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arXiv 1003.0553cond-mat.str-elcond-mat.other
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NMR ~(61)Ni在La2NiO4 .17和K2NiF4中的磁化率- Knight-shift关系

The susceptibility - Knight-shift relation in La2NiO4.17 and K2NiF4 by 61Ni NMR

J. J. van der Klink, H. B. Brom

摘要:

用~(61)Ni-核磁共振(~(61)Ni-NMR)研究了空穴掺杂高温超导体La{2-x} SrxCuO_4的近亲La_2NiO_(4.17)中的NiO_4片晶。掺杂和未掺杂的斑被区分的NMR共振的移位,导致一个小的线分裂,这几乎不依赖于温度或磁化率。这种效应的微小性是Schussler-Langenheine等人推断的孔洞位置的额外证据,物理修订版信函95,156402(2005)。随着温度的降低,线宽的增加显示了局部场的重新分布,与电荷密度波或条纹的形成相一致。为了比较,我们特别研究了所有平面反铁磁体的祖母K2 NiF在顺磁状态下使用天然丰富的61 Ni。在两个二维化合物的超精细场似乎是非常小的,这是很好地解释了超(转移)超精细相互作用。在K2 NiF 4的磁化率和奈特位移的温度依赖性不能被带到一个简单的标度曲线。这种独特的功能是归因于这两个参数的相关性的不同的敏感性。

英文摘要:

The NiO4 plaquettes in La2NiO4.17, a cousin of the hole-doped high-temperature superconductor La{2-x}SrxCuO4, have been studied by 61Ni-NMR in 14 T in a single crystal enriched in 61Ni. Doped and undoped plaquettes are discriminated by the shift of the NMR resonance, leading to a small line splitting, which hardly depends on temperature or susceptibility. The smallness of the effect is additional evidence for the location of the holes as deduced by Schussler-Langenheine et al., Phys. Rev. Lett. 95, 156402 (2005). The increase in linewidth with decreasing temperature shows a local field redistribution, consistent with the formation of charge density waves or stripes. For comparison, we studied in particular the grandmother of all planar antiferromagnets K2NiF in the paramagnetic state using natural abundant 61Ni. The hyperfine fields in both 2-dimensional compounds appear to be remarkably small, which is well explained by super(transferred) hyperfine interaction. In K2NiF4 the temperature dependence of the susceptibility and Knight shift cannot be brought onto a simple scaling curve. This unique feature is ascribed to a different sensitivity for correlations of these two parameters.

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