We show that the energy gap induced by ferromagnetically aligned magnetic impurities on the surface of a topological insulator can be filled, due to scattering off the non-magnetic potential of the impurities. In both a continuum surface model and a three-dimensional tight-binding lattice model, we find that the energy gap disappears already at weak potential scattering as impurity resonances add spectral weight at the Dirac point. This can help explain seemingly contradictory experimental results as to the existence of a gap.
Chern insulators arguably provide the simplest examples of topological phases. They are characterized by a topological invariant and can be identified by the presence of protected edge states. In this article, we show that a local impurity in a Chern insulator induces a twofold response: bound states that carry a chiral current and a net current circulating around the impurity. This is a manifestation of broken time symmetry and persists even for an infinitesimal impurity potential. To illustrate this, we consider a Coulomb impurity in the Haldane model. Working in the low-energy long-waveleng…
Charge transport in topological insulators is primarily characterised by so-called topologically projected helical edge states, where charge carriers are correlated in spin and momentum. In principle, dissipation-less current can be carried by these edge states as backscattering from impurities and defects is suppressed as long as time-reversal symmetry is not broken. However, applied magnetic fields or underlying nuclear spin-defects in the substrate can break this time reversal symmetry. In particular, magnetic impurities lead to back-scattering by spin-flip processes. We have investigated t…
We investigate the effect of a non-magnetic donor impurity located at the surface of the SnTe topological crystalline insulator. In particular, the changes on the surface states due to a Sb impurity atom are analyzed by means of ab initio simulations of pristine and impurity-doped SnTe. Both semi-infinite and slab geometries are considered within the first-principles approach. Furthermore, minimal and Green's function continuum models are proposed with the same goal. We find that the Dirac cones are shifted down in energy upon doping; this shift strongly depends on the position of the impurity…
We consider a Kondo-like impurity interacting with fermions on a honeycomb lattice at half-filling, as in the case of graphene. We derive from the lattice model an effective one-dimensional continuum theory which has, in general, four flavors with angular momentum mixing in the presence of internode scattering processes and six couplings in the spin-isotropic case. Under particular conditions, however, it can be reduced to a single-coupling multichannel pseudogap Kondo model. We finally calculate, in the presence of an energy dependent Fermi velocity, induced by Coulomb interaction, the critic…
We show that the local in-gap Greens function of a band insulator $\mathbf{G}_0 (ε,\mathbf{k}_{\parallel},\mathbf{r}_{\perp}=0)$, with $\mathbf{r}_\perp$ the position perpendicular to a codimension-1 or -2 impurity, reveals the topological nature of the phase. For a topological insulator, the eigenvalues of this Greens function attain zeros in the gap, whereas for a trivial insulator the eigenvalues remain nonzero. This topological classification is related to the existence of in-gap bound states along codimension-1 and -2 impurities. Whereas codimension-1 impurities can be viewed as 'soft edg…
We consider the effects of impurities on topological insulators and superconductors. We start by identifying the general conditions under which the eigenenergies of an arbitrary Hamiltonian H belonging to one of the Altland-Zirnbauer symmetry classes undergo a robust zero energy crossing as a function of an external parameter which can be, for example, the impurity strength. We define a generalized root of \det H, and use it to predict or rule out robust zero-energy crossings in all symmetry classes. We complement this result with an analysis based on almost degenerate perturbation theory, whi…
We demonstrate that a quantum spin Hall current, spontaneously generated at the edge of a two-dimensional topological insulator, acts as a source of spin-pumping for a magnetic impurity with uniaxial anisotropy. One can then manipulate the impurity spin direction by means of an electrical current without using either magnetic electrodes or an external magnetic field. Furthermore we show that the unique properties of the quantum spin Hall topological state have profound effects on the inelastic electron tunneling spectrum of the impurity. For low current densities inelastic spin-flip events do …
We theoretically investigate the exchange interaction between magnetic impurities in ultrathin Bi$_2$Se$_3$ topological insulator films by taking into account the low-energy states produced by the impurities. We find that the locally induced impurity resonances strongly influence the exchange interaction between magnetic moments. In particular, we find a non-collinear alignment being more favorable than the collinear ferromagnetic alignment preferred when impurity states are ignored and only the pristine topological insulator band structure is considered. Moreover, we show that by applying of …
For atomic thin layer insulating materials we provide an exact analytic form of the two-dimensional screened potential. In contrast to three-dimensional systems where the macroscopic screening can be described by a static dielectric constant in 2D systems the macroscopic screening is non local (q-dependent) showing a logarithmic divergence for small distances and reaching the unscreened Coulomb potential for large distances. The cross-over of these two regimes is dictated by 2D layer polarizability that can be easily computed by standard first-principles techniques. The present results have st…
Prototypes of quantum impurities (QI), such as NV and SiV centers in diamond, have been recently growing in popularity due to their minimally invasive and high-resolution magnetic field sensing. Here, we focus on quantum-impurity relaxometry as a method to probe collective excitations in magnetic insulators. We develop a general framework that relates the experimentally-measurable quantum-impurity relaxation rates to the properties of a magnetic system via the noise emitted by the latter. We suggest that, when the quantum-impurity frequency lies within the spin-wave gap, quantum-impurity relax…
We study the higher-order Fermi-liquid relations of Kondo systems for arbitrary impurity-electron fillings, extending the many-body quantum theoretical approach of Yamada-Yosida. It includes partly a microscopic clarification of the related achievements based on Nozières' phenomenological description: Filippone, Moca, von Delft, and Mora [Phys.\ Rev.\ B {\bf 95}, 165404 (2017)]. In our formulation, the Fermi-liquid parameters such as the quasi-particle energy, damping, and transport coefficients are related to each other through the total vertex $Γ_{σσ';σ'σ} (ω, ω'; ω', ω)$, which may be regar…
Current-phase relation in a Josephson junction formed by putting two s-wave superconductors on the same edge of a two dimensional topological insulator is investigated. We consider the case that the junction length is finite and magnetic impurity exists. The similarity and difference with conventional Josephson junction is discussed. The current is calculated in the semiconductor picture. Both the $2π$- and $4π$-period current-phase relations ($I_{2π}(ϕ), I_{4π}(ϕ)$) are studied. There is a sharp jump at $ϕ=π$ and $ϕ=2π$ for $I_{2π}$ and $I_{4π}$ respectively in the clean junction. For $I_{2π}…
We theoretically investigate the spin resolved Friedel oscillation (FO) and quasiparticle interference (QPI) in graphene induced by an Anderson impurity. Once the impurity becomes magnetic, the resulted FO becomes spin dependent, which gives rise to a local magnetic moment oscillation with an envelop decaying as $r^{-2}$ in real space in the doping cases. Meanwhile, at half filling, the charge density and local magnetic moment will not oscillate but decay as $r^{-3}$. Such spin resolved FO has both sublattice and spin asymmetry. Interestingly, the local magnetic moment decay at half filling on…
An Anderson impurity in a Hubbard model on chains with finite length is studied using the density-matrix renormalization group (DMRG) technique. In the first place, we analyzed how the reduction of electron density from half-filling to quarter-filling affects the Kondo resonance in the limit of Hubbard repulsion U=0. In general, a weak dependence with the electron density was found for the local density of states (LDOS) at the impurity except when the impurity, at half-filling, is close to a mixed valence regime. Next, in the central part of this paper, we studied the effects of finite Hubbard…
We report a detailed study on low-frequency 1/f-noise in large-area molecular-beam epitaxy grown thin (10 nm) films of topological insulators as a function of temperature, gate voltage, and magnetic field. When the Fermi energy is within the bulk valence band, the temperature dependence reveals a clear signature of generation-recombination noise in the defect states in the bulk band gap. However, when the Fermi energy is tuned to the bulk band gap, the gate voltage dependence of noise shows that the resistance fluctuations in surface transport are caused by correlated mobility-number density f…
Injection of spins into semiconductors is essential for the integration of the spin functionality into conventional electronics. Insulating layers are often inserted between ferromagnetic metals and semiconductors for obtaining an efficient spin injection, and it is therefore crucial to distinguish between signatures of electrical spin injection and impurity-driven effects in the tunnel barrier. Here we demonstrate an impurity-assisted tunneling magnetoresistance effect in nonmagnetic-insulator-nonmagnetic and ferromagnetic-insulator-nonmagnetic tunnel barriers. In both cases, the effect refle…
The ground state properties of a high spin magnetic impurity and its interaction with an electronic spin are probed via Andreev reflection. We see that through the charge and spin conductance one can effectively estimate the interaction strength, the ground state spin and magnetic moment of any high spin magnetic impurity. We show how a high spin magnetic impurity at the junction between a normal metal and superconductor can contribute to superconducting spintronics applications. Particularly, while spin conductance is absent below the gap for Ferromagnet-Insulator-Superconductor junctions we …
By generalizing the Kubo-Streda formula for calculating electrical conductivities to the thermoelectric coefficients, we theoretically study the anomalous Nernst effect (ANE) on the surface of a topological insulator induced by a finite concentration of magnetic impurities. The ANE is found to be modulated by the impurity scattering and thermal fluctuations, simultaneously, and so exhibits rich structures in the energy space. While the anomalous Hall conductivity is half-integer quantized with the Fermi level across the magnetic-impurity-induced gap, the anomalous Nernst signal (ANS) is fully …
Traditional ionic/covalent compound insulators arise from a commensuration between electron count and system volume. On the other hand, conventional topological insulators, outside of quantum hall effect systems, do not typically display such a commensuration. Tnstead, they can undergo a phase transition to a trivial insulator that preserves the electron filling. Nevertheless, in some crystalline insulators, termed filling-enforced quantum band insulators (feQBIs), electron filling can dictate nontrivial topology in the insulating ground state. Currently, little is known about the relation bet…
Scanning tunneling spectroscopic studies of Bi2Se3 epitaxial films on Si (111) substrates reveal highly localized unitary impurity resonances associated with non-magnetic quantum impurities. The strength of the resonances depends on the energy difference between the Fermi level ({E_F}) and the Dirac point ({E_D}) and diverges as {E_F} approaches {E_D}. The Dirac-cone surface state of the host recovers within ~ 2Å spatial distance from impurities, suggesting robust topological protection of the surface state of topological insulators against high-density impurities that preserve time reversal s…
We study the ground-state entanglement properties of nanostructured Kondo systems consisting of a pair of impurity spins coupled to a background of confined electrons. The competition between the RKKY-like coupling and the Kondo effect determines the development of quantum correlations between the different parts of the system. A key element is the electronic filling due to confinement. An even electronic filling leads to results similar to those found previously for extended systems, where the properties of the reduced impurity-spin subsystem are uniquely determined by the spin correlation fu…
We extend the microscopic Fermi-liquid theory for the Anderson impurity [Phys.\ Rev.\ B {\bf 64}, 153305 (2001)] to explore non-equilibrium transport at finite magnetic fields. Using the Ward identities in the Keldysh formalism with the analytic and anti-symmetric properties of the vertex function, the spin-dependent Fermi-liquid corrections of order $T^2$ and $(eV)^2$ are determined at low temperatures $T$ and low bias voltages $eV$. Away from half-filling, these corrections can be expressed in terms of the linear and non-linear static susceptibilities which represent the two-body and three-b…
The influence of individual impurities of Fe on the electronic properties of topological insulator Bi$_2$Se$_3$ is studied by Scanning Tunneling Microscopy. The microscope tip is used in order to remotely charge/discharge Fe impurities. The charging process is shown to depend on the impurity location in the crystallographic unit cell, on the presence of other Fe impurities in the close vicinity, as well as on the overall doping level of the crystal. We present a qualitative explanation of the observed phenomena in terms of tip-induced local band bending. Our observations evidence that the spec…
We calculate the anomalous Hall conductivity $σ_{xy}$ of the surface states {in cubic topological Kondo insulators}. We consider a generic model for the surface states with three Dirac cones on the (001) surface. The Fermi velocity, the Fermi momentum and the Zeeman energy in different Dirac pockets may be unequal. The microscopic impurity potential mediates mixed intra and interband extrinsic scattering processes. Our calculation of $σ_{xy}$ is based on the Kubo-Streda diagrammatic approach. It includes diffractive skew scattering contributions originating from the rare two-impurity complexes…
Using a three-dimensional microscopic lattice model of a strong topological insulator (TI) we study potential impurities and vacancies in surface and subsurface positions. For all impurity locations we find impurity-induced resonance states with energy proportional to the inverse of the impurity strength, although the impurity strength needed for a low-energy resonance state increases with the depth of the impurity. For strong impurities and vacancies as deep as 15 layers into the material, resonance peaks will appear at and around the Dirac point in the surface energy spectrum, splitting the …
We address the electronic structure of the surface states of topological insulator thin films with embedded local non-magnetic and magnetic impurities. Using the $T$-matrix expansion of the real space Green's function, we derive the local density of electrons states and corresponding spin resolved densities. We show that the effects of the impurities can be tuned by applying an electric field between the surface layers. The emerging magnetic states are expected to play an important role both in ferromagnetic mechanism of magnetic topological insulators as well as in its transport properties. I…
We consider periodically driven potential impurities coupled to the surface states of a two-dimensional topological insulator. The problem is addressed by means of two models, out which the first model is an effective continuum Hamiltonian for the surface states, whereas the Kane-Mele lattice model is our second approach. While both models result in drastic changes in the local density of electron states with increasing amplitude and frequency of the driving field, the linearly low energy local density of electron states remains in the continuum model, however, with an increased Fermi velocity…
We calculate exact zero-temperature real space properties of a substitutional magnetic impurity coupled to the edge of a zigzag silicene-like nanoribbon. Using a Lanczos transformation [Phys. Rev. B 91, 085101 (2015)] and the density matrix renormalization group method, we obtain a realistic description of stanene and germanene that includes the bulk and the edges as boundary one-dimensional helical metallic states. Our results for substitutional impurities indicate that the development of a Kondo state and the structure of the spin correlations between the impurity and the electron spins in t…
A two-dimensional superconductor (SC) on surfaces of topological insulators (TIs) is a mixture of s-wave and helical p-wave components when induced by s-wave interactions, since spin and momentum are correlated. On the basis of the Abrikosov-Gor'kov theory, we reveal that unconventional SCs on the surfaces of TIs are stable against time-reversal symmetric (TRS) impurities within a region of small impurity concentration. Moreover, we analyze the stability of the SC on the surfaces of TIs against impurities beyond the perturbation theory by solving the real-space Bogoliubov-de Gennes equation fo…
The massless Dirac electrons found at topological insulator surfaces are thought to be influenced very little by weak, non-magnetic disorder. However, a resonance effect of strongly perturbing non-magnetic impurities has been theoretically predicted to change the dispersion and physical nature of low-energy quasiparticles, resulting in unique particle-like states that lack microscopic translational symmetry. Here we report the direct observation of impurities reshaping the surface Dirac cone of the model 3D topological insulator Bi2Se3. For the first time, a pronounced kink-like dispersion fea…
We study weak anti-localization (WAL) effect in topological insulator Bi2Te3 thin films at low temperatures. Two-dimensional WAL effect associated with surface carriers is revealed in the tilted magnetic field dependence of magneto-conductance. Our data demonstrates that the observed WAL is robust against deposition of non-magnetic Au impurities on the surface of the thin films. But it is quenched by deposition of magnetic Fe impurities which destroy the pi Berry's phase of the topological surface states. The magneto-conductance data of a 5 nm Bi2Te3 film suggests that a crossover from symplec…
Motivated by recent scanning tunneling microscopy experiments on surfaces of Bi$_{1-x}$Sb$_{x'}$\cite{yazdanistm,gomesstm} and Bi$_2$Te$_3$,\cite{kaptunikstm,xuestm} we theoretically study the electronic structure of a 3-dimensional (3D) topological insulator in the presence of a local impurity or a domain wall on its surface using a 3D lattice model. While the local density of states (LDOS) oscillates significantly in space at energies above the bulk gap, the oscillation due to the in-gap surface Dirac fermions are very weak. The extracted modulation wave number as a function of energy satisf…
We theoretically address the impact of a random distribution of non-magnetic impurities on the surface states formed at the interface between a trivial and a topological insulator. The interaction of electrons with the impurities is accounted for by a separable pseudo-potential method that allows us to obtain closed expressions for the density of states. Spectral properties of surface states are assessed by means of the Green's function averaged over disorder realizations. For comparison purposes, the configurationally averaged Green's function is calculated by means of two different self-cons…
We present a microscopic Fermi-liquid view on the low-energy transport through an Anderson impurity with $N$ discrete levels, at arbitrary electron filling $N_d$. It is applied to nonequilibrium current fluctuations, for which the two-quasiparticle collision integral and the three-body correlations that determine the quasiparticle energy shift play important roles. Using the numerical renormalization group up to $N=6$, we find that for strong interactions the three-body fluctuations are determined by a single parameter other than the Kondo energy scale in a wide filling range $1 \lesssim N_d \…
While standard scaling arguments show that a system of non-interacting electrons in two dimensions and in the presence of uncorrelated disorder is insulating, in this work we discuss the case where inter-impurity correlations are included. We find that for point-like impurities and an infinite inter-impurity correlation length a mobility edge exists in 2D even if the individual impurity potentials are random. In the uncorrelated system we recover the scaling results, while in the intermediate regime for length scales comparable to the correlation length, the system behaves like a metal but wit…
We determine conditions on the filling of electrons in a crystalline lattice to obtain the equivalent of a band insulator -- a gapped insulator with neither symmetry breaking nor fractionalized excitations. We allow for strong interactions, which precludes a free particle description. Previous approaches that extend the Lieb-Schultz-Mattis argument invoked spin conservation in an essential way, and cannot be applied to the physically interesting case of spin-orbit coupled systems. Here we introduce two approaches, the first an entanglement based scheme, while the second studies the system on a…
Topological insulators (TIs) are said to be stable against non-magnetic impurity scattering due to suppressed backscattering in the Dirac surface states. We solve a lattice model of a three-dimensional TI in the presence of strong potential impurities and find that both the Dirac point and low-energy states are significantly modified: low-energy impurity resonances are formed that produce a peak in the density of states near the Dirac point, which is destroyed and split into two nodes that move off-center. The impurity-induced states penetrate up to 10 layers into the bulk of the TI. These fin…
We study the low-energy behavior of the vertex function of a single Anderson impurity away from half-filling for finite magnetic fields, using the Ward identities with careful consideration of the anti-symmetry and analytic properties. The asymptotic form of the vertex function $Γ_{σσ';σ'σ}^{}(iω,iω';iω',iω)$ is determined up to terms of linear order with respect to the two frequencies $ω$ and $ω'$, as well as the $ω^2$ contribution for anti-parallel spins $σ'\neq σ$ at $ω'=0$. From these results, we also obtain a series of the Fermi-liquid relations beyond those of Yamada-Yosida. The $ω^2$ re…
Band structures of topological insulators are characterized by non-local topological invariants. Consequently, proposals for the experimental detection using local probes are rare. A recent paper [Slager et al., Phys. Rev. B 92, 085126 (2015)] has argued, based on theoretical results for a particular class of models, that insulators with topologically trivial and non-trivial band structures in two space dimensions display a qualitatively different response to point-like impurities. Here we present a comprehensive investigation of the impurity response of a large set of models of non-interactin…
We solve the problem of a magnetic impurity coupled to a U(1) quantum spin liquid with spinon Fermi surface and compute the impurity spectral function. Using the slave rotor mean field approach combined with gauge field fluctuations, we find that a peak located at the top of the lower Hubbard band and one at the bottom of the upper Hubbard band can emerge in the impurity spectral function. The peaks at the Hubbard band edges arise from the gauge field fluctuations induced spinon chargon binding inside the spinon Kondo screening cloud of the magnetic impurity. For a magnetic impurity embedded i…
We theoretically study an emergent SU(2) symmetry which is suggested by recent magneto-transport measurements, carried out near two electrons filling of a carbon nanotube quantum dot. It emerges in the case where the spin and orbital Zeeman splittings cancel each other out for two of the one-particle dot levels among four. Using the Wilson numerical renormalization group, we show that a crossover from the SU(4) to SU(2) Fermi-liquid behavior occurs at two impurity-electrons filling as magnetic field increases. We also find that the quasiparticles are significantly renormalized as the remaining…
Quantum spin-orbital liquids are elusive strongly correlated states of matter that emerge from quantum frustration between spin and orbital degrees of freedom. A promising route towards the observation of those states is the creation of artificial Mott insulators where antiferromagnetic correlations between spins and orbitals can be designed. We show that Coulomb impurity lattices on the surface of gapped honeycomb substrates, such as graphene on SiC, can be used to simulate SU(4) symmetric spin-orbital lattice models. We exploit the property that massive Dirac fermions form mid-gap bound stat…
Impurity-induced thermal crossover in fractional Chern insulators
City University of Hong Kong（香港城市大学）；University of Maryland（马里兰大学）；Joint Quantum Institute（联合量子研究所）；Kavli Institute for Theoretical Physics（卡弗里理论物理研究所）；University of California, Santa Barbara（加州大学圣塔芭芭拉分校）
Anyon-Impurity Bound States in Quantum-Engineered Fractional Chern Insulators
International Solvay Institutes（国际索尔维研究所）；Center for Nonlinear Phenomena and Complex Systems, Université Libre de Bruxelles（布鲁塞尔自由大学非线性现象与复杂系统中心）；Department of Physics and Arnold Sommerfeld Center for Theoretical Physics (ASC), Ludwig-Maximilians-Universität München（慕尼黑大学物理系及阿诺德·索末菲理论物理中心）；Munich Center for Quantum Science and Technology (MCQST)（慕尼黑量子科学与技术中心）
We prove the existence of low energy excitations in insulating systems at general filling factor under certain conditions, and discuss in which cases these may be identified as topological excitations. This proof is based on previously proven locality results. In the case of half-filling it provides a significantly shortened proof of the recent higher dimensional Lieb-Schultz-Mattis theorem.
We compute the multifractal spectra associated to local density of states (LDOS) fluctuations due to weak quenched disorder, for a single Dirac fermion in two spatial dimensions. Our results are relevant to the surfaces of Z_2 topological insulators such as Bi_2Se_3 and Bi_2Te_3, where LDOS modulations can be directly probed via scanning tunneling microscopy. We find a qualitative difference in spectra obtained for magnetic versus non-magnetic disorder. Randomly polarized magnetic impurities induce quadratic multifractality at first order in the impurity density; by contrast, no operator exhib…
We investigate the ground state and quantum dynamics of an interacting bosonic chain with the nonreciprocal hopping. In sharp contrast to its Hermitian counterpart, the ground state can support Mott insulators in systems with noninteger filling due to the competition between nonreciprocal hopping and the on-site interaction. For the quantum dynamics, conservation laws for non-Hermitian systems manifest a stark difference from their Hermitian counterpart. In particular, for any Hermitian operator that commutes with the Hamiltonian operator, its expectation value is guaranteed to be nonconserved…
We present a combined experimental and theoretical study of twisted double bilayer graphene with twist angles between 1° and 1.35°. Consistent with moiré band structure calculations, we observe insulators at integer moiré band fillings one and three, but not two. An applied transverse electric field separates the first moiré conduction band from neighbouring bands, and favors the appearance of correlated insulators at 1/4, 1/2, and 3/4 band filling. Insulating states at 1/4 and 3/4 band filling emerge only in a parallel magnetic field (B_{||}), whereas the resistance at half band filling is we…
