We propose a review of recent developments on entanglement and non-classical effects in collective two-atom systems and present a uniform physical picture of the many predicted phenomena. The collective effects have brought into sharp focus some of the most basic features of quantum theory, such as nonclassical states of light and entangled states of multiatom systems. The entangled states are linear superpositions of the internal states of the system which cannot be separated into product states of the individual atoms. This property is recognized as entirely quantum-mechanical effect and have played a crucial role in many discussions of the nature of quantum measurements and, in particular, in the developments of quantum communications. Much of the fundamental interest in entangled states is connected with its practical application ranging from quantum computation, information processing, cryptography, and interferometry to atomic spectroscopy.
We report an exhaustive numerical analysis of violations of local realism by two qutrits in all possible pure entangled states. In Bell type experiments we allow any pairs of local unitary U(3) transformations to define the measurement bases. Surprisingly, Schmidt rank-2 states, resembling pairs of maximally entangled qubits, lead to the most noise-robust violations of local realism. The phenomenon seems to be even more pronounced for four and five dimensional systems, for which we tested a few interesting examples.
Photon-number correlation measurements are performed on bright squeezed vacuum states using a standard Bell-test setup, and quantum correlations are observed for conjugate polarization-frequency modes. We further test the entanglement witnesses for these states and demonstrate the violation of the separability criteria, which infers that all the macroscopic Bell states, containing typically $10^6$ photons per pulse, are polarization entangled. The study also reveals the symmetry of macroscopic Bell states with respect to local polarization transformations.
We develop a theoretical model to study the Intensity-Intensity correlation of polarization entangled photons emitted in a biexciton-exciton cascade. We calculate the degree of correlation and show how polarization correlation are affected by the presence of dephasing and energy level splitting of the excitonic states. Our theoretical calculations are in agreement with the recent observation of polarization dependent Intensity-Intensity correlations from a single semiconductor quantum dot [R. M. Stevenson et. al., Nature 439, 179 (2006)] . Our model can be extended to study polarization entang…
The relation between genuine multipartite entanglement in the pure state of a collection of N qubits and the nonclassical correlations in its two-qubit subsystems is studied. Quantum discord is used as the quantifier of nonclassical correlations in the subsystem while the generalised geometric measure (GGM) [Phys. Rev. A. 81, 012308 (2010)] is used to quantify global entanglement in the N-qubit state. While no definite discernible dependence between the two can be found for randomly generated global states, for those with additional structure like weighted graph states we find that local disco…
We demonstrate several new results for the nonlinear interferometer, which emerge from a formalism which describes in an elegant way the output field of the nonlinear interferometer as two-mode entangled coherent states. We clarify the relationship between squeezing and entangled coherent states, since a weak nonlinear evolution produces a squeezed output, while a strong nonlinear evolution produces a two-mode, two-state entangled coherent state. In between these two extremes exist superpositions of two-mode coherent states manifesting varying degrees of entanglement for arbitrary values of th…
We present an efficient scheme to generate two-mode SU(2) macroscopic quantum superposition (Schrödinger cat) states, entangled number states and entangled coherent states for the vibrational motion of an ion trapped in a two-dimensional harmonic potential well. We also show that the same scheme can be used to realize a Fredkin gate operation.
Proposals for solid state quantum computing are extremely promising as they can be used to built room temperature quantum computers. If such a quantum computer is ever built it would require in-built sources of nonclassical states required for various quantum information processing tasks. Possibilities of generation of such nonclassical states are investigated here for a physical system composed of a monochromatic light coupled to a two-band semiconductor with direct band gap. The model Hamiltonian includes both photon-exciton and exciton-exciton interactions. Time evolution of the relevant bo…
Localized radiation sources are analyzed with respect to the relation of nonclassicality and quantum entanglement of the emitted light. The source field parts of the radiation emitted in different directions are closely related to each other. As a consequence, nonclassicality of the light fields in one direction directly implies entanglement of the field modes in different directions. This implication can be extended to multipartite-entanglement and multi-time quantum correlations. Given that a nonclassical effect is observed, our approach explicitly yields the multipartite entanglement witnes…
We consider a family of continuous variable (CV) states being a superposition of displaced number states with equal modulo but opposite in sign displacement amplitudes. Either an even or odd CV state is mixed with a delocalized photon at a beam splitter with arbitrary transmittance and reflectance coefficients with the subsequent registration of the measurement outcome in an auxiliary mode to deterministically generate hybrid entanglement. We show that at certain values of the experimental parameters maximally entangled states are generated. The considered approach is also applicable to trunca…
We propose a scheme in which broadband nanostructures allow to generate squeezed light and entanglement of quantum emitters that are extremely far detuned. It is shown that the reduced fluctuations of the electromagnetic field arising from collective resonance fluorescence provide also a means to detect the entanglement between the emitters. Due to the near-field enhancement in the proposed hybrid systems, these nonclassical effects can be encountered outside both the extremely close separations limiting the observation in free space and narrow frequency bands in high-Q cavities. Our approach …
The thesis is divided into three parts. In the first part a new theoretical analysis of interferometric experiments by Alley-Shih, Ou-Mandel and the entanglement swapping experiment is performed. It is shown that the double- and single-photon distinguishability is not necessary for the experiments to be genuine tests against local realism. In the second part, basing on simple geometrical properties of Hilbert space, new, stronger Bell inequalities for M qubits in a maximally entangled state are derived. Application of the same method to two maximally entangled qubits yields an inequality for a…
The ground state of quantum Rabi model (QRM) exhibits rich nonclassical states including squeezed state, cat state, and entangled state in different parameter regimes. In this paper, we firstly use the polaron picture to figure out the process of superradiant phase transition (SPT) in view of the nonclassical states. According to the polaron wave functions, the squeezed state extends to whole parameter regimes, and a small but non-zero weighted antipolaron is necessary to form novel semi-cat states. Moreover, the behavior of superradiance in the QRM can be viewed as the same displacement of th…
The nonclassicality of primordial gravitational waves (PGWs) is characterized in terms of sub-Poissonian graviton statistics. The sub-Poissonian statistics are realized when quantum states are squeezed coherent states. In the presence of matter fields, the Universe experiences the squeezed coherent state during inflation. The condition to realize the sub-Poissonian graviton statistics is translated into the frequency range of gravitational waves. If the initial state is the Bunch-Davies vacuum, there is another necessary condition between phases of squeezing and coherent parameters. Here, we e…
The interaction of two identical three-level atoms of the types $V$, $Ξ$ and $Λ$ with a quantized cavity field as well as a driving external classical field is studied. Under two certain unitary transformations, the system is converted to a typical form of the Jaynes-Cummings model for two three-level atoms. The exact analytical solutions of the wave function for different considered atom-field systems are exactly obtained with the help of the Laplace transform technique, when the atoms are initially prepared in the topmost excited state and the quantized field is in a coherent state. In order…
Mode-entanglement based criteria and measures become insufficient for broadband emission, e.g. from spasers (plasmonic nano-lasers). We introduce criteria and measures for the (i) total entanglement of two wavepackets, (ii) entanglement of a wavepacket with an ensemble and (iii) total nonclassicality of a wavepacket~(WP). We discuss these criteria in the context of (i) entanglement of two WPs emitted from two initially entangled cavities (or two initially entangled atoms) and (ii) entanglement of an emitted WP with the ensemble/atom for the spontaneous emission and the single-photon superradia…
Quantum teleportation establishes a correspondence between an entangled state shared by two separate par- ties that can communicate classically and the presence of a quantum channel connecting the two parties. The standard benchmark for quantum teleportation, based on the average fidelity between the input and output states, indicates that some entangled states do not lead to channels which can be certified to be quantum. It was re- cently shown that if one considers a finer-tuned witness, then all entangled states can be certified to produce a non-classical teleportation channel. Here we expe…
A novel method of macroscopically entangled light-pair generation is presented for a quantum laser using randomness-based deterministic phase control of coherent light in a Mach-Zehnder interferometer (MZI). Unlike the particle nature-based quantum correlation in conventional quantum mechanics, the wave nature of photons is applied for collective phase control of coherent fields, resulting in a deterministically controllable nonclassical phenomenon. For the proof of principle, the entanglement between output light fields from an MZI is examined using the Hong-Ou-Mandel-type anticorrelation tec…
We propose a scheme to generate nonclassical states of a quantum system, which is composed of the one-dimensional trapped ion motion and a single cavity field mode. We show that two-mode SU(2) Schrödinger-cat states, entangled coherent states, two-mode squeezed vacuum states and their superposition can be generated. If the vibration mode and the cavity mode are used to represent separately a qubit, a quantum phase gate can be implemented.
We show that correlations inconsistent with any locally causal description can be a generic feature of measurements on entangled quantum states. Specifically, spatially-separated parties who perform local measurements on a maximally-entangled state using randomly chosen measurement bases can, with significant probability, generate nonclassical correlations that violate a Bell inequality. For n parties using a Greenberger-Horne-Zeilinger state, this probability of violation rapidly tends to unity as the number of parties increases. We also show that, even with both a randomly chosen two-qubit p…
We report nonclassical aspects of the collective behaviour of two atoms in a cavity by investigating the photon statistics and photon distribution in a very broad domain of parameters. Starting with the dynamics of two atoms radiating in phase into the cavity, we study the photon statistics for arbitrary interatomic phases as revealed by the second-order intensity correlation function at zero time $g^{(2)}(0)$ and the Mandel $Q$ parameter. We find that the light field can be tuned from antibunched to (super-)bunched as well as nonclassical to classical behaviour by merely modifying the atomic …
Description of nonclassicality of states has hitherto been through violation of Bell inequality and non-separability, with the latter being a stronger constraint. In this paper, we show that this can be further sharpened, by introducing the concept of classical simulation. A state admits classical simulation if it can be mimicked fully by a separable state of higher dimension. A nonclassical state, which we call exceptional, does not admit classical simulation. Focusing on two qubit states, we show that exceptionality is more stringent than violation of Bell inequality, and involves an intrica…
We show that two-time, second-order correlations of scattered photons from planar arrays and chains of atoms display nonclassical features that can be described by a superatom picture of the canonical single-atom $g_2(τ)$ resonance fluorescence result. For the superatom, the single-atom linewidth is replaced by the linewidth of the underlying collective low light-intensity eigenmode. Strong light-induced dipole-dipole interactions lead to a correlated response, suppressed joint photon detection events, and dipole blockade that inhibits multiple excitations of the collective atomic state. For t…
We briefly review the ideas that have shaped modern optics and have led to various applications of light ranging from spectroscopy to astrophysics, and street lights to quantum communication. The review is primarily focused on the modern applications of classical light and nonclassical light. Specific attention has been given to the applications of squeezed, antibunched, and entangled states of radiation field. Applications of Fock states (especially single photon states) in the field of quantum communication are also discussed.
Although nonclassical quantum states are important both conceptually and as a resource for quantum technology, it is often difficult to test whether a given quantum system displays nonclassicality. A simple method to certify nonclassicality is introduced, based on easily accessible collective atomic quadrature measurements, without the need of full state tomography. The statistics is analyzed beyond the ground-state noise level, by direct sampling of a regularized atomic quadrature quasiprobability. Nonclassicality of a squeezed ensemble of 2x10^5 Cesium atoms is demonstrated, with a significa…
The question whether all entangled states can be used as a nonclassical resource has remained open so far. Here we provide a conclusive answer to this problem for the case of systems shared by two parties. We show that any entangled state $σ$ can enhance the teleportation power of some other state. This holds even if the state $σ$ is bound entangled.
We theoretically study the dynamics of entangled states created in a beam splitter with a nonlinear Kerr medium placed into one input arm. Entanglement dynamics of initial classical and nonclassical states are studied and compared. Signatures of revival and fractional revival phenomena exhibited during the time evolution of states in the Kerr medium are captured in the entangled states produced by the beam splitter. Maximum entanglement is obtained at the instants of collapses of wave packets in the medium. Our analysis shows increase in entanglement with increase in the degree of nonclassical…
The interaction of mesoscopic interference devices with nonclassical electromagnetic fields is studied. The external quantum fields induce a phase factor on the electric charges. This phase factor, which is a generalization of the standard Aharonov-Bohm phase factor, is in the case of nonclassical electromagnetic fields a quantum mechanical operator. Its expectation value depends on the density matrix describing the nonclassical photons and determines the interference. Several examples are discussed, which show that the quantum noise of the nonclassical photons destroys slightly the electron i…
We consider macroscopic correlations in a bipartite system consisting of 2N particles described by a generalised probabilistic theory. In particular, we discuss a case of N PR-boxes shared between two parties. We characterise macroscopic measurements as collective measurements of the same property on all the boxes in the same region. Such measurements are assumed to reveal only the average value of the measured collective property. We show that for two measurements per observer and N greater or equal 2 there always exist a joint probability distribution explaining all observable data and there…
Photonic crystal cavities can localize light into nanoscale volumes with high quality factors. This permits a strong interaction between light and matter, which is important for the construction of classical light sources with improved properties (e.g., low threshold lasers) and of nonclassical light sources (such as single and entangled photon sources) that are crucial pieces of hardware of quantum information processing systems. This article will review some of our recent experimental and theoretical results on the interaction between single quantum dots and photonic crystal cavity fields, a…
Over the last twenty years of research on quantum game theory have given us many ideas of how quantum games could be played. One of the most prominent ideas in the field is a model of quantum playing a 2x2 game introduced by J. Eisert, M. Wilkens and M. Lewenstein. The scheme assumes that players' strategies are unitary operations the players act on the maximally entangled two-qubit state. The quantum nature of the scheme has been under discussion since the article by Eisert et al. came out. The aim of our paper is to identify some of non-classical features of the quantum scheme.
We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the…
Relative and center of mass cordinates are used to generalize mutually unbiased bases (MUB) and define mutually unbiased bases (MUCB). Maximal entangled states are given as product staes in the collective varibles
We propose a method to generate nonclassical states of light in multimode microwave cavities. Our approach considers two-photon processes that take place in a system composed of two extended cavities and an ultrastrongly coupled light-matter system. Under specific resonance conditions, our method generates, in a deterministic manner, product states of uncorrelated photon pairs, Bell states, and W states. We demonstrate improved generation times when increasing the number of multimode cavities, and prove the generation of genuine multipartite entangled states when coupling an ancillary system t…
Quantum technologies exploit entanglement to revolutionize computing, measurements, and communications. This has stimulated the research in different areas of physics to engineer and manipulate fragile many-particle entangled states. Progress has been particularly rapid for atoms. Thanks to the large and tunable nonlinearities and the well developed techniques for trapping, controlling and counting, many groundbreaking experiments have demonstrated the generation of entangled states of trapped ions, cold and ultracold gases of neutral atoms. Moreover, atoms can couple strongly to external forc…
We present a new and feasible test proving quantum contextuality in four-dimensional Hiltbert space. In our scheme, a contradiction between quantum mechanics and noncontextual hidden variables is revealed through the measurement statistics of two joint measurements of an ensemble of non-entangled qubits. The origin of nonclassicality is fully attributed to the measurement process. Quantum optical realization using photon pairs and linear optics are presented.
Reassessing the boundary between classical and nonclassical for individual quantum processes
Institute for Quantum Computing, University of Waterloo（滑铁卢大学量子计算研究所）；Perimeter Institute for Theoretical Physics（理论物理前沿研究所）；Department of Physics & Astronomy, University of Waterloo（滑铁卢大学物理与天文学系）
We study an experimental scheme to generate Gaussian two-mode entangled states via beam splitter. Specifically, we consider a nonclassical Gaussian state (squeezed state) and a thermal state as two input modes, and evaluate the degree of entanglement at the output. Experimental conditions to generate entangled outputs are completely identified and the critical thermal noise to destroy entanglement is analytically obtained. By doing so, we discuss the possibility to link the resistance to noise in entanglement generation with the degree of single-mode nonclassicality.
We motivate and introduce a class of "hierarchical" quantum superposition states of $N$ coupled quantum oscillators. Unlike other well-known multimode photonic Schrödinger cat states such as entangled coherent states, the hierarchical superposition states are characterized as two-branch superpositions of tensor products of single-mode Schrödinger cat states. In addition to analyzing the photon statistics and quasiprobability distributions of prominent examples of these nonclassical states, we consider their usefulness for high-precision quantum metrology of nonlinear optical Hamiltonians and q…
We derive a master equation describing the collective decay of two-level atoms inside a single mode cavity in the dispersive limit. By considering atomic decay in the collective thermostat, we found a decoherence-free subspace of the multiparticle entangled states of the W-like class. We present a scheme for writing and storing these states in collective thermostat.
Nonclassical Many-Body Superradiant States with Interparticle and Spin-Momentum Entanglement
JILA and Department of Physics, University of Colorado（科罗拉多大学物理系与JILA）；Theoretische Physik, Universität des Saarlandes（萨尔兰州立大学理论物理学）；Physikalisches Institut, University of Bonn（波恩大学物理研究所）
Most experimental demonstrations of entanglement require nonclassical states and correlated measurements of single-photon detection events. It is shown here that entanglement can produce a large decrease in the rate of two-photon absorption for a classical input state that can be observed using classical detectors. These effects can be interpreted as being due to the creation of entangled photon holes that are somewhat analogous to the holes of semiconductor theory.
Ensembles of alkali or noble-gas atoms at room temperature and above are widely applied in quantum optics and metrology owing to their long-lived spins. Their collective spin states maintain nonclassical nonlocal correlations, despite the atomic thermal motion in the bulk and at the boundaries. Here we present a stochastic, fully-quantum description of the effect of atomic diffusion in these systems. We employ the Bloch-Heisenberg-Langevin formalism to account for the quantum noise originating from diffusion and from various boundary conditions corresponding to typical wall coatings, thus mode…
The quantum teleportation process is composed of a joint measurement performed upon two subsystems A and B (uncorrelated), followed by a unitary transformation (parameters of which depend on the outcome of the measurement) performed upon a third subsystem C (EPR correlated with system B). The information about the outcome of the measurement is transferred by classical means. The measurement performed upon the systems A and B collapses their joint wavefunction into one of the four {\it entangled} Bell states. It is shown here that this measurement process plus a possible measurement on the thir…
Quantum teleportation is a method for utilizing quantum measurements and the maximally entangled Einstein-Podolsky-Rosen (EPR) pair to transmit an unknown quantum state. It is well known that all entangled states demonstrate so-called "nonclassical teleportation" that cannot be simulated by the seminal classical measure-prepare strategy. Herein, we propose a new benchmark which reveals that not all nonclassical teleportations are truly quantum-mechanical. Rather, there exists a more robust classical-teleportation model, which includes the measure-prepare mimicry as a special case, that can des…
Nonclassical motional states of matter are of interest both from a fundamental perspective but also for their potential technological applications as resources in various quantum processing tasks such as quantum teleportation, sensing, communication, and computation. In this work we explore the motional effects of a harmonically trapped, excited two-level emitter coupled to a one-dimensional (1D) photonic system. As the emitter decays it experiences a momentum recoil that entangles its motion with the emitted photon pulse. In the long-time limit the emitter relaxes to its electronic ground sta…
We introduce a new method of investigating qutrit nonclassicality by translating qutrit operators to symmetric two-qubit operators. We show that this procedure partially resolves the discrepancy between maximal qutrit entanglement and maximal nonclassicality of qutrit correlations. Namely we express Bell operators corresponding to qutrit Bell inequalities in terms of symmetric two-qubit operators, and analyze the maximal quantum violation of a given Bell inequality from the qubit perspective. As an example we show that the two-qutrit CGLMP(Collins-Gisin-Linden-Massar-Popescu) Bell inequality c…
We present a fully quantum mechanical treatment of recent experiments on creation of collective quantum memory and generation of non-classically correlated photon pairs from an atomic ensemble via the protocol of Duan et al. [Nature {\bf 414,} 413(2001)]. The temporal evolution of photon numbers, photon statistics and cross-correlation between the Stokes and anti-Stokes fields is found by solving the equation of motion for atomic spin-wave excitations. We consider a low-finesse cavity model with collectively enhanced signal-to-noise ratio, which remains still considerably large in the free-spa…
A system of two two-level atoms interacting with a squeezed vacuum field can exhibit stationary entanglement associated with nonclassical two-photon correlations characteristic of the squeezed vacuum field. The amount of entanglement present in the system is quantified by the well known measure of entanglement called concurrence. We find analytical formulas describing the concurrence for two identical and nonidentical atoms and show that it is possible to obtain a large degree of steady-state entanglement in the system. Necessary conditions for the entanglement are nonclassical two-photon corr…
The notion of entanglement is the most well-known nonclassical correlation in quantum mechanics and a fundamental resource in quantum information and computation. This correlation, which is displayed by certain classes of quantum states, is of utmost importance when dealing with protocols such as quantum teleportation, cryptography, and quantum key distribution. In this paper, we exploit a classification of tripartite entanglement by introducing the concepts of entangled hypergraph and evolving entangled hypergraph as data structures suitable to model quantum protocols which use entanglement. …
We analyze nonclassical correlations between outcomes of measurements conducted on two spatial radiation modes. These correlations cannot be simulated with statistical mixtures of coherent states or, more generally, with non-negative phase-space functions of quantum states and measurements. We argue that nonclassical correlations are naturally related to Bell nonlocality, the former being a more general class of quantum correlations. Indeed, it is known that local realistic as well as noncontextual models correspond to non-negative solutions to a system of linear equations for the joint probab…
A simple model allows us to study the nonclassical behavior of slowly moving atoms interacting with a quantized field. Atom and field become entangled and their joint state can be identified as a mesoscopic "Schroedinger-cat". By introducing appropriate observables for atom and field and by analyzing correlations between them based on a Bell-type inequality we can show the corresponding nonclassical behavior.
We experimentally demonstrate sum-frequency generation (SFG) with entangled photon-pairs, generating as many as 40,000 SFG photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a linear intensity-dependence of the nonlinear process. The key element in our scheme is the generation of an ultrahigh flux of entangled photons while maintaining their nonclassical properties. This is made possible by generating the down-converted photons as broadband as possible, orders of magnitude wider than the pump. This approach is readily applicable for ot…
We demonstrate the generation of multi-photon quantum states of light by cavity-enhanced parametric down-conversion in the high-repetition-rate pulsed regime. An external enhancement cavity resonant with the spectral comb of modes of a mode-locked pump laser provides a coherent build-up of the pump intensity and greatly enhances the parametric gain without sacrificing its high repetition rate and comb structure. We probe the parametric gain enhancement by the conditional generation and tomographic analysis of two-photon Fock states. Besides its potential impact to efficiently generate highly-n…
We experimentally demonstrated entanglement extraction scheme by using photons at the telecommunication band for optical-fiber-based quantum communications. We generated two pairs of non-degenerate polarization entangled photons at 780~nm and 1551~nm by spontaneous parametric down-conversion and distributed the two photons at 1551~nm through a collective phase damping channel which gives the same amount of random phase shift on the two photons. Through local operation and classical communication, we extracted an entangled photon pair from two phase-disturbed photon pairs. An observed fidelity …
We investigate the states generated in continuous variable (CV) optical fields on operating them with a number-conserving operator of the type $s\hat{a}\hat{a}^†+ t\hat{a}^†\hat{a}$, formed by the generalised superposition of products of field annihilation ($\hat{a}$) and creation ($\hat{a}^†$) operators, with $s^2+t^2=1$. Such an operator is experimentally realizable and can be suitably manipulated to generate nonclassical optical states when applied on single- and two-mode coherent, thermal, and squeezed input states. At low intensities, these nonclassical states can interact with a secondar…
