This article reports nonintuitive characteristic of a splashing drop on a solid surface discovered through extracting image features using a feedforward neural network (FNN). Ethanol of area-equivalent radius about 1.29 mm was dropped from impact heights ranging from 4 cm to 60 cm (splashing threshold 20 cm) and impacted on a hydrophilic surface. The images captured when half of the drop impacted the surface were labeled according to their outcome, splashing or nonsplashing, and were used to train an FNN. A classification accuracy higher than 96% was achieved. To extract the image features identified by the FNN for classification, the weight matrix of the trained FNN for identifying splashing drops was visualized. Remarkably, the visualization showed that the trained FNN identified the contour height of the main body of the impacting drop as an important characteristic differentiating between splashing and nonsplashing drops, which has not been reported in previous studies. This feature was found throughout the impact, even when one and three-quarters of the drop impacted the surface. To confirm the importance of this image feature, the FNN was retrained to classify using only the main body without checking for the presence of ejected secondary droplets. The accuracy was still higher than 82%, confirming that the contour height is an important feature distinguishing splashing from nonsplashing drops. Several aspects of drop impact are analyzed and discussed with the aim of identifying the possible mechanism underlying the difference in contour height between splashing and nonsplashing drops.
Tokyo University of Agriculture and Technology（东京农工大学）
This paper reports the features of a splashing drop on a solid surface and the temporal evolution, which are extracted through image-sequence classification using a highly interpretable feedforward neural network (FNN) with zero hidden layer. The image sequences used for training-validation and testing of the FNN show the early-stage deformation of milli-sized ethanol drops that impact a hydrophilic glass substrate with the Weber number ranges between 31-474 (splashing threshold about 173). Specific videographing conditions and digital image processing are performed to ensure the high similari…
Tokyo University of Agriculture and Technology（东京农工大学）
The impact of a drop on a solid surface is an important phenomenon that has various implications and applications. However, the multiphase nature of this phenomenon causes complications in the prediction of its morphological evolution, especially when the drop splashes. While most machine-learning-based drop-impact studies have centred around physical parameters, this study used a computer-vision strategy by training an encoder-decoder to predict the drop morphologies using image data. Herein, we show that this trained encoder-decoder is able to successfully generate videos that show the morph…
When a droplet hits a surface fast enough, droplet splashing can occur: smaller secondary droplets detach from the main droplet during impact. While droplet splashing on smooth surfaces is by now well understood, the surface roughness also affects at which impact velocity a droplet splashes. In this study, the influence of the surface roughness on droplet splashing is investigated. By changing the root mean square roughness of the impacted surface, we show that the droplet splashing velocity is only affected when the droplet roughness is large enough to disrupt the spreading droplet lamella an…
We investigate the impact velocity beyond which the ejection of smaller droplets from the main droplet (splashing) occurs for droplets impacting a smooth surface. We examine its dependence on the surface wetting properties and droplet surface tension. We show that the splashing velocity is independent of the wetting properties of the surface, but increases roughly linearly with increasing surface tension of the liquid. A preexisting splashing model is considered that predicts the splashing velocity by incorporating the air viscosity. The model is consistent with our data, but the calculation i…
Correlation between morphological evolution of splashing drop and exerted impact force revealed by interpretation of explainable artificial intelligence
Tokyo University of Agriculture and Technology（东京农工大学）
A drop impacting a solid surface with sufficient velocity will emit many small droplets creating a splash. However, splashing is completely suppressed if the surrounding gas pressure is lowered. The mechanism by which the gas affects splashing remains unknown. We use high-speed interference imaging to measure the air beneath all regions of a spreading viscous drop as well as optical absorption to measure the drop thickness. Although an initial air bubble is created on impact, no significant air layer persists until the time a splash is created. This suggests that splashing in our experimentall…
When a fast-moving drop impacts onto a smooth substrate, splashing will be produced at the edge of the expanding liquid sheet. This ubiquitous phenomenon lacks a fundamental understanding. Combining experiment with model, we illustrate that the ultrathin air film trapped under the expanding liquid front triggers splashing. Because this film is thinner than the mean free path of air molecules, the interior airflow transfers momentum with an unusually high velocity comparable to the speed of sound and generates a stress 10 times stronger than the airflow in common situations. Such a large stress…
A liquid drop impacting a dry solid surface with sufficient kinetic energy will splash, breaking apart into numerous secondary droplets. This phenomenon shows many similarities to forced wetting, including the entrainment of air at the contact line. Because of these similarities and the fact that forced wetting has been shown to depend on the wetting properties of the surface, existing theories predict splashing to depend on wetting properties as well. However, using high-speed interference imaging we observe that at high capillary numbers wetting properties have no effect on splashing for var…
We experimentally investigated the splashing of dense suspension droplets impacting a solid surface, extending prior work to the regime where the viscosity of the suspending liquid becomes a significant parameter. The overall behavior can be described by a combination of two trends. The first one is that the splashing becomes favored when the kinetic energy of individual particles at the surface of a droplet overcomes the confinement produced by surface tension. This is expressed by a particle-based Weber number $We_p$. The second is that splashing is suppressed by increasing the viscosity of …
Even a small fraction of nanoparticles in fluids affects the splashing behavior of a droplet upon impact on a smooth surface. Nanofluid drop impact onto a smooth sapphire substrate is experimentally investigated over wide ranges of Reynolds ($10^2<\mathrm{Re}<10^4$) and Weber ($50<\mathrm{We}<500$) numbers for three nanofluid mass concentrations (0.01%, 0.1%, 1%) using high-speed photography. Nanofluids are prepared by diluting a commercial Al$_2$O$_3$-water nanofluid in aqueous glycerol solutions without dispersants. In total, 30 samples are prepared and 1799 data points are acquired. Every s…
A liquid drop impacting a solid surface may splash by emitting a thin liquid sheet that subsequently breaks apart or by promptly ejecting droplets from the advancing liquid-solid contact line. Using high-speed imaging, we show that air pressure and surface roughness influence both splash mechanisms. Roughness increases prompt splashing at the advancing contact line but inhibits the formation of the thin sheet. If the air pressure is lowered, droplet ejection is suppressed not only during thin-sheet formation but for prompt splashing as well. The threshold pressure depends on impact velocity, l…
We explore the evolution of a splash when a liquid drop impacts a smooth, dry surface. There are two splashing regimes that occur when the liquid viscosity is varied, as is evidenced by its dependence on ambient gas pressure. A high-viscosity drop splashes by emitting a thin sheet of liquid from a spreading liquid lamella long after the drop has first contacted the solid. Likewise, we find that there is also a delay in the ejection of a thin sheet when a low-viscosity drop splashes. We show how the ejection time of the thin sheet depends on liquid viscosity and ambient gas pressure.
We experimentally investigate the splashing mechanism of a millimeter-sized ethanol drop impinging on a structured solid surface, comprised of micro-pillars, through side-view and top-view high speed imaging. By increasing the impact velocity we can tune the impact outcome from a gentle deposition to a violent splash, at which tiny droplets are emitted as the liquid sheet spreads laterally. We measure the splashing threshold for different micropatterns and find that the arrangement of the pillars significantly affects the splashing outcome. In particular, directional splashing in direction in …
The dynamics of drop impact on solid surfaces can be changed significantly by tuning the elasticity of the solid. Most prominently, the substrate deformation causes an increase in the splashing threshold as compared to impact onto perfectly rigid surfaces, and can thus lead to splash suppression. Here, we experimentally determine the splashing threshold for impact on thin membranes as a function of the tension in the membrane and its elastic properties. The drop dynamics is correlated to the membrane deformation, which is simultaneously measured using a laser profilometry technique. The experi…
At atmospheric pressure, a drop of ethanol impacting on a solid surface produces a splash. Reducing the ambient pressure below its atmospheric value suppresses this splash. The origin of this so-called pressure effect is not well understood and this is the first study to present an in-depth comparison between various theoretical models that aim to predict splashing and simulations. In this work the pressure effect is explored numerically by resolving the Navier-Stokes equations at a 3-nm resolution. In addition to reproducing numerous experimental observations, it is found that different model…
After impact onto a smooth dry surface, a drop of viscous liquid initially spreads in the form of a thick lamella. If the drop splashes, it first emits a thin fluid sheet that can ultimately break up into droplets causing the splash. Ambient gas is crucial for creating this thin sheet. The time for sheet ejection, $t_{ejt}$, depends on impact velocity, liquid viscosity, gas pressure and molecular weight. A central air bubble is trapped below the drop at pressures even below that necessary for this sheet formation. In addition, air bubbles are entrained underneath the spreading lamella when the…
We present fluid dynamics videos illustrating wetting splashing-produced by water drop impact onto hydrophobic microstructures at high impact velocity ($\sim 3$ ms$^{-1}$). The substrate consists of regular and transparent microtextures in square or hexagonal lattice, yielding a high contact angle of $\sim 150 ^\circ$. Our high speed top-or-bottom view recordings through the transparent surface shed light on the solid-liquid-air interfaces at impact. Despite the superhydrophobicity of the latticed micropillars (of a periodicity of $10 μm), water droplet wets a certain central area and moreover…
Oblique impact of drops onto a solid or liquid surface is frequently observed in nature. Most studies on drop impact and splashing, however, focus on perpendicular impact. Here, we study oblique impact of 100-micrometer drops onto a deep liquid pool, where we quantify the splashing threshold, maximum cavity dimensions and cavity collapse by high-speed imaging above and below the water surface. Gravity can be neglected in these experiments. Three different impact regimes are identified: smooth deposition onto the pool, splashing in the direction of impact only, and splashing in all directions. …
Drop impacts on solid and liquid surfaces exhibit complex dynamics due to the competition of inertial, viscous, and capillary forces. After impact, a liquid lamella develops and expands radially, and under certain conditions, the outer rim breaks up into an irregular arrangement of filaments and secondary droplets. We show experimentally that the lamella expansion and subsequent break up of the outer rim can be controlled by length scales that are of comparable dimension to the impacting drop diameter. Under identical impact parameters, ie. fluid properties and impact velocity, we observe uniq…
Droplets splash when they impact dry, flat substrates above a critical velocity that depends on parameters such as droplet size, viscosity and air pressure. By imaging ethanol drops impacting silicone gels of different stiffnesses we show that substrate stiffness also affects the splashing threshold. Splashing is reduced or even eliminated: droplets on the softest substrates need over 70\% more kinetic energy to splash than they do on rigid substrates. We show that this is due to energy losses caused by deformations of soft substrates during the first few microseconds of impact. We find that s…
Because splashing is such a violent process, one might naively expect that neither the direction of droplet emission nor the amount of ejected material can be controlled with any precision. Even though it is observed countless times in the course of a day, drop splashing is highly non-intuitive: for example, it is surprising that the surrounding air pressure determines whether a drop will splash when hitting a smooth surface. Here we describe a discovery with significant practical ramifications: the direction, as well as the number, of the ejected droplets can be controlled by the texture of a…
The impact of droplets at increased environmental pressure is important in many industrial applications. Previous studies mainly considered the impact process at standard or reduced environmental pressure, and the effect of high environmental pressure is unclear. In this study, we experimentally investigate the impact of ethanol droplets on dry smooth surfaces at increased environmental pressure. The effects of the environmental pressure on the splashing and rupture of the crown during the impact process are analyzed. The results show that surrounding gas with high environmental pressure can l…
The splashing of a drop impacting onto a liquid pool produces a range of different sized micro-droplets. At high impact velocities, the most significant source of these droplets is a thin liquid jet emerging at the start of the impact from the neck that connects the drop to the pool. We use ultra-high-speed video imaging in combination with high-resolution numerical simulations to show how the ejecta gives way to irregular splashing. At higher Reynolds number, its base becomes unstable, shedding vortex rings into the liquid from the free surface in an axisymmetric von Kármán vortex street, thu…
Experimental and modelling study is presented for the effect of a wide range of liquid viscosities on the droplet impact on a smooth solid surface at atmospheric pressure. A non-monotonic variation of threshold between droplet deposition and splash was observed experimentally. Specifically, the critical Weber number separating deposition from splashing decreases and then increases with increasing the Ohnesorge number. The observations of splash in low viscosity region and receding breakup in high viscosity region were analyzed qualitatively from the perspectives of Kelvin-Helmholtz instability…
The ambient gas pressure is determined for the onset of splashing of low-viscosity liquid drops on smooth dry surfaces as we change the control parameters: drop impact velocity, drop radius, viscosity, surface tension, density, and gas molecular weight. This threshold pressure indicates that there are two distinct regimes when drop impact velocity is varied. By rescaling data using functions of only three dimensionless numbers, the commonly used Reynolds and Weber numbers, as well as the ratio of drop radius to gas mean free path, all data is collapsed to a single curve that encompasses both r…
We study experimentally the enhancement of splashing due to solidification. Investigating the impact of water drops on dry smooth surfaces, we show that the transition velocity to splash can be drastically reduced by cooling the surface below the liquid melting temperature. We find that at very low temperatures (below $-60 ^\circ \rm C$), the splashing behaviour becomes independent of surface undercooling and presents the same characteristics as on ambient temperature superhydrophobic surfaces. This resemblance arises from an increase of the dynamic advancing contact angle of the lamella with …
Vertical drop impacts of ferrofluids onto glass slides in a non-uniform magnetic field have been studied using high-speed photography. Outcomes have been classified based on the motion of the fluid-surface contact lines, and formation of peaks (Rosensweig instabilities) which affect the height of the spreading drop. The largest peaks are nucleated at the edge of a spreading drop, similarly to crown-rim instabilities in drop impacts with conventional fluids, and remain there for an extended time. Impact Weber numbers ranged from 18.0 to 489, and the vertical component of the B-field was varied …
The impact of nanometer sized drops on solid surfaces is studied using molecular dynamics simulations. Equilibrated floating drops consisting of short chains of Lennard-Jones liquids with adjustable volatility are directed normally onto an atomistic solid surface where they are observed to bounce, stick, splash or disintegrate, depending on the initial velocity and the nature of the materials involved. Drops impacting at low velocity bounce from non-wetting surfaces but stick and subsequently spread slowly on wetting surfaces. Higher velocity impacts produce an prompt splash followed by disint…
Drops impacting on a surface are ubiquitous in our everyday experience. This impact is understood within a commonly accepted hydrodynamic picture: it is initiated by a rapid shock and a subsequent ejection of a sheet leading to beautiful splashing patterns. However, this picture ignores the essential role of the air that is trapped between the impacting drop and the surface. Here we describe a new imaging modality that is sensitive to the behavior right at the surface. We show that a very thin film of air, only a few tens of nanometers thick, remains trapped between the falling drop and the su…
The rich structures arising from the impingement dynamics of water drops onto solid substrates at high velocities are investigated numerically. Current methodologies in the aircraft industry estimating water collection on aircraft surfaces are based on particle trajectory calculations and empirical extensions thereof in order to approximate the complex fluid-structure interactions. We perform direct numerical simulations (DNS) using the volume-of-fluid method in three dimensions, for a collection of drop sizes and impingement angles. The high speed background air flow is coupled with the motio…
