(La1-yPry)0.7Ca 0.3Mn 16/18 O3中Griffiths相的形核与相竞争的关系
Correlation Between Phase Competition and the Nucleation of a Griffiths Phase in (La1-yPry)0.7Ca0.3Mn16/18O3
摘要:
对典型相分离的(La 1-yPry)0.7Ca 0.3Mn 16/18 O3(0 < y < 1)的温度依赖性零场交流磁化率的详细分析揭示了与格里菲斯相(GP)的存在一致的特征,即,逆磁化率的特征在于当y朝向yc < 0.85减小时,0.05超过yc = 0.85,GP被抑制。这些数据,与以前的中子衍射测量相结合,使相图总结了该系统的组成GP的演变;特别地,它表明与这种相的建立相关的无序与相分离的反铁磁和铁磁组分的相对体积分数密切相关,即使超过最近估计的双交换(DE)关联的逾渗阈值。电子-声子耦合的影响也可以通过氧同位素效应看到。
英文摘要:
Detailed analyses of the temperature-dependent zero field ac susceptibility of prototypical phase-separated (La1-yPry)0.7Ca0.3Mn16/18O3, 0 < y < 1, reveal features consistent with the presence of a Griffiths phase (GP), viz., an inverse susceptibility characterized by power law with 0.05 < lamda < 0.33 as y decreases towards yc < 0.85. Beyond yc = 0.85, the GP is suppressed. These data, combined with previous neutron diffraction measurements, enable a phase diagram summarizing the evolution of the GP with composition to be constructed for this system; in particular, it shows that the disorder relevant for the establishment of such a phase is linked closely to the relative volume fractions of the phase separated antiferromagnetic and ferromagnetic components, even when the recently estimated double exchange (DE) linked percolation threshold is exceeded. The influence of electron-phonon coupling can also be seen through oxygen isotope effects.
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