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arXiv 2610.20128cond-mat.str-el
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Sr2FeRuO6中无序诱导的类Griffiths相与电荷局域化

Disorder-Induced Griffiths like Phase and Charge Localization in Sr2FeRuO6

South China University of Technology(华南理工大学);Institute of Engineering and Management, Sector-V(维 sector 工程管理学院);University of Engineering and Management, Newtown(纽敦工程与管理大学);Saha Institute of Nuclear Physics, A CI of Homi Bhabha National Institute(萨哈核物理研究所,霍米·巴巴国立学院成员机构);Department of Physics, Aditya University(阿迪蒂亚大学物理系)

Koustav Pal, Shuvendu Ghosh, I. Das

AI总结:

研究Sr2FeRuO6中结构无序、阻挫磁性与电荷输运的相互作用,发现其存在类Griffiths相与电荷局域化行为,为自旋电子材料设计提供了典型体系。

摘要:

全面理解复杂过渡金属氧化物是设计具有定制化磁性与输运功能的下一代自旋电子材料的关键。我们研究3d-4d混合双钙钛矿Sr2FeRuO6中结构无序、阻挫磁性与局域电荷输运之间的相互作用。该化合物采用单斜晶结构,存在显著的B位反位无序,这是其非常规行为的驱动因素。磁性测量揭示出在有序温度以上仍延伸的稳定Griffiths相,证明无序基质中存在稳定的短程铁磁团簇。电输运始终处于强局域化状态,在高温下从小极化子跳跃转变为中温下的变程跳跃。这些结果表明Sr2FeRuO6是一类典型的3d-4d混合体系,其中淬火无序稳定了自旋不均匀性,同时还观测到极化子与跳跃输运现象。

英文摘要:

A comprehensive understanding of complex transition-metal oxides is key to designing next-generation spintronic materials with tailored magnetic and transport functionalities. We investigate the interplay among structural disorder, frustrated magnetism, and localized charge transport in the 3d-4d hybrid double perovskite Sr2FeRuO6. The compound adopts a monoclinic structure with significant B-site antisite disorder that drives its unconventional behavior. Magnetic measurements uncover a robust Griffiths phase extending well above the ordering temperature, evidencing stable short-range ferromagnetic clusters within a disordered matrix. Electrical transport remains strongly localized, transitioning from small-polaron hopping at high temperatures to variable-range hopping at intermediate temperatures. These results position Sr2FeRuO6 as a representative 3d-4d hybrid system in which quenched disorder stabilizes spin inhomogeneity, while polaronic and hopping transport are also observed.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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