We consider the counting statistics of electron transport through a double quantum dot with special emphasis on the dephasing induced by a nearby charge detector. The double dot is embedded in a dissipative enviroment, and the presence of electrons on the double dot is detected with a nearby quantum point contact. Charge transport through the double dot is governed by a non-Markovian generalized master equation. We describe how the cumulants of the current can be obtained for such problems, and investigate the difference between the dephasing mechanisms induced by the quantum point contact and the coupling to the external heat bath. Finally, we consider various open questions of relevance to future research.
We present a theory of full counting statistics for electron transport through interacting electron systems with non-Markovian dynamics. We illustrate our approach for transport through a single-level quantum dot and a metallic single-electron transistor to second order in the tunnel-coupling strength, and discuss under which circumstances non-Markovian effects appear in the transport properties.
We present a general technique to obtain the zero temperature full counting statistics of charge transfer in interacting impurity models out of equilibrium from time-dependent simulations on a lattice. We demonstrate the technique with application to the self-dual interacting resonant level model, where very good agreement between numerical simulations using the density matrix renormalization group and those obtained analytically from the thermodynamic Bethe ansatz is found. We show from the exact form of counting statistics that the quasiparticles involved in transport carry charge $2e$ in th…
A mesoscopic Coulomb blockade system with two identical transport channels is studied in terms of full counting statistics. It is found that the average current cannot distinguish the quantum constructive interference from the classical non-interference, but the shot noise and skewness are more sensitive to the nature of quantum mechanical interference and can fulfill that task. The interesting super-Poisson shot noise is found and is demonstrated as a consequence of constructive interference, which induces an effective system with fast-and-slow transport channels. Dephasing effects on the cou…
We study the full charge counting statistics of a charge pump based on a nearly open single electron transistor. The problem is mapped onto an exactly soluble problem of a g=1/2 non-equilibrium Luttinger liquid with an impurity. We obtain an analytic expression for the generating function of the transmitted charge for an arbitrary pumping strength. Even though this model contains fractionally charged excitations only integer transmitted charges can be observed during finite observation times.
We examine the full counting statistics of quantum dots, which display super-Poissonian shot noise. By an extension to a generic situation with many excited states we identify the underlying transport process. The statistics is a sum of independent Poissonian processes of bunches of different sizes, which leads to the enhanced noise. The obtained results could be useful to determine transport characteristics in molecules and large quantum dots, since the noise (and higher cumulants) allow to identify the internal level structure, which is not visible in the average current.
Electron counting statistics of a current pump in an open system has universal form in the weak pumping current regime. In the time domain, charge transmission is described by two uncorrelated Poisson processes, corresponding to electron transmission in the right and left direction. Overall noise is super-poissonian, and can be reduced to poissonian by tuning the amplitude and phase of driving signal so that current to noise ratio is maximized. Measuring noise in this regime provides a new method for determining charge quantum in an open system without any fitting parameters.
It is shown that a one-channel mesoscopic conductor in an ohmic environment can be mapped to the problem of a backscattering impurity in a Tomonaga-Luttinger liquid (TLL). This allows to determine non perturbatively the effect of the environment on $I-V$ curves, and to find an exact relationship between dynamic Coulomb blockade and shot noise. We investigate critically how this relationship compares to recent proposals in the literature. The full counting statistics is determined at zero temperature.
We calculate the full counting statistics (FCS) of a subsystem energy in free fermionic systems by means of the Grassmann variables. We demonstrate that the generating function of these systems can be written as a determinant formula with respect to the Hamiltonian couplings and by employing the Bell's polynomials, we derive exact formulas for the subsystem energy moments. In addition, we discuss the same quantities in the quantum XY spin chain, and we demonstrate that at the critical regimes the fluctuations of the energy moments decay like a power-law as we expect from the conformal field th…
We evaluate the current distribution for a single-electron transistor with intermediate strength tunnel conductance. Using the Schwinger-Keldysh approach and the drone (Majorana) fermion representation we account for the renormalization of system parameters. Nonequilibrium effects induce a lifetime broadening of the charge-state levels, which suppress large current fluctuations.
Using the Schwinger-Keldysh approach and the drone (Majorana) fermion representation, we evaluate current distribution in a single-electron transistor in a regime where a total tunnel resistance is small. Nonequilibrium quantum fluctuations of charge induce a lifetime broadening of charge-state level, as well as renormalization of system parameters. We find that the lifetime broadening effect may suppress the probability of relatively large current.
We analyze the full counting statistics of a multiorbital Kondo effect in a quantum dotwith the SU(N) symmetry in the framework of the renormalized perturbation theory. The current probability distribution function is calculated for an arbitrary dot-site Coulomb repulsion $U$ in the particle-hole symmetric case. The resulting cumulant up to the leading nonlinear term of applied bias voltages indicates two types of electron transfer, respectively carrying charge $e$ and $2e$, with different $N$-dependences. The cross correlation between different orbital currents shows exponential enhancement w…
We calculate the spin current distribution function for a Kondo dot in two different regimes. In the exactly solvable Toulouse limit the linear response, zero temperature statistics of the spin transfer is trinomial, such that all the odd moments vanish and the even moments follow a binomial distribution. On the contrary, the corresponding spin-resolved distribution turns out to be binomial. The combined spin and charge statistics is also determined. In particular, we find that in the case of a finite magnetic field or an asymmetric junction the spin and charge measurements become statisticall…
We discuss the counting statistics and current noise associated with the double Josephson quasiparticle resonance point in a superconducting single electron transistor. The counting statistics are in general phase-dependent, despite the fact that the average current has no dependence on phase. Focusing on parameter regimes where the counting statistics have no phase-dependence, we use a general relation first derived by MacDonald in 1948 to obtain the full frequency-dependent shot noise directly from the counting statistics, without any further approximations. We comment on problems posed by t…
We review the relations between the full counting statistics and the field theory of electric circuits. We demonstrate that for large conductances the counting statistics is determined by non-trivial saddle-point of the field. Coulomb effects in this limit are presented as quantum corrections that can stongly renormalize the action at low energies.
We study analytically the full counting statistics of charge transport through single molecules, strongly coupled to a weakly damped vibrational mode. The specifics of transport in this regime - a hierarchical sequence of avalanches of transferred charges, interrupted by "quiet" periods - make the counting statistics strongly non-Gaussian. We support our findings for the counting statistics as well as for the frequency-dependent noise power by numerical simulations, finding excellent agreement.
We present a theory of modified reduced dynamics in the presence of counting fields. Reduced dynamics techniques are useful for describing open quantum systems at long emergent timescales when the memory timescales are short. However, they can be difficult to formulate for observables spanning the system and its environment, such as those characterizing transport properties. A large variety of mixed system--environment observables, as well as their statistical properties, can be evaluated by considering counting fields. Given a numerical method able to simulate the field-modified dynamics over…
In the hot electron regime, electron-electron scattering strongly modifies not only the shot noise but also the full counting statistics. We employ a method based on a stochastic path integral to calculate the counting statistics of two systems in which noise in the hot electron regime has been experimentally measured. We give an analytical expression for the counting statistics of a chaotic cavity and find that heating due to electron-electron scattering renders the distribution of transmitted charge symmetric in the shot noise limit. We also discuss the frequency dispersion of the third orde…
We present measurements of the time-dependent fluctuations in electrical current in a voltage-biased tunnel junction. We were able to simultaneously extract the first three moments of the tunnel current counting statistics. Detailed comparison of the second and the third moment reveals that counting statistics is accurately described by the Poissonian distribution expected for spontaneous current fluctuations due to electron charge discreteness, realized in tunneling transport at negligible coupling to environment.
Full counting statistics is a powerful tool to characterize the noise and correlations in transport through mesoscopic systems. In this work, we propose the theory of conditional spin counting statistics, i.e., the statistical fluctuations of spin-up (down) current given the observation of the spin-down (up) current. In the context of transport through a single quantum dot, it is demonstrated that a strong Coulomb interaction leads to a conditional spin counting statistics that exhibits a substantial change in comparison to that without Coulomb repulsion. It thus can be served as an effective …
We derive the full counting statistics of charge transfer through a voltage biased superconducting junction. We find that for measurement times much longer than the inverse Josephson frequency, the counting statistics describes a correlated transfer of quanta of multiple electron charges, each quantum associated with the transfer of a single quasiparticle. An expression for the the counting statistics in terms of the quasiparticle scattering amplitudes is derived.
Full counting statistics is a fundamentally new concept in quantum transport. After a review of basic statistics theory, we introduce the powerful Green's function approach to full counting statistics. To illustrate the concept we consider a number of examples. For generic two-terminal contacts we show how counting statistics elucidates the common (and different) features of transport between normal and superconducting contacts. Finally, we demonstrate how correlations in multi-terminal structures are naturally included in the formalism.
We present a stochastic path integral method to calculate the full counting statistics of conductors with energy conserving dephasing probes and dissipative voltage probes. The approach is explained for the experimentally important case of a Mach-Zehnder interferometer, but is easily generalized to more complicated setups. For all geometries where dephasing may be modeled by a single one-channel dephasing probe we prove that our method yields the same full counting statistics as phase averaging of the cumulant generating function.
Recent experiments [Nature 521, 196 (2015) and Nat. Commun. 8, 395 (2017)] have presented evidence for electron pairing in a quantum dot beyond the superconducting regime. Here, we show that the impact of an attractive electron-electron interaction on the full counting statistics of electron transfer through a quantum dot is qualitatively different from the case of a repulsive interaction. In particular, the sign of higher-order (generalized) factorial cumulants reveals more pronounced correlations, which even survive in the limit of fast spin relaxation.
We discuss how threshold detectors can be used for a direct measurement of the full counting statistics (FCS) of current fluctuations and how to implement Jose phson junctions in this respect. We propose a scheme to characterize the full co unting statistics from the current dependence of the escape rate measured. We il lustrate the scheme with explicit results for tunnel, diffusive and quasi-ballis tic mesoscopic conductors.
We present a theory for the full distribution of current fluctuations in incoherent diffusive superconducting junctions, subjected to a voltage bias. This theory of full counting statistics of incoherent multiple Andreev reflections is valid for arbitrary applied voltage. We present a detailed discussion of the properties of the first four cumulants as well as the low and high voltage regimes of the full counting statistics. The work is an extension of the results of Pilgram and the author, Phys. Rev. Lett. 94, 086806 (2005).
Using a microscopic model for stochastic transport through a single quantum dot that is modified by the Coulomb interaction of environmental (weakly coupled) quantum dots, we derive generic properties of the full counting statistics for multi-stable Markovian transport systems. We study the temporal crossover from multi-modal to broad uni-modal distributions depending on the initial mixture, the long-term asymptotics and the divergence of the cumulants in the limit of a large number of transport branches. Our findings demonstrate that the counting statistics of a single resonant level may be u…
We explore the full counting statistics of single electron tunneling through a quantum dot using a quantum point contact as non-invasive high bandwidth charge detector. The distribution of counted tunneling events is measured as a function of gate and source-drain-voltage for several consecutive electron numbers on the quantum dot. For certain configurations we observe super-Poissonian statistics for bias voltages at which excited states become accessible. The associated counting distributions interestingly show a bimodal characteristic. Analyzing the time dependence of the number of electron …
We study the full counting statistics of current of large open systems through the application of random matrix theory to transition-rate matrices. We develop a method for calculating the ensemble-averaged current-cumulant generating functions based on an expansion in terms of the inverse system size. We investigate how different symmetry properties and different counting schemes affect the results.
Full counting statistics of electron transport is a powerful diagnostic tool for probing the nature of quantum transport beyond what is obtainable from the average current or conductance measurement alone. In particular, the non-Markovian dynamics of quantum dot molecule plays an important role in the nonequilibrium electron tunneling processes. It is thus necessary to understand the non-Markovian full counting statistics in a quantum dot molecule. Here we study the non-Markovian full counting statistics in two typical quantum dot molecules, namely, serially coupled and side-coupled double qua…
We describe a method for calculating the counting statistics of electronic transport through nanoscale devices with both sequential and cotunneling contributions. The method is based upon a perturbative expansion of the von Neumann equation in Liouvillian space, with current cumulants calculated from the resulting nonMarkovian master equation without further approximation. As application, we consider transport through a single quantum dot and discuss the effects of cotunneling on noise and skewness, as well as the properties of various approximation schemes.
We study the full counting statistics of heterostructures consisting of normal metal parts connected to a superconducting terminal. Assuming that coherent superconducting correlations are suppressed in the normal metals we show, using Keldysh-Nambu Green's functions, that the system can be mapped onto a purely normal system with twice the number of elements. For a superconducting beam splitter with several normal terminals we obtain general results for the counting statistics.
We investigate the effect of weak interactions on the full counting statistics of charge transfer through an arbitrary mesoscopic conductor. We show that the main effect can be incorporated into an energy dependence of the transmission eigenvalues and study this dependence in a non-perturbative approach. An unexpected result is that all mesoscopic conductors behave at low energies like either a single or a double tunnel junction, which divides them into two broad classes.
Destructive interference of single-electron tunneling between three quantum dots can trap an electron in a coherent superposition of charge on two of the dots. Coupling to external charges causes decoherence of this superposition, and in the presence of a large bias voltage each decoherence event transfers a certain number of electrons through the device. We calculate the counting statistics of the transferred charges, finding a crossover from sub-Poissonian to super-Poissonian statistics with increasing ratio of tunnel and decoherence rates.
We present here a quantum mechanical framework for defining the statistics of measurements of time integrals of A(t), A(t) being a quantum mechanical variable. This is a generalization of the so-called full counting statistics proposed earlier for DC electric currents. We develop an influence functional formalism that allows us to study the quantum system along with the measuring device thus fully accounting for the action of the detector on the system to be measured. We define the full counting statistics of an arbitrary variable by means of an evolution operator that relates initial and fina…
We use the inchworm Quantum Monte Carlo method to investigate the full counting statistics of particle and energy currents in a strongly correlated quantum dot. Our method is used to extract the heat fluctuations and entropy production of a quantum thermoelectric device, as well as cumulants of the particle and energy currents. The energy--particle current cross correlations reveal information on the preparation of the system and the interplay of thermal and electric currents. We furthermore demonstrate the signature of a crossover from Coulomb blockade to Kondo physics in the energy current f…
We consider current shot noise and the full counting statistics in a chain of quantum dots which exhibits a continuous non-equilibrium phase transition as a function of the tunnel couplings of the chain with the electrodes. Using a combination of analytical and numerical methods, we establish that the full counting statistics is conventional away from the phase transition, but becomes, in a well-defined sense, essentially non-Gaussian on the critical line, where the current fluctuations are controlled by the dynamic critical exponent $z$. We find that signatures of the critical full counting s…
The joint probability distribution in the full counting statistics (FCS) for noninteracting electrons is discussed for an arbitrary number of initially separate subsystems which are connected at t=0 and separated at a later time. A simple method to obtain the leading order long time contribution to the logarithm of the characteristic function is presented which simplifies earlier approaches. New explicit results for the determinant involving the scattering matrices are found. The joint probability distribution for two leads is discussed for Y-junctions and dots connected to four leads.
We investigate the dynamics of electron spin qubits in quantum dots. Measurement of the qubit state is realized by a charge current through the dot. The dynamics is described in the framework of the quantum trajectory approach, widely used in quantum optics, and we show that it can be applied successfully to problems in condensed matter physics. The relevant master equation dynamics is unravelled to simulate stochastic tunneling events of the current through the dot.Quantum trajectories are then used to extract the counting statistics of the current. We show how, in combination with an electro…
We study the full counting statistics of electric current to several drain terminals with spin-dependent entrance conductances. We show that the statistics of charge transfers can be interpreted in terms of single electrons and spin-singlet pairs coming from the source. If the source contains transport channels of high transparency, a significant fraction of electrons comes in spin-singlet pairs.
We review several ways of defining the statistics of charge that is transmitted through an electric circuit, the so-called "counting statistics". We first pursue two approaches that explain the origin of "negative probabilities" that have been found earlier in this context. The first analysis involves degrees of freedom of the electric circuit only. In the second approach an idealized charge detector is introduced. We study then general linear detectors and how their back action on the electric conductor affects the statistics of transferred charge. Phase-coherent conductors in the presence of…
Exact numerical results for the full counting statistics (FCS) of a one-dimensional tight-binding model of noninteracting electrons are presented at finite temperatures using an identity recently presented by Abanov and Ivanov. A similar idea is used to derive a new expression for the cumulant generating function for a system consisting of two quasi-one-dimensional leads connected by a quantum dot in the long time limit. This provides a generalization of the Levitov-Lesovik formula for such systems.
We derive a stochastic path integral representation of counting statistics in semi-classical systems. The formalism is introduced on the simple case of a single chaotic cavity with two quantum point contacts, and then further generalized to find the propagator for charge distributions with an arbitrary number of counting fields and generalized charges. The counting statistics is given by the saddle point approximation to the path integral, and fluctuations around the saddle point are suppressed in the semi-classical approximation. We use this approach to derive the current cumulants of a chaot…
We study the effect of Coulomb interaction on the full counting statistics of an Aharonov-Bohm (AB) interferometer with a single-level quantum dot in one arm in the regime of weak dot-lead and lead-lead tunnel couplings. In the absence of Coulomb interaction, the interference processes are of nonresonant nature with an even AB flux dependence and obey bidirectional Poissonian statistics. For large charging energy, the statistic of these processes changes. In addition, processes of resonant nature with an odd flux dependence appear. In the limit of strongly asymmetric tunnel couplings from the …
In order to fully characterize the noise associated with electron transport, with its severe consequences for solid-state quantum information systems, the theory of full counting statistics has been developed. It accounts for correlation effects associated with the statistics and effects of entanglement, but it remains a non-trivial task to account for interaction effects. In this article we present two examples: we describe electron transport through quantum dots with strong charging effects beyond perturbation theory in the tunneling, and we analyze current fluctuations in a diffusive intera…
The full counting statistics of a molecular level weakly interacting with a local phonon mode is derived. We find an analytic formula that gives the behavior of arbitrary irreducible moments of the distribution upon phonon excitation. The underlying competition between quasi-elastic and inelastic processes results in the formation of domains in parameter space characterized by a given sign in the jump of the irreducible moments. In the limit of perfect transmission, the corresponding distribution is distorted from Gaussian statistics for electrons to Poissonian transfer of holes above the inel…
We develop a self-consistent version of perturbation theory in Liouville space which seeks to combine the advantages of master equation approaches in quantum transport with the nonperturbative features that a self-consistent treatment brings. We describe how counting fields may be included in a self-consistent manner in this formalism such that the full counting statistics can be calculated. NonMarkovian effects are also incorporated. Several different self-consistent approximations are introduced and we discuss their relative strengths with a simple example.
We propose a theory that treats the current, noise, and, generally, the full current statistics of electron transfer in a mesoscopic system in a unified, simple and efficient way. The theory appears to be a circuit theory of $2\times 2$ matrices associated with Keldysh Green functions. We illustrate the theory by considering the big fluctuations of currents in various three-terminal circuits.
We examine the full counting statistics of electron transport through double quantum dots coupled in series, with particular attention being paid to the unique features originating from level renormalization. It is clearly illustrated that the energy renormalization gives rise to a dynamic charge blockade mechanism, which eventually results in super-Poissonian noise. Coupling of the double dots to an external heat bath leads to dephasing and relaxation mechanisms, which are demonstrated to suppress the noise in a unique way.
We study the charge transfer in a small grain oscillating between two leads. Coulomb blockade restricts the charge fluctuations in such a way that only zero or one additional electrons can sit on the grain. The system thus acts as a charge shuttle. We obtain the full counting statistics of charge transfer and discuss its behavior. For large oscillation amplitude the probability of transferring $\tilde n$ electrons per cycle is strongly peaked around one. The peak is asymmetric since its form is controlled by different parameters for $\tilde n>1$ and $\tilde n < 1$. Under certain conditions the…
The article develops a powerful theoretical tool to obtain the full counting statistics. By a slight extension of the standard Keldysh method we can access immediately all correlation functions of the current operator. Embedded in a quantum generalization of the circuit theory of electronic transport, we are able to study the full counting statistics of a large class of two-terminal contacts and multi-terminal structures, containing superconductors and normal metals as elements. The practical use of the method is demonstrated in many examples.
Non-adiabatic charge pumping through a single-level quantum dot with periodically modulated parameters is studied theoretically. By means of a quantum-master-equation approach the full counting statistics of the system is obtained. We find a trinomial-probability distribution of the charge transfer, which adequately describes the reversal of the pumping current by sweeping the driving frequency. Further, we derive equations of motion for current and noise, and solve those numerically for two different driving schemes. Both show interesting features which can be fully analyzed due to the simple…
We propose to describe correlations in classical and quantum systems in terms of full counting statistics of a suitably chosen discrete observable. The method is illustrated with two exactly solvable examples: the classical one-dimensional Ising model and the quantum spin-1/2 XY chain. For the one-dimensional Ising model, our method results in a phase diagram with two phases distinguishable by the long-distance behavior of the Jordan-Wigner strings. For the quantum XY chain, the method reproduces the previously known phase diagram.
We developed a theoretical framework which extends the method of \textit{full counting statistics} (FCS) from conventional single channel Kondo screening schemes to multi-channel Kondo paradigm. The developed idea of FCS has been demonstrated considering an example of two-stage Kondo (2SK) model. We analyzed the charge transferred statistics in the strong-coupling regime of a 2SK model using non-equilibrium Keldysh formulation. A bounded value of Fano factor, $1\leq F\leq 5/3$, confirmed the cross-over regimes of charge transfered statistics in 2SK effect, from Poissonian to super-Poissonian. …
We consider full counting statistics of spin in matrix product states. In particular, we study the approach to gaussian distribution for magnetization. We derive the asymptotic corrections to the central limit theorem for magnetization distribution for finite but large blocks in analogy to the Edgeworth series. We also show how central limit theorem like behavior is modified for certain states with topological characteristics such as the AKLT state.
We propose a derivation of the full counting statistics of electronic current based on a positive-operator-valued measure. Our approach justifies the Levitov-Lesovik formula in the long-time limit, but can be generalized to the detection of finite-frequency noise correlations. The combined action of the projection postulate and the quantum formula for current noise at high frequencies imply an additional white noise. Estimates for this additional noise are in accordance with known experiments. We propose an experimental test of our conjecture by a simultaneous measurement of high- and low-freq…
Time-dependent driving influences the quantum and thermodynamic fluctuations of a system, changing the familiar physical picture of electronic noise which is an important source of information the about microscopic mechanism of quantum transport. Giving access to all cumulants of the current, the full counting statistics (FCS) is the powerful theoretical method to study fluctuations in nonequilibrium quantum systems. In this paper, we propose the application of FCS to consider periodic driven junctions. The combination of Floquet theory for time dynamics and nonequilibrium counting-field Green…
We calculate the charge transport in a flux biased dissipative Cooper pair pump using the method of full counting statistics (FCS). This is instead of a more traditional technique of integrating a very small expectation value of the instantaneous current over the pumping period. We show that the rotating wave approximation (RWA), which fails in the traditional technique, produces accurate results within the FCS method.
We have measured the full counting statistics (FCS) of current fluctuations in a semiconductor quantum dot (QD) by real-time detection of single electron tunneling with a quantum point contact (QPC). This method gives direct access to the distribution function of current fluctuations. Suppression of the second moment (related to the shot noise) and the third moment (related to the asymmetry of the distribution) in a tunable semiconductor QD is demonstrated experimentally. With this method we demonstrate the ability to measure very low current and noise levels.
