Quantum light is a key resource for promoting quantum technology. One such class of technology aims to improve the precision of optical measurements using engineered quantum states of light. In this study, we investigate transmission measurement of frequency-entangled broadband photon pairs generated via parametric down-conversion with a monochromatic laser. It is observed that state-to-state dynamics in the system under study are temporally resolved by adjusting the path difference between the entangled twin beams when the entanglement time is sufficiently short. The non-classical photon correlation enables time-resolved spectroscopy with monochromatic pumping. It is further demonstrated that the signal corresponds to the spectral information along anti-diagonal lines of, for example, two-dimensional Fourier-transformed photon echo spectra. This correspondence inspires us to anticipate that more elaborately engineered photon states would broaden the availability of quantum light spectroscopy.
Multidimensional optical signals are commonly recorded by varying the delays between time ordered pulses. These control the evolution of the density matrix and are described by ladder diagrams. We propose a new non-time-ordered protocol based on following the time evolution of the wavefunction and described by loop diagrams. The time variables in this protocol allow to observe different types of resonances and reveal information about intraband dephasing not readily available by time ordered techniques. The time variables involved in this protocol become coupled when using entangled light, whi…
We find that multidimensional determinants "hyperdeterminants", related to entanglement measures (the so-called concurrence or 3-tangle for the 2 or 3 qubits, respectively), are derived from a duality between entangled states and separable states. By means of the hyperdeterminant and its singularities, the single copy of multipartite pure entangled states is classified into an onion structure of every closed subset, similar to that by the local rank in the bipartite case. This reveals how inequivalent multipartite entangled classes are partially ordered under local actions. In particular, the …
Entangled photon pair excitation and time-frequency-filtered multidimensional photon correlation spectroscopy as a probe for dissipative exciton kinetics
Center for Free-Electron Laser Science CFEL, Deutsches Elektronen-Synchrotron DESY（自由电子激光科学中心，德国电子同步加速器）；University of California, Irvine（加州大学尔湾分校）
We demonstrate how the Hong-Ou-Mandel (HOM) interference with polarization-entangled photons can be used to probe ultrafast dephasing. We can infer the optical properties like the real and imaginary parts of the complex susceptibility of the medium from changes in the position and the shape of the HOM dip. From the shift of the HOM dip, we are able to measure 22 fs dephasing time using a continuous-wave (CW) laser even with optical loss > 97%, while the HOM dip visibility is maintained at 92.3~\% (which can be as high as 96.7%). The experimental observations, which are explained in terms of a …
We present an input/output analysis of photon-correlation experiments whereby a quantum mechanically entangled bi-photon state interacts with a material sample placed in one arm of a Hong-Ou-Mandel (HOM) apparatus. We show that the output signal contains detailed information about subsequent entanglement with the microscopic quantum states in the sample. In particular, we apply the method to an ensemble of emitters interacting with a common photon mode within the open-system Dicke Model. Our results indicate considerable dynamical information concerning spontaneous symmetry breaking can be rev…
Quantum entangled photons provide a sensitive probe of many-body interactions and offer an unique experimental portal for quantifying many-body correlations in a material system. In this paper, we present a theoretical demonstration of how photon-photon entanglement can be generated via interactions between coupled qubits. Here we develop a model for the scattering of an entangled pair of photons from a molecular dimer. We develop a diagrammatic theory for the scattering matrix and show that one can correlate the von Neumann entropy of the outgoing bi-photon wave function to exciton exchange a…
We propose a probabilistic scheme to prepare a maximally entangled state between a pair of two-level atoms inside a leaking cavity, without requiring precise time-controlling of the system evolution and initial atomic state. We show that the steady state of this dissipative system is a mixture of two parts: either the atoms being in their ground state or in a maximally entangled one. Then, by applying a weak probe field on the cavity mode we are able to distinguish those states without disturbing the atomic system, i.e., performing a quantum non-demolition measurement via the cavity transmissi…
Correlated photons inspire abundance of metrology-related platforms, which benefit from quantum (anti-) correlations and outperform their classical-light counterparts. While such demonstrations mainly focus on entanglement, the role of photon exchange-phase and degree of distinguishability have not been widely utilized in quantum-enhanced applications. Using an interferometric setup we show that even at low degree entanglement, when a two-photon wave-function is coupled to matter, it is encoded with a reliable "which pathway?" information. An interferometric exchange-phase-cycling protocol is …
We explore the structure of multipartite quantum systems which are entangled in multiple degrees of freedom. We find necessary and sufficient conditions for the characterization of tripartite systems and necessary conditions for any number number of parties. Furthermore we develop a framework of multi-level witnesses for efficient discrimination and quantification of multidimensional entanglement that is applicable for an arbitrary number of systems and dimensions.
We propose a multidimensional quantum information encoding approach based on temporal modulation of single photons, where the Hilbert space can be spanned by an in-principle infinite set of orthonormal temporal profiles. We analyze two specific realizations of such modulation schemes, and show that error rate per symbol can be smaller than 1% for practical implementations. Temporal modulation may enable multidimensional quantum communication over the existing fiber optical infrastructure, as well as provide an avenue for probing high-dimensional entanglement approaching the continuous limit.
For the quantum depolarizing channel with any finite dimension, we compare three schemes for channel identification: unentangled probes, probes maximally entangled with an external ancilla, and maximally entangled probe pairs. This comparison includes cases where the ancilla is itself depolarizing and where the probe is circulated back through the channel before measurement. Compared on the basis of (quantum Fisher) information gained per channel use, we find broadly that entanglement with an ancilla dominates the other two schemes, but only if entanglement is cheap relative to the cost per ch…
Quantum walks in atomic systems, owing to their continuous nature, are especially well-suited for the simulation of many-body physics and can potentially offer an exponential speedup in solving certain black box problems. Photonics offers an alternate route to simulating such nonclassical behavior in a more robust platform. However, in photonic implementations to date, an increase to the depth of a continuous quantum walk requires modifying the footprint of the system. Here we report continuous walks of a two-photon quantum frequency comb with entanglement across multiple dimensions. The coupl…
Wave function collapse models are considered as the modified theories of standard quantum mechanics at the macroscopic level. By introducing nonlinear stochastic terms in the Schrödinger equation, these models make predictions, differently from those of standard quantum mechanics, that it is fundamentally impossible to prepare macroscopic systems in macroscopic superpositions. The validity of these models can only be examined by experiments and hence efficient protocols for this kind of experiments are highly needed. Here we provide a protocol that is able to probe the postulated collapse effe…
We introduce and define a set of functions on pure bipartite states called entanglement moments. Usual entanglement measures tell you if two systems are entangled, while entanglement moments tell you both if and how two systems are entangled. They are defined with respect to a measurement basis in one system (e.g., a measuring device), and output numbers describing how a system (e.g., a qubit) is entangled with that measurement basis. The moments utilize different distance measures on the Hilbert space of the measured system, and can be generalized to any N-dimensional Hilbert space. As an app…
The experimental realization of multidimensional quantum states may lead to unexplored and interesting physics, as well as advanced quantum communication protocols. The orbital angular momentum of photons is a well suitable discrete degree of freedom for implementing high-dimensional quantum systems. The standard method to generate and manipulate such photon modes is to use bulk and fixed optics. Here the authors demonstrate the utilization of a spatial light modulator to manipulate the orbital angular momentum of entangled photons generated in spontaneous parametric downconversion. They show …
The ability to control multidimensional quantum systems is key for the investigation of fundamental science and for the development of advanced quantum technologies. Here we demonstrate a multidimensional integrated quantum photonic platform able to robustly generate, control and analyze high-dimensional entanglement. We realize a programmable bipartite entangled system with dimension up to $15 \times 15$ on a large-scale silicon-photonics quantum circuit. The device integrates more than 550 photonic components on a single chip, including 16 identical photon-pair sources. We verify the high pr…
This theoretical research aims to examine areas of the Compton cross section of entangled annihilation photons for the purpose of testing for possible break down of theory, which could have consequences for predicted optimal capabilities of Compton PET systems.We provide maps of the cross section for entangled annihilation photons for experimental verification.We introduce a strategy to derive cross sections in a relatively straight forward manner for the Compton scattering of a hypothetical separable, mixed and entangled states. To understand the effect that entanglement has on the cross sect…
Quadratic Quantum Polarimetry with Entangled Photon Pairs
ARC Centre of Excellence for Transformative Meta-Optical Systems (TMOS), Department of Electronic Materials Engineering, Research School of Physics, The Australian National University（澳大利亚国立大学）；Institute of Applied Physics, Abbe Center of Photonics, Friedrich Schiller University Jena（耶拿弗里德里希·席勒大学应用物理研究所）；Opto-Electronics and Measurement Techniques, Advanced Electronics Centre, Faculty of Information Technology and Electrical Engineering, University of Oulu（奥卢大学信息技术与电气工程学院高级电子中心光电子与测量技术部门）；Institute of Quantum Precision Measurement, State Key Laboratory of Radio Frequency Heterogeneous Integration, College of Physics and Optoelectronic Engineering, Shenzhen University（深圳大学物理与光电工程学院量子精密测量研究所）；Aston Institute of Photonic Technologies, Aston University（阿斯顿大学光子技术研究所）
Addressing the feasibilty of quantum communication with electrons we consider entangled spin states of electrons in a double-dot which is weakly coupled to in--and outgoing leads. We show that the entanglement of two electrons in the double-dot can be detected in mesoscopic transport and noise measurements. In the Coulomb blockade and cotunneling regime the singlet and triplet states lead to phase-coherent current and noise contributions of opposite signs and to Aharonov-Bohm and Berry phase oscillations in response to magnetic fields. These oscillations are a genuine two-particle effect and p…
Multidimensional photonic graph states, such as cluster states, have prospective applications in quantum metrology, secure quantum communication, and measurement-based quantum computation. However, to date, generation of multidimensional cluster states of photonic qubits has relied on probabilistic methods that limit the scalability of typical generation schemes in optical systems. Here we present an experimental implementation in the microwave domain of a resource-efficient scheme for the deterministic generation of 2D photonic cluster states. By utilizing a coupled resonator array as a slow-…
Dynamically probing systems of ultrastrongly coupled light and matter by advanced coherent control has been recently proposed as a unique tool for detecting peculiar quantum features of this regime. Coherence allows in principle on-demand conversion of virtual photons dressing the entangled eigenstates of the system to real ones, with unitary efficiency and remarkable robustness. Here we study this effect in the presence of decoherence, showing that also in far from ideal regimes is it possible to probe such peculiar features.
Making measurements on single quantum systems is considered difficult, almost impossible if the state is a-priori unknown. Protective measurements suggest a possibility to measure single quantum systems and gain some new information in the process. Protective measurement is described, both in the original and generalized form. The degree to which the system and the apparatus remain entangled in a protective measurement, is assessed. A possible experimental test of protective measurements is discussed.
Cluster states are useful in many quantum information processing applications. In particular, universal measurement-based quantum computation (MBQC) utilizes 2D cluster states, and topologically fault-tolerant MBQC requires cluster states with three or higher dimensions. This work proposes a protocol to deterministically generate multidimensional photonic cluster states using a single atom-cavity system and time-delay feedback. The dimensionality of the cluster state increases linearly with the number of time-delay feedback. We firstly give a diagrammatic derivation of the tensor network state…
A new type of quantum entangled interferometer was recently realized that employs parametric amplifiers as the wave splitting and recombination elements. The quantum entanglement stems from the parametric amplifiers, which produce quantum correlated fields for probing the phase change signal in the interferometer. This type of quantum entangled interferometer exhibits some unique properties that are different from traditional beam splitter-based interferometers such as Mach-Zehnder interferometers. Because of these properties, it is superior to the traditional interferometers in many aspects, …
Quantum steering enables one party to communicate with another remote party even if the sender is untrusted. Such characteristics of quantum systems not only provide direct applications to quantum information science, but are also conceptually important for distinguishing between quantum and classical resources. While concrete illustrations of steering have been shown in several experiments, quantum steering has not been certified for higher dimensional systems. Here, we introduce a simple method to experimentally certify two different kinds of quantum steering: Einstein-Podolsky-Rosen (EPR) s…
We have recently calculated shot noise for entangled and spin-polarized electrons in novel beam-splitter geometries with a local Rashba s-o interaction in the incoming leads. This interaction allows for a gate-controlled rotation of the incoming electron spins. Here we present an alternate simpler route to the shot noise calculation in the above work and focus on only electron pairs. Shot noise for these shows continuous bunching and antibunching behaviors. In addition, entangled and unentangled triplets yield distinctive shot noise oscillations. Besides allowing for a direct way to identify t…
We propose an entanglement detector composed of two quantum spin Hall insulators and a side gate deposited on one of the edge channels. For an ac gate voltage, the differential noise contributed from the entangled electron pairs exhibits the nontrivial step structures, from which the spin entanglement concurrence can be easily obtained. The possible spin dephasing effects in the quantum spin Hall insulators are also included.
Variational quantum circuits (VQCs) built upon noisy intermediate-scale quantum (NISQ) hardware, in conjunction with classical processing, constitute a promising architecture for quantum simulations, classical optimization, and machine learning. However, the required VQC depth to demonstrate a quantum advantage over classical schemes is beyond the reach of available NISQ devices. Supervised learning assisted by an entangled sensor network (SLAEN) is a distinct paradigm that harnesses VQCs trained by classical machine-learning algorithms to tailor multipartite entanglement shared by sensors for…
We demonstrate a different scheme to perform optical sectioning of a sample based on the concept of induced coherence [Zou et al., Phys. Rev. Lett. 67, 318 (1991)]. This can be viewed as a different type of optical coherence tomography scheme where the varying reflectivity of the sample along the direction of propagation of an optical beam translates into changes of the degree of first-order coherence between two beams. As a practical advantage the scheme allows probing the sample with one wavelength and measuring photons with another wavelength. In a bio-imaging scenario, this would result in…
We theoretically propose a biphoton entanglement-enhanced multidimensional spectroscopic technique as a probe for the dissipative polariton dynamics in the ultrafast regime. It is applied to the cavity-confined monomeric photosynthetic complex that represents a prototypical multi-site excitonic quantum aggregate. The proposed technique is shown to be particularly sensitive to inter-manifold polariton coherence between the two and one-excitation subspaces. It is demonstrated to be able to monitor the dynamical role of cavity-mediated excitonic correlations, and dephasing in the presence of phon…
Characterizing high-dimensional entangled states is of crucial importance in quantum information science and technology. Recent theoretical progress has been made to extend the Hardy's paradox into a general scenario with multisetting multidimensional systems, which can surpass the bound limited by the original version. Hitherto, no experimental verification has been conducted to verify such a Hardy's paradox, as most of previous experimental efforts were restricted to two-dimensional systems. Here, based on two-photon high-dimensional orbital angular momentum (OAM) entanglement, we report the…
We propose a method to detect the microwave magnetic-field gradient by using a pair of entangled two-component Bose-Einstein condensates. We consider the two spatially separated condensates to be coupled to the two different magnetic fields. The magnetic-field gradient can be determined by measuring the variances of population differences and relative phases between the two-component condensates in two wells. The precision of measurement can reach the Heisenberg limit. We study the effects of one-body and two-body atom losses on the detection. We find that the entangled atoms can outperform th…
We experimentally demonstrate that it is impossible to simulate quantum bipartite correlations with a deterministic universal Turing machine. Our approach is based on the Normalized Information Distance (NID) that allows the comparison of two pieces of data without detailed knowledge about their origin. Using NID, we derive an inequality for output of two local deterministic universal Turing machines with correlated inputs. This inequality is violated by correlations generated by a maximally entangled polarization state of two photons. The violation is shown using a freely available lossless c…
We propose a method to produce pure single photons with an arbitrary designed temporal shape in a heralded, lossless and scalable way. As the indispensable resource, the method uses pairs of time-energy entangled photons. To accomplish the shaping, one photon of a pair undergoes temporal modulation according to the desired shape. Subsequent frequency-resolving detection of the photon heralds its entangled counterpart in a pure quantum state with a temporal shape non-locally affected by the modulation. We found conditions for the shape of the heralded photon to reproduce the modulation function…
Correlations between spacelike separated measurements on entangled quantum systems are stronger than any classical correlations and are at the heart of numerous quantum technologies. In practice, however, spacelike separation is often not guaranteed and we typically face situations where measurements have an underlying time order. Here we aim to provide a fair comparison of classical and quantum models of temporal correlations on a single particle, as well as timelike-separated correlations on multiple particles. We use a causal modeling approach to show, in theory and experiment, that quantum…
High harmonic spectroscopy has the potential to combine attosecond temporal with sub-Angstrom spatial resolution of the early nuclear and multielectron dynamics in molecules. It involves strong field ionization of the molecule by the IR laser field followed by time-delayed recombination of the removed electron with the molecular ion. The time-delay is controlled on the attosecond time scale by the oscillation of the IR field and is mapped into the harmonic number, providing a movie of molecular dynamics between ionization and recombination. One of the challenges in the analysis of high harmoni…
We show that the interaction of a pulsed laser light with a mechanical oscillator through the radiation pressure results in an opto-mechanical entangled state in which the photon number is correlated with the oscillator position. Interestingly, the mechanical oscillator can be delocalized over a large range of positions when driven by an intense laser light. This provides a simple yet sensitive method to probe hypothetic post-quantum theories including an explicit wave function collapse model, like the Diosi and Penrose model. We propose an entanglement witness to reveal the quantum nature of …
Quantum entanglement shared between more than two particles is essential to foundational questions in quantum mechanics, and upcoming quantum information technologies. So far, up to 14 two-dimensional qubits have been entangled, and an open question remains if one can also demonstrate entanglement of higher-dimensional discrete properties of more than two particles. A promising route is the use of the photon orbital angular momentum (OAM), which enables implementation of novel quantum information protocols, and the study of fundamentally new quantum states. To date, only two of such multidimen…
Quantum two-level systems interacting with the surroundings are ubiquitous in nature. The interaction suppresses quantum coherence and forces the system towards a steady state. Such dissipative processes are captured by the paradigmatic spin-boson model, describing a two-state particle, the "spin", interacting with an environment formed by harmonic oscillators. A fundamental question to date is to what extent intense coherent driving impacts a strongly dissipative system. Here we investigate experimentally and theoretically a superconducting qubit strongly coupled to an electromagnetic environ…
Multiplexed quantum memories and high-dimensional entanglement can improve the performance of quantum repeaters by promoting the entanglement generation rate and the quantum communication channel capacity. Here, we experimentally generate a high-dimensional entangled state between a photon and a collective spin wave excitation stored in the multiplexed atomic quantum memory. We verify the entanglement dimension by the quantum witness and the entanglement of formation. Then we use the high-dimensional entangled state to test the violation of the Bell-type inequality. Our work provides an effect…
We establish a novel approach to probing spatially resolved multi-time correlation functions of interacting many-body systems, with scalable experimental overhead. Specifically, designing nonlinear measurement protocols for multidimensional spectra in a chain of trapped ions with single-site addressability enables us, e.g., to distinguish coherent from incoherent transport processes, to quantify potential anharmonicities, and to identify decoherence-free subspaces.
Bell's theorem implies that the outcomes of local measurements on two maximally entangled systems cannot be simulated without classical communication between the parties. The communication cost is finite for n Bell states, but it grows exponentially in n. Three simple protocols are presented that provide approximate simulations for low-dimensional entangled systems and require a linearly growing amount of communication. We have tested them by performing some simulations for a family of measurements. The maximal error is less than 1% in three dimensions and grows sublinearly with the number of …
