We introduce a deductive statistical mechanics approach for granular materials which is formally built from few realistic physical assumptions. The main finding is an universal behavior for the distribution of the density fluctuations. Such a distribution is the equivalent of the Maxwell-Boltzmann's distribution in the kinetic theory of gasses. The comparison with a very extensive set of experimental and simulation data for packings of monosized spherical grains, reveals a remarkably good quantitative agreement with the theoretical predictions for the density fluctuations both at the grain level and at the global system level. Such agreement is robust over a broad range of packing fractions and it is observed in several distinct systems prepared by using different methods. The equilibrium distributions are characterized by only one parameter ($k$) which is a quantity very sensitive to changes in the structural organization. The thermodynamical equivalent of $k$ and its relation with the `granular temperature' are also discussed.
Granular segregation is ubiquitous in industrial, geological or daily-life context, but there is still no unifying theoretical approach. In this review, we examine two examples of granular segregation -- shallow rapid flows and rotating drums -- which suggest that the dynamics of systems at intermediate and high density might be amenable to a statistical mechanics approach.
The {\em hydrodynamic} approach to a continuum mechanical description of granular behavior is reviewed and elucidated. By considering energy and momentum conservation simultaneously, the general formalism of {\em hydrodynamics} provides a systematic method to {derive} the structure of constitutive relations, including all gradient terms needed for nonuniform systems. An important input to arrive at different relations (say, for Newtonian fluid, solid and granular medium) is the energy, especially the number and types of its variables. Starting from a careful examination of the physics underlyi…
This paper models the increase of density of a virgin loose granular sample submitted to a progressive axisymmetric compression (either isotropic or anisotropic) as an irreversible process which destroys the larger voids; a statistical mechanics approach similar to the one proposed by Boutreux & de Gennes is performed which leads to the equation of the density of normally consolidated states as a function of pressure; this equation is in agreement with experimental data and the typical variation of e (void index) or v (specific volume) vs. ln(p) .
This paper aims to justify the use of statistical mechanics tools in situations where the system is out of equilibrium and jammed. Specifically, we derive a Boltzmann equation for a jammed granular system and show that the Boltzmann's analysis can be used to produce a ``Second Law'', $\dot{S}\ge 0$ for jammed systems. We highlight the fundamental questions in this area of physics and point to the key quantities in characterising a packing of particles, accessible through a novel experimentation method which we also present here.
Magic Sand, a hydrophobic toy granular material, is widely used in popular science instructions because of its non-intuitive mechanical properties. A detailed study of the failure of an underwater column of magic sand shows that these properties can be traced to a single phenomenon: the system self-generates a cohesive skin that encapsulates the material inside. The skin, consists of pinned air-water-grain interfaces, shows multi-scale mechanical properties: they range from contact-line dynamics in the intra-grain roughness scale, plastic flow at the grain scale, all the way to the sample-scal…
Changes in the mechanical properties of granular materials, induced by variations in the intrinsic compressibility of the particles, are investigated by means of numerical simulations based on the combination of the Finite Element and Contact Dynamics methods. Assemblies of athermal 2D particles are subjected to quasi-static uni-axial compactions up to packing fractions close to $1$. Inspired by the contact mechanics in the Hertz's limit, we show that the effect of the compressibility of the particles both on the global and the local stresses, can be described by considering only the packing f…
A new first-principles statistical mechanics formulation is proposed to describe slow and dilated granular fluids, where prolonged intergranular contacts vitiate collision theory. The contacts, where all the important physics takes place, are regarded as quasi-particles that can appear and disappear. A contact potential, $ν$, is defined as a measure of the fluctuations and the mean coordination number per particle and its fluctuations are calculated as a function of it. This formulation extends the Edwards statistical mechanics to slow dynamic systems and converges to it when the motion stops.…
"Granular elasticity," useful for calculating static stress distributions in granular media, is generalized by including the effects of slowly moving, deformed grains. The result is a hydrodynamic theory for granular solids that agrees well with models from soil mechanics.
In the present letter a method to find a proper expression for the force distribution inside a granular sample in static equilibrium is proposed. The method is based in statistical mechanics and the force distribution is obtained by studying how the potential elastic energy is divided among the different contacts between grains. It is found with DEM simulations with spheres that the elastic potential energy distribution follows a Bose Einstein law from which the force distribution is deduced. The present letter open a way in which granular materials can be studied with the tools provided by st…
By detailed Molecular Dynamics and Monte Carlo simulations %of a realistic model we show that granular materials at rest can be described as thermodynamics systems. First we show that granular packs can be characterized by few parameters, as much as fluids or solids. Then, in a second independent step, we demonstrate that these states can be described in terms of equilibrium distributions which coincide with the Statistical Mechanics of powders first proposed by Edwards. We also derive the system equation of state as a function of the ``configurational temperature'', its new intensive thermody…
We employ a novel fluid-particle model to study the shearing behavior of granular soils under different saturation levels, ranging from the dry material via the capillary bridge regime to higher saturation levels with percolating clusters. The full complexity of possible liquid morphologies is taken into account, implying the formation of isolated arbitrary-sized liquid clusters with individual Laplace pressures that evolve by liquid exchange via films on the grain surface. Liquid clusters can grow in size, shrink, merge and split, depending on local conditions, changes of accessible liquid an…
Under external perturbations, inter-particle forces in disordered granular media are well known to form a heterogeneous distribution with filamentary patterns. Better understanding these forces and the distribution is important for predicting the collective behavior of granular media, the media second only to water as the most manipulated material in global industry. However, studies in this regard so far have been largely confined to granular media exhibiting only geometric heterogeneity, leaving the dimension of mechanical heterogeneity a rather uncharted area. Here, through a FEM contact me…
The behavior of an ultrasonic shot peening process is observed and analyzed by using a model of inelastic hard spheres in a gravitational field that are fluidized by a vibrating bottom wall (sonotrode) in a cylindrical chamber. A marked heterogeneous distribution of impacts appears when the collision between the shot and the side wall becomes inelastic with constant dissipation. This effect is one order of magnitude larger than the simple heterogeneity arising from boundary collision on the cylinder. Variable restitution coefficients bring the simulation closer to the general observation and a…
We use an analogy with the statistical mechanics of gas to build the statistical mechanics of granular media. The case of an isotropic disordered packing of equal spheres submitted to an isotropic stress is considered. We use the assumption of a maximal disorder and the method of the Lagrange multipliers to demonstrate that the distribution of the force moduli decreases exponentially and obeys an exponential-decay statistics. This distribution results from the above hypotheses and from the existence of a mean stress, which acts as a constraint. This distribution is confirmed by experiments and…
Statistical equivalence of reduced gravity and enhanced friction in granular packings
Shanghai Jiao Tong University（上海交通大学）；The Hong Kong University of Science and Technology（香港科技大学）；East China Normal University（华东师范大学）；Chengdu University of Technology（成都理工大学）
Recent work on suspension flows has shown that contact mechanics plays a role in suspension flow dynamics. The contact mechanics between particulate matter in dispersions should depend sensitively on the composition of the dispersed phase: evidently emulsion droplets interact differently with each other than angular sand particles. We therefore ask: what is the role of contact mechanics in dispersed media flow? We focus on slow flows, where contacts are long-lasting and hence contact mechanics effects should be most visible. To answer our question, we synthesize soft hydrogel particles with di…
Tunable mechanical properties and air-based lubrication in an acoustically levitated granular material
James Franck Institute, University of Chicago（詹姆斯·弗兰克研究所，芝加哥大学）；Department of Physics, University of Chicago（芝加哥大学物理系）；Department of Physics, Drexel University（德雷塞尔大学物理系）；Department of Chemistry, Stanford University（斯坦福大学化学系）；Department of Radiology, Stanford University（斯坦福大学放射学系）；Department of Chemical Engineering, Stanford University（斯坦福大学化学工程系）
An self-contained elastic theory is derived which accounts both for mechanical yield and shear-induced volume dilatancy. Its two essential ingredients are thermodynamic instability and the dependence of the elastic moduli on compression.
Confinement of a slender body into a granular array induces stress localization in the geometrically nonlinear structure, and jamming, reordering, and vertical dislocation of the surrounding granular medium. By varying the initial packing density of grains and the length of a confined elastica, we identify the critical length necessary to induce jamming, and demonstrate an intricate coupling between folds that localize along grain boundaries. Above the jamming threshold, the characteristic length of elastica deformation is shown to scale with the length over which force field fluctuations prop…
Classical soil mechanics results are used to propose the equation of the jamming transition surface in the (stress, specific volume) space. Taking axis-ymmetric conditions, labelling q the deviatoric stress and p' the mean pressure applied on the granular skeleton, and considering normal range of pressure (10 kPa-10MPa) the equation of the surface of jamming transition is v = vo-m ln(p'/p'o)+ md ln(1+q q/(M' M' p' p')); M' is related to the friction angle, m and md are two constants which depend on soil characteristics; p'o is a "unit" pressure.
A zero-temperature critical point has been invoked to control the anomalous behavior of granular matter as it approaches jamming or mechanical arrest. Criticality manifests itself in an anomalous spectrum of low-frequency normal modes and scaling behavior near the jamming transition. The critical point may explain the peculiar mechanical properties of dissimilar systems such as glasses and granular materials. Here, we study the critical scenario via an experimental measurement of the normal modes frequencies of granular matter under stress from a pole decomposition analysis of the effective ma…
We study the mechanical response generated by local deformations in jammed packings of rigid disks. Based on discrete element simulations we determine the critical force of the local perturbation that is needed to break the mechanical equilibrium and examine the generated displacement field. Displacements decay as a power law of the distance from the perturbation point. The decay exponent and the critical force exhibit nontrivial dependence on the friction: Both quantities are nonmonotonic and have a sharp maximum at the friction coefficient 0.1. We find that the mechanical response properties…
It is proposed a simple non linear incremental modelling of the axi-symmetric compression of granular materials and powders. It describes the main features of undrained compression and of oedometric compression using the results of compression tests at constant lateral stress . It generalises the concept of characteristic state. It shows that trajectories arriving at a given critical state shall pertain to a single surface in the (v,q,p) space, which confirms the recent result demonstrating that Hvorslev's and Roscoe's surfaces are part of the same surface. Effects of induced anisotropy are di…
Granular fluids consist of collections of activated mesoscopic or macroscopic particles (e.g., powders or grains) whose flows often appear similar to those of normal fluids. To explore the qualitative and quantitative description of these flows an idealized model for such fluids, a system of smooth inelastic hard spheres, is considered. The single feature distinguishing granular and normal fluids being explored in this way is the inelasticity of collisions. The dominant differences observed in real granular fluids are indeed captured by this feature. Following a brief introductory description …
The impact dynamics between wet surfaces, which dominates the mechanical properties of wet granular matter, is studied both experimentally and theoretically. It is shown that the hysteretic formation and rupture of liquid capillary bridges between adjacent grains accounts reasonably well for most relevant cases of wet granular matter. The various dissipation mechanisms are discussed with particular emphasis on their relevance. Variations of the rupture energy loss with the impact energy are quantified and discussed.
DEM simulations were used to study the sensitivity of a granular system to the change of the mechanical properties of the grains, applied to the penetration of a cylindrical intruder near a vertical wall. The simulations reproduce a real experimental setup, changing the friction, the Young modulus and the restitution coefficient of the particles.
We study the behavior of an assembly of $N$ granular particles contained in two compartments within a simple kinetic approach. The particles belonging to each compartment collide inelastically with each other and are driven by a stochastic heat bath. In addition, the fastest particles can change compartment at a rate which depends on their kinetic energy. Via a Boltzmann velocity distribution approach we first study the dynamics of the model in terms of a coupled set of equations for the populations in the containers and their granular temperatures and find a crossover from a symmetric high-te…
This paper investigates the effect of initial volume fraction on the runout characteristics of collapse of granular columns on slopes in fluid. Two-dimensional sub-grain scale numerical simulations are performed to understand the flow dynamics of granular collapse in fluid. The Discrete Element (DEM) technique is coupled with the Lattice Boltzmann Method (LBM), for fluid-grain interactions, to understand the evolution of submerged granular flows. The fluid phase is simulated using Multiple- Relaxation-Time LBM (LBM-MRT) for numerical stability. In order to simulate interconnected pore space in…
Using the recent incremental modelling, it is shown that the trajectory of a sample in the phase space of soil mechanics in the vicinity of the critical state is not governed by the rigidity matrix, but by its variations. The characteristics are used to predict that pseudo Young modulus tends to 0 as B -M-1 tends to 0, i.e. near the critical point, where B is the vertical-to-lateral-stress ratio during an axi-symmetric test. An attempt to understand and predict unstable behaviours is done using the same modelling. Compatibility of this modelling with results on soil liquefaction is emphasised.
Theoretical treatments of frictional granular matter often assume that it is legitimate to invoke classical elastic theory to describe its coarse-grained mechanical properties. Here we show, based on experiments and numerical simulations, that this is generically not the case since stress auto-correlation functions decay more slowly than the elastic Green's function. It was shown theoretically that standard elastic decay demands pressure and torque density fluctuations to be normal, with possibly one of them being hyperuniform. Generic compressed frictional assemblies exhibit however abnormal …
The paper addresses the underlying source of two forms of induced anisotropy in granular materials: contact orientation anisotropy and contact force anisotropy. A rational, mathematical structure is reviewed for the manner in which fabric anisotropy emerges and evolves during loading. Fabric is expressed as an orientation density, and transport phenomena such as convection, contact generation, and diffusion control the rate of fabric evolution during loading. The paper proposes specific measurable forms for all terms, based upon the micro-mechanics of particle interactions. Discrete element (D…
The question when and how dense granular materials start to flow under stress, despite many industrial and geophysical applications, remains largely unresolved. We develop and test a simple equation for the onset of quasi-static flows of granular materials which is based on the frictional aging of the granular packing. The result is a non-monotonic stress-strain relation which - akin to classical friction - is independent of the shear rate. This relation suffices to understand the below-threshold deformations of aging granular media, and its solid-to-liquid transition. Our results also elucida…
A systematic and mechanistic connection between granular materials' macroscopic and grain level behaviors is developed for monodisperse systems of spherical elastic particles under die compaction. The Granular Micromechanics Approach (GMA) with static assumption is used to derive the stiffness tensor of transversely isotropic materials, from the average behavior of particle-particle interactions in all different directions at the microscale. Two particle-scale directional density distribution functions, namely the directional distribution of a combined mechano-geometrical property and the dire…
Granular matter is comprised of a large number of particles whose collective behavior determines macroscopic properties such as flow and mechanical strength. A comprehensive theory of the properties of granular matter, therefore, requires a statistical framework. In molecular matter, equilibrium statistical mechanics, which is founded on the principle of conservation of energy, provides this framework. Grains, however, are small but macroscopic objects whose interactions are dissipative since energy can be lost through excitations of the internal degrees of freedom. In this work, we construct …
Structural organization and correlations are studied in very large packings of equally sized acrylic spheres, reconstructed in three-dimensions by means of X-ray computed tomography. A novel technique, devised to analyze correlations among more than two spheres, shows that the structural organization can be conveniently studied in terms of a space-filling packing of irregular tetrahedra. The study of the volume distribution of such tetrahedra reveals an exponential decay in the region of large volumes; a behavior that is in very good quantitative agreement with theoretical prediction. I argue …
The dissipation properties of a fine sand system are investigated by a low-frequency mechanical spectroscopy. The experiments show many interesting profiles of the relative energy dissipation, which imply that some structural transition of force chains in dense granular media has occurred. The following data and discussion indicate that the transition of force chains will lead to the small deformation of arrangement in the granular system, which is responsible for the historical effects. We hope this research can improve our knowledge of the microstructure of the granular materials.
Using X-ray tomography, we experimentally investigate granular packings subject to mechanical tapping for three types of beads with different friction coefficients. We validate Edwards volume ensemble in these three-dimensional granular systems and establish a granular version of thermodynamic zeroth law. Within Edwards framework, we also explicitly clarify how friction influences granular statistical mechanics as modifying the density of states, which allows us to determine the entropy as a function of packing fraction and friction subsequently. Additionally, we obtain a granular jamming phas…
We discuss the statistical mechanics of granular matter and derive several significant results. First, we show that, contrary to common belief, the volume and stress ensembles are inter-dependent, necessitating the use of both. We use the combined ensemble to calculate explicitly expectation values of structural and stress-related quantities for two-dimensional systems. We thence demonstrate that structural properties may depend on the angoricity tensor and that stress-based quantities may depend on the compactivity. This calls into question previous statistical mechanical analyses of static g…
The physical properties of granular materials have been extensively studied in recent years. So far, however, there exists no theoretical framework which can explain the observations in a unified manner beyond the phenomenological jamming diagram [1]. This work focuses on the case of static granular matter, where we have constructed a statistical ensemble [2] which mirrors equilibrium statistical mechanics. This ensemble, which is based on the conservation properties of the stress tensor, is distinct from the original Edwards ensemble and applies to packings of deformable grains. We combine it…
The mechanical yield of dense granular materials is a fascinating rheological phenomenon, beyond which stress no longer increases with strain at a sufficiently large deformation. Understanding the behavior of mechanical responses associated with yielding is a fundamental goal in granular physics, and other related fields including glassy physics, material sciences, geophysics, and active matter biophysics. However, despite nearly half a century of theoretical efforts, the nature of yielding in amorphous solids remains largely elusive compared to its crystalline counterpart. Here, we experiment…
A thermodynamic formulation of jammed matter is reviewed. Experiments and simulations of compressed emulsions and granular materials are then used to provide a foundation for the thermodynamics.
This textbook in French describes the rheology of granular materials in the quasi static regime at a macroscopic scale. It starts defining cohesion, friction and the Coulomb approach, from the large-strain range. Then it focuses on the range of small and intermediate deformation when the medium can dilate if it is dense; different specific typical tests (oedometric, constant pressure, constant volume) are defined, the behaviours they lead are carefully described and their dependences upon initial density recalled. Roles of friction and dilatancy are exemplified and their link with the deviator…
Dependence of structural self-organization of granular materials on preparation and grain parameters is key to predictive modelling. We study 60 different mechanically equilibrated polydisperse disc packs, generated numerically by two protocols. We show that, for same-variance disc size distributions (DSDs): 1. the mean coordination number of rattler-free packs vs. the packing fraction is a function independent of initial conditions, friction and the DSD: 2. all quadron volume and cell order distributions collapse to universal forms, also independent of the above. We conclude that, contrary to…
We study the geometrically induced cohesion of ensembles of granular "u-particles" which mechanically entangle through particle interpenetration. We vary the length-to-width ratio $l/w$ of the u-particles and form them into free-standing vertical columns. In laboratory experiment we monitor the response of the columns to sinusoidal vibration (frequency $f$, peak acceleration $Γ$). Column collapse occurs in a characteristic time, $τ$, which follows the relation $τ= f^{-1} \exp(Δ/ Γ)$. $Δ$ resembles an activation energy and is maximal at intermediate $l/w$. Simulation reveals that optimal streng…
In general, the mechanics of granular matter is described using continuum mechanics approach; this requires to introduce the concepts of stress and strain, which are averaged quantities, so that this needs also to introduce the notion of representative elementary volume (REV) above which averaged quantities have some physical meaning. As local quantities fluctuate spatially in granular matter; a local measure of stress and strain shall exhibit fluctuations too, whose typical amplitude depends on the sampling size L. This paper discusses this problem and the causes for large scale correlation. …
Mechanical impulse propagation in granular media depends strongly on the imposed confinement conditions. In this work, the propagation of sound in a granular packing contained by flexible walls that enable confinement under hydrostatic pressure conditions is investigated. This configuration also allows the form of the input impulse to be controlled by means of an instrumented impact pendulum. The main characteristics of mechan- ical wave propagation are analyzed, and it is found that the wave speed as function of the wave amplitude of the propagating pulse obeys the predictions of the Hertz co…
Experiments and computer simulations are carried out to investigate ordering principles in a granular gas which phase separates under vibration. The densities of the dilute and the dense phase are found to follow a lever rule. A Maxwell construction is found to predict both the coexisting pressure and binodal densities remarkably well, despite the fact that the pressure-volume characteristic $P(v)$ is not an isotherm. Although the system is far from equilibrium and energy conservation is strongly violated, we derive the construction from the minimization of mechanical work and fluctuating part…
We enumerate and classify nearly all of the possible mechanically stable (MS) packings of bidipserse mixtures of frictionless disks in small sheared systems. We find that MS packings form continuous geometrical families, where each family is defined by its particular network of particle contacts. We also monitor the dynamics of MS packings along geometrical families by applying quasistatic simple shear strain at zero pressure. For small numbers of particles (N < 16), we find that the dynamics is deterministic and highly contracting. That is, if the system is initialized in a MS packing at a gi…
In 1989, Sir Sam Edwards made the visionary proposition to treat jammed granular materials using a volume ensemble of equiprobable jammed states in analogy to thermal equilibrium statistical mechanics, despite their inherent athermal features. Since then, the statistical mechanics approach for jammed matter has garnered an extraordinary amount of attention by both theorists and experimentalists. Here, we review a systematic approach to jammed matter based on the Edwards statistical mechanical ensemble. We discuss the construction of microcanonical and canonical ensembles based on the volume fu…
We developed a novel experimental technique to generate mechanically stable (MS) packings of frictionless granular disks. We performed a series of coordinated experiments and numerical simulations to enumerate the MS packings in small 2D systems composed of bidisperse disks. We find that frictionless MS packings occur as discrete, well-separated points in configuration space and obtain excellent quantitative agreement between MS packings generated in experiments and simulations. In addition, we observe that MS packing probabilities can vary by many orders of magnitude and are robust with respe…
An understanding of homogeneous nucleation of crystalline structure from a disordered medium such as a liquid remains an important unsolved problem in condensed matter physics. Guided by the results from a number of experiments on granular and colloidal systems in the past two decades, including in particular observations of homogeneous nucleation in colloidal and granular systems, we suggest an alternative to the statistical mechanics approach to static granular matter initiated by Edwards and Oakeshott in 1989.
