We experimentally demonstrate sum-frequency generation (SFG) with entangled photon-pairs, generating as many as 40,000 SFG photons per second, visible even to the naked eye. The nonclassical nature of the interaction is exhibited by a linear intensity-dependence of the nonlinear process. The key element in our scheme is the generation of an ultrahigh flux of entangled photons while maintaining their nonclassical properties. This is made possible by generating the down-converted photons as broadband as possible, orders of magnitude wider than the pump. This approach is readily applicable for other nonlinear interactions, and may be applicable for various quantum-measurement tasks.
High-quality entangled photon pairs generated via spontaneous parametric down-conversion have made great contributions to the modern quantum information science and the fundamental tests of quantum mechanics. However, the quality of the entangled states decreases sharply when moving from biphoton to multiphoton experiments, mainly due to the lack of interactions between photons. Here, for the first time, we generate a four-photon Greenberger-Horne-Zeilinger state with a fidelity of $98\%$, which is even comparable to the best fidelity of biphoton entangled states. Thus, it enables us to demons…
In this letter, we report a compact, low-power laser diode-pumped, all-fiber polarization-entangled photon pair source based on periodically-poled silica fiber technology. The all-fiber source offers room-temperature, alignment-free, turn-key operation, with low power consumption, and is packaged into a fanless, portable enclosure. It features a broad biphoton spectrum of more than 100nm with a concurrence that is greater than 0.96 for polarization entanglement. The source is stable over at least 10 hours of continuous operation, achieving coincidence-to-accidental ratios of more than 2000 con…
We experimentally demonstrate a source of polarization entangled photon-pairs based on a single periodically-poled potassium titanyl phosphate (PPKTP) crystal pumped with a broadband, free running laser diode.The crystal is placed within a linear beam-displacement interferometer, and emits photon-pairs based ontype-0 spontaneous parametric downconversion (SPDC). We observe pair rates of 0.56 Mpairs/s/mW in a single spatial mode with a polarization visibility of 97.7% over a spectral range of 100 nm. This experiment demonstrates a pathway towards observing Gigacount rates of polarization entang…
We present a proof-of-principle experimental demonstration of a reconfigurable entanglement distribution scheme utilizing a poled fiber-based source of broadband polarization-entangled photon pairs and dense wavelength-division multiplexing. A large bandwidth (> 90 nm, centered at 1555 nm) and highly spectrally correlated nature of the entangled source can be exploited to allow for the generation of more than 25 frequency-conjugate entangled pairs when aligned to the standard 200 GHz ITU grid. In this work, three frequency-conjugate entangled pairs are used to demonstrate quantum key distribut…
Generating entangled photons from a monolithic chip is a major milestone towards real-life applications of optical quantum information processing including quantum key distribution and quantum computing. Ultrabroadband entangled photons are of particular interest to various applications such as quantum metrology and multi-party entanglement distribution. In this work, we demonstrate the direct generation of broadband wavelength multiplexed polarization entangled photons from a semiconductor chip for the first time. Without the use of any on-chip compensation, interferometry, entangled photons …
We present a new approach to engineering broadband sources of entangled photon pairs for quantum interferometry. The source is based on quasi-phase-matched spontaneous parametric down conversion in a titanium diffused periodically poled lithium niobate waveguide with a strongly-chirped poling period. The proposed non-standard asymmetric poling mitigates phase distortions associated with the process of chirping. Asymmetric poling significantly broadens the entangled source bandwidth while preserving high visibility quantum interferometric sensing.
We experimentally investigate the properties of light generated by the sequential processes of spontaneous parametric downconversion followed by upconversion. By interfering the upconverted photons with the original pump light, we show that the processes preserve the coherence of the light. Moreover, we observe interferences with doubled phase sensitivity when changing the phase of the downconverted entangled light, although its coherence length is several orders of magnitude shorter than the one of the pump light. Finally the statistics of the upconverted light is expected to be super-poisson…
In this letter, we report a polarization-entangled photon-pair source based on type-II spontaneous parametric down conversion at telecom O-band in periodically poled silica fiber (PPSF). The photon-pair source exhibits more than 130 nm (~24 THz) emission bandwidth centered at 1306.6 nm. The broad emission spectrum results in a short biphoton correlation time and we experimentally demonstrate a Hong-Ou-Mandel interference dip with a full width of 26.6 fs at half maximum. Owing to the low birefringence of the PPSF, the biphotons generated from type-II SPDC are polarization-entangled over the ent…
The rising demand for transmission capacity in optical networks has motivated steady interest in expansion beyond the standard C-band (1530-1565 nm) into the adjacent L-band (1565-1625 nm), for an approximate doubling of capacity in a single stroke. However, in the context of quantum networking, the ability to leverage the L-band will require advanced tools for characterization and management of entanglement resources which have so far been lagging. In this work, we demonstrate an ultrabroadband two-photon source integrating both C- and L-band wavelength-selective switches for complete control…
We experimentally demonstrate a polarization-entangled photon source at 810 nm using a type-II phase-matched PPKTP crystal pumped by a low-cost, broadband laser diode with a central wavelength of 405 nm and a typical bandwidth of 0.53 nm. The PPKTP crystal is placed in a Sagnac-loop to realize the compact size and high stability. The downconverted biphotons, the signal and the idler, have typical bandwidths of 5.57 nm and 7.32 nm. We prepare two Bell states |Psi+> and |Psi-> with the fidelities of 0.948+-0.004 and 0.963+-0.002. In polarization correlation measurement, the visibilities are all …
Entangled microwave photons form a fundamental resource for quantum information processing and sensing with continuous variables. We use a low-loss Josephson metamaterial comprising superconducting, non-linear, asymmetric inductive elements to generate frequency-entangled photons from vacuum fluctuations at a rate of 2 giga entangled bits per second spanning over 4 GHz bandwidth. The device is operated as a traveling wave parametric amplifier under Kerr-relieving biasing conditions. Furthermore, we realize the first successfully demonstration of single-mode squeezing in such devices -- $3.1\pm…
We report, for the first time, the generation of entangled photon pairs via type-0 spontaneous parametric down conversion in an ultra-thin wafer of lithium niobate in which momentum between the pump photon and daughter photons is not conserved. The characteristics of the emission are investigated using several techniques. We find that non-phase matched SPDC is a promising source of ultra-broadband two photon radiation that exhibits remarkably tight correlation widths in both the spatial and temporal domains.
Highly Efficient and Broadband Optical Delay Line towards a Quantum Memory
National University of Singapore（新加坡国立大学）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）；Thales Research and Technology（泰雷兹研究技术）；Department of Physics, National University of Singapore（新加坡国立大学物理系）
Laboratoire Matériaux et Phénomènes Quantiques, Université Paris Cité（量子物质与现象实验室，巴黎西岱大学）；Centre de Nanosciences et Nanotechnologies, Université Paris-Saclay（纳米科学与纳米技术研究中心，巴黎萨克雷大学）；STMicroelectronics（意法半导体）
We demonstrate the capability to discretize the frequency spectrum of broadband energy-time entangled photons by means of a spatial light modulator to encode qudits in various bases. Exemplarily, we implement three different discretization schemes, namely frequency bins, time bins and Schmidt modes. Entangled qudits up to dimension $d=4$ are then revealed by two-photon interference experiments with visibilities violating a $d$-dimensional Bell inequality.
The concept of `flat optics' is quickly conquering different fields of photonics, but its implementation in quantum optics is still at infancy. In particular, polarization entanglement, which is central to quantum photonics due to the simplicity of polarization qubit encoding and control, is so far not realized on flat platforms. Meanwhile, relaxed phase matching of flat nonlinear optical sources enables enormous freedom in tailoring their polarization properties. Here we use this freedom to generate photon pairs with tunable polarization entanglement via spontaneous parametric down-conversion…
We experimentally study the violation of the CGLMP inequality for entangled 2-qubit and 2-qutrit states with different degrees of entanglement using numerically optimized measurement settings. The qudits are encoded and manipulated in the frequency spectrum of broadband energy-time entangled photons by taking into account a spatial light modulator. The latter allows to discretize the spectrum into bins. By controlling each frequency bin individually, the generation of maximally and non-maximally entangled qutrits is verified through quantum state tomography.
Entangled pairs of microwave photons are commonly produced in the narrow frequency band of a resonator, which represents a modified vacuum density of states. We use a broadband, semi-infinite transmission line terminated by a superconducting quantum interference device (SQUID). A weak pump signal modulates the SQUID inductance, resulting in a single time-varying boundary condition. We detect both quadratures of the microwave radiation emitted at two different frequencies separated by 0.7~GHz. We determine the type and purity of entanglement from the noise correlations and an in-situ noise and …
Semiconductor quantum dots embedded in hybrid circular Bragg gratings are a promising platform for the efficient generation of nonclassical light. The scalable fabrication of multiple devices with similar performance is highly desirable for their practical use as sources of single and entangled photons, while the ability to operate at telecom wavelength is essential for their integration with the existing fiber infrastructure. In this work we combine the promising properties of broadband hybrid circular Bragg gratings with a membrane-transfer process performed on 3" wafer scale. We develop and…
We present a technique to completely characterise the spectral-temporal wave function of a broadband photon pair using spectral-shearing interferometry. Our method is fully self-referencing and is generalisable across a wide range of wavelengths. To demonstrate, we generate an entangled photon pair with controllable time-frequency entanglement and perform a full reconstruction. These results allow previously unobservable features of quantum states to be measured and utilised for the first time. We foresee this will unlock new opportunities in high-dimensional quantum technology, enabling the d…
We experimentally study entangled two-photon absorption in Rhodamine 6G as a function of the spatial properties of a high flux of broadband entangled photon pairs. We first demonstrate a key signature dependence of the entangled two-photon absorption rate on the type of entangled pair flux attenuation: linear, when the laser pump power is attenuated, and quadratic, when the pair flux itself experiences linear loss. We then perform a fluorescence-based Z-scan measurement to study the influence of beam waist size on the entangled two-photon absorption process and compare this to classical single…
High gain parametric amplifier with a single-pass pulsed pump is known to generate broadband twin photon fields that are entangled in amplitude and phase but have complicated spectral correlation. Fortunately, they can be decomposed into independent temporal modes. But the common treatment of parametric interaction Hamiltonian does not consider the issue of time ordering problem of interaction Hamiltonian and thus leads to incorrect conclusion that the mode structure and the temporal mode functions do not change as the gain increases. In this paper, we use an approach that is usually employed …
We present an analytical quantum theoretic model for non-resonant molecular two-photon absorption (TPA) of broadband, spectrally multi-mode squeezed vacuum, including low-gain (isolated entangled photon pairs or EPP) and high-gain (bright squeezed vacuum or BSV) regimes. The results are relevant to the potential use of entangled-light TPA as a spectroscopic and imaging method. We treat the scenario that the exciting light is spatially single-mode and is non-resonant with all intermediate molecular states. In the case of high gain, we find that in the case that the linewidth of the final molecu…
The realization of a future quantum Internet requires processing and storing quantum information at local nodes, and interconnecting distant nodes using free-space and fibre-optic links. Quantum memories for light are key elements of such quantum networks. However, to date, neither an atomic quantum memory for non-classical states of light operating at a wavelength compatible with standard telecom fibre infrastructure, nor a fibre-based implementation of a quantum memory has been reported. Here we demonstrate the storage and faithful recall of the state of a 1532 nm wavelength photon, entangle…
It is well known that the reduced state of a two-mode squeezed vacuum state is a thermal state---i.e. a state whose photon-number statistics obey a geometric distribution. More exotic \emph{broadband} states can be realized as the reduced state of two spectrally-entangled beams generated using nonlinear optics. We show that these broadband "pseudothermal" states are tensor products of states in spectral Schmidt modes, whose photon-number statistics obey a geometric distribution. We study the spectral and temporal coherence properties of these states and show that their spectral coherence can b…
We propose a scheme in which broadband nanostructures allow to generate squeezed light and entanglement of quantum emitters that are extremely far detuned. It is shown that the reduced fluctuations of the electromagnetic field arising from collective resonance fluorescence provide also a means to detect the entanglement between the emitters. Due to the near-field enhancement in the proposed hybrid systems, these nonclassical effects can be encountered outside both the extremely close separations limiting the observation in free space and narrow frequency bands in high-Q cavities. Our approach …
On-chip bright quantum sources with multiplexing ability are extremely high in demand for the integrated quantum networks with unprecedented scalability and complexity. Here, we demonstrate an ultrabright and broadband biphoton quantum source generated in a lithium niobate microresonator system.Without introducing the conventional domain poling, the on-chip microdisk produces entangled photon pairs covering a broad bandwidth promised by natural phase matching in spontaneous parametric down conversion.Experimentally, the multiplexed photon pairs are characterized by $30\ \rm nm$ bandwidth limit…
Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission measurement of frequency-entangled broadband photon pairs generated via parametric down-conversion with a monochromatic laser. It is observed that state-to-state dynamics in the system under study are temporally resolved by adjusting the path difference between the entangled twin beams when the entanglement time is sufficiently short. The non-classical photon corr…
We propose an application of quantum temporal imaging to restoring the indistinguishability of the signal and the idler photons produced in type-II spontaneous parametric down-conversion with a pulsed broadband pump. It is known that in this case, the signal and the idler photons have different spectral and temporal properties. This effect deteriorates their indistinguishability and the visibility of the Hong-Ou-Mandel interference, respectively. We demonstrate that inserting a time lens in one arm of the interferometer and choosing properly its magnification factor restores perfect indistingu…
Quantum interference, like Hong-Ou-Mandel interference, has played an important role to test fundamental concepts in quantum physics. We experimentally show that the multiple quantum interference effects enable the generation of high-performance polarization entangled photons. These photons have a high-emission rate, are degenerate, have a broadband distribution, and are postselection free. A quantum interferometric scheme, based on a round-trip configuration of a double-pass polarization Sagnac interferometer, makes it possible to use the large generation efficiency of polarization entangled …
An outstanding goal in quantum optics and scalable photonic quantum technology is to develop a source that each time emits one and only one entangled photon pair with simultaneously high entanglement fidelity, extraction efficiency, and photon indistinguishability. By coherent two-photon excitation of a single InGaAs quantum dot coupled to a circular Bragg grating bullseye cavity with broadband high Purcell factor up to 11.3, we generate entangled photon pairs with a state fidelity of 0.90(1), pair generation rate of 0.59(1), pair extraction efficiency of 0.62(6), and photon indistinguishabili…
While two-photon absorption (TPA) and other forms of nonlinear interactions of molecules with isolated time-frequency-entangled photon pairs (EPP) have been predicted to display a variety of fascinating effects, their potential use in practical quantum-enhanced molecular spectroscopy requires close examination. This paper presents a detailed theoretical study of quantum-enhanced TPA by both photon-number correlations and spectral correlations, including an account of the deleterious effects of dispersion. While such correlations in EPP created by spontaneous parametric down conversion can incr…
Cluster state plays a crucial role in the one-way quantum computation. Here, we propose and experimentally demonstrate a new scheme to prepare an ultrahigh-fidelity four-photon linear cluster state via spontaneous parametric down-conversion process. The state fidelity is measured to be $0.9517\pm0.0027$. Our scheme can be directly extended to more photons to generate N-qubit linear cluster state. Furthermore, our scheme is optimal for generating photonic linear cluster states in the sense of achieving the maximal success probability and having the simplest strategy. The key idea is that the ph…
