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arXiv 1804.01403cond-mat.mtrl-scicond-mat.mes-hall
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费米-狄拉克分布电子气超快形成的解码

Decoding the ultrafast formation of a Fermi-Dirac distributed electron gas

Gerald Rohde, Ankatrin Stange, Arne Müller, Marcel Behrendt, Lars-Philip Oloff, Kerstin Hanff, Thies Albert, Petra Hein, Kai Rossnagel, Michael Bauer

摘要:

利用时间分辨和角度分辨的光电子能谱学(13 fs)研究了石墨吸收7 fs强激光脉冲后形成Fermi-Dirac分布电子气的不同阶段。在激发后的第一个50 fs内,解决了一系列时间帧,其特征在于所涉及的光子,电子和声子自由度之间的不同能量和动量交换过程。实验结果表明,由于与所涉及的相互作用过程相关的不同的时间尺度,从新生的非热向热电子分布的过渡的复杂性。

英文摘要:

Time- and angle-resolved photoelectron spectroscopy with 13 fs temporal resolution is used to follow the different stages in the formation of a Fermi-Dirac distributed electron gas in graphite after absorption of an intense 7 fs laser pulse. Within the first 50 fs after excitation a sequence of time frames is resolved which are characterized by different energy and momentum exchange processes among the involved photonic, electronic, and phononic degrees of freedom. The results reveal experimentally the complexity of the transition from a nascent non-thermal towards a thermal electron distribution due to the different timescales associated with the involved interaction processes.

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