Generation and nonclassicality of entangled states via the interaction of two three-level atoms with a quantized cavity field assisted by a driving external classical field
H. R. Baghshahi, M. K. Tavassoly, S. J. Akhtarshenas
The interaction of two identical three-level atoms of the types $V$, $Ξ$ and $Λ$ with a quantized cavity field as well as a driving external classical field is studied. Under two certain unitary transformations, the system is converted to a typical form of the Jaynes-Cummings model for two three-level atoms. The exact analytical solutions of the wave function for different considered atom-field systems are exactly obtained with the help of the Laplace transform technique, when the atoms are initially prepared in the topmost excited state and the quantized field is in a coherent state. In order to examine the nonclassicality features of the deduced states, the dynamics of the entanglement between subsystems is discussed via two well-known measures, namely, von Neumann entropy of the reduced state and negativity. In addition, we pay attention to the temporal behaviour of quantum statistics of the photons of the field and squeezing phenomenon. Meanwhile, the influence of the external classical field on the latter physical quantities is analyzed in detail. The results show that the mentioned quantities can be sensitively controlled via the external classical field. Also, numerical computations imply the fact that the nonclassicality features in $Ξ$-type three-level atomic system is more visible than the other two configurations. In addition, it is shown that in the particular case of $Λ$-type atomic system, the rank of the reduced density matrix of the three-level atoms is no larger than three, so that negativity fully captures the entanglement of this system and that such entanglement is distillable.
We report an exhaustive numerical analysis of violations of local realism by two qutrits in all possible pure entangled states. In Bell type experiments we allow any pairs of local unitary U(3) transformations to define the measurement bases. Surprisingly, Schmidt rank-2 states, resembling pairs of maximally entangled qubits, lead to the most noise-robust violations of local realism. The phenomenon seems to be even more pronounced for four and five dimensional systems, for which we tested a few interesting examples.
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
Mode-entanglement based criteria and measures become insufficient for broadband emission, e.g. from spasers (plasmonic nano-lasers). We introduce criteria and measures for the (i) total entanglement of two wavepackets, (ii) entanglement of a wavepacket with an ensemble and (iii) total nonclassicality of a wavepacket~(WP). We discuss these criteria in the context of (i) entanglement of two WPs emitted from two initially entangled cavities (or two initially entangled atoms) and (ii) entanglement of an emitted WP with the ensemble/atom for the spontaneous emission and the single-photon superradia…
Localized radiation sources are analyzed with respect to the relation of nonclassicality and quantum entanglement of the emitted light. The source field parts of the radiation emitted in different directions are closely related to each other. As a consequence, nonclassicality of the light fields in one direction directly implies entanglement of the field modes in different directions. This implication can be extended to multipartite-entanglement and multi-time quantum correlations. Given that a nonclassical effect is observed, our approach explicitly yields the multipartite entanglement witnes…
The quantum nature of the state of a bosonic quantum field manifests itself in its entanglement, coherence, or optical nonclassicality which are each known to be resources for quantum computing or metrology. We provide quantitative and computable bounds relating entanglement measures with optical nonclassicality measures. These bounds imply that strongly entangled states must necessarily be strongly optically nonclassical. As an application, we infer strong bounds on the entanglement that can be produced with an optically nonclassical state impinging on a beam splitter. For Gaussian states, we…
We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the…
We introduce a kind of entangled state---photon-addition two-mode squeezed thermal state (TMSTS) by adding photons to each mode of the TMSTS. Using the P-representation of thermal state, the compact expression of the normalization factor is derived, a Jacobi polynomial. The nonclassicality is investigated by exploring especially the negativity of Wigner function. The entanglement is discussed by using Shchukin-Vogel criteria. It is shown that the photon-addtion to the TMSTS may be more effective for the entanglement enhancement than the photon-subtraction from the TMSTS. In addition, the quant…
We introduce a new method of investigating qutrit nonclassicality by translating qutrit operators to symmetric two-qubit operators. We show that this procedure partially resolves the discrepancy between maximal qutrit entanglement and maximal nonclassicality of qutrit correlations. Namely we express Bell operators corresponding to qutrit Bell inequalities in terms of symmetric two-qubit operators, and analyze the maximal quantum violation of a given Bell inequality from the qubit perspective. As an example we show that the two-qutrit CGLMP(Collins-Gisin-Linden-Massar-Popescu) Bell inequality c…
Systems of on-off detectors are well established for measuring radiation fields in the regime of small photon numbers. We propose to combine these detector systems with unbalanced homodyning with a weak local oscillator. This approach yields phase-space functions, which represent the click counterpart of the s parametrized quasiprobabilities of standard photoelectric detection theory. This introduced class of distributions can be directly sampled from the measured click counting statistics. Therefore, our technique visualizes nonclassical effects without further data processing. Surprisingly, …
We study the relation between single-mode nonclassicality and two-mode entanglement in a beam-splitter. We show that not all of the nonclassicality (entanglement potential) is transformed into two-mode entanglement for an incident single-mode light. Some of the entanglement potential remains as single-mode nonclassicality in the two entangled output modes. Two-mode entanglement generated in the process can be equivalently quantified as the increase in the minimum uncertainty widths (or decrease in the squeezing) of the output states compared to the input states. We use the nonclassical depth a…
The interaction between a $\diamondsuit$-type four-level atom and a single-mode field in the presence of Kerr medium with intensity-dependent coupling involving multi-photon processes has been studied. Using the generalized (nonlinear) Jaynes-Cummings model, the exact analytical solution of the wave function for the considered system under particular condition, has been obtained when the atom is initially excited to the topmost level and the field is in a coherent state. Some physical properties of the atom-field entangled state such as linear entropy showing the entanglement degree, Mandel pa…
Various lower- and higher-order nonclassical properties have been studied for two physical systems- (i) an optomechanical system composed of a Fabry-Perot cavity with one nonlinearly oscillating mirror and (ii) an optomechanical-like system formed using a Bose-Einstein condensate (BEC) trapped inside an optical cavity. The investigation is performed using a perturbation method that leads to closed form analytic expressions for the time evolution of the relevant bosonic operators. In the first system, it is observed that the radiation pressure coupling leads to the emergence of lower- and highe…
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of identical two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled $W$ states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations as one needs to e…
Shiv Nadar Institution of Eminence（希夫纳德卓越机构）；ICFO-Institut de Ciencies Fotoniques, The Barcelona Institute of Science and Technology（ICFO-光子科学研究所，巴塞罗那科学技术研究院）；ETH Zürich（苏黎世联邦理工学院）；University College London（伦敦大学学院）
Description of nonclassicality of states has hitherto been through violation of Bell inequality and non-separability, with the latter being a stronger constraint. In this paper, we show that this can be further sharpened, by introducing the concept of classical simulation. A state admits classical simulation if it can be mimicked fully by a separable state of higher dimension. A nonclassical state, which we call exceptional, does not admit classical simulation. Focusing on two qubit states, we show that exceptionality is more stringent than violation of Bell inequality, and involves an intrica…
Recently, in [Phys. Rev. A 97, 043806 (2018)], the detuned and nonlinear Jaynes-Cummings model describing the quantized motion of a trapped ion was introduced and its corresponding dynamics was solved via considering the driving laser in a quantized manner. In this work we reconsider this model and show that it can likewise be solved with a classical driving laser field. Using the exact solution we investigate the quantum time-ordering effects of the system with respect to nonclassicality of the motional states of the ion. Furthermore, we use the Magnus expansion to analyze the impact of certa…
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a g…
We present a study of photon statistics associated with high-order harmonic generation (HHG) involving one-mode and intermodal correlations of the high harmonic photons. The aim of the paper is to give insight into the nonclassical properties of high-order harmonic modes. To this end, we use a simplified model describing an elementary quantum emitter: the model of a two-level atom. While the material system is extremely simplified in this description, the conclusions and the methods may be generalized for more complex cases. Our primary interest is an effective model of HHG in which the exciti…
We study the evolution of entangled coherent states of the two quantized electromagnetic fields under dissipation. Characteristic time scales for the decay of the negativity are found in the case of large values of the phase space distance among the states of each mode. We also study how the entanglement emerges among the reservoirs.
We propose and design a high-brightness, ultra-compact electrically pumped GaSb-based laser source of entangled photons generated by mode-matched intracavity parametric down-conversion of lasing modes. To describe the nonlinear mixing in highly dispersive and dissipative waveguides, we develop a nonperturbative quantum theory of parametric down-conversion of waveguide modes which takes into account the effects of modal dispersion, group and phase mismatch, propagation, dissipation, and coupling to noisy reservoirs. We extend our theory to the regime of quantized pump fields with a new approach…
In this paper, we follow our presented model in J. Opt. Soc. Am. B {\bf 30}, 1109--1117 (2013), in which the interaction between a $Λ$-type three-level atom and a quantized two-mode radiation field in a cavity in the presence of nonlinearities is studied. After giving a brief review on the procedure of obtaining the state vector of the atom-field system, some further interesting and important physical features (which are of particular interest in the quantum optics field of research) of the whole system state, i.e., the number-phase entropic uncertainty relation (based on the two-mode Pegg-Bar…
Rigorous results on approach to thermal equilibrium, entanglement, and nonclassicality of an optical quantum field mode scattering from the elements of a non-equilibrium quantum reservoir
We study quantum dynamics of many-qubit systems strongly coupled to a quantized electromagnetic cavity field in the presence of decoherence and dissipation for both fermions and cavity photons, and taking into account the varying coupling strength of different qubits to the cavity field and the spread of their transition frequencies. Compact analytic solutions for time-dependent quantum state amplitudes and observables are derived for a broad class of open quantum systems in Lindblad approximation with the use of the stochastic Schroedinger equation approach. We show that depending on the init…
Nonclassical states of a quantized light are described in terms of Glauber-Sudarshan P distribution which is not a genuine classical probability distribution. Despite several attempts, defining a uniform measure of nonclassicality (NC) for the single mode quantum states of light is yet an open task. In our previous work [Phys. Rev. A 95, 012330 (2017)] we have shown that the existing well-known measures fail to quantify the NC of single mode states that are generated under multiple NC-inducing operations. Recently, Ivan et. al. [Quantum. Inf. Process. 11, 853 (2012)] have defined a measure of …
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We study the resonance interaction between two entangled identical atoms coupled to a quantized scalar field vacuum, and accelerating between two mirrors. We show how radiative processes of the two-atom entangled state can be manipulated by the atomic configuration undergoing noninertial motion. Incorporating the Heisenberg picture with symmetric operator ordering, the vacuum fluctuation and the self-reaction contributions are distinguished. We evaluate the resonance energy shift and the relaxation rate of energy of the two atom system from the self-reaction contribution in the Heisenberg equa…
Proposals for solid state quantum computing are extremely promising as they can be used to built room temperature quantum computers. If such a quantum computer is ever built it would require in-built sources of nonclassical states required for various quantum information processing tasks. Possibilities of generation of such nonclassical states are investigated here for a physical system composed of a monochromatic light coupled to a two-band semiconductor with direct band gap. The model Hamiltonian includes both photon-exciton and exciton-exciton interactions. Time evolution of the relevant bo…
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We have constructed a theoretical framework of the biexciton-resonant hyperparametric scattering for the pursuit of high-power and high-quality generation of entangled photon pairs. Our framework is applicable to nano-to-bulk crossover regime where the center-of-mass motion of excitons and biexcitons is confined. Material surroundings and the polarization correlation of generated photons can be considered. We have analyzed the entangled-photon generation from CuCl film, by which ultraviolet entangled-photon pairs are generated, and from dielectric microcavity embedding a CuCl layer. We have re…
We propose a novel scheme for the efficient production of "NOON states" based on the resonant interaction of a pair of quantized cavity modes with an ensemble of atoms. We show that in the strong-coupling regime the adiabatic evolution of the system tends to a limiting state that describes mesoscopic entanglement between photons and atoms which can easily be converted to a purely photonic or atomic NOON state. We also demonstrate the remarkable property that the efficiency of this scheme increases exponentially with the cavity cooperativity factor, which gives efficient access to high number N…
We develop the analytic theory describing the formation and evolution of entangled quantum states for a fermionic quantum emitter coupled to a quantized electromagnetic field in a nanocavity and quantized phonon or mechanical vibrational modes. The theory is applicable to a broad range of cavity quantum optomechanics problems and emerging research on plasmonic nanocavities coupled to single molecules and other quantum emitters. The optimal conditions for a tri-state entanglement are realized near the parametric resonances in a coupled system. The model includes decoherence effects due to coupl…
Photons may have homogeneous polarization and may carry quantized orbital angular momentum (OAM). Photon entanglement has been realized in various degrees of freedom such as polarization and OAM. Using a pair of orthogonally polarized states carrying opposite-handedness quantized OAMs could create "quantized" vector polarization states with space-variant polarization structures. It is thus possible to extend the polarization degree of freedom from two dimensional space to indefinite dimensional discrete Hilbert space. We present a class of vector-polarization entangled Bell states, which use t…
The interaction between two $Ξ$-type three-level atoms and a single-mode cavity field in the intensity dependent coupling regime has been studied. Exact analytical solution of the wave function for the considered atoms-field system has been obtained by using the Laplace transform technique when the atoms are initially prepared in the excited state and the field is in a coherent state. The presented structure has the potential ability to generate various new classes of entangled states depending on the chosen nonlinearity function. Two forms of intensity-dependent coupling as well as constant c…
We study quantum dynamics of many-qubit systems strongly coupled to a quantized electromagnetic cavity mode, in the presence of decoherence and dissipation for both fermions and cavity photons. The analytic solutions are derived for a broad class of open quantum systems in Lindblad approximation. They include identical qubits, an ensemble of qubits with a broad distribution of transition frequencies, and multi-level electron systems. Compact analytic solutions for time-dependent quantum state amplitudes and observables become possible with the use of the stochastic equation of evolution for th…
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The quantum photodynamics of a simple diatomic molecule with a permanent dipole immersed within an optical cavity containing a quantized radiation field is studied in detail. The chosen molecule under study, lithium fluoride (LiF), is characterized by the presence of an avoided crossing between the two lowest $^1Σ$ potential energy curves (covalent-ionic diabatic crossing). Without field, after prompt excitation from the ground state $1\; ^1Σ$, the excited nuclear wave packet moves back and forth in the upper $2\; ^1Σ$ state, but in the proximity of the avoided crossing, the non-adiabatic coup…
Quantum-mechanically correlated (entangled) states of many particles are of interest in quantum information, quantum computing and quantum metrology. Metrologically useful entangled states of large atomic ensembles have been experimentally realized, but these states display Gaussian spin distribution functions with a non-negative Wigner function. Non-Gaussian entangled states have been produced in small ensembles of ions, and very recently in large atomic ensembles. Here, we generate entanglement in a large atomic ensemble via the interaction with a very weak laser pulse; remarkably, the detec…
In the present paper an example of entanglement between two different kinds of interacting particles, photons and electrons is analysed. The initial-value problem of the Schroedinger equation is solved non-perturbatively for the system of a free electron interacting with a quantized mode of the electromagnetic radiation. Wave packets of the dressed states so obtained are constructed in order to describe the spatio-temporal separation of the subsystems before and after the interaction. The joint probability amplitudes are calculated for the detection of the electron at some space-time location …
We investigate the quantum deformation of the Wheeler--DeWitt equation of a Schwarzchild black hole. Specifically, the quantum deformed black hole is a quantized model constructed from the quantum Heisenberg--Weyl $U_q(h_4)$ group. We show that the event horizon area and the mass are quantized, degenerate, and bounded. The degeneracy of states indicates entangled quantum black hole/white hole states. Accordingly, quantum deformation provides a new framework to examine Einstein--Rosen wormhole solutions. Besides, we obtain the mass, the temperature, and the entropy of the q-deformed quantum Sch…
Second-quantized numerical simulations of tunable entanglement in quantum high harmonic generation
Max Planck Institute for the Structure and Dynamics of Matter（马克斯·普朗克物质与结构动力学研究所）；Center for Computational Quantum Physics, The Flatiron Institute（平顿研究院计算量子物理中心）；Technion - Israel Institute of Technology（以色列理工学院）
In this paper, we study the interaction between a three-level atom and a quantized single-mode field with $` `$intensity-dependent coupling$"$ in a $` `$Kerr medium$"$. The three-level atom is considered to be in a $Λ$-type configuration. Under particular initial conditions, which may be prepared for the atom and the field, the dynamical state vector of the entire system will be explicitly obtained, for arbitrary nonlinearity function $f(n)$ associated to any physical system. Then, after evaluating the variation of the field entropy against time, we will investigate the quantum statistics as w…
