We discuss the magnetic and topological properties of bulk crystals and quasi-two-dimensional thin films formed by stacking intrinsic magnetized topological insulator ( for example Mn(Sb$_{x}$Bi$_{1-x}$)$_2$X$_4$ with X = Se,Te, including MnBi$_2$Te$_4$) septuple layers and topological insulator quintuple layers in arbitrary order. Our analysis makes use of a simplified model that retains only Dirac-cone degrees of freedom on both surfaces of each septuple or quintuple layer. We demonstrate the model's applicability and estimate its parameters by comparing with {\it ab initio } density-functional-theory(DFT) calculations. We then employ the coupled Dirac cone model to provide an explanation for the dependence of thin-film properties, particularly the presence or absence of the quantum anomalous Hall effect, on film thickness, magnetic configuration, and stacking arrangement, and to comment on the design of Weyl superlattices.
We present an analytical theory to describe three-dimensional magnetic textures in perpendicularly magnetized magnetic multilayers that arise in the presence of magnetostatic interactions and the Dzyaloshinskii-Moriya interaction (DMI). We demonstrate that domain walls in multilayers develop a complex twisted structure, which persists even for films with strong DMI. The origin of this twist is surface-volume stray field interactions that manifest as a depth-dependent effective field whose form mimics the DMI effective field. We find that the wall twist has a minor impact on the equilibrium sky…
Current induced domain wall (DW) motion has been investigated in a 600-nm wide nanowire using multilayer film with a structure of Ta(5 nm)/Pd(5 nm)/[CoFe(0.4 nm)/Pd(1.2 nm)]$_{15}$/Ta(5 nm)in terms of anomalous Hall effect measurements. It is found that motion of DWs can be driven by a current density as low as 1.44$\times$10$^{11}$ A.m$^{-2}$. The effect of the Oersted field ($H_{Oe}$) and spin transfer torque field ($H_{ST}$), which are considered as effective fields for DW motion, has been quantitatively separated from the dependence of depinning fields on the current. The results show that…
Two-dimensional magnetic insulators can be promising hosts for topological magnons. In this study, we show that ABC-stacked honeycomb lattice multilayers with alternating Dzyaloshinskii-Moriya interaction (DMI) reveal a rich topological magnon phase diagram. Based on our bandstructure and Berry curvature calculations, we demonstrate jumps in the thermal Hall behavior that corroborate with topological phase transitions triggered by adjusting the DMI and interlayer coupling. We connect the phase diagram of generic multilayers to a bilayer and a trilayer system. We find an even-odd effect amongst…
Based on $k\cdot p$ analysis and realistic tight-binding calculations, we find that time-reversal-breaking Weyl semimetals can be realized in magnetically-doped (Mn, Eu, Cr etc.) Sn$_{1-x}$Pb$_x$(Te,Se) class of topological crystalline insulators. All the Weyl points are well separated in momentum space and possess nearly the same energy due to high crystalline symmetry. Moreover, both the Weyl points and Fermi arcs are highly tunable by varying Pb/Sn composition, pressure, magnetization, temperature, surface potential etc., opening up the possibility of manipulating Weyl points and rewiring t…
Tailoring Ultrathin Magnetic Multilayers at Terraced Topologically Insulating Interfaces for Perpendicularly Magnetized Domains
University of Leeds（利兹大学）；ISIS Neutron and Muon Source, STFC Rutherford Appleton Laboratory（STFC卢瑟福阿普尔顿实验室中子与μ子源）；Diamond Light Source（钻石光源）；Imperial College London（伦敦帝国理工学院）
Spin-orbit torque (SOT) magnetization switching of ferromagnets with large perpendicular magnetic anisotropy has a great potential for the next-generation non-volatile magnetoresistive random-access memory (MRAM). It requires a high-performance pure spin current source with a large spin Hall angle and high electrical conductivity, which can be fabricated by a mass production technique. In this work, we demonstrate ultrahigh efficient and robust SOT magnetization switching in all-sputtered BiSb topological insulator - perpendicularly magnetized Co/Pt multilayers. Despite fabricated by the indus…
We present a study of the temperature dependence of the switching fields in Co/Ni-based perpendicularly magnetized spin-valves. While magnetization reversal of all-perpendicular Co/Ni spin valves at ambient temperatures is typically marked by a single sharp step change in resistance, low temperature measurements can reveal a series of resistance steps, consistent with non-uniform magnetization configurations. We propose a model that consists of domain nucleation, propagation and annihilation to explain the temperature dependence of the switching fields. Interestingly, low temperature (<30 K) s…
Chirally stacked $N$-layer graphene is a semimetal with $\pm p^N$ band-touching at two nonequivalent corners in its Brillioun zone. We predict that an off-resonant circularly polarized light (CPL) drives chirally stacked $N$-layer graphene into a Floquet Chern Insulators (FCIs), a.k.a. quantum anomalous Hall insulators, with tunable high Chern number $C_F=\pm N$ and large gaps. A topological phase transition between such a FCI and a valley Hall (VH) insulator with high valley Chern number $C_v=\pm N$ induced by a voltage gate can be engineered by the parameters of the CPL and voltage gate. We …
We explore the scattering of Dirac electrons in a double-gated topological insulator in the presence of magnetic proximity effects and warped surface states. It is found that a magnetic field can shift the Dirac cone in momentum space and deform the constant-energy contour, or opens up a band gap at the Dirac point, depending on the magnetization orientation. The double gate voltage induces quantum wells and/or quantum barriers on the surface of topological insulators, generating surface resonant tunnelling states. It is found that the hexagonal warping effect can increase the electronic trans…
Centro Atómico Bariloche（巴里洛切原子中心）；Instituto Balseiro, Universidad Nacional de Cuyo–CNEA（巴尔塞罗研究所，门多萨国立大学-国家原子能委员会）；Instituto de Nanociencia y Materiales de Aragón (INMA-CSIC)（阿拉贡纳米与材料研究所）；Universidad de Zaragoza（萨拉戈萨大学）
One-dimensional (1D) topologically protected states are usually formed at the interface between two-dimensional (2D) materials with different topological invariants. Therefore, 1D chiral interface channels (CICs) can be created at the boundary of two quantum anomalous Hall (QAH) insulators with different Chern numbers. Such a QAH junction can function as a chiral edge current distributer at zero magnetic field, but its realization remains challenging. Here, by employing an in-situ mechanical mask, we use molecular beam epitaxy (MBE) to synthesize QAH insulator junctions, in which two QAH insul…
The transverse anisotropy constant and the related Döring mass density are key parameters of the one-dimensional model to describe the motion of magnetic domain walls. So far, no general framework is available to determine these quantities from static characterizations such as magnetometry measurements. Here, we derive a universal analytical expression to calculate the transverse anisotropy constant for the important class of perpendicular magnetic multilayers. All the required input parameters of the model, such as the number of repeats, the thickness of a single magnetic layer, and the layer…
We propose a different route to time-reversal invariant Weyl semimetals employing multilayer heterostructures comprising ordinary "trivial" insulators and nontrivial insulators with \textit{pairs} of protected Dirac cones on the surface. We consider both the case of weak topological insualtors, where surface Dirac cones are pinned to time-reversal invariant momenta, and of topological crystalline insulators with unpinned surface Dirac cones. For both realizations we explain phenomenologically how the proposed construction leads to the emergence of a Weyl semimetal phase. We further formulate e…
This is a Reply to a Comment by Tanaka and Machida. We provide some details of the derivation of the effective field theory for integer quantum Hall transitions using the non-Abelian chiral anomaly.
We use the Dirac cone model to explore the high Chern number (C) phases that are realized in the magnetic-doped topological insulator (TI) multilayer structures by Zhao et al. [Nature 588, 419 (2020)]. The Chern number is calculated by capturing the evolution of the phase boundaries with the parameters and then the Chern number phase diagrams of the TI multilayer structures are obtained. The high-C behavior is attributed to the band inversion of the renormalized Dirac cones, along with which the spin polarization at the Γpoint will get increased. Moreover, another two TI multilayer structures …
While the experimental progress on three dimensional topological insulators is rapid, the development of their two dimensional counterparts has been comparatively slow, despite their technological promise. The main reason is materials challenges of the to date only realizations of two-dimensional topological insulators, in semiconductor quantum wells. Here we identify a two dimensional topological insulator in a material which does not face similar challenges and which is by now most widely available and well-charaterized: graphene. For certain commensurate interlayer twists graphene multilaye…
The high-Chern number phases with a Chern number C>1 have been observed in a recent experiment that performed on the topological insulator (TI) multilayer structures, consisting of the alternating magnetic-doped and undoped TI layers. In this paper, we develop an effective method to determine the Chern numbers in the TI multilayer structures and then make a systematic study on the Chern number phase diagrams that are modulated by the magnetic doping and the middle layer thickness. We point out that in the multilayer structure, the high-C behavior can be attributed to the band inversion mechani…
We propose a simple realization of the three-dimensional (3D) Weyl semimetal phase, utilizing a multilayer structure, composed of identical thin films of a magnetically-doped 3D topological insulator (TI), separated by ordinary-insulator spacer layers. We show that the phase diagram of this system contains a Weyl semimetal phase of the simplest possible kind, with only two Dirac nodes of opposite chirality, separated in momentum space, in its bandstructure. This particular type of Weyl semimetal has a finite anomalous Hall conductivity, chiral edge states, and occurs as an intermediate phase b…
We develop a minimal theory for the recently observed metal-insulator transition (MIT) in two-dimensional (2D) moiré multilayer transition metal dichalcogenides (mTMD) using Coulomb disorder in the environment as the underlying mechanism. In particular, carrier scattering by random charged impurities leads to an effective 2D MIT approximately controlled by the Ioffe-Regel criterion, which is qualitatively consistent with the experiments. We find the necessary disorder to be around $5$-$10\times10^{10}$cm$^{-2}$ random charged impurities in order to quantitatively explain much, but not all, of …
Spin pumping in Yttrium-iron-garnet (YIG)/nonmagnetic-metal (NM) layer systems under ferromagnetic resonance (FMR) conditions is a popular method of generating spin current in the NM layer. A good understanding of the spin current source is essential in extracting spin Hall angle of the NM and in potential spintronics applications. It is widely believed that spin current is pumped from precessing YIG magnetization into NM layer. Here, by combining microwave absorption and DC-voltage measurements on YIG/Pt and YIG/NM1/NM2 (NM1=Cu or Al, NM2=Pt or Ta), we unambiguously showed that spin current i…
In ultra-thin film of topological insulator, the hybridization between the top and bottom surfaces opens an energy gap and forms two degenerate quantum anomalous Hall states, which give rise to a quantum spin Hall state. In this paper, we demonstrate that a Weyl semimetal can be realized in an ultra-thin film of topological insulator heterostructure in a similar way to that of the surface state of a strong three-dimensional (3D) topological insulator studied by Burkov and Balents . We find that the system realizes both 3D quantum anomalous Hall phase and 3D quantum spin Hall phase, and the Wey…
A multilayer edge molecular electronics device (MEMED), which utilize the two metal electrodes of a metal-insulator-metal tunnel junction as the two electrical leads to molecular channels, can overcome the long standing fabrication challenges for developing futuristic molecular devices. However, producing ultrathin insulator is the most challenging step in MEMED fabrication. A simplified molecular device approach was developed by avoiding the need of depositing a new materiel on the bottom electrode for growing ultrathin insulator. This paper discuss the approach for MEMED's insulator growth b…
The so called quantum spin Hall phase is a topologically non trivial insulating phase that is predicted to appear in graphene and graphene-like systems. In this work we address the question of whether this topological property persists in multilayered systems. We consider two situations: purely multilayer graphene and heterostructures where graphene is encapsulated by trivial insulators with a strong spin-orbit coupling. We use a four orbital tight-binding model that includes the full atomic spin-orbit coupling and we calculate the $Z_{2}$ topological invariant of the bulk states as well as th…
Employing a Keldysh-Eilenberger technique, we theoretically study the generation of a sponta- neous supercurrent and the appearance of the $ϕ$0 phase shift parallel to uniformly in-plane mag- netized superconducting interfaces made of the surface states of a three-dimensional topological insulator. We consider two weakly coupled uniformly magnetized superconducting surfaces where a macroscopic phase difference between the s-wave superconductors can be controlled externally. We find that, depending on the magnetization strength and orientation on each side, a spontaneous supercurrent due to the…
We calculate the energy of the magnetostatic interaction between two ferromagnetic films with uniform magnetization and correlated interfaces (the "orange-peel" effect). The "orange-peel" coupling is anisotropic: the interaction is ferromagnetic when the films are magnetized in-plane; and it is antiferromagnetic when magnetization is out-of-plane. The interaction anisotropy can be used to distinguish the "orange-peel" effect from the interlayer exchange coupling.
We investigate an ultra-thin film of topological insulator (TI) multilayer as a model for a three-dimensional (3D) Weyl semimetal. We introduce tunneling parameters $t_S$, $t_\perp$, and $t_D$, where the former two parameters couple layers of the same thin film at small and large momenta, and the latter parameter couples neighbouring thin film layers along the $z$-direction. The Chern number is computed in each topological phase of the system and we find that for $t_S,t_D>0$, the tunneling parameter $t_\perp$ changes from positive to negative as the system transits from Weyl semi-metallic phas…
We experimentally study the interlayer interaction in a magnetic multilayer system ferromagnet/insulator/ferromagnet with different spacer thickness. We demonstrate that the sign and the magnitude of the interaction can be deduced from the FMR peak shape rather than from the FMR peak shift. The proposed technique allows studying the interlayer interaction using a single sample (without a reference sample for comparison).
Charge imprinting biases topology of correlated insulator in hBN-aligned rhombohedral multilayer graphene
University of Chinese Academy of Sciences（中国科学院大学）；Kavli Institute for Theoretical Sciences, University of Chinese Academy of Sciences（中国科学院理论科学 kavli 研究所）；ShanghaiTech University（上海科技大学）；Liaoning Academy of Materials（辽宁省材料研究院）
We investigate multilayer systems of a normal insulator and a Weyl semimetal. We calculate the bulk band structure and determine phase diagrams by changing the thickness of the normal insulator and that of the Weyl semimetal layer using two models; one is from the effective model for a Weyl semimetal, and the other is the lattice model. We compare the results between the two models, and found that they agree well. As a result, we find that the multilayer system shows a qualitatively different behavior depending on the stacking direction relative to the displacement vector connecting between tw…
The quantum anomalous Hall (QAH) state is a two-dimensional topological insulating state that has quantized Hall resistance of h/Ce2 and vanishing longitudinal resistance under zero magnetic field, where C is called the Chern number. The QAH effect has been realized in magnetic topological insulators (TIs) and magic-angle twisted bilayer graphene. Despite considerable experimental efforts, the zero magnetic field QAH effect has so far been realized only for C = 1. Here we used molecular beam epitaxy to fabricate magnetic TI multilayers and realized the QAH effect with tunable Chern number C up…
Topological insulators (TIs) are bulk insulators with exotic 'topologically protected' surface conducting modes. It has recently been pointed out that when stacked together, interactions between surface modes can induce diverse phases including the TI, Dirac semimetal, and Weyl semimetal. However, currently a full experimental understanding of the conditions under which topological modes interact is lacking. Here, working with multilayers of the TI Sb$_2$Te$_3$ and the band insulator GeTe, we provide experimental evidence of a multiple topological modes in a single Sb$_2$Te$_3$-GeTe-Sb$_2$Te$_…
Spinmotive force induced by domain wall motion in perpendicularly magnetized nanowires is numerically demonstrated. We show that using nanowires with large magnetic anisotropy can lead to a high stability of spinmotive force under strong magnetic fields. We observe spinmotive force in the order of tens of microvolt in a multilayered Co/Ni nanowire and in the order of several hundred microvolt in a FePt nanowire; the latter is two orders of magnitude greater than that in permalloy nanowires reported previously. The narrow structure and low mobility of a domain wall under magnetic fields in perp…
The metal-insulator transition temperature in CMR manganites has been altered and brought close to the room temperature by preparing La$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (LSMO)/ Nd$_{0.67}$Sr$_{0.33}$MnO$_{3}$ (NSMO) multilayers with ultra thin individual layers of LSMO and NSMO. The LSMO/NSMO multilayers with ultra thin individual layers of thickness of about $10Å$ exhibits 150% magnetoresistance at 270 K whereas LSMO/NSMO multilayers with moderate individual layer thickness of about $40Å$ each exhibits a mere 15% magnetoresistance at the same temperature. We have shown that the reduction in thick…
Fractional Chern insulators in alternating twisted multilayer MoTe$_{2}$
Huazhong University of Science and Technology（华中科技大学）；Wuhan National High Magnetic Field Center, Huazhong University of Science and Technology（华中科技大学武汉国家高能磁场中心）；Hubei Fundamental Research Center for Physics（湖北省物理基础研究中心）
We theoretically study the correlated insulator states, quantum anomalous Hall (QAH) states, and field-induced topological transitions between different correlated states in twisted multilayer graphene systems. Taking twisted bilayer-monolayer graphene and twisted double-bilayer graphene as examples, we show that both systems stay in spin polarized, $C_{3z}$-broken insulator states with zero Chern number at 1/2 filling of the flat bands under finite displacement fields. In some cases these spin polarized, nematic insulator states are in the quantum valley Hall phase by virtue of the nontrivial…
Mainstream among topological insulators, GaSb/InAs quantum wells present a broken gap alignment for the energy bands which supports the quantum spin Hall insulator phase and forms an important building block in the search of exotic states of matter. Such structures allow the band-gap inversion with electrons and holes confined in adjacent layers, providing a fertile ground to tune the corresponding topological properties. Using a full 3D 8-band ${\bf k}\cdot{\bf p}$ method we investigate the inverted band structure of GaSb/InAs/GaSb and InAs/GaSb/InAs multilayers and the behavior of the helica…
In this work, we predict a hinged quantum spin-Hall (HQSH) effect featured by a pair of helical hinge modes in antiferromagnetic (AFM) topological insulator (TI) multilayers. This pair of helical hinge modes are localized on the hinges of the top and bottom surfaces of the AFM TI multilayers. Unlike the conventional QSH effect, the HQSH effect survives the breaking of time-reversal symmetry (TRS) and thus represents a different kind of topological phenomenon. The helical hinge modes are sustainable to inelastic scattering and TRS-breaking disorder, which can be observed in macroscopic samples.…
The metal-insulator transition (MIT) is one of the remarkable electrical transport properties of atomically thin molybdenum disulphide (MoS2). Although the theory of electron-electron interactions has been used in modeling the MIT phenomena in MoS2, the underlying mechanism and detailed MIT process still remain largely unexplored. Here, we demonstrate that the vertical metal-insulator-semiconductor (MIS) heterostructures built from atomically thin MoS2 (monolayers and multilayers) are ideal capacitor structures for probing the electron states in MoS2. The vertical configuration of MIS heterost…
Chern insulators are two-dimensional magnetic topological materials that conduct electricity along their edges via the one-dimensional chiral modes. The number of these modes is a topological invariant called the first Chern number $C$, that defines the quantized Hall conductance as $S_{xy}= C e^2/h$. Increasing $C$ is pivotal for the realization of low-power-consumption topological electronics, but there has been no clear-cut solution of this problem so far, with the majority of existing Chern insulators showing $C=1$. Here, by using state-of-the-art theoretical methods, we propose an efficie…
Deterministic current-induced spin-orbit torque (SOT) switching of magnetization in a heavy transition metal/ferromagnetic metal/oxide magnetic heterostructure with the ferromagnetic layer being perpendicularly-magnetized typically requires an externally-applied in-plane field to break the switching symmetry. We show that by inserting an in-plane magnetized ferromagnetic layer CoFeB underneath the conventional W/CoFeB/MgO SOT heterostructure, deterministic SOT switching of the perpendicularly-magnetized top CoFeB layer can be realized without the need of in-plane bias field. Kerr imaging study…
Dirac points in two-dimensional electronic structures are a source for topological electronic states due to the $\pm π$ Berry phase that they sustain. Here we show that two rutile multilayers (namely (WO$_2$)$_2$/(ZrO$_2$)$_n$ and (PtO$_2$)$_2$/(ZrO$_2$)$_n$, where an active bilayer is sandwiched by a thick enough (n=6 is sufficient) band insulating substrate, show semi-metallic Dirac dispersions with a total of four Dirac cones along the $Γ-M$ direction. These become gapped upon the introduction of spin-orbit coupling, giving rise to an insulating ground state comprising four edge states. We …
Topological edge states at the boundary of quantum spin Hall (QSH) insulators hold great promise for dissipationless electron transport. The device application of topological edge states has several critical requirements for the QSH insulator materials, e.g., large band gap, appropriate insulating substrates, and multiple conducting channels. In this paper, based on first-principle calculations, we show that Bi$_{4}$Br$_{4}$ is a suitable candidate. Single-layer Bi$_{4}$Br$_{4}$ was demonstrated to be QSH insulator with sizable gap recently. Here, we find that, in multilayer systems, both the …
Second-order topological insulators (SOTIs) are the topological phases of matter in d dimensions that manifest (d-2)-dimensional localized modes at the intersection of the edges. We show that SOTIs can be designed via stacked Chern insulators with opposite chiralities connected by interlayer coupling. To characterize the bulk-corner correspondence, we establish a Jacobian-transformed nested Wilson loop method and an edge theory that are applicable to a wider class of higher-order topological systems. The corresponding topological invariant admits a filling anomaly of the corner modes with frac…
Graphene multilayers with flat moiré minibands can exhibit the quantized anomalous Hall effect due to the combined influence of spontaneous valley polarization and topologically non-trival valley-projected bands. The sign of the Hall effect in these Chern insulators can be reversed either by applying an external magnetic field, or by driving a transport current through the system. We propose a current-driven mechanism whereby reversal occurs along lines in the (current $I$, magnetic-field $B$) control parameter space with slope $dI/dB = (e/h)\, M A_{M} \, (1-γ^2)/γ$, where $M$ is the magnetiza…
Spin-polarized Superconductivity and High-Chern Insulators in Twisted Rhombohedral Graphene Family
International Center for Quantum Materials, School of Physics, Peking University（北京大学物理学院量子材料国际中心）；State Key Laboratory for Mesoscopic Physics, Frontiers Science Centre for Nano-optoelectronics, School of Physics, Peking University（北京大学物理学院介观物理国家重点实验室纳米光电子前沿科学中心）；Research Center for Electronic and Optical Materials, National Institute for Material Science（日本国立物质材料研究所电子与光学材料研究中心）；Research Center for Materials Nanoarchitectonics, National Institute for Material Science（日本国立物质材料研究所材料纳米结构研究中心）；Interdisciplinary Institute of Light-Element Quantum Materials and Research Centre for Light-Element Advanced Materials, Peking University（北京大学轻元素量子材料交叉研究院轻元素先进材料研究中心）
The advent of topological phases of matter revealed a variety of observed boundary phenomena, such as chiral and helical modes found at the edges of two-dimensional (2D) topological insulators. Antichiral states in 2D semimetals, i.e., copropagating edge modes on opposite edges compensated by a counterpropagating bulk current, are also predicted, but, to date, no realization of such states in a solid-state system has been found. Here, we put forward a procedure to realize antichiral states in twisted van der Waals multilayers, by combining the electronic Dirac-cone spectra of each layer throug…
