Drop impacts on solid and liquid surfaces exhibit complex dynamics due to the competition of inertial, viscous, and capillary forces. After impact, a liquid lamella develops and expands radially, and under certain conditions, the outer rim breaks up into an irregular arrangement of filaments and secondary droplets. We show experimentally that the lamella expansion and subsequent break up of the outer rim can be controlled by length scales that are of comparable dimension to the impacting drop diameter. Under identical impact parameters, ie. fluid properties and impact velocity, we observe unique splashing dynamics by varying the target cross-sectional geometry. These behaviors include: (i) geometrically-shaped lamellae and (ii) a transition in splashing stability, from regular to irregular splashing. We propose that regular splashes are controlled by the azimuthal perturbations imposed by the target cross-sectional geometry and that irregular splashes are governed by the fastest-growing unstable Plateau-Rayleigh mode.
When a droplet hits a surface fast enough, droplet splashing can occur: smaller secondary droplets detach from the main droplet during impact. While droplet splashing on smooth surfaces is by now well understood, the surface roughness also affects at which impact velocity a droplet splashes. In this study, the influence of the surface roughness on droplet splashing is investigated. By changing the root mean square roughness of the impacted surface, we show that the droplet splashing velocity is only affected when the droplet roughness is large enough to disrupt the spreading droplet lamella an…
The impact and splash of liquid drops on solid substrates are ubiquitous in many important fields. However, previous studies have mainly focused on spherical drops while the non-spherical situations, such as raindrops, charged drops, oscillating drops, and drops affected by electromagnetic field, remain largely unexplored. Using ferrofluid, we realize various drop shapes and illustrate the fundamental role of shape in impact and splash. Experiments show that different drop shapes produce large variations in spreading dynamics, splash onset, and splash amount. However, underlying all these vari…
We investigate the impact velocity beyond which the ejection of smaller droplets from the main droplet (splashing) occurs for droplets impacting a smooth surface. We examine its dependence on the surface wetting properties and droplet surface tension. We show that the splashing velocity is independent of the wetting properties of the surface, but increases roughly linearly with increasing surface tension of the liquid. A preexisting splashing model is considered that predicts the splashing velocity by incorporating the air viscosity. The model is consistent with our data, but the calculation i…
Splashing occurs when a liquid drop hits a dry solid surface at high velocity. This paper reports experimental studies of how the splash depends on the roughness and the texture of the surfaces as well as the viscosity of the liquid. For smooth surfaces, there is a "corona" splash caused by the presence of air surrounding the drop. There are several regimes that occur as the velocity and liquid viscosity are varied. There is also a "prompt" splash that depends on the roughness and texture of the surfaces. A measurement of the size distribution of the ejected droplets is sensitive to the surfac…
A drop impacting a solid surface with sufficient velocity will emit many small droplets creating a splash. However, splashing is completely suppressed if the surrounding gas pressure is lowered. The mechanism by which the gas affects splashing remains unknown. We use high-speed interference imaging to measure the air beneath all regions of a spreading viscous drop as well as optical absorption to measure the drop thickness. Although an initial air bubble is created on impact, no significant air layer persists until the time a splash is created. This suggests that splashing in our experimentall…
The corona splash due to the impact of a liquid drop on a smooth dry substrate is investigated with high speed photography. A striking phenomenon is observed: splashing can be completely suppressed by decreasing the pressure of the surrounding gas. The threshold pressure where a splash first occurs is measured as a function of the impact velocity and found to scale with the molecular weight of the gas and the viscosity of the liquid. Both experimental scaling relations support a model in which compressible effects in the gas are responsible for splashing in liquid solid impacts.
Experiments of water droplets impacting small geometric posts of equal dimension to the drop diameter are shown in this fluid dynamics video. High speed photography shows that the dynamics of drop splashing are significantly affected by the geometrical boundary of the target and that finger formation and drop break up are accurately controlled.
The impact of a drop onto a liquid layer and the subsequent splash has important implications for diverse physical processes such as air-sea gas transfer, cooling, and combustion. In the {\it crown splash} parameter regime, the splash pattern is highly regular. We focus on this case as a model for the mechanism that leads to secondary droplets, and thus explain the drop size distribution resulting from the splash. We show that the mean number of secondary droplets is determined by the most unstable wavelength of the Rayleigh-Plateau instability. Variations from this mean are governed by the wi…
We investigate the impact of droplets of dense suspensions onto a solid substrate. We show that a global hydrodynamic balance is unable to predict the splash onset and propose to replace it by an energy balance at the level of the particles in the suspension. We experimentally verify that the resulting, particle-based Weber number gives a reliable, particle size and density dependent splash onset criterion. We further show that the same argument also explains why in bimodal systems smaller particles are more likely to escape than larger ones.
Experimental and modelling study is presented for the effect of a wide range of liquid viscosities on the droplet impact on a smooth solid surface at atmospheric pressure. A non-monotonic variation of threshold between droplet deposition and splash was observed experimentally. Specifically, the critical Weber number separating deposition from splashing decreases and then increases with increasing the Ohnesorge number. The observations of splash in low viscosity region and receding breakup in high viscosity region were analyzed qualitatively from the perspectives of Kelvin-Helmholtz instability…
A liquid drop impacting a dry solid surface with sufficient kinetic energy will splash, breaking apart into numerous secondary droplets. This phenomenon shows many similarities to forced wetting, including the entrainment of air at the contact line. Because of these similarities and the fact that forced wetting has been shown to depend on the wetting properties of the surface, existing theories predict splashing to depend on wetting properties as well. However, using high-speed interference imaging we observe that at high capillary numbers wetting properties have no effect on splashing for var…
When a fast-moving drop impacts onto a smooth substrate, splashing will be produced at the edge of the expanding liquid sheet. This ubiquitous phenomenon lacks a fundamental understanding. Combining experiment with model, we illustrate that the ultrathin air film trapped under the expanding liquid front triggers splashing. Because this film is thinner than the mean free path of air molecules, the interior airflow transfers momentum with an unusually high velocity comparable to the speed of sound and generates a stress 10 times stronger than the airflow in common situations. Such a large stress…
We investigate the interplay between substrate roughness and surrounding gas pressure in controlling the dynamics of splashing when a liquid drop hits a dry solid surface. We associate two distinct forms of splashing with each of these control parameters: prompt splashing is due to surface roughness and corona splashing is due to instabilities produced by the surrounding gas. The size distribution of ejected droplets reveals the length scales of the underlying droplet-creation process in both cases.
This is an entry for the Gallery of Fluid Motion of the 61st Annual Meeting of the APS-DFD (fluid dynamics videos). This video shows the collision and rebound of viscoelastic drops against a solid wall. Using a high speed camera, the process of approach, contact and rebound of drops of a viscoelastic liquid is observed. We found that these drops first splash, similar to what is observed in Newtonian colliding drops; after a few instants, the liquid recoils, recovering its original drop shape and bounce off the wall.
Because splashing is such a violent process, one might naively expect that neither the direction of droplet emission nor the amount of ejected material can be controlled with any precision. Even though it is observed countless times in the course of a day, drop splashing is highly non-intuitive: for example, it is surprising that the surrounding air pressure determines whether a drop will splash when hitting a smooth surface. Here we describe a discovery with significant practical ramifications: the direction, as well as the number, of the ejected droplets can be controlled by the texture of a…
Droplets splash when they impact dry, flat substrates above a critical velocity that depends on parameters such as droplet size, viscosity and air pressure. By imaging ethanol drops impacting silicone gels of different stiffnesses we show that substrate stiffness also affects the splashing threshold. Splashing is reduced or even eliminated: droplets on the softest substrates need over 70\% more kinetic energy to splash than they do on rigid substrates. We show that this is due to energy losses caused by deformations of soft substrates during the first few microseconds of impact. We find that s…
The impact of droplets on liquid pools is ubiquitous in nature and many industrial applications. Most previous studies of droplet impact focus on Newtonian fluids, while less attention has been paid to the impact dynamics of non-Newtonian droplets, even though non-Newtonian fluids are widely used in many applications. In this study, the splashing dynamics of shear-thinning droplets with yield stress are studied by combined experiments and simulations. The formation and the propagation of the ejecta sheet produced during the splashing process are considered, and the velocity, the radius, and th…
We investigate the dynamics of drop impact on a thin liquid film at short times in order to identify the mechanisms of splashing formation. Using numerical simulations and scaling analysis, we show that the splashing formation depends both on the inertial dynamics of the liquid and the cushioning of the gas. Two asymptotic regimes are identified, characterized by a new dimensionless number $J$: when the gas cushioning is weak, the jet is formed after a sequence of bubbles are entrapped and the jet speed is mostly selected by the Reynolds number of the impact. On the other hand, when the air cu…
Making use of experimental and theoretical considerations, in this Letter we deduce a criterion to determine the critical velocity for which a drop impacting a smooth dry surface either spreads over the substrate or disintegrates into smaller droplets. The derived equation, which expresses the splash threshold velocity as a function of the material properties of the two fluids involved, the drop radius and the mean free path of the molecules composing the surrounding gaseous atmosphere, has been thoroughly validated experimentally at normal atmospheric conditions using eight different liquids,…
In this work simulations are presented of low viscosity ethanol and high viscosity silicone oil droplets impacting on a dry solid surface at atmospheric and reduced ambient pressure. The simulations are able to capture both the effect of the ambient gas pressure and liquid viscosity on droplet impact and breakup. The results suggests that the early time droplet impact and gas film behavior for both low and high viscosity liquids share the same physics. However, for later time liquid sheet formation and breakup high and low viscosity liquids behave differently. These results explain why for bot…
A liquid drop impacting a solid surface may splash by emitting a thin liquid sheet that subsequently breaks apart or by promptly ejecting droplets from the advancing liquid-solid contact line. Using high-speed imaging, we show that air pressure and surface roughness influence both splash mechanisms. Roughness increases prompt splashing at the advancing contact line but inhibits the formation of the thin sheet. If the air pressure is lowered, droplet ejection is suppressed not only during thin-sheet formation but for prompt splashing as well. The threshold pressure depends on impact velocity, l…
After impact onto a smooth dry surface, a drop of viscous liquid initially spreads in the form of a thick lamella. If the drop splashes, it first emits a thin fluid sheet that can ultimately break up into droplets causing the splash. Ambient gas is crucial for creating this thin sheet. The time for sheet ejection, $t_{ejt}$, depends on impact velocity, liquid viscosity, gas pressure and molecular weight. A central air bubble is trapped below the drop at pressures even below that necessary for this sheet formation. In addition, air bubbles are entrained underneath the spreading lamella when the…
At atmospheric pressure, a drop of ethanol impacting on a solid surface produces a splash. Reducing the ambient pressure below its atmospheric value suppresses this splash. The origin of this so-called pressure effect is not well understood and this is the first study to present an in-depth comparison between various theoretical models that aim to predict splashing and simulations. In this work the pressure effect is explored numerically by resolving the Navier-Stokes equations at a 3-nm resolution. In addition to reproducing numerous experimental observations, it is found that different model…
We have studied the splashing dynamics of water drops impacting granular layers. Depending on the drop kinetic energy, various shapes are observed for the resulting craters. Experimental parameters that have been considered are : the size of the millimetric droplets; the height of the free fall, ranging from 1.5 cm to 100 cm; and the diameter of the grains. As the drop is impacting the granular layer, energy is dissipated and a splash of grain occurs. Meanwhile, surface tension, inertia and viscosity compete, leading to strong deformations of the drop which depend on the experimental condition…
In nature, high-speed raindrops often impact and spread on particulate surfaces (e.g., soil, plant leaves with spores or pollen). We study the dynamics of droplet impact on a loosely packed monolayer of particles by combining experimental and mathematical approaches. We find that the presence of mobile particles lowers the critical impact velocity at which the droplet exhibits corona splashing, as the particle area fraction is systematically increased. We rationalize this experimental observation by considering the jamming of frictional particles at the spreading rim. Elucidating the splashing…
Droplet Impact on Microparticle Raft: Wettability, density and size govern splashing and microplastic ejection from rafts under raindrop impact
University College London（伦敦大学学院）；University of Oxford（牛津大学）；Instituto de Investigaciones en Materiales, Universidad Nacional Autónoma de México（墨西哥国立自治大学材料研究所）
We experimentally investigate the splashing mechanism of a millimeter-sized ethanol drop impinging on a structured solid surface, comprised of micro-pillars, through side-view and top-view high speed imaging. By increasing the impact velocity we can tune the impact outcome from a gentle deposition to a violent splash, at which tiny droplets are emitted as the liquid sheet spreads laterally. We measure the splashing threshold for different micropatterns and find that the arrangement of the pillars significantly affects the splashing outcome. In particular, directional splashing in direction in …
Tokyo University of Agriculture and Technology（东京农工大学）
The impact of a drop on a solid surface is an important phenomenon that has various implications and applications. However, the multiphase nature of this phenomenon causes complications in the prediction of its morphological evolution, especially when the drop splashes. While most machine-learning-based drop-impact studies have centred around physical parameters, this study used a computer-vision strategy by training an encoder-decoder to predict the drop morphologies using image data. Herein, we show that this trained encoder-decoder is able to successfully generate videos that show the morph…
We investigate both experimentally and numerically the impact of liquid drops on deep pools of aqueous glycerol solutions with variable pool viscosity and air pressure. With this approach we are able to address drop impacts on substrates that continuously transition from low-viscosity liquids to almost solids. We show that the generic corolla spreading out from the impact point consists of two distinct sheets, namely an ejecta sheet fed by the drop liquid and a second sheet fed by the substrate liquid, which evolve on separated timescales. These two sheets contribute to a varying extent to the…
We present fluid dynamics videos illustrating wetting splashing-produced by water drop impact onto hydrophobic microstructures at high impact velocity ($\sim 3$ ms$^{-1}$). The substrate consists of regular and transparent microtextures in square or hexagonal lattice, yielding a high contact angle of $\sim 150 ^\circ$. Our high speed top-or-bottom view recordings through the transparent surface shed light on the solid-liquid-air interfaces at impact. Despite the superhydrophobicity of the latticed micropillars (of a periodicity of $10 μm), water droplet wets a certain central area and moreover…
The oblique impact of a liquid droplet onto a deep liquid pool is studied numerically with the adaptive volume-of-fluid solver Basilisk. The splashing threshold, cavity formation, cavity evolution and the maximum cavity dimensions are quantified as a function of the Weber number and the impact angle. We compare the numerical results with recent experimental work by Gielen et al. [Phys. Rev. Fluids 2, 083602 (2017)]. Similarly to the experimental results, three different impact regimes are observed: deposition of the droplet onto the pool, single-sided splashing in the direction of the impact a…
We explore the evolution of a splash when a liquid drop impacts a smooth, dry surface. There are two splashing regimes that occur when the liquid viscosity is varied, as is evidenced by its dependence on ambient gas pressure. A high-viscosity drop splashes by emitting a thin sheet of liquid from a spreading liquid lamella long after the drop has first contacted the solid. Likewise, we find that there is also a delay in the ejection of a thin sheet when a low-viscosity drop splashes. We show how the ejection time of the thin sheet depends on liquid viscosity and ambient gas pressure.
Oblique impact of drops onto a solid or liquid surface is frequently observed in nature. Most studies on drop impact and splashing, however, focus on perpendicular impact. Here, we study oblique impact of 100-micrometer drops onto a deep liquid pool, where we quantify the splashing threshold, maximum cavity dimensions and cavity collapse by high-speed imaging above and below the water surface. Gravity can be neglected in these experiments. Three different impact regimes are identified: smooth deposition onto the pool, splashing in the direction of impact only, and splashing in all directions. …
The video exhibits experimental qualitative and quantitative results of water/glycerol (50%/50% by mass) droplet impact on two types of micro-patterned superhydrophobic surfaces. The two types of surfaces used were 80% cavity fraction ribs and posts with a periodic spacing of 40 μm and 32 μm, respectively. All surfaces were manufactured through photolithography. The impact Weber number is used as the dynamic parameter to compare splash and rebound behaviors between the two types of surfaces. While droplets exhibit similar dynamics at low Weber numbers, rebound jet speed (normalized by droplet …
We experimentally investigated the splashing of dense suspension droplets impacting a solid surface, extending prior work to the regime where the viscosity of the suspending liquid becomes a significant parameter. The overall behavior can be described by a combination of two trends. The first one is that the splashing becomes favored when the kinetic energy of individual particles at the surface of a droplet overcomes the confinement produced by surface tension. This is expressed by a particle-based Weber number $We_p$. The second is that splashing is suppressed by increasing the viscosity of …
The ambient gas pressure is determined for the onset of splashing of low-viscosity liquid drops on smooth dry surfaces as we change the control parameters: drop impact velocity, drop radius, viscosity, surface tension, density, and gas molecular weight. This threshold pressure indicates that there are two distinct regimes when drop impact velocity is varied. By rescaling data using functions of only three dimensionless numbers, the commonly used Reynolds and Weber numbers, as well as the ratio of drop radius to gas mean free path, all data is collapsed to a single curve that encompasses both r…
Even a small fraction of nanoparticles in fluids affects the splashing behavior of a droplet upon impact on a smooth surface. Nanofluid drop impact onto a smooth sapphire substrate is experimentally investigated over wide ranges of Reynolds ($10^2<\mathrm{Re}<10^4$) and Weber ($50<\mathrm{We}<500$) numbers for three nanofluid mass concentrations (0.01%, 0.1%, 1%) using high-speed photography. Nanofluids are prepared by diluting a commercial Al$_2$O$_3$-water nanofluid in aqueous glycerol solutions without dispersants. In total, 30 samples are prepared and 1799 data points are acquired. Every s…
Tokyo University of Agriculture and Technology（东京农工大学）
This article reports nonintuitive characteristic of a splashing drop on a solid surface discovered through extracting image features using a feedforward neural network (FNN). Ethanol of area-equivalent radius about 1.29 mm was dropped from impact heights ranging from 4 cm to 60 cm (splashing threshold 20 cm) and impacted on a hydrophilic surface. The images captured when half of the drop impacted the surface were labeled according to their outcome, splashing or nonsplashing, and were used to train an FNN. A classification accuracy higher than 96% was achieved. To extract the image features ide…
Correlation between morphological evolution of splashing drop and exerted impact force revealed by interpretation of explainable artificial intelligence
Tokyo University of Agriculture and Technology（东京农工大学）
We study the formation, growth, and disintegration of jets following impact of a drop on a thin film of the same liquid for We < 1000 and Re < 2000 using a combination of numerical simulations and linear stability theory (Agbaglah et al. 2013). Our simulations faithfully capture this phenomena and are in good agreement with experimental profiles obtained from high-speed X-ray imaging.We obtain scaling relations from our simulations and use these as inputs to our stability analysis. The resulting prediction for the most unstable wavelength are in excellent agreement with experimental data. Our …
Would a raindrop impacting on a coarse beach behave differently from that impacting on a desert of fine sand? We study this question by a series of model experiments, where the packing density of the granular target, the wettability of individual grains, the grain size, the impacting liquid, and the impact speed are varied. We find that by increasing the grain size and/or the wettability of individual grains the maximum droplet spreading undergoes a transition from a capillary regime towards a viscous regime, and splashing is suppressed. The liquid-grain mixing is discovered to be the underlyi…
Tokyo University of Agriculture and Technology（东京农工大学）
This paper reports the features of a splashing drop on a solid surface and the temporal evolution, which are extracted through image-sequence classification using a highly interpretable feedforward neural network (FNN) with zero hidden layer. The image sequences used for training-validation and testing of the FNN show the early-stage deformation of milli-sized ethanol drops that impact a hydrophilic glass substrate with the Weber number ranges between 31-474 (splashing threshold about 173). Specific videographing conditions and digital image processing are performed to ensure the high similari…
The dynamics of drop impact on solid surfaces can be changed significantly by tuning the elasticity of the solid. Most prominently, the substrate deformation causes an increase in the splashing threshold as compared to impact onto perfectly rigid surfaces, and can thus lead to splash suppression. Here, we experimentally determine the splashing threshold for impact on thin membranes as a function of the tension in the membrane and its elastic properties. The drop dynamics is correlated to the membrane deformation, which is simultaneously measured using a laser profilometry technique. The experi…
Impacts of drops on liquids are ubiquitous in nature and in a range of applications in healthcare, agriculture and industry. They can lead to splash and generation of secondary droplets important for a range of coating, dispersal or contaminant problems. The physics of splash, despite being more than a century old problem, still has a number of unanswered questions. We study the sequence of events occurring upon drop impact on a deep, inviscid liquid pool. We particularly focus on the air cavity formed below the liquid surface and the liquid sheet of the crown, which forms and rises above the …
Droplet impact on a surface is practically relevant to a variety of fields in nature and industry, while a complete control of its outcomes remains challenging due to various unmanageable factors. In this work, we propose the quantum simulation of droplet impact outcomes in the platform of ultracold atoms. Specifically, we study the quantum-fluctuation-driven dynamics (QFDD) of two-dimensional Bose-Bose mixtures from an initial Townes soliton towards the formation of a quantum droplet. By tuning the fluctuation energy of the initial Townes state through its size and number, the subsequent QFDD…
The splashing of a drop impacting onto a liquid pool produces a range of different sized micro-droplets. At high impact velocities, the most significant source of these droplets is a thin liquid jet emerging at the start of the impact from the neck that connects the drop to the pool. We use ultra-high-speed video imaging in combination with high-resolution numerical simulations to show how the ejecta gives way to irregular splashing. At higher Reynolds number, its base becomes unstable, shedding vortex rings into the liquid from the free surface in an axisymmetric von Kármán vortex street, thu…
The impact of droplets at increased environmental pressure is important in many industrial applications. Previous studies mainly considered the impact process at standard or reduced environmental pressure, and the effect of high environmental pressure is unclear. In this study, we experimentally investigate the impact of ethanol droplets on dry smooth surfaces at increased environmental pressure. The effects of the environmental pressure on the splashing and rupture of the crown during the impact process are analyzed. The results show that surrounding gas with high environmental pressure can l…
In this article, the fluid dynamics of room temperature liquid metal (RTLM) droplet impacting onto a pool of the same liquid in ambient air was investigated. A series of experiments were conducted in order to disclose the influence of the oxidation effect on the impact dynamics. The droplet shape and impact phenomenology were recorded with the aid of a high-speed digital camera. The impact energy stored in the splash structures was estimated via a theoretical model and several morphological parameters obtained from instantaneous images of the splash. It was observed that the droplet shape and …
In this paper we analyze the impact of a circular disc on a free surface using experiments, potential flow numerical simulations and theory. We focus our attention both on the study of the generation and possible breakup of the splash wave created after the impact and on the calculation of the force on the disc. We have experimentally found that drops are only ejected from the rim located at the top part of the splash --giving rise to what is known as the crown splash-- if the impact Weber number exceeds a threshold value $\Weber_{crit}\simeq 140$. We explain this threshold by defining a local…
The impact of nanometer sized drops on solid surfaces is studied using molecular dynamics simulations. Equilibrated floating drops consisting of short chains of Lennard-Jones liquids with adjustable volatility are directed normally onto an atomistic solid surface where they are observed to bounce, stick, splash or disintegrate, depending on the initial velocity and the nature of the materials involved. Drops impacting at low velocity bounce from non-wetting surfaces but stick and subsequently spread slowly on wetting surfaces. Higher velocity impacts produce an prompt splash followed by disint…
We study experimentally the enhancement of splashing due to solidification. Investigating the impact of water drops on dry smooth surfaces, we show that the transition velocity to splash can be drastically reduced by cooling the surface below the liquid melting temperature. We find that at very low temperatures (below $-60 ^\circ \rm C$), the splashing behaviour becomes independent of surface undercooling and presents the same characteristics as on ambient temperature superhydrophobic surfaces. This resemblance arises from an increase of the dynamic advancing contact angle of the lamella with …
