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arXiv 2302.13845cond-mat.str-el
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F掺杂LaMnO3中的铁磁性与金属-绝缘体转变

Ferromagnetism and Metal-Insulator transition in F-doped LaMnO3

Ekta Yadav, Pramod Ghising, K. P. Rajeev, Z. Hossain

AI总结:

本文研究F掺杂LaMnO3,发现LaMnO2.5F0.5具有约239 K居里温度的铁磁金属行为和-64%磁电阻,归因于F掺杂诱导混合价Mn离子实现双交换,并在213 K以下发现可能存在两种不同电阻的双交换跳跃路径。

摘要:

我们介绍了对氟掺杂LaMnO3(LaMnO3-yFy)多晶样品的研究。LaMnO2.5F0.5表现出显著的磁性和电学性质。它显示出铁磁性和金属行为,居里温度高达约239 K,磁电阻高达-64%。与纯LaMnO3相比,这种磁性质的剧烈变化归因于F在O位点的掺杂所驱动的混合价态Mn离子的存在,这使得LMOF中能够发生双交换(DE)作用。此外,电阻率数据分别在239 K和213 K处显示出两个电阻率峰。我们的结果表明,在213 K以下,样品中可能同时存在两种不同电阻的多重双交换跳跃路径。

英文摘要:

We present our studies on polycrystalline samples of fluorine doped LaMnO3 (LaMnO3-yFy). LaMnO2.5F0.5 exhibits remarkable magnetic and electrical properties. It shows ferromagnetic and metallic behavior with a high Curie temperature of ~ 239 K and a high magnetoresistance of -64. This drastic change in magnetic properties in comparison to pure LaMnO3 is ascribed to the presence of mixed-valence Mn ions driven by the F-doping at the O-sites, which enables double exchange (DE) in LMOF. Furthermore, the resistivity data exhibits two resistivity peaks at 239 K and 213 K, respectively. Our results point towards the possibility of multiple double exchange hopping paths of two distinct resistances existing simultaneously in the sample below 213 K.

机构、总结、中文摘要均由AI分析而来,可能存在错误,请以论文正文为准。

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