Within a gauge-invariant microscopic kinetic theory, we study the electromagnetic response in the superconducting states. Both superfluid and normal-fluid dynamics are involved. We predict that the normal fluid is present only when the excited superconducting velocity $v_s$ is larger than a threshold $v_L=|Δ|/k_F$. Interestingly, with the normal fluid, we find that there exists friction between the normal-fluid and superfluid currents. Due to this friction, part of the superfluid becomes viscous. Therefore, a three-fluid model: normal fluid, non-viscous and viscous superfluids, is proposed. For the stationary magnetic response, at $v_s<v_L$ with only the non-viscous superfluid, the Meissner supercurrent is excited and the gap equation can reduce to Ginzburg-Landau equation. At $v_s{\ge}v_L$, with the normal fluid, non-viscous and viscous superfluids, in addition to the directly excited Meissner supercurrent in the superfluid, normal-fluid current is also induced through the friction drag with the viscous superfluid current. Due to the normal-fluid and viscous superfluid currents, the penetration depth is influenced by the scattering effect. In addition, a modified Ginzburg-Landau equation is proposed. We predict an exotic phase in which both the resistivity and superconducting gap are {\em finite}. As for the optical response, the excited ${v_s}$ oscillates with time. When $v_s<v_L$, only the non-viscous superfluid is present whereas at $v_s{\ge}v_L$, normal fluid, non-viscous and viscous superfluids are present. We show that the excited normal-fluid current exhibits the Drude-model behavior while the superfluid current consists of the Meissner supercurrent and Bogoliubov quasiparticle current. Due to the friction between the superfluid and normal-fluid currents, the optical conductivity is captured by the three-fluid model. ......
A broad review of theoretical research work involving different types of microscopic mechanism in various classes of superconductors, carried out in our research group over a decade or so, is presented. These mechanisms include both conventional as well as exotic ones. Special emphasis is placed on the possible applications to the experimental situations. Moreover, comparison of our works with various theoretical proposals made by various other researchers, with regard to high temperature superconductivity in particular, is made. The crucial importance and special significance of our results a…
It is widely believed that, in contrast to its electron doped counterparts, the hole doped compound Ba1-xKxFe2As2 exhibits a mesoscopic phase separation of magnetism and superconductivity in the underdoped region of the phase diagram. Here, we report a combined high-resolution x-ray powder diffraction and volume sensitive muon spin rotation study of underdoped Ba1-xKxFe2As2 (0 \leq x \leq 0.25) showing that this paradigm is wrong. Instead we find a microscopic coexistence of the two forms of order. A competition of magnetism and superconductivity is evident from a significant reduction of the …
Finding of unconventional superconductivity (USC) in FeSe in an electronic "normal" state with broken $C_{4v}$ rotational symmetry testifies to the diversity of pairing states in Fe-based superconductors. Moreover, such USC emerges as a direct instability of a normal state without Landau Fermi liquid quasiparticles, increasingly dubbed a `strange' metal. Here, we combine inputs from a first-principles correlated electronic structure method (LDA+DMFT) and symmetry analyses to propose a novel mechanism for unconventional nodal superconductivity as a direct instability of an incoherent bad-metal …
The discovery of the interface enhanced superconductivity in the single layer film of FeSe epitaxially grown on SrTiO3 substrates has triggered a flurry of activity in the field of superconductivity. It raised the hope to find more conventional high-Tc superconductors which are purely driven by the electron-phonon interaction at ambient pressure. Here we report the experimental evidence from the measurement of scanning tunneling spectroscopy for the interface enhanced high-Tc superconductivity in the Pb thin film islands grown on SrTiO3 substrates. The superconducting energy gap of the Pb film…
On the basis of the periodic Anderson model the microscopic Ginzburg-Landau equations for heavy-fermion superconductors in the coexistence phase of superconductivity and antiferromagnetism have been derived. The obtained expressions are valid in the vicinity of quantum critical point of heavy-fermion superconductors when the onset temperatures of antiferromagnetism and superconductivity are sufficiently close to each other. It is shown that the formation of antiferromagnetic ordering causes a decrease of the critical temperature of superconducting transition and order parameter in the phase of…
Using the standard Bardeen-Cooper-Schrieffer (BCS) theory, we revise microscopic derivation of the superconductor-insulator boundary conditions for the Ginzburg-Landau (GL) model. We obtain a negative contribution to free energy in the form of surface integral. Boundary conditions for the conventional superconductor have the form $\textbf{n} \cdot \nabla ψ= \text{const} ψ$. These are shown to follow from considering the order parameter reflected in the boundary. The boundary conditions are also derived for more general GL models with higher-order derivatives and pair-density-wave states. It sh…
Microscopic gauge-invariant theory of the c-axis infrared response of bilayer cuprate superconductors and the origin of the superconductivity induced absorption bands
A consistent microscopic theory of pseudogap phenomena and novel Bose-liquid superconductivity (superfluidity) is presented, based on the fact that in high-$T_c$ cuprates and related systems the energy $\varepsilon_A$ of the effective attraction between fermions is comparable with their Fermi energy $\varepsilon_F$ and the bosonic Cooper pairs are formed above $T_c$ and then a part of such Cooper pairs condense into a Bose superfluid at $T_c$. High-$T_c$ cuprates and other systems with low Fermi energies ($\varepsilon_F\sim\varepsilon_A$) are bosonic superconductors/superfluids and exhibit pse…
The electron paramagnetic resonance study for an organic superconductor $β''$-(BEDT-TTF)$_{4}$[(H$_3$O)Ga(C$_2$O$_4$)$_3$]$\cdot$C$_6$H$_5$NO$_2$ reveals that superconductivity coexists uniformly with the charge ordered state in one material. In the charge ordered state, the interplane spin exchange is gapped, while the in-plane conductivity is not significantly modified. This anisotropic behavior is explained by the exotic charge ordered state, in which molecular-site selective carrier localization coexists with conducting carriers on other molecules. Relationship between superconductivity an…
Shortly after the Gor'kov microscopic derivation of the Ginzburg-Landau (GL) model via a small order parameter expansion in Bardeen-Cooper-Schrieffer theory of superconductivity, the derivation was carried to next-to-leading order in that parameter and its spatial derivatives. The aim was to obtain a generalized GL free energy that approximates the microscopic model better. Since 1960s, multiple works have claimed or implicitly assumed that this extended GL model corresponds to the free energy and has solutions in the form of local minima describing superconductivity, such as vortex solutions.…
Driving a conventional superconductor with an appropriately tuned classical electromagnetic field can lead to an enhancement of superconductivity via a redistribution of the quasiparticles into a more favorable non-equilibrium distribution -- a phenomenon known as the Eliashberg effect. Here we theoretically consider coupling a two-dimensional superconducting film to the quantized electromagnetic modes of a microwave resonator cavity. As in the classical Eliashberg case, we use a kinetic equation to study the effect of the fluctuating, dynamical electromagnetic field on the Bogoliubov quasipar…
The standing wave model describes the well-known phenomenon of superconductivity in a new way [1]. Starting from a new definition of superconductivity, a microscopic London relation is derived from first principles. The relation between the macroscopic electric current and the field is derived from this microscopic relation. The coherence length as function of the superfluid density is derived from the microscopic theory. The critical temperature as function of the superfluid density is thus obtained. These results are compared to the experimental work of Bozovic et. al. [2].
The close interplay between superconductivity and antiferromagnetism in several quantum materials can lead to the appearance of an unusual thermodynamic state in which both orders coexist microscopically, despite their competing nature. A hallmark of this coexistence state is the emergence of a spin-triplet superconducting gap component, called $π$-triplet, which is spatially modulated by the antiferromagnetic wave-vector, reminiscent of a pair-density wave. In this paper, we investigate the impact of these $π$-triplet degrees of freedom on the phase diagram of a system with competing antiferr…
The recent Comment by Vorontsov [arXiv:2007.13696] claims that surface pair-density-wave superconductivity with critical temperature higher than the bulk FFLO critical temperature is not supported by microscopic theory. The conclusion is reached by using an approximate semi-microscopic quasiclassical approach. Here we show that a fully microscopic approach unambiguously demonstrates the existence of surface pair-density-wave superconductivity.
Ginzburg-Landau (GL) equations and GL free energy for flux phase and superconductivity are derived microscopically from the $t-J$ model on a square lattice. Order parameter (OP) for the flux phase has direct coupling to a magnetic field, in contrast to the superconducting OP which has minimal coupling to a vector potential. Therefore, when the flux phase OP has unidirectional spatial variation, staggered currents would flow in a perpendicular direction. The derived GL theory can be used for various problems in high-$T_c$ cuprate superconductors, e.g., states near a surface or impurities, and t…
The phenomenon of oxygen incorporation induced superconductivity in iron telluride (Fe1+yTe, with antiferromagnetic (AFM) orders) is intriguing and quite different from the case of FeSe. Until now, the microscopic origin of the induced superconductivity and the role of oxygen are far from clear. Here, by combining in-situ scanning tunneling microscopy/spectroscopy (STM/STS) and x-ray photoemission spectroscopy (XPS) on oxygenated FeTe, we found physically adsorbed O2 molecules crystallized into c(2/3x2) structure as an oxygen overlayer at low temperature, which was vital for superconductivity.…
Rock-salt type niobium nitride ($δ$-NbN) is a well-known superconductor having superconducting transition temperature (Tc) $\approx$ 18\,K and a large superconducting gap $\approx$3\,meV. The Tc of $δ$-NbN thin film exhibits a large scattering irrespective of the growth conditions and lattice parameter. In this work, we investigate the atomic origin of suppression of Tc in $δ$-NbN thin film by employing combined methods of experiments and ab-initio simulations. Sputtered $δ$-NbN thin films with different disorder were analyzed through electrical resistivity and x-ray absorption spectroscopy. A…
We present a microscopic study of superconductivity in OsB2 , and discuss the origin and characteristic length scales of the superconducting state. From first-principles we show that OsB2 is characterized by three different Fermi sheets, and we prove that this fermiology complies with recent quantum-oscillation experiments. Using the found microscopic properties, and experimental data from the literature, we employ Ginzburg-Landau relations to reveal that OsB2 is a distinctly type-I superconductor with very low Ginzburg-Landau parameter kappa - a rare property among compound materials. We show…
The recent successful experimental observation of quantum anomalous Hall effect in graphene under laser irradiation demonstrates the feasibility of controlling single particle band structure by lasers. Here we study superconductivity in a Hubbard honeycomb model in the presence of an electromagnetic drive. We start with Hubbard honeycomb model in the presence of an electromagnetic field drive, both circularly and linearly polarized light and map it onto a Floquet $t$-$J$ model. We explore conditions on the drive under which one can induce superconductivity (SC) in the system. We study the Floq…
Coexistence of a new-type antiferromagnetic (AFM) state, the so-called hedgehog spin-vortex crystal (SVC), and superconductivity (SC) is evidenced by $^{75}$As nuclear magnetic resonance study on single-crystalline CaK(Fe$_{0.951}$Ni$_{0.049}$)$_4$As$_4$. The hedgehog SVC order is clearly demonstrated by the direct observation of the internal magnetic induction along the $c$ axis at the As1 site (close to K) and a zero net internal magnetic induction at the As2 site (close to Ca) below an AFM ordering temperature $T_{\rm N}$ $\sim$ 52 K. The nuclear spin-lattice relaxation rate 1/$T_1$ shows a…
Recently the evidence of the helical magnetic structure modulated along $c$-axis with the period of four lattice parameters was obtained in easy $ab$ plane ferromagnetic superconductor EuRbFe$_4$As$_4$ [K. Iida et al., Phys. Rev. B 100, 014506 (2019)]. We argue that such structure may appear due to the presence of superconductivity. In spite of the very small value of the exchange field acting on the superconducting electrons in EuRbFe$_4$As$_4$, the exchange mechanism of interaction between superconductivity and ferromagnetism could dominate over the electromagnetic one and this circumstance …
Motivated by the observation of nematic superconductivity in several systems, we revisit the problem of the leading pairing instability of two-component unconventional superconductors on the triangular lattice -- such as $(p_{x},\,p_{y})$-wave and $(d_{x^{2}-y^{2}},\,d_{xy})$-wave. Such a system has two possible superconducting states: the chiral state (e.g. $p+ip$ or $d+id$), which breaks time-reversal symmetry, and the nematic state (e.g. $p+p$ or $d+d$), which breaks the threefold rotational symmetry of the lattice. Weak-coupling calculations generally favor the chiral over the nematic supe…
