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arXiv 1001.3370cond-mat.mes-hall
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双层石墨烯拉曼光谱中朗道能级间跃迁的光谱特征

Spectral features due to inter-Landau-level transitions in the Raman spectrum of bilayer graphene

M. Mucha-Kruczynski, O. Kashuba, V. I. Fal'ko

摘要:

研究了入射光子能量Ω>> 1 eV时,低能电子激发对双层石墨烯拉曼光谱的贡献。从四带紧束缚模型出发,导出了一个有效的散射振幅,它可以被纳入常用的两带近似。由于高能带的影响,这种有效的散射振幅是不同的接触相互作用的振幅内的两个带模型单独获得。然后,我们计算的非弹性光散射的光谱密度的电子空穴对的激发双层石墨烯。在没有磁场的情况下,由于双层晶体中低能带的抛物线色散,这种贡献是恒定的,并且在掺杂结构中具有两倍于费米能的阈值。在外部磁场中,占主导地位的拉曼活性模式是n_{-}到n_{+}的朗道能级间跃迁,具有输入/输出光子的交叉极化。我们估计了在10 T磁场下单次n_{-}到n_{+}跃迁的量子效率为I_{ n_{-}到n_{+} }~10^{-12}。

英文摘要:

We investigate the contribution of the low-energy electronic excitations towards the Raman spectrum of bilayer graphene for the incoming photon energy Omega >> 1eV. Starting with the four-band tight-binding model, we derive an effective scattering amplitude that can be incorporated into the commonly used two-band approximation. Due to the influence of the high-energy bands, this effective scattering amplitude is different from the contact interaction amplitude obtained within the two-band model alone. We then calculate the spectral density of the inelastic light scattering accompanied by the excitation of electron-hole pairs in bilayer graphene. In the absence of a magnetic field, due to the parabolic dispersion of the low-energy bands in a bilayer crystal, this contribution is constant and in doped structures has a threshold at twice the Fermi energy. In an external magnetic field, the dominant Raman-active modes are the n_{-} to n_{+} inter-Landau-level transitions with crossed polarisation of in/out photons. We estimate the quantum efficiency of a single n_{-} to n_{+} transition in the magnetic field of 10T as I_{n_{-} to n_{+}}~10^{-12}.

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