogenides (TMDs) are optically active layered materials providing potential for fast optoelectronics and on-chip photonics. We demonstrate electrically driven single-photon emission from localised sites in tungsten diselenide (WSe2) and tungsten disulphide (WS2). To achieve this, we fabricate a light emitting diode structure comprising single layer graphene, thin hexagonal boron nitride and TMD mono- and bi-layers. Photon correlation measurements are used to confirm the single-photon nature of the spectrally sharp emission. These results present the TMD family as a platf…
Quantum systems combining indistinguishable photon generation and spin-based quantum information processing are essential for remote quantum applications and networking. However, identification of suitable systems in scalable platforms remains a challenge. Here, we investigate the silicon vacancy centre in silicon carbide and demonstrate controlled emission of indistinguishable and distinguishable photons via coherent spin manipulation. Using strong off-resonant excitation and collecting photons from the ultra-stable zero-phonon line optical transitions, we show a two-photon interference contr…
Temporal photon correlation measurement, instrumental to probing the quantum properties of light, typically requires multiple single photon detectors. Progress in single photon avalanche diode (SPAD) array technology highlights their potential as high performance detector arrays for quantum imaging and photon number resolving (PNR) experiments. Here, we demonstrate this potential by incorporating a novel on-chip SPAD array with 55% peak photon detection probability, low dark count rate and crosstalk probability of 0.14% per detection, in a confocal microscope. This enables reliable measurement…
An on-demand source of indistinguishable and entangled photon pairs is a fundamental component for different quantum information applications such as optical quantum computing, quantum repeaters, quantum teleportation and quantum communication. Parametric down-conversion and four-wave mixing sources of entangled photons have shown high degrees of entanglement and indistinguishability but the probabilistic nature of their generation process also creates zero or multiple photon pairs following a Poissonian distribution. This limits their use in complex algorithms where many qubits and gate opera…
We implement an InGaAs/InP single-photon avalanche diode (SPAD) for single-photon detection with the fastest gating frequency reported so far, of 2.23 GHz, which approaches the limit given by the bandwidth of the SPAD - 2.5 GHz. We propose a useful way to characterize the afterpulsing distribution for rapid gating that allows for easy comparison with conventional gating regimes. We compare the performance of this rapid gating scheme with free-running detector and superconducting single-photon detector (SSPD) for the coherent one-way quantum key distribution (QKD) protocol. The rapid gating sys…
In this letter, we report a compact, low-power laser diode-pumped, all-fiber polarization-entangled photon pair source based on periodically-poled silica fiber technology. The all-fiber source offers room-temperature, alignment-free, turn-key operation, with low power consumption, and is packaged into a fanless, portable enclosure. It features a broad biphoton spectrum of more than 100nm with a concurrence that is greater than 0.96 for polarization entanglement. The source is stable over at least 10 hours of continuous operation, achieving coincidence-to-accidental ratios of more than 2000 con…
We demonstrate a straightforward implementation of a push-button like single-photon source which is based on a strongly coupled atom-cavity system. The device operates intermittently for periods of up to 100 microseconds, with single-photon repetition rates of 1.0 MHz and an efficiency of 60 %. Atoms are loaded into the cavity using an atomic fountain, with the upper turning point near the cavity's mode centre. This ensures long interaction times without any disturbances induced by trapping potentials. The latter is the key to reaching deterministic efficiencies as high as obtained in probabal…
In this letter, we present a detailed, all optical study of the influence of different excitation schemes on the indistinguishability of single photons from a single InAs quantum dot. For this study, we measure the Hong-Ou-Mandel interference of consecutive photons from the spontaneous emission of an InAs quantum dot state under various excitation schemes and different excitation conditions and give a comparison.
A reliable source of identical (indistinguishable) photons is a prerequisite for exploiting interference effects, which is a necessary component for linear optical based quantum computing, and applications thereof such as Boson sampling. Generally speaking, the degree of distinguishability will determine the efficacy of the particular approach, for example by limiting the fidelity of constructed resource states, or reducing the complexity of an optical circuits output distribution. It is therefore of great practical relevance to engineer heralded sources of highly pure and indistinguishable ph…
On-chip indistinguishable photons using III-V nanowire/SiN hybrid integration
该研究将含量子点的单根III-V纳米线集成到硅基SiN波导上，实现片上不可区分光子产生，并揭示不同激发条件下时间抖动、光谱扩散和纯退相对干涉可见度的限制。
We propose an application of quantum temporal imaging to restoring the indistinguishability of the signal and the idler photons produced in type-II spontaneous parametric down-conversion with a pulsed broadband pump. It is known that in this case, the signal and the idler photons have different spectral and temporal properties. This effect deteriorates their indistinguishability and the visibility of the Hong-Ou-Mandel interference, respectively. We demonstrate that inserting a time lens in one arm of the interferometer and choosing properly its magnification factor restores perfect indistingu…
Highly efficient sources of indistinguishable single photons that can operate at room temperature would be very beneficial for many applications in quantum technology. We show that the implementation of such sources is a realistic goal using solid-state emitters and ultrasmall mode volume cavities. We derive and analyze an expression for photon indistinguishability that accounts for relevant detrimental effects, such as plasmon-induced quenching and pure-dephasing. We then provide the general cavity and emitter conditions required to achieve efficient indistinguishable photon emission, and als…
Single molecules in solid-state matrices have been proposed as sources of single-photon Fock states back 20 years ago. Their success in quantum optics and in many other research fields stems from the simple recipes used in the preparation of samples, with hundreds of nominally identical and isolated molecules. Main challenges as of today for their application in photonic quantum technologies are the optimization of light extraction and the on-demand emission of indistinguishable photons. We here present Hong-Ou-Mandel experiments with photons emitted by a single molecule of dibenzoterrylene in…
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