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arXiv 2602.21986cond-mat.mes-hall
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多层石墨烯-铁改性氧化铋忆阻器中的量子抗性用于类脑计算

Quantum Resistance in Multilayer Graphene-BiFeO3 Memristor for Brain-Inspired Computing

Institute of Physics(印度物理研究所);Homi Bhabha National Institute(霍米·巴巴国立研究所);Sambalpur University(桑巴尔普尔大学);Chalmers University of Technology(查尔姆斯理工大学);Centre de Nanosciences et de Nanotechnologies, CNRS, Université Paris-Saclay(巴黎萨克雷大学纳米科学和纳米技术中心,法国国家科学研究中心);Institute of Nano Science and Technology(纳米科学与技术研究所);Indian Institute of Technology Madras(马德拉斯印度理工学院)

Suman Roy, Priyanka Sahu, Subhabrata Das, Sameer Kumar Mallik, Susmita Jana, Alok Kumar, Himadri Nandan Mohanty, Kaushik Ghosh, B. R. K. Nanda, Satyaprakash Sahoo

AI总结:

本研究通过多层石墨烯-铁改性氧化铋忆阻器实现量子抗性,展示了高阶可调性及在类脑计算中的应用潜力。

摘要:

在大数据和物联网时代,量子级导电状态的控制为高密度数据存储和类脑神经形态计算提供了有前途的途径。尽管量子导电(QC)现象已在各种金属氧化物忆阻器中得到展示,但实现可靠且精确的量子化状态控制仍处于初级阶段。在这里,我们展示了多功能铁改性氧化铋(BFO)钙钛矿忆阻器与多层石墨烯接触的双向量子导电状态,实现了更高的可调性,并揭示了钙钛矿-二维异质结构在量子工程记忆和计算设备中的潜力。XPS分析提供了关于BFO中氧空位动态的详细见解,而第一性原理密度泛函理论计算清楚地揭示了石墨烯-BFO界面处的强局域电场。我们的设备表现出由量子点接触形成促进的电流控制的高阶QC过渡,在设置和重置过程中产生量子化导电状态。时间滞后相关图谱量化了在动态电压脉冲调制方案下QC状态的随机演变。值得注意的是,量子化导电状态有效地模拟了突触增强和抑制,实现了高精度图像和数字识别的卷积神经网络中的精确权重调节。这些发现确立了钙钛矿-二维异质结构作为QC驱动的电阻开关的有前景的候选者,并展示了其在开发可控量子忆阻器中的潜力。

英文摘要:

In the era of big data and the Internet of Things, quantum-level control of conductance states offers a promising route toward high-density data storage and brain-inspired neuromorphic computing. Although quantum conductance (QC) phenomena have been demonstrated in various metal oxide memristors, achieving reliable and precise control over quantized states remains in its infancy. Here, we demonstrate bidirectional quantum conductance states in multifunctional BiFeO3 (BFO) perovskite memristors integrated with multilayer-graphene contacts, enabling higher-order tunability and revealing the potential of perovskite-2D heterostructures for quantum-engineered memory and computing devices. XPS analysis provides detailed insights into oxygen vacancy dynamics in BFO, whereas first-principles density functional theory calculations clearly reveal a strong localized electric field at the graphene-BFO interface. Our devices exhibit current-controlled higher-order QC transitions facilitated by quantum point contact formation, giving rise to quantized conductance states during both SET and RESET processes. Time-lag correlation maps quantify the stochastic evolution of QC states under dynamic voltage-pulse tuning schemes. Notably, the quantized conductance states effectively emulate synaptic potentiation and depression, enabling precise weight modulation for high-accuracy image and digit recognition in convolutional neural networks. These findings establish perovskite-2D heterostructures as promising candidates for QC-driven resistive switching and demonstrate their potential for developing controllable quantum memristors.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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