Narrow-gap higher mobility semiconducting alloys In_{1-x}Mn_{x}Sb were synthesized in polycrystalline form and their magnetic and transport properties have been investigated. Ferromagnetic response in In_{0.98}Mn_{0.02}Sb was detected by the observation of clear hysteresis loops up to room temperature in direct magnetization measurements. An unconventional (reentrant) magnetization versus temperature behavior has been found. We explained the observed peculiarities within the frameworks of recent models which suggest that a strong temperature dependence of the carrier density is a crucial parameter determining carrier-mediated ferromagnetism of (III,Mn)V semiconductors. The correlation between magnetic states and transport properties of the sample has been discussed. The contact spectroscopy method is used to investigate a band structure of (InMn)Sb near the Fermi level. Measurements of the degree of charge current spin polarization have been carried out using the point contact Andreev reflection (AR) spectroscopy. The AR data are analyzed by introducing a quasiparticle spectrum broadening, which is likely to be related to magnetic scattering in the contact. The AR spectroscopy data argued that at low temperature the sample is decomposed on metallic ferromagnetic clusters with relatively high spin polarization of charge carriers (up to 65% at 4.2K) within a cluster.
There are two competing views of itinerant ferromagnetism, the first viewing ferromagnetism as resulting from the indirect coupling between local moments via the itinerant carrier dynamics, the so-called RKKY mechanism, while in the alternative picture, ferromagnetism results from the spin polarization of itinerant carriers by the strong atomic Hund interaction - the so-called double exchange (DE) scenario. Which view describes the ferromagnetism in diluted magnetic semiconductors, materials with promise for spintronic applications, is still unclear. Here, we describe the detailed physical res…
For modeling the magnetic properties of concentrated and diluted magnetic semiconductors, we use the Kondo-lattice model. The magnetic phase diagram is derived by inspecting the static susceptibility of itinerant band electrons, which are exchange coupled to localized magnetic moments. It turns out that rather low band occupations favour a ferromagnetic ordering of the local moment systems due to an indirect coupling mediated by a spin polarization of the itinerant charge carriers. The disorder in diluted systems is treated by adding a CPA-type concept to the theory. For almost all moment conc…
We investigate the itinerant ferromagnetism using a diluted spin-fermion model, derived from a repulsive Hubbard model, where itinerant fermions are coupled antiferromagnetically to auxiliary fields in a three-dimensional simple cubic lattice. We focus, in particular, on understanding the spin-dependent transport properties of the itinerant fermions in the impurity band by taking positional disorder of the auxiliary fields into account. For on-site repulsion $U$ $\sim$ bandwidth the density of the itinerant carriers confined to the impurity band, play a key role in determining the kinetic ener…
Carrier-induced ferromagnetism is investigated in a diluted Hubbard model for ordered impurity arrangements. The delicate competition between particle-hole processes contributing to the spin couplings results in a rich variety of behaviour. The ferromagnetic transition temperature obtained within the spin-fluctuation theory is in good agreement with reported values for $\rm Ga_{1-x} Mn_x N$.
Being a wide band gap system GaMnN attracted considerable interest after the discovery of highest reported ferromagnetic transition temperature $T_C$ $\sim$ 940 K among all diluted magnetic semiconductors. Later it become a debate due to the observation of either a ferromagnetic state with very low $T_C$ $\sim$ 8 K or sometimes no ferromagnetic state at all. We address these issues by calculating the ferromagnetic window, $T_C$ Vs $p$, within a $t-t'$ Kondo lattice model using a spin-fermion Monte-Carlo method on a simple cubic lattice. We exploit the next-nearest-neighbor hopping $t'$ to tune…
Ion implantation of Mn ions into hole-doped GaP has been used to induce ferromagnetic behavior above room temperature for optimized Mn concentrations near 3 at.%. The magnetism is suppressed when the Mn dose is increased or decreased away from the 3 at.% value, or when n-type GaP substrates are used. At low temperatures the saturated moment is on the order of one Bohr magneton, and the spin wave stiffness inferred from the Bloch-law T^3/2 dependence of the magnetization provides an estimate Tc = 385K of the Curie temperature that exceeds the experimental value, Tc = 270K. The presence of ferro…
We report on a cooperative phenomenon of ferromagnetism and unconventional superconductivity (SC) in UGe$_2$ through the measurements of $^{73}$Ge nuclear-quadrupole-resonance (NQR) under pressure ($P$). The NQR spectra evidenced phase separation into ferromagnetic and paramagnetic phases in the vicinity of $P_c\sim 1.5$ GPa, pointing to a first-order transition. The measurements of nuclear-spin-lattice-relaxation-rate $1/T_1$ revealed that SC emerges under the background of ferromagnetism, but not of the paramagnetic phase.
An investigation of La and Ca doped Sr4Ru3O10, featuring a coexistence of interlayer ferromagnetism and intralayer metamagnetism, is presented. La doping readily changes magnetism between ferromagnetism and metamagnetism by tuning the density of states. It also results in different Curie temperatures for the c-axis and the basal plane, highlighting a rare spin-orbit coupling with the crystal field states. In contrast, Ca doping enhances the c-axis ferromagnetism and the magnetic anisotropy. La doping also induces a dimensional crossover in the interlayer transport whereas Ca doping exhibits a …
We have examined whether the Co ions crystallographically substitute on the Ti sites in rutile and anatase Ti_{1-x}$Co$_{x}$O$_{2-delta}$ thin films that exhibit room-temperature ferromagnetism. Intensities of the x-ray Bragg reflection from the films were measured around the $K$-absorption-edge of Co. If the Co ions randomly substitute on the Ti sites, the intensity should exhibit an anomaly due to the anomalous dispersion of the atomic scattering factor of Co. However, none of the anatase and rutile samples did exhibit an anomaly, unambiguously showing that the Co ions in Ti$_{1-x}$Co$_{x}$O…
We calculate magnetic couplings in the $J_{pd}$ model for dilute magnets, in order both to identify the relevant parameters which control ferromagnetism and also to bridge the gap between first principle calculations and model approaches. The magnetic exchange interactions are calculated non-perturbatively and disorder in the configuration of impurities is treated exacly, allowing us to test the validity of effective medium theories. Results differ qualitatively from those of weak coupling. In contrast to mean field theory, increasing $J_{pd}$ may not favor high Curie temperatures: $T_C$ scale…
We argue, in contrast to recent studies, that the antiferromagnetic superexchange coupling between nearest neighbour spins does not fully destroy the ferromagnetism in dilute magnets with long-ranged ferromagnetic couplings. Above a critical coupling, we find a \textit{canted} ferromagnetic phase with unsaturated moment. We have calculated the transition temperature using a simplified local Random Phase Approximation procedure which accounts for the canting. For the dilute magnetic semiconductors, such as GaMnAs, using \textit{ab-initio} couplings allows us to predict the existence of a canted…
Unconventional ferromagnetism and superconductivity in the imbalanced kagome-lattice Hubbard model are investigated by the mean-field theory and determinant quantum Monte Carlo method. Due to the asymmetric band structure of kagome lattice, the spin-$z$ ferromagnetic order intrinsically exists in the system, which is first enhanced by the interaction, and then continuously destructed after reaching a maximum at a moderate interaction strength. In contrast, the $xy$-plane ferromagnetism develops only above a critical interaction, which is estimated to be $U_c/t=3.65 \pm 0.05$ by finite-size sca…
For nearly a century, the Stoner model has dominated research in itinerant ferromagnetism, yet recent work on ultracold, optically trapped Fermi gases suggests that phase separation of spins occurs independent of long-range magnetic order. In this paper, we consider the breakdown of the Stoner criterion in a Landau-Fermi liquid with weak non-zero gauge field. Due to a process analogous to Kohn's theory of a metal-insulator transition, we find the stability of a Fermi liquid phase in the absence of non-quasiparticle contributions to the response is strongly dependent on Landau parameters of mix…
We calculate Curie temperatures and study the stability of ferromagnetism in diluted magnetic materials, taking as a model for the exchange between magnetic impurities a damped Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction and a shor t range term representing the effects of superexchange. To properly include effects of spin and thermal fluctuations as well as geometric disorder, we solve the effective Heisenberg Hamiltonian by means of a recently developed semi-analytical approach. This approach, ``self-consistent local Random Phase Approximation (SC-L RPA)'', is explained. We show that pre…
Ground state properties of the repulsive Hubbard model on a cubic lattice are investigated by means of the auxiliary-field quantum Monte Carlo method. We focus on low-density systems with varying on-site interaction $U/t$, as a model relevant to recent experiments on itinerant ferromagnetism in a dilute Fermi gas with contact interaction. Twist-average boundary conditions are used to eliminate open-shell effects and large lattice sizes are studied to reduce finite-size effects. The sign problem is controlled by a generalized constrained path approximation. We find no ferromagnetic phase transi…
We present a theory for carrier induced ferromagnetism in diluted magnetic semi-conductor (DMS). Our approach treats on equal footing quantum fluctuations within the RPA approximation and disorder within CPA. This method allows for the calculation of $T_c$, magnetization and magnon spectrum as a function of hole, impurity concentration and temperature. It is shown that, sufficiently close to $T_c$, and within our decoupling scheme (Tyablicov type) the CPA for the itinerant electron gas reduces to the Virtual Crystal Approximation. This allows, in the low impurity concentration and low density …
The 5d-electron based BaIrO3 is a nonmetallic weak ferromagnet with a Curie temperature at Tc=175 K. Its largely extended orbitals generate strong electron-lattice coupling, and magnetism and electronic structure are thus critically linked to the lattice degree of freedom. Here we report results of our transport and magnetic study on slightly Sr doped BaIrO3. It is found that dilute Sr-doping drastically suppresses Tc, and instantaneously leads to a nonmetal-metal transition at high temperatures. All results highlight the instability of the ground state and the subtle relation between magnetic…
We solve the double exchange model in the presence of arbitrary substitutional disorder by using a self consistently generated effective Hamiltonian for the spin degrees of freedom. The magnetic properties are studied through classical Monte Carlo while the effective exchange, $D_{ij}$, are calculated by solving the disordered fermion problem, and renormalised self-consistently with increasing temperature. We present exact results on the conductivity, magnetoresistance, optical response and `real space' structure of the inhomogeneous ferromagnetic state, and compare our results with charge dyn…
Thin films of the optimally electron-doped $T'$-phase superconductor La$_{1.89}$Ce$_{0.11}$CuO$_{4\pm \d}$ are investigated by dilute Co doping, formed as La$_{1.89}$Ce$_{0.11}$(Cu$_{1-x}$Co$_{x}$)O$_{4\pm\d}$ (LCCCO) with $x$ = 0.01 -- 0.05. The following results are obtained for the first time: for the whole dilute Co doping range, LCCCO thin films show long-range ferromagnetic ordering at the temperature range from 5 K to 300 K, which is likely due to the RKKY interaction; in the very dilute Co doping, $x$ = 0.01 and 0.02, the superconductivity is maitained, the system shows the coexistence…
Linear Ensemble-Constrained Quantum Monte Carlo: From Dilute Fermi Gas to Flat-Band Ferromagnetism
Key Laboratory of Artificial Structures and Quantum Control (Ministry of Education) School of Physics and Astronomy, Shanghai Jiao Tong University(上海交通大学物理与天文学院人工结构量子控制教育部重点实验室);Institute of Theoretical Physics, Chinese Academy of Sciences(中国科学院理论物理研究所);Hefei National Laboratory(合肥国家实验室)
We study the possibility of d0 ferromagnetism in the compound MgO doped with nitrogen (N). The Haldane-Anderson impurity model is formulated within the tight-binding approximation for determining the host band-structure and the impurity-host hybridization. Using the quantum Monte Carlo technique, we observe a finite local moment for an N impurity, and long-range ferromagnetic correlations between two N impurities. The ferromagnetic correlations are strongly influenced by the impurity bound state. When the ferromagnetic correlation between a pair of impurities is mapped onto the isotropic Heise…
We report on the itinerant ferromagnetic superconductor UGe_2 through ^73Ge-NQR measurements under pressure (P). The P dependence of the NQR spectrum signals a first-order transition from the low-temperature (T) and low-P ferromagnetic phase (FM2) to high-T and high-P one (FM1) around a critical pressure of P_x ~ 1.2 GPa. The superconductivity exhibiting a maximum value of T_sc=0.7 K at P_x ~ 1.2 GPa, was found to take place in connection with the P-induced first-order transition. The nuclear spin-lattice relaxation rate 1/T_1 has probed the ferromagnetic transition, exhibiting a peak at the C…
Diluted magnetic semiconductors possessing intrinsic static magnetism at high temperatures represent a promising class of multifunctional materials with high application potential in spintronics and magneto-optics. In the hexagonal Fe-doped diluted magnetic oxide, 6H-BaTiO$_{3-δ}$, room-temperature ferromagnetism has been previously reported. Ferromagnetism is broadly accepted as an intrinsic property of this material, despite its unusual dependence on doping concentration and processing conditions. However, the here reported combination of bulk magnetization and complementary in-depth local-p…
The state of art in the theoretical and experimental studies of transition metal doped oxides (dilute magnetic dielectrics) is reviewed. The available data show that the generic non-equilibrium state of oxide films doped with magnetic impurities may either favor ferromagnetism with high Curie temperature or result in highly inhomogeneous state without long-range magnetic order. In both case concomitant defects (vacancies, interstitial ions play crucial part.
Diluted ferromagnetic semiconductors (DMSs) that combine the properties of semiconductors with ferromagnetism have potential application in spin-sensitive electronics (spintronics) devices. The search for DMS materials exploded after the observation of ferromagnetic ordering in III-V (Ga,Mn)As films. Recently, a series of DMS compounds isostructural to iron-based superconductors have been reported. Among them, the highest Curie temperature $T_C$ of 230 K has been achieved in (Ba,K)(Zn,Mn)$_2$As$_2$. However, most DMSs, including (Ga,Mn)As, are p-type, i.e., the carriers that mediate ferromagne…
A review is given for the recent progress of research in the field of oxide-based diluted magnetic semiconductor (DMS), which was triggered by combinatorial discovery of transparent ferromagnet. The possible advantages of oxide semiconductor as a host of DMS are described in comparison with conventional compound semiconductors. Limits and problems for identifying novel ferromagnetic DMS are described in view of recent reports in this field. Several characterization techniques are proposed in order to eliminate unidentified ferromagnetism of oxide-based DMS (UFO). Perspectives and possible devi…
We have studied the electronic structure of Zn$_{0.9}$Fe$_{0.1}$O nano-particles, which have been reported to show ferromagnetism at room temperature, by x-ray photoemission spectroscopy (XPS), resonant photoemission spectroscopy (RPES), x-ray absorption spectroscopy (XAS) and x-ray magnetic circular dichroism (XMCD). From the experimental and cluster-model calculation results, we find that Fe atoms are predominantly in the Fe$^{3+}$ ionic state with mixture of a small amount of Fe$^{2+}$ and that Fe$^{3+}$ ions are dominant in the surface region of the nano-particles. It is shown that the roo…
Despite the recent success in the realization of the quantum anomalous Hall effect, the underlying physical mechanism of the long range Ferromagnetism is still unclear. Based on our density functional theory calculations, we discovered an intriguing long-range ferromagnetic order in Cr-doped, carrier-free Bi2Te3, with the separation between dopants more than 8 Å. We found that this magnetic coupling is facilitated by an anti-bonding state originated from the lone pair of a Te 5p state and a Bi 6s state, despite this anti-bonding state lies below the valence band maximum. Such a state serves as…
Using a recently developed semi-analytical method (Self-Consistent Local RPA or SC-LRPA) we study the stability of the ferromagnetic phase in diluted magnetic systems where the exchange coupling between magnetic impurities are of RKKY form. A short discussion of the relevance of these calculations with respect to the ferromagnetism observed in diluted ferromagnetic materials is provided. Then, within a two step approach, we study ferromagnetism in $Zn_{1-x}Cr_{x}Te$. In the first step of our study, we calculate the magnetic couplings between Mn impurities within the LDA. In the second step, we…
We have performed x-ray magnetic circular dichroism (XMCD) and valence-band photoemission studies of the diluted ferromagnetic semiconductor Zn$_{1-x}$Cr$_x$Te. XMCD signals due to ferromagnetism were observed at the Cr 2p absorption edge. Comparison with atomic multiplet calculations suggests that the magnetically active component of the Cr ion was divalent under the tetrahedral crystal field with tetragonal distortion along the crystalline a-, b-, and c-axes. In the valence-band spectra, spectral weight near the Fermi level was strongly suppressed, suggesting the importance of Jahn-Teller ef…
The electronic structure of the Cr ions in the diluted ferromagnetic semiconductor Zn$_{1-x}$Cr$_x$Te ($x=0.03$ and 0.15) thin films has been investigated using x-ray magnetic circular dichroism (XMCD) and photoemission spectroscopy (PES). Magnetic-field ($H$) and temperature ($T$) dependences of the Cr $2p$ XMCD spectra well correspond to the magnetization measured by a SQUID magnetometer. The line shape of the Cr $2p$ XMCD spectra is independent of $H$, $T$, and $x$, indicating that the ferromagnetism is originated from the same electronic states of the Cr ion. Cluster-model analysis indicat…
We report on tunneling magnetoresistance (TMR) experiments that demonstrate the existence of a significant spin polarization in Co-doped (La,Sr)TiO3-d (Co-LSTO), a ferromagnetic diluted magnetic oxide system (DMOS) with high Curie temperature. These TMR experiments have been performed on magnetic tunnel junctions associating Co-LSTO and Co electrodes. Extensive structural analysis of Co-LSTO combining high-resolution transmission electron microscopy and Auger electron spectroscopy excluded the presence of Co clusters in the Co-LSTO layer and thus, the measured ferromagnetism and high spin pola…
Films of ZnO doped with magnetic ions, Mn and Co and, in some cases, with Al have been fabricated with a very wide range of carrier densities. Ferromagnetic behaviour is observed in both insulating and metallic films, but not when the carrier density is intermediate. Insulating films exhibit variable range hopping at low temperatures and are ferromagnetic at room temperature due to the interaction of the localised spins with static localised states. The magnetism is quenched when carriers in the localised states become mobile. In the metallic (degenerate semiconductor) range, robust ferromagne…
We have performed ab initio calculations within the density-functional theory for Ga_{1-x}Mn_xAs diluted semiconductors. Total energy results unambiguously show that a quasi-localized down-spin hole, with strong p-like character, surrounds the fully polarized Mn up-spin d^5-electrons. Calculations indicate that the holes form an essentially dispersionless impurity band, thus rendering effective-mass descriptions of hole states open to challenge. We obtain estimates both for the s = 1/2 hole and S = 5/2 Mn exchange coupling, and for the distance dependence of the effective Mn-Mn exchange intera…
The realization of semiconductors that are ferromagnetic above room temperature will potentially lead to a new generation of spintronic devices with revolutionary electrical and optical properties. Transition temperatures in doped ZnO are high but, particularly for Mn doping, the reported moments have been small. We show that by careful control of both oxygen deficiency and aluminium doping the ferromagnetic moments measured at room temperature in n-type ZnMnO and ZnCoO are close to the ideal values of 5mB and 3mB respectively. Furthermore a clear correlation between the magnetisation per tran…
Here by combining a symmetry-based analysis with numerical computations we predict a new kind of magnetic ordering - antichiral ferromagnetism. The relationship between chiral and antichiral magnetic order is conceptually similar to the relationship between ferromagnetic and antiferromagnetic order. Without loss of generality, we focus our investigation on crystals with full tetrahedral symmetry where chiral interaction terms - Lifshitz invariants - are forbidden by symmetry. However, we demonstrate that leading chirality-related term leads to nontrivial smooth magnetic textures in the form of…
While ferromagnetism at relatively high temperatures is seen in diluted magnetic semiconductors such as Ga_(1-x)Mn_(x)As, doped semiconductors without magnetic ions have not shown evidence for ferromagnetism. Using a generalized disordered Hubbard model designed to characterize hydrogenic centers in semiconductors, we find that such systems may also exhibit a ferromagnetic ground state, at least on the nanoscale. This is found most clearly in a regime inaccessible to bulk systems, but attainable in quantum dots as well as heterostructures. We present numerical results demonstrating the occurre…
The puzzling observation of room temperature ferromagnetism in double perovskites (A$_2$BB$'$O$_6$), despite having the magnetic lattice of B-ions diluted by non-magnetic B$'$-ions, have been examined for Sr$_2$FeReO$_6$. {\it Ab-initio} spin spiral electronic structure calculations along various high symmetry directions in reciprocal space are used to determine the exchange interactions entering an extended Heisenberg model, which is then solved classically using Monte Carlo simulations to determine the ferromagnetic transition temperature T$_c$. We find that one must consider onsite Coulomb …
A brief review of theory of ferromagnetism of dilute magnetic semiconductors of the form (A,Mn)B based on the double exchange model is first given. A systematic investigation of the phenomena extending the current theory is outlined. We begin with an investigation of the regions of instability of the nonmagnetic towards the ferromagnetic state of a system of Mn-atoms doped in AB-type semiconductor. A self-consistent many-body theory of the ferromagnetic state is then developed, going beyond the mean field approaches by including fluctuations of the Mn-spins and the itinerant hole-gas. A functi…
Ferromagnetism is observed at and above room temperature in pulsed laser deposited epitaxial films of Co-doped Ti-based oxide perovskite (La1-xSrxTiO3-d). The system has the characteristics of an intrinsic diluted magnetic semiconductor (metal) at low concentrations (<~ 2 %), but develops inhomogeneity at higher cobalt concentrations. The films range from being opaque metallic to transparent semiconducting depending on the oxygen pressure during growth and are yet ferromagnetic.
A lattice spin-fermion model for diluted magnetic semiconductors (DMS) is investigated numerically, improving on previously used mean-field (MF) approximations. Curie temperatures are obtained varying the Mn-spin x and hole n densities, and the impurity-hole exchange J in units of the hopping amplitude t. Optimal values are found in the subtle intermediate regime between itinerant and localized carriers. Our main result is the behavior of the Curie temperature at large J/t, where a "clustered" state is observed and ferromagnetism is suppressed. Formal analogies between DMS and manganites are a…
Colossal low-field negative magnetoresistance in CaAl$_{2}$Si$_{2}$-type diluted magnetic semiconductors (Ba,K)(Cd,Mn)$_{2}$As$_{2}$
Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences(中国科学院物理研究所凝聚态物理国家实验室);Collaborative Innovation Center of Quantum Matter(量子物质协同创新中心)
We present a theory to model carrier mediated ferromagnetism in concentrated or diluted local moment systems. The electronic subsystem of the Kondo lattice model is described by a combined equation of motion / coherent potential approximation method. Doing this we can calculate the free energy of the system and its minimum according to the magnetization of the local moments. Thus also the Curie temperature can be determined and its dependence on important model parameters. We get qualitative agreement with the Curie temperatures' experimental values of Ga$_{1-x}$Mn$_x$As for a proper hole dens…
The present work reproduces the room temperature ferromagnetism by doping magnetic Mn atoms in diamagnetic ZnO. The ferromagnetic ordering is extended up to 640 K in mechanical milled Zn0.95Mn0.05O samples. The bulk and nanocrystalline samples are stabilized in hexagonal crystal structure with space group p63mc. The grain size and lattice strain of the samples, estimated from XRD spectrum using Williamson-Hall plot, showed a significant variation with milling time. Surface structure (morphology, distribution of grains and elements) is observed to be reasonably good from SEM picture and EDX spe…
Carrier induced ferromagnetism in diluted III-V semi-conductor is analyzed within a two step approach. First, within a single site CPA formalism, we calculate the element resolved averaged Green's function of the itinerant carrier. Then using a generalized RKKY formula we evaluate the Mn-Mn long-range exchange integrals and the Curie temperature as a function of the exchange parameter, magnetic impurity concentration and carrier density. The effect of the disorder (impurity scattering) appears to play a crucial role. The standard RKKY calculation (no scattering processes), strongly underestima…
Superconductivity has again become a challenge following the discovery of unconventional superconductivity. Resistance-free currents have been observed in heavy-fermion materials, organic conductors and copper oxides. The discovery of superconductivity in a single crystal of $UGe_2$, $ZrZn_2$ and $URhGe$ revived the interest in the coexistence of superconductivity and ferromagnetism. The experiments indicate that: i)The superconductivity is confined to the ferromagnetic phase. ii)The ferromagnetic order is stable within the superconducting phase (neutron scattering experiments). iii) The speci…
Recent results about the coexistence of ferromagnetism and unconventional superconductivity with spin-triplet Cooper pairing are reviewed on the basis of the quasi-phenomenological Ginzburg-Landau theory. The superconductivity in the mixed phase of coexistence of ferromagnetism and unconventional superconductivity is triggered by the spontaneous magnetization. The mixed phase is stable whereas the other superconducting phases that usually exist in unconventional superconductors are either unstable or metastable at relatively low temperatures in a quite narrow domain of the phase diagram and th…
Motivated by the unconventional properties and rich phase diagram of NaxCoO2 we consider the electronic and magnetic properties of a two-dimensional Hubbard model on an isotropic triangular lattice doped with electrons away from half-filling. Dynamical mean-field theory (DMFT) calculations predict that for negative inter-site hopping amplitudes (t<0) and an on-site Coulomb repulsion, U, comparable to the bandwidth, the system displays properties typical of a weakly correlated metal. In contrast, for t>0 a large enhancement of the effective mass, ferromagnetism and a Curie-Weiss magnetic suscep…