We develop a quantum noise approach to study quantum transport through nanostructures. The nanostructures, such as quantum dots, are regarded as artificial atoms, subject to quasi-equilibrium fermionic reservoirs of electrons in biased leads. Noise operators characterizing the quantum fluctuation in the reservoirs are related to the damping and fluctuation of the artificial atoms through the quantum Langevin equation. The average current and current noise are derived in terms of the reservoir noise correlations. In the white-noise limit, we show that the current and current noise can be exactly calculated by the quantum noise approach, even in the presence of interaction such as Coulomb blockade. As a typical application, the average current and current noise through a single quantum dot are studied.
It is shown that the electron coupling to photons in field-dressed nanostructures can result in the ground electron-photon state with a nonzero electric current. Since the current is associated with the ground state, it flows without the Joule heating of the nanostructure and is nondissipative. Such a dissipationless electron transport can be realized in strongly coupled electron-photon systems with the broken time-reversal symmetry - particularly, in quantum rings and chiral nanostructures dressed by circularly polarized photons.
Metallic nanostructures (the nanofilms and nanowires) are widely used in electronic devices, and their thermal transport properties are crucial for heat dissipation. However, there are still gaps in understanding thermal transport in metallic nanostructures, especially regarding the size effect and validity of the Wiedemann-Franz law. In this work, we perform mode-by-mode first-principles calculations combining the Boltzmann transport equation to understand thermal transport in metallic nanostructures. We take the gold (Au) and tungsten (W) nanostructures as prototypes. It is found that when t…
This review summarizes recent studies of thermal transport in nanoscaled semiconductors. Different from bulk materials, new physics and novel thermal properties arise in low dimensional nanostructures, such as the abnormal heat conduction, the size dependence of thermal conductivity, phonon boundary/edge scatterings. It is also demonstrated that phonons transport super-diffusively in low dimensional structures, in other words, Fourier's law is not applicable. Based on manipulating phonons, we also discuss envisioned applications of nanostructures in a broad area, ranging from thermoelectrics, …
Geometric symmetries cause orbital degeneracies in a molecule's spectrum. In a single-molecule junction, these degeneracies are lifted by various symmetry-breaking effects. We study quantum transport through such nanostructures with an almost degenerate spectrum. We show that the master equation for the reduced density matrix must be derived within the singular-coupling limit as opposed to the conventional weak-coupling limit. This results in signatures of the density matrix's off-diagonal elements in the transport characteristics.
I. Introduction (Preface, Nanostructures in Si Inversion Layers, Nanostructures in GaAs-AlGaAs Heterostructures, Basic Properties). II. Diffusive and Quasi-Ballistic Transport (Classical Size Effects, Weak Localization, Conductance Fluctuations, Aharonov-Bohm Effect, Electron-Electron Interactions, Quantum Size Effects, Periodic Potential). III. Ballistic Transport (Conduction as a Transmission Problem, Quantum Point Contacts, Coherent Electron Focusing, Collimation, Junction Scattering, Tunneling). IV. Adiabatic Transport (Edge Channels and the Quantum Hall Effect, Selective Population and De…
In this review we focus on electronic transport through semiconductor nanostructures which are driven by ac fields. Along the review we describe the available experimental information on different nanostructures, like resonant tunneling diodes, superlattices or quantum dots, together with the theoretical tools needed to describe the observed features. These theoretical tools such as, for instance, the Floquet formalism, the non-equilibrium Green's function technique or the density matrix technique, are suitable for tackling with photon-assisted transport problems where the interplay of differe…
We review experimental and theoretical results on thermal transport in semiconductor nanostructures (multilayer thin films, core/shell and segmented nanowires), single- and few-layer graphene, hexagonal boron nitride, molybdenum disulfide and black phosphorus. Different possibilities of phonon engineering for optimization of electrical and heat conductions are discussed. The role of the phonon energy spectra modification on the thermal conductivity in semiconductor nanostructures is revealed. The dependence of thermal conductivity in graphene and related two-dimensional (2D) materials on tempe…
We present a numerical investigation of energy and charge distributions during electron-beam-induced growth of W nanostructures on SiO2 substrates using Monte Carlo simulation of electron transport. This study gives a quantitative insight into the deposition of energy and charge in the substrate and in already existing metallic nanostructures in the presence of the electron beam. We analyze electron trajectories, inelastic mean free paths, and distribution of backscattered electrons in different deposit compositions and depths. We find that, while in the early stages of the nanostructure growt…
Transparent boundary conditions for the time-dependent Schrodinger equation are implemented using the R-matrix method. The employed scattering formalism is suitable for describing open quantum systems and provides the framework for the time-dependent coherent transport. Transmission and reflection of wave functions at the edges of a finite quantum system are essential for an accurate and efficient description of the time-dependent processes on large time scales. The approach is used here to describe time-dependent transport across nanostructured interfaces relevant for photovoltaic application…
We study the coupled current and magnetization noise in magnetic nanostructures by magnetoelectronic circuit theory. Spin current fluctuations, which depend on the magnetic configuration, are found to be an important source of magnetization noise and damping in thinly layered systems. The enhanced magnetization fluctuations in spin valves can be directly measured by their effect on the resistance noise.
Stationary electric transport in semiconductor nanostructures is studied by the method of nonequilibrium Green functions. In the case of sequential tunneling the results are compared with density matrix theory, providing almost identical results. Nevertheless, the method of Green functions is easier to handle due to the availability of an absolute energy scale. It is demonstrated, that the transport in complicated structures, like quantum cascade lasers, can be described in reasonable agreement with experiment.
In this review article, we present a non-equilibrium quantum transport theory for transient electron dynamics in nanodevices based on exact master equation derived with the path integral method in the fermion coherent-state representation. Applying the exact master equation to nanodevices, we also establish the connection of the reduced density matrix and the transient quantum transport current with the Keldysh nonequilibrium Green functions. The theory enables us to study transient quantum transport in nanostructures with back-reaction effects from the contacts, with non-Markovian dissipation…
Organic and carbon-based materials are attractive for spintronics because their small spin-orbit coupling and low hyperfine interaction is expected to give rise to large spin-relaxation times. However, the corresponding spin-relaxation length is not necessarily large when transport is via weakly interacting molecular orbitals. Here we use graphite as a model system and study spin transport in the direction perpendicular to the weakly bonded graphene sheets. We achieve injection of highly (75%) spin-polarized electrons into graphite nanostructures of 300-500 nm across and up to 17 nm thick, and…
We present the theory of the electronic transfer and the optical properties of the quasi-zero dimensional quantum nanostructures, like quantum dots or the DNA molecule. The theory is based on the multiple scattering of the charge carriers in the quasi-zero dimensional nanostructures leading to the manifestation of the nonadiabatic influence of the atomic lattice on the charge carriers. The theory is based on the nonequilibrium Green's functions and the quantum kinetic equations. Three examples of the electronic motion in the small systems are presented, together with a comparison of the theore…
We investigate the effect of a scanning gate tip in the nonlinear quantum transport properties of nanostructures. Generally, we predict that the symmetry of the current-voltage characteristic in reflection-symmetric samples is broken by a tip-induced rectifying conductance correction. Moreover, in the case of a quantum point contact (QPC), the tip-induced rectification term becomes dominant as compared to the change of the linear conductance at large tip-QPC distances. Calculations for a weak tip probing a QPC modeled by an abrupt constriction show that these effects are experimentally observa…
Transport properties of a gated nanostructure depend crucially on the coupling of its states to the states of electrodes. In the case of a single quantum dot the coupling, for a given quantum state, is constant or can be slightly modified by additional gating. In this paper we consider a concentric dot-ring nanostructure (DRN) and show that its transport properties can be drastically modified due to the unique geometry. We calculate the dc current through a DRN in the Coulomb blockade regime and show that it can efficiently work as a single electron transistor or a current rectifier. In both c…
Magnetoelectronics is mainly digital, i.e. governed by up and down magnetizations. In contrast, analogue magnetoelectronics makes use of phenomena occuring for non-collinear magnetization configurations. Here we review theories which have recently been applied to the transport in non-collinear magnetic nanostructures in two and multiterminal structures, viz. random matrix and circuit theory. Both are not valid for highly transparent systems in a resistive environment like perpendicular metallic spin valves. The solution to this problem is a renormalization of the conventional and spin-mixing c…
We studied phase coherent phenomena in mesoscopic Permalloy samples by exploring low temperature transport. Both, differential conductance as a function of bias voltage and magnetoconductance of individual wires display conductance fluctuations. Analysis of these fluctuations yields a phase coherence length of $\sim250$ nm at 25 mK as well as a $1/\sqrt{T}$ temperature dependence. To suppress conductance fluctuations by ensemble averaging we investigated low temperature transport in wire arrays and extended Permalloy films. In these samples we have measured conductance corrections which stem f…
Recent experimental progress has made it possible to detect in real-time single electrons tunneling through Coulomb blockade nanostructures, thereby allowing for precise measurements of the statistical distribution of the number of transferred charges, the so-called full counting statistics. These experimental advances call for a solid theoretical platform for equally accurate calculations of distribution functions and their cumulants. Here we develop a general framework for calculating zero-frequency current cumulants of arbitrary orders for transport through nanostructures with strong Coulom…
We study the non-equilibrium transport properties of a one-dimensional array of dissipative quantum dots. Using the Keldysh formalism, we show that the dots' dissipative nature leads to a spatial variation of the chemical potential, which in disordered arrays, breaks the invariance of the current, I, under bias reversal. Moreover, the array's nanoscopic size results in an algebraic low-temperature dependence of I. Finally, we show that a local Coulomb interaction splits the dots' electronic levels, resulting in a Coulomb blockade, which is softened with increasing dissipation and array size.
By scattering theory we show that spin current noise in normal electric conductors in contact with nanoscale ferromagnets increases the magnetization noise by means of a fluctuating spin-transfer torque. Johnson-Nyquist noise in the spin current is related to the increased Gilbert damping due to spin pumping, in accordance with the fluctuation-dissipation theorem. Spin current shot noise in the presence of an applied bias is the dominant contribution to the magnetization noise at low temperatures.
Transport through semiconductor nanostructures is a quantum-coherent process. This paper focuses on systems in which the electron's dynamics is ballistic and the transport is dominated by the scattering from structure boundaries. Opposite to the well-known case of the nuclear reactions, the potentials defining semiconductor structures are nonspherically symmetric and the asymptotic motion of the electrons is determined by the different potential levels in the contacts. For this special type of potential the mathematical foundations for the scattering theoretical description of the transport ph…
We theoretically investigate the role of spin fluctuations in charge transport through a magnetic junction. Motivated by recent experiments that measure a nonlinear dependence of the current on electrical bias, we develop a systematic understanding of the interplay of charge and spin dynamics in nanoscale magnetic junctions. Our model captures two distinct features arising from these fluctuations: magnon-assisted transport and the effect of spin-transfer torque on the magnetoconductance. The latter stems from magnetic misalignment in the junction induced by spin-current fluctuations. As the te…
The transport properties of micrometer scale structures fabricated from high-mobility HgTe quantum-wells have been investigated. A special photoresist and Ti masks were used, which allow for the fabrication of devices with characteristic dimensions down to 0.45 $μ$m. Evidence that the transport properties are dominated by ballistic effects in these structures is presented. Monte Carlo simulations of semi-classical electron trajectories show good agreement with the experiment.
Unlike classical heat diffusion at the macroscale, nanoscale heat transport can occur without energy dissipation because phonons can travel in straight lines for hundreds of nanometres. Despite recent experimental evidence of such ballistic phonon transport, control over its directionality, and thus its practical use, remains a challenge, as the directions of individual phonons are chaotic. Here, we show a way to control the directionality of ballistic phonon transport using silicon thin-films with arrays of holes. First, we demonstrate the formation of directional heat fluxes in the passages …
Because of high surface-to-volume ratio, the most prominent size effect limiting thermal transport originates from phonon-surface scattering in nanostructures. Herein we propose the mechanism of phonon scattering by the bond strength imperfections on surface of nanostructures, and derive the phonon scattering rate of this mechanism by quantum perturbation theory combining with bond order theory. By incorporating this phonon-surface scattering mechanism to phonon Boltzmann transport equation, we calculate the thermal conductivity of silicon thin films and silicon nanowires, and find that the ca…
Landauer-Büttiker formula describes the electronic quantum transports in nanostructures and molecules. It will be numerically demanding for simulations of complex or large size systems due to, for example, matrix inversion calculations. Recently, Chebyshev polynomial method has attracted intense interests in numerical simulations of quantum systems due to the high efficiency in parallelization, because the only matrix operation it involves is just the product of sparse matrices and vectors. Many progresses have been made on the Chebyshev polynomial representations of physical quantities for is…
Recent progress in physics on spin dependent transport in magnetic nanostructures is reviewed. Special attention is paid on the spin accumulation and spin current caused by spin injection into non-magnetic metals and semiconductors and superconductors. A variety of phenomena induced in nano-superconductor/ferromagnet devices are proposed, examining the spin-charge separation in superconductors.
Understanding phonon transport mechanisms in nanostructures is of great importance for delicately tailoring thermal properties. Combining phonon particle and wave effects through different strategies, previous studies have obtained ultra-low thermal conductivity in nanostructures. However, phonon particle and wave effects are coupled together, that is their individual contributions to phonon transport cannot be figured out. Here, we present how to quantify the particle and wave effects on phonon transport by combining Monte Carlo and atomic green function methods. We apply it to 1D silicon nan…
We consider the question of how to distinguish quantum from classical transport through nanostructures. To address this issue we have derived two inequalities for temporal correlations in nonequilibrium transport in nanostructures weakly coupled to leads. The first inequality concerns local charge measurements and is of general validity; the second concerns the current flow through the device and is relevant for double quantum dots. Violation of either of these inequalities indicates that physics beyond that of a classical Markovian model is occurring in the nanostructure.
We have developed a quantum noise approach to study the phonon transport through nanostructures. The nanostructures acting as phonon channels are attached to two phonon reservoirs. And the temperature drop between the two reservoirs drives the phonon transport through the channels. We have derived a quantum Langevin equation(QLE) to describe the phonon transport with the quantum noise originated from the thermal fluctuation of the reservoirs. Within the Markov approximation, the QLE is used to get the thermal conductivity $κ$ of the nanostructures and the finite size effect of the $κ$ then is …
The Braess paradox, known for traffic and other classical networks, lies in the fact that adding a new route to a congested network in an attempt to relieve congestion can counter-intuitively degrade the overall network performance. Recently, we have extended the concept of Braess paradox to semiconductor mesoscopic networks, whose transport properties are governed by quantum physics. In this paper, we demonstrate theoretically that, alike in classical systems, congestion plays a key role in the occurrence of a Braess paradox in mesoscopic networks.
We study coherent transport in a system of a periodic linear chain of quantum dots placed between two parallel quantum wires. We show that resonant-tunneling conductance between the wires exhibits a Rabi splitting of the resonance peak as a function of Fermi energy in the wires indicating the emergence of strong coupling between the system constituents. The underlying mechanism of the strong coupling regime is conservation of the quasimomentum in a periodic system that leads to transition resonances between electron states in a quantum dot chain and quantum wires. A perpendicular magnetic fiel…
Using an approach to open quantum systems based on the effective non-Hermitian Hamiltonian, we fully describe transport properties for a paradigmatic model of a coherent quantum transmitter: a finite sequence of square potential barriers. We consider the general case of asymmetric external barriers and variable coupling strength to the environment. We demonstrate that transport properties are very sensitive to the degree of opening of the system and determine the parameters for maximum transmission at any given degree of asymmetry. Analyzing the complex eigenvalues of the non-Hermitian Hamilto…
Graphene is an interesting material for spintronics, showing long spin relaxation lengths even at room temperature. For future spintronic devices it is important to understand the behavior of the spins and the limitations for spin transport in structures where the dimensions are smaller than the spin relaxation length. However, the study of spin injection and transport in graphene nanostructures is highly unexplored. Here we study the spin injection and relaxation in nanostructured graphene with dimensions smaller than the spin relaxation length. For graphene nanoislands, where the edge length…
A summary is given of a talk on the physics and technology of hybrid metallic nanostructures, with a view to metallic nanoelectronics. In the beginning of the talk it was noted that the majority of the presentations at the conference were not concerned with electronics but the physics of sensors, since they were devoted to studies of the influence of temperature, magnetic field, whereas electronics is all about modulation of electrical conductance by electrical means. An overview was given of the latest research into electric field effects in metals, including quantum field effects and effects…
Hierarchical material nanostructuring is considered to be a very promising direction for high performance thermoelectric materials. In this work we investigate thermal transport in hierarchically nanostructured silicon. We consider the combined presence of nanocrystallinity and nanopores, arranged under both ordered and randomized positions and sizes, by solving the Boltzmann transport equation using the Monte Carlo method. We show that nanocrystalline boundaries degrade the thermal conductivity more drastically when the average grain size becomes smaller than the average phonon mean free path…
Two-dimensional (2D) materials for their versatile band structures and strictly 2D nature have attracted considerable attention over the past decade. Graphene is a robust material for spintronics owing to its weak spin-orbit and hyperfine interactions, while monolayer transition metal dichalcogenides (TMDs) possess a Zeeman effect-like band splitting in which the spin and valley degrees of freedom are nondegenerate. The surface states of topological insulators (TIs) exhibit a spin-momentum locking that opens up the possibility of controlling the spin degree of freedom in the absence of an exte…
Electron transport through nanodevices of atoms in a single-layer rectangular arrangement with free (open) boundary conditions parallel to the direction of the current flow is studied within the single-band tight binding model. The Landauer formula gives the electrical conductance to be a function of the electron transmission probability, ${\cal T}(E)$, as a function of the energy $E$ of the incoming electron. A quantum dragon nanodevice is one which has a perfectly conducting channel, namely ${\cal T}(E)=1$ for all energies which are transmitted by the external leads even though there may be …
We present a comparative study of the (magneto)transport properties, including Hall effect, of bulk, thin film and nanostructured MnSi. In order to set our results in relation to published data we extensively characterize our materials, this way establishing a comparatively good sample quality. Our analysis reveals that in particular for thin film and nanostructured material, there are extrinsic and intrinsic contributions to the electronic transport properties, which by modeling the data we separate out. Finally, we discuss our Hall effect data of nanostructured MnSi under consideration of th…
We present measurements of low frequency charge noise and conductance drift in modulation doped GaAs/AlGaAs heterostructures grown by molecular beam epitaxy in which the silicon doping density has been varied from $2.4\times 10^{18} cm^{-3}$ (critically doped) to $6.0\times 10^{18} cm^{-3}$ (overdoped). Quantum point contacts were used to detect charge fluctuations. A clear reduction of both short time scale telegraphic noise and long time scale conductance drift with decreased doping density was observed. These measurements indicate that the {\it neutral} doping region plays a significant rol…
All-electrical generation and detection of pure spin currents is a promising way towards controlling the diffusive magnon transport in magnetically ordered insulators. We quantitatively compare two measurement schemes, which allow to measure the magnon spin transport in a three-terminal device based on a yttrium iron garnet thin film. We demonstrate that the dc charge current method based on the current reversal technique and the ac charge current method utilizing first and second harmonic lock-in detection can both efficiently distinguish between electrically and thermally injected magnons. I…
In this colloquia review we discuss methods for thermal transport calculations for nanojunctions connected to two semi-infinite leads served as heat-baths. Our emphases are on fundamental quantum theory and atomistic models. We begin with an introduction of the Landauer formula for ballistic thermal transport and give its derivation from scattering wave point of view. Several methods (scattering boundary condition, mode-matching, Piccard and Caroli formulas) of calculating the phonon transmission coefficients are given. The nonequilibrium Green's function (NEGF) method is reviewed and the Caro…
Our primary goal is to provide a rigorous treatment of scattering nonlocality in semiconductor nanostructures. On the one hand, starting from the conventional density-matrix formulation and employing as ideal instrument for the study of the semiclassical limit the well-known Wigner-function picture, we shall perform a fully quantum-mechanical derivation of the space-dependent Boltzmann equation. On the other hand, we shall examine the validity limits of such semiclassical framework, pointing out, in particular, regimes where scattering-nonlocality effects may play a relevant role; to this end …
At low temperatures when the phonon modes are effectively frozen, photon transport is the dominating mechanism of thermal relaxation in metallic systems. Starting from a microscopic many-body Hamiltonian, we develop a nonequilibrium Green's function method to study energy transport by photons in nanostructures. A formally exact expression for the energy current between a metallic island and a one-dimensional electromagnetic field is obtained. From this expression we derive the quantized thermal conductance as well as show how the results can be generalized to nonequilibrium situations. General…
Imaging heat transport in suspended diamond nanostructures with integrated spin defect thermometers
Swiss Federal Institute of Technology Lausanne (EPFL)（洛桑联邦理工学院）；PROUD SA（PROUD公司）；Istituto Nazionale di Ricerca Metrologica (INRiM)（意大利国家计量研究所）；University of Stuttgart（斯图加特大学）
We derive an $n$-resolved Master equation for quantum transport that includes a dependence on the number $n$ of tunneled electrons in system parameters such as tunnel rates and energy levels. We apply the formalism to describe dynamical changes due to random backaction effects, for example due to local fluctuations of the electrostatic landscape during the transport process. We quantify the amount of additional noise on top of electron shot noise due to these fluctuations by giving explicit expressions both for sequential and coherent tunneling examples.
This work summarizes recent progress on the thermal transport properties of three-dimensional (3D) nanostructures, with an emphasis on experimental results. Depending on the applications, different 3D nanostructures can be prepared or designed to either achieve a low thermal conductivity for thermal insulation or thermoelectric devices, or a high thermal conductivity for thermal interface materials used in the continuing miniaturization of electronics. A broad range of 3D nanostructures have been discussed, ranging from colloidal crystals/assemblies, array structures, holey structures, hierarc…
We observe large amplitude changes in the resistance of ferromagnetic (F) wires at the onset of superconductivity of adjacent superconductors (S). New sharp peaks of large amplitude are found in the magnetoresistance of the F-wires. We discuss a new mechanism for the long-range superconducting proximity effect in F/S nanostructures based on the analysis of the topologies of actual Fermi-surfaces in ferromagnetic metals.
We present a theory of finite-frequency noise in non-equilibrium conductors. It is shown that Non-Markovian correlations are essential to describe the physics of quantum noise. In particular, we show the importance of a correct treatment of the initial system-bath correlations, and how these can be calculated using the formalism of quantum master equations. Our method is particularly important in interacting systems, and when the measured frequencies are larger that the temperature and applied voltage. In this regime, quantum-noise steps are expected in the power spectrum due to vacuum fluctua…
Electron transport in branched semiconductor nanostructures provides many possibilities for creating fundamentally new devices. We solve the problem of its calculation using a quantum network model. The proposed scheme consists of three computational parts: S-matrix of the network junction, S-matrix of the network in terms of its junctions' S-matrices, electric currents through the network based on its S-matrix. To calculate the S-matrix of the network junction, we propose scattering boundary conditions in a clear integro-differential form. As an alternative, we also consider the Dirichlet-to-…
We report an experimental investigation of the edge effect on the room-temperature transport in graphene nanoribbon and graphene sheet (both single-layer and bilayer). By measuring the resistance scaling behaviors at both low and high carrier densities, we show that the transport of single-layer nanoribbons lies in a strong localization regime, which can be attributed to an edge effect. We find that this edge effect can be weakened by enlarging the width, decreasing the carrier densities or adding an extra layer. From graphene nanoribbon to graphene sheet, the data show a dimensional crossover…
Nanoscience offers a unique opportunity to design modern materials from the bottom up, via low-cost, solution processed assembly of nanoscale building blocks. These systems promise electronic band structure engineering using not only the nanoscale structural modulation, but also the mesoscale spatial patterning, although experimental realization of the latter has been challenging. Here we design and fabricate a new type of artificial solid by stacking graphene on a self-assembled, nearly periodic array of nanospheres, and experimentally observe superlattice miniband effects. We find conductanc…
We study transport properties of graphene nanostructures consisted of alternating slabs of gapless and gapped graphene in the presence of piecewise constant external potential equal to zero in the gapless regions. The transmission through single-, double-barrier structures and superlattices has been studied. It was revealed that any n-barrier structure is perfectly transparent at certain conditions defining the positions of new Dirac points created in the superlattice. The conductance and the shot noise were as well computed and investigated for the considered graphene systems. In a general ca…
We study a structure consisting of a ferromagnetic (F) layer coupled to two normal metal (N) leads. The system is driven out of equilibrium by the simultaneous application of external dc and ac voltages across the N/F/N structure. Using the Keldysh diagrammatic approach, and modeling the ferromagnet as a classical spin of size S >> 1, we derive the Langevin equation for the magnetization dynamics and calculate the noise correlator. We find that the noise has an explicit frequency dependence in addition to depending on the characteristics of the ac and dc drive. Further, we calculate the curren…
