We investigate the Casimir free energy of a metallic film either sandwiched between two dielectric plates or in vacuum. It is shown that even for a thin film of several tens of nanometer thickness the Casimir free energy and pressure calculated with the Lifshitz theory using the Drude model and the plasma model approaches take significantly different values and can be easily discriminated. According to our results, the classical limit is already achieved for films of about 100\,nm thickness if the Drude model approach is used in calculations. In this case the classical expressions for the Casimir free energy and pressure are common for both configurations considered. If the plasma model approach is used, the classical limit is not achieved for any film thickness. Instead, the Casimir free energy and pressure are decreasing exponentially to zero. When the plasma frequency goes to infinity, the Casimir free energy obtained using the Drude model approach goes to a nonzero limit in contradiction with expectations. If the plasma model approach is used the free energy of metallic film goes to zero in the limit of infinitely large plasma frequency. All analytic results are accompanied by numerical computations performed for a Au film and sapphire plates. The possibilities to observe the predicted effects discriminating between the Drude and plasma model approaches are discussed.
The Casimir force is calculated between Au thin films that are described by a Drude model with a frequency dependent damping function. The model parameters are obtained from available experimental data for Au thin films. Two cases are considered; annealed and nonannealed films that have a different damping function. Compared with the calculations using a Drude model with a constant damping parameter, we observe changes in the Casimir force of a few percent. This behavior is only observed in films of no more than 300 $Å$ thick.
We compute the Casimir interaction between a plane and a sphere, the configuration employed in the most precise experiments. The scattering formula is developed by taking a suitably chosen plane-wave and multipole basis and is valid for arbitrary values of the sphere radius, inter-plate distance, temperature and arbitrary dielectric functions for both sphere and plate. Our analytical and numerical results for metallic surfaces show a non-trivial interplay between the effects of curvature, temperature, finite conductivity and dissipation.
We give a rigorous analytical derivation of low-temperature behavior of the Casimir entropy in the framework of the Lifshitz formula combined with the Drude dielectric function. An earlier result that the Casimir entropy at zero temperature is not equal to zero and depends on the parameters of the system is confirmed, i.e. the third law of thermodynamics (the Nernst heat theorem) is violated. We illustrate the resolution of this thermodynamical puzzle in the context of the surface impedance approach by several calculations of the thermal Casimir force and entropy for both real metals and diele…
Analytic expressions that describe Casimir interactions over the entire range of separations have been limited to planar surfaces. Here we derive analytic expressions for the classical or high-temperature limit of Casimir interactions between two spheres (interior and exterior configurations), including the sphere-plane geometry as a special case, using bispherical coordinates. We consider both Dirichlet boundary conditions and metallic boundary conditions described by the Drude model. At short distances, closed-form expansions are derived from the exact result, displaying an intricate structu…
We derive an exact analytic expression for the high-temperature limit of the Casimir interaction between two Drude spheres of arbitrary radii. Specifically, we determine the Casimir free energy by using the scattering approach in the plane-wave basis. Within a round-trip expansion, we are led to consider the combinatorics of certain partitions of the round trips. The relation between the Casimir free energy and the capacitance matrix of two spheres is discussed. Previously known results for the special cases of a sphere-plane geometry as well as two spheres of equal radii are recovered. An asy…
We calculate the Casimir force between a Ge plate and a Ge spherical lens with neglected and included free charge carriers. Computations with included carriers are performed using the Drude, plasma, and diffusion models. It is shown that the plasma and the Drude models lead to almost identical computational results, while the results obtained using the diffusion model are sandwiched between those obtained with neglected charge carriers and with charge carriers described by the plasma or Drude models.
In view of the current discussion on the subject, an effort is made to show very accurately both analytically and numerically how the Drude dispersive model, assuming the relaxation is nonzero at zero temperature (which is the case when impurities are present), gives consistent results for the Casimir free energy at low temperatures. Specifically, we find that the free energy consists essentially of two terms, one leading term proportional to T^2, and a next term proportional to T^{5/2}. Both these terms give rise to zero Casimir entropy as T -> 0, thus in accordance with Nernst's theorem.
We calculate the Casimir force and its gradient between a spherical and a planar gold surface. Significant numerical improvements allow us to extend the range of accessible parameters into the experimental regime. We compare our numerically exact results with those obtained within the proximity force approximation (PFA) employed in the analysis of all Casimir force experiments reported in the literature so far. Special attention is paid to the difference between the Drude model and the dissipationless plasma model at zero frequency. It is found that the correction to PFA is too small to explai…
A recent experiment [J. L. Garrett, D. A. T. Somers, and J. N. Munday, Phys. Rev. Lett {\bf 120}, 040401 (2018)] measured for the first time the gradient of the Casimir force between two gold spheres in vacuum at room temperature, and placed a bound on the magnitude of the deviation of the measured force from the proximity force approximation (PFA). The present work extends a previous theoretical analysis of this experiment [G. Bimonte, Phys. Rev. D {\bf 97}, 085011 (2018)], by analyzing in detail how the magnitude of the deviation from PFA is affected by the inclusion or neglect of ohmic diss…
We derive an analytic behavior of the Casimir free energy, entropy and pressure of metallic films in vacuum at low temperature. It is shown that this behavior differs significantly depending on whether the plasma or the Drude model is used to describe the dielectric properties of film metal. For metallic films described by the lossless plasma model the thermal corrections to the Casimir energy and pressure drop to zero exponentially fast with increasing film thickness. There is no classical limit in this case. The Casimir entropy satisfies the Nernst heat theorem. For metallic films with perfe…
For the first time, we have studied the impact of magnetic polarizability of a neutral metallic particle on the dynamical Casimir-Polder force, when the particle is uniformly moving with relativistic velocity parallel to the surface of an ideally conducting plate. The material properties of particle are taken into account within the Drude model approach.
We describe a Casimir apparatus based on a differential force measurement between a Au-coated sphere and a planar slab divided in two regions, one of which is made of high-resistivity (dielectric) Si, and the other of Au. The crucial feature of the setup is a semi-transparent plane parallel conducting over-layer, covering both regions. The setup offers two important advantages over existing Casimir setups. On one hand it leads to a large amplification of the difference between the Drude and the plasma prescriptions that are currently used to compute the thermal Casimir force. On the other hand…
We discuss theoretical predictions for the thermal Casimir force and compare them with available experimental data. Special attention is paid to the recent claim of the observation of that effect, as predicted by the Drude model approach. We show that this claim is in contradiction with a number of experiments reported so far. We suggest that the experimental errors, as reported in support of the observation of the thermal Casimir force, are significantly underestimated. Furthermore, the experimental data at separations above $3\,μ$m are shown to be in agreement not with the Drude model approa…
Recently V. A. Yampol'skii, S. Savel'ev, Z. A. Mayselis, S. S. Apostolov, and F. Nori [Phys. Rev. Lett., v.101, 096803 (2008),arXiv:0712.1395] claimed that the Casimir force between a thin metal film described by the Drude model and an ideal metal semispace can decrease with temperature whereas for bulk samples the Casimir force increases with temperature. On this basis the experimental observation of the decreasing temperature dependence of the Casimir force magnitude between a film and a bulk ideal metal was proposed. We demonstrate that, contrary to what is claimed by the authors, the magni…
An extended Drude model, termed as the Gurzhi model, which takes into account the electron-phonon and electron-electron interactions, is applied to calculate the Casimir force between two metallic plates. It is shown that although the dielectric permittivity of the Gurzhi model has a first order pole in the upper half-plane of complex frequencies and, thus, violates the causality principle, it can be used in a restricted frequency interval in combination with the experimental permittivity determined by the optical data for the complex index of refraction. The imaginary part of the Gurzhi diele…
We perform detailed comparison of the experimental data of the experiment on the determination of the Casimir pressure between two parallel Au plates with the theoretical values computed using the Lifshitz formula at zero temperature. Computations are done using the optical data for the complex index of refraction of Au extrapolated to low frequencies by means of the Drude model with both most often used and other suggested Drude parameters. It is shown that the experimental data exclude the Lifshitz formula at zero temperature at a 70% confidence level if the Drude model with most often used …
The Casimir interactions in the solid-liquid-solid systems as a function of separation distance have been studied by the Lifshitz theory. The dielectric permittivity functions for a wide range of materials are described by Drude, Drude-Lorentz and oscillator models. We find that the Casimir forces between gold and silica or MgO materials are both the repulsive and attractive. We also find the stable forms for the systems. Our studies would provide a good guidance for the future experimental studies on the dispersion interactions.
We calculate the Casimir energy and entropy for two spheres described by the perfect metal model, plasma model, and Drude model in the large separation limit. We obtain nonmonotonic behavior of the Helmholtz free energy with separation and temperature for the perfect metal and plasma models, leading to parameter ranges with negative entropy, and also nonmonotonic behavior of the entropy with temperature and the separation between the spheres. This nonmonotonic behavior has not been found for Drude model. The appearance of this anomalous behavior of the entropy is discussed as well as its therm…
The situation with the temperature corrections to the Casimir force between real metals of finite conductivity is reported. It is shown that the plasma dielectric function is well adapted to the Lifshitz formula and leads to reasonable results for real conductors. The Drude dielectric function which describes media with dissipation is found not to belong to the application range of the Lifshitz formula at nonzero temperature. For Drude metals the special modification of the zero-frequency term of this formula is suggested. The contradictory results on the subject in recent literature are analy…
We derive analytically the asymptotic behavior of the Casimir interaction between a sphere and a plate when the distance between them, $d$, is much smaller than the radius of the sphere, $R$. The leading order and next-to-leading order terms are derived from the exact formula for the Casimir interaction energy. They are found to depend nontrivially on the dielectric functions of the objects. As expected, the leading order term coincides with that derived using the proximity force approximation. The result on the next-to-leading order term complements that found by Bimonte, Emig and Kardar [App…
We demonstrate the Casimir interaction between two ferromagnetic boundary surfaces using the dynamic atomic force microscope. The experimental data are found to be in excellent agreement with the predictions of the Lifshitz theory for magnetic boundary surfaces combined with the plasma model approach. It is shown that for magnetic materials the role of hypothetical patch potentials is opposite to that required for reconciliation of the data with the Drude model.
We study the Casimir interaction between a dielectric nanosphere and a metallic plane, using the multiple scattering theory. Exact results are obtained with the dielectric described by a Sellmeier model and the metal by a Drude model. Asymptotic forms are discussed for small spheres, large or small distances. The well-known Casimir-Polder formula is recovered at the limit of vanishingly small spheres, while an expression better behaved at small distances is found for any finite value of the radius. The exact results are of particular interest for the study of quantum states of nanospheres in t…
Recently J.S. Hoye, I.Brevik, J.B. Aarseth, and K.A. Milton [Phys. Rev. E v.67, 056116 (2003); quant-ph/0212125] proposed that if the Lifshitz formula is combined with the Drude model, the transverse electric zero mode does not contribute to the result for real metals and there arises a linear temperature correction to the Casimir force at small temperatures. The authors claim that in spite of the fact that the Casimir entropy in their approach is negative, the Nernst heat theorem is satisfied. In the present Comment we show that the authors' conclusion regarding the Nernst heat theorem is in …
We examine the Casimir free energy and pressure of magnetic metal films, which are free-standing in vacuum, sandwiched between two dielectric plates, and deposited on either nonmagnetic or magnetic metallic plates. All calculations are performed using both the Drude and plasma model approaches to the Lifshitz theory. According to our results, the Casimir free energies and pressures calculated using both theoretical approaches are significantly different in the magnitude and sign even for thin films of several tens of nanometers thickness. Thus, for the Ni film of 47\,nm thickness deposited on …
It is well known that the Casimir force calculated at large separations using the Lifshitz theory differs by a factor of 2 for metals described by the Drude or plasma models. We argue that this difference is entirely determined by the contribution of transverse electric (s) evanescent waves. Taking into account that there is a lack of experimental information on the electromagnetic response of metals to low-frequency evanescent waves, we propose an experiment on measuring the magnetic field of an oscillating magnetic dipole spaced in vacuum above a thick metallic plate. According to our result…
It was recently found that thermodynamic anomalies which arise in the Casimir effect between metals described by the Drude model can be attributed to the interaction of fluctuating Foucault (or eddy) currents [Phys. Rev. Lett. 103, 130405 (2009)]. We show explicitly that the two leading terms of the low-temperature correction to the Casimir free energy of interaction between two plates, are identical to those pertaining to the Foucault current interaction alone, up to a correction which is very small for good metals. Moreover, a mode density along real frequencies is introduced, showing that t…
Zero-frequency Casimir theory is analyzed from different viewpoints, focusing on the Drude-plasma issue that turns up when one considers thermal corrections to the Casimir force. The problem is that the plasma model, although leaving out dissipation in the material, apparently gives the best agreement with recent experiments. We consider a dielectric plate separated from a dielectric half-space by a vacuum gap, both media being similar. We consider the following categories: (1) Making use of the statistical mechanical method developed by Høye and Brevik (1998), implying that the quantized elec…
We present results on the determination of the differential Casimir force between an Au-coated sapphire sphere and the top and bottom of Au-coated deep silicon trenches performed by means of the micromechanical torsional oscillator in the range of separations from 0.2 to 8 $\upmu$m. The random and systematic errors in the measured force signal are determined at the 95\% confidence level and combined into the total experimental error. The role of surface roughness and edge effects is investigated and shown to be negligibly small. The distribution of patch potentials is characterized by Kelvin p…
The analytic expressions for the free energy and entropy of the Casimir-Polder interaction between a polarizable and magnetizable atom and a graphene sheet are found in the limiting case of low temperature. In so doing, the response of graphene to electromagnetic fluctuations is described in the framework of the Dirac model by means of the polarization tensor in (2+1)-dimensional space-time. It is shown that the dominant contribution to the low-temperature behavior is given by an explicit dependence of the polarization tensor on temperature as a parameter. We demonstrate that the Lifshitz theo…
We extend our approach to the Casimir effect between absorbing dielectric multilayers [M. S. Tomas, Phys. Rev. A 66, 052103 (2002)] to magnetodielectric systems. The resulting expression for the force is used to numerically explore the effect of the medium dispersion on the attractive/repulsive force in a metal-magnetodielectric system described by the Drude-Lorentz permittivities and permeabilities.
We derive perturbation analytic expressions for the Casimir free energy and entropy between two dissimilar ferromagnetic plates which are applicale at arbitrarily low temperature. The dielectric properties of metals are described using either the nondissipative plasma model or the Drude model taking into account the dissipation of free charge carriers. Both cases of constant and frequency-dependent magnetic permeability are considered. It is shown that for ferromagnetic metals described by the plasma model the Casimir entropy goes to zero when the temperature vanishes, i.e., the Nernst heat th…
We study the Casimir interaction in the plane-sphere geometry in the classical limit of high temperatures. In this limit, the finite conductivity of the metallic plates needs to be taken into account. For the Drude model, the classical Casimir interaction is nevertheless found to be independent of the conductivity so that it can be described by a single universal function depending only on the aspect ratio $x=L/R$ where $L$ is the interplate distance and $R$ the sphere radius. This universal function differs from the one found for perfect reflectors and is in principle amenable to experimental…
Differential force measurements between spheres coated with either nickel or gold and rotating disks with periodic distributions of nickel and gold are reported. The rotating samples are covered by a thin layer of titanium and a layer of gold. While titanium is used for fabrication purposes, the gold layer (nominal thicknesses of 21, 37, 47 and 87 nm) provides an isoelectronic environment, and is used to nullify the electrostatic contribution but allow the passage of long wavelength Casimir photons. A direct comparison between the experimental results and predictions from Drude and plasma mode…
We investigate the thermodynamical aspects of the Casimir effect in the case of plane parallel plates made of real metals. The thermal corrections to the Casimir force between real metals were recently computed by several authors using different approaches based on the Lifshitz formula with diverse results. Both the Drude and plasma models were used to describe a real metal. We calculate the entropy density of photons between metallic plates as a function of the surface separation and temperature. Some of these approaches are demonstrated to lead to negative values of entropy and to nonzero en…
We use the extended Lifshitz theory to study the behaviors of the Casimir forces between finite-thickness effective medium slabs. We first study the interaction between a semi-infinite Drude metal and a finite-thickness magnetic slab with or without substrate. For no substrate, the large distance $d$ dependence of the force is repulsive and goes as $1/d^5$; for the Drude metal substrate, a stable equilibrium point appears at an intermediate distance which can be tuned by the thickness of the slab. We then study the interaction between two identical chiral metamaterial slabs with and without su…
We investigate the Casimir force between two dissimilar plane mirrors the material properties of which are described by Drude or Lorentz models. We calculate analytically the short and long distance asymptote of the force and relate its behavior to the influence of interacting surface plasmons. In particular we discuss conditions under which Casimir repulsion could be achieved.
The low-temperature asymptotic expressions for the Casimir interaction between two real metals described by Leontovich surface impedance are obtained in the framework of thermal quantum field theory. It is shown that the Casimir entropy computed using the impedance of infrared optics vanishes in the limit of zero temperature. By contrast, the Casimir entropy computed using the impedance of the Drude model attains at zero temperature a positive value which depends on the parameters of a system, i.e., the Nernst heat theorem is violated. Thus, the impedance of infrared optics withstands the ther…
Quantum theory predicts the existence of the Casimir force between macroscopic bodies, due to the zero-point energy of electromagnetic field modes around them. This quantum fluctuation-induced force has been experimentally observed for metallic and semiconducting bodies, although the measurements to date have been unable to clearly settle the question of the correct low-frequency form of the dielectric constant dispersion (the Drude model or the plasma model) to be used for calculating the Casimir forces. At finite temperature a thermal Casimir force, due to thermal, rather than quantum, fluct…
We present theoretical calculations of the Casimir force for Au thin films near the insulator-conductor transition that has been observed experimentally. The dielectric function of the Au thin films is described by the Drude-Smith model. The parameters needed to model the dielectric function such as the relaxation time, plasma frequency and the backscattering constant depend on the thickness of the film. The Casimir force decreases as the film thickness decreases until it reaches a minimum after which the force increases again. The minimum of the force coincides with the critical film thicknes…
We carefully re-examine the conditions of validity for the consistent derivation of the Lifshitz-Matsubara sum formula for the Casimir pressure between metallic plane mirrors. We recover the usual expression for the lossy Drude model, but not for the lossless plasma model. We give an interpretation of this new result in terms of the modes associated with the Foucault currents which play a role in the limit of vanishing losses, in contrast to common expectations.
We investigate the Casimir force acting between real metals at nonzero temperature. It is shown that the zero-frequency term of Lifshitz formula has interpretation problem in the case of real metal described by Drude model. It happens because the scattering theory underlying Lifshitz formula is not well formulated when the dielectric permittivity takes account of dissipation. To give the zeroth term of Lifshitz formula the definite meaning different prescriptions were used recently by different authors with diversed results. These results are shown to be improper and in disagreement with exper…
Difference between bulk material and deposited film is shown to have an appreciable influence on the Casimir force. Analysis of the optical data on gold films unambiguously demonstrates the sample dependence: the dielectric functions of the films deposited in different conditions are different on the level that cannot be ignored in high precision prediction of the force. It is argued that the precise values of the Drude parameters are crucial for accurate evaluation of the force. The dielectric function of perfect single crystalline gold is discussed. It is used to establish the upper limit on…
The Casimir free energy and pressure of thin metal films deposited on metallic plates are considered using the Lifshitz theory and the Drude and plasma model approaches to the role of conduction electrons. The bound electrons are taken into account by using the complete optical data of film and plate metals. It is shown that for films of several tens of nanometers thickness the Casimir free energy and pressure calculated using these approaches differ by hundreds and thousands percent and can be easily discriminated experimentally. According to our results, the free energy of a metal film does …
Negative entropy has been known in Casimir systems for some time. For example, it can occur between parallel metallic plates modeled by a realistic Drude permittivity. Less well known is that negative entropy can occur purely geometrically, say between a perfectly conducting sphere and a conducting plate. The latter effect is most pronounced in the dipole approximation, which is reliable when the size of the sphere is small compared to the separation between the sphere and the plate. Therefore, here we examine cases where negative entropy can occur between two electrically and magnetically pol…
The thermal Casimir force between two metallic plates is known to depend on the description of material properties. For large separations the dissipative Drude model leads to a force a factor of 2 smaller than the lossless plasma model. Here we show that the plane-sphere geometry, in which current experiment are performed, decreases this ratio to a factor of 3/2, as revealed by exact numerical and large distance analytical calculations. For perfect reflectors, we find a repulsive contribution of thermal photons to the force and negative entropy values at intermediate distances.
Based on calculations involving an idealized boundary condition, it has long been assumed that the stress on a spherical conducting shell is repulsive. We use the more realistic case of a Drude dielectric to show that the stress is attractive, matching the generic behavior of Casimir forces in electromagnetism. We trace the discrepancy between these two cases to interactions between the electromagnetic quantum fluctuations and the dielectric material.
We analyze the conditions for getting the Casimir repulsion between two nonequal plates. The force between plates with magnetic permeability defined by Drude or Lorentz models is calculated. The short and long distance limits of the force are derived. The Casimir set-up with the hypothetical perfect matching metamaterial is discussed. We put into question the possibility of getting repulsion within the design of metamaterials based on metallic inclusions.
We study the lateral Casimir force between corrugated dielectric plates. We use the dielectric contrast perturbation theory [R. Golestanian, {\it Phys. Rev. Lett.} {\bf 95}, 230601, (2005)], which allows us to consider arbitrary deformations with large amplitudes. We consider sinusoidal, rectangular, and sawtooth corrugations, for samples made of silicon and gold. We use the plasma and Drude-Lorentz models for the permittivity of gold and silicon, respectively. For these geometries and materials, the lateral Casimir force is {\it not} a sinusoidal function of the relative lateral displacement …
We calculate the Casimir force between slabs of finite thickness made of intrinsic and doped silicon with different concentration of carriers and compare the results to those obtained for gold slabs. We use the Drude and the plasma models to describe the dielectric function for the carriers in doped Si. We discuss the possibility of experimentally testing the appropriateness of these models. We also investigate the influence of finite thickness on $VO_2$, which has recently been proposed for Casimir effect measurements testing the metal-insulator transition.
We investigate the thermal Casimir interaction of a suspended graphene described by the Dirac model with a plate made of dielectric or metallic materials. The reflection coefficients on graphene expressed in terms of a temperature-dependent polarization tensor are used. We demonstrate that for a graphene with nonzero mass gap parameter the Casimir free energy remains nearly constant (and the thermal correction negligibly small) over some temperature interval. For the interaction of graphene with metallic plate, the free energy is nearly the same, irrespective of whether the metal is nonmagneti…
We consider a dielectric medium with an ultraviolet behavior as it follows from the Drude model. Compared with dilute models, this has the advantage that, for large frequencies, two different media behave the same way. As a result one expects the Casimir energy to contain less divergencies than for the dilute media approximation. We show that the Casimir energy of a spherical dielectric ball contains just one divergent term, a volume one, which can be renormalized by introducing a contact term analogous to the volume energy counterterm needed in bag models. PACS: 12.20.Ds, 03.70.+k, 77.22.Ch
The physical reasons why the Drude dielectric function is not compatible with the Lifshitz formula, as opposed to the generalized plasma-like permittivity, are presented. Essentially, the problem is connected with the finite size of metal plates. It is shown that the Lifshitz theory combined with the generalized plasma-like permittivity is thermodynamically consistent.
Recently, Høye, Brevik, Ellingsen and Aarseth (quant-ph/0703174) claimed that the use of the Drude dielectric function leads to zero Casimir entropy at zero temperature in accordance with Nernst's theorem. We demonstrate that their proof is not applicable to metals with perfect crystal lattices having no impurities. Thus there is no any contradiction with previous results in the literature proving that the Drude dielectric function violates the Nernst theorem for the Casimir entropy in the case of perfect crystal lattices. We also indicate mistakes in the coefficients of their asymptotic expre…
The new approach to the theoretical description of the thermal Casimir force between real metals is presented. It uses the plasma-like dielectric permittivity that takes into account the interband transitions of core electrons. This permittivity precisely satisfies the Kramers-Kronig relations. The respective Casimir entropy is positive and vanishes at zero temperature in accordance with the Nernst heat theorem. The physical reasons why the Drude dielectric function, when substituted in the Lifshitz formula, is inconsistent with electrodynamics are elucidated. The proposed approach is the sing…
Precise optical properties of metals are very important for accurate prediction of the Casimir force acting between two metallic plates. Therefore we measured ellipsometrically the optical responses of Au films in a wide range of wavelengths from 0.14 mum to 33 mum. The films at various thickness were deposited at different conditions on silicon or mica substrates. Considerable variation of the frequency dependent dielectric function from sample to sample was found. Detailed analysis of the dielectric functions was performed to check the Kramers-Kronig consistency, and extract the Drude parame…
