Nonclassical correlations of phase noise and photon number in quantum nondemolition measurements
Holger F. Hofmann
备注：
16 pages, 5 figures, final version to be published in Phys. Rev. A, Clarifications of the nature of the measurement result and the noise added in section II
The continuous transition from a low resolution quantum nondemolition measurement of light field intensity to a precise measurement of photon number is described using a generalized measurement postulate. In the intermediate regime, quantization appears as a weak modulation of measurement probability. In this regime, the measurement result is strongly correlated with the amount of phase decoherence introduced by the measurement interaction. In particular, the accidental observation of half integer photon numbers preserves phase coherence in the light field, while the accidental observation of quantized values increases decoherence. The quantum mechanical nature of this correlation is discussed and the implications for the general interpretation of quantization are considered.
It is shown that the quantum jumps in the photon number n from zero to one or more photons induced by backaction evasion quantum nondemolition measurements of a quadrature component x of the vacuum light field state are strongly correlated with the quadrature component measurement results. This correlation corresponds to the operator expectation value <xnx> which is equal to one fourth for the vacuum even though the photon number eigenvalue is zero. Quantum nondemolition measurements of a quadrature component can thus provide experimental evidence of the nonclassical operator ordering dependen…
While quantum mechanics exquisitely describes the behavior of microscopic systems, one ongoing challenge is to explore its applicability to systems of larger size and mass. Unfortunately, quantum states of increasingly macroscopic objects are more easily corrupted by unintentional measurements from the classical environment. Additionally, even the intentional measurements from the observer can further perturb the system. In optomechanics, coherent light fields serve as the intermediary between the fragile mechanical states and our inherently classical world by exerting radiation pressure force…
We discuss the feasibility of a quantum nondemolition measurement (QND) of photon number based on cross phase modulation due to the Kerr effect in Photonic Crystal Waveguides (PCWs). In particular, we derive the equations for two modes propagating in PCWs and their coupling by a third order nonlinearity. The reduced group velocity and small cross-sectional area of the PCW lead to an enhancement of the interaction relative to bulk materials. We show that in principle, such experiments may be feasible with current photonic technologies, although they are limited by material properties. Our analy…
In this paper, we propose a resources-optimal linear-optical scheme for quantum nondemolition detection of single-photon presence. By measuring the state of ancillary photons, the presence of a photon in signal mode is revealed with a success probability of 1/2 without any disturbance to its state. We also show how to tune the setup to perform quantum nondemolition measurement of the signal photon state, and we provide tradeoff between the extracted information and the signal state disturbance. Moreover, the optimality of resources and methods by which to increase the success probability are d…
Experimental results stated in quant-ph/0612031 are seminal: The authors have realized nondemolition measurements of the photon number. As to the interpretation of the results, it seems to be less than convincing: The treatment of the system state and of the role of measurement is not compatible with the conventional point of view. We propose an adequate treatment, in which the experimental results are a manifestation of a partial Zeno effect (a slowdown of relaxation).
Quantum nondemolition (QND) measurements of photons is a much pursued endeavor in the field of quantum optics and quantum information processing. Here we propose a novel hybrid optoelectromechanical platform that integrates a cavity system with a hybrid electromechanical probe for QND photon counting. Building upon a mechanical-mode-mediated nonperturbative electro-optical dispersive coupling, our protocol performs the QND photon counting measurement by means of the current-voltage characteristics of the probe. In particular, we show that the peak voltage shift of the differential conductance …
Optical quantum nondemolition devices can provide essential tools for quantum information processing. Here, we describe several optical interferometers that signal the presence of a single photon in a particular input state without destroying it. We discuss both entanglement-assisted and non-entanglement-assisted interferometers, with ideal and realistic detectors. We found that existing detectors with 88% quantum efficiency and single-photon resolution can yield output fidelities of up to 89%, depending on the input state. Furthermore, we construct expanded protocols to perform QND detections…
Finite resolution quantum nondemolition (QND) measurements allow a determination of light field properties while preserving some of the original quantum coherence of the input state. It is thus possible to measure correlations between the photon number and a quadrature component of the same light field mode. Nonclassical features emerge as photon number quantization is resolved. In particular, a strong anti-correlation of quantization and coherence is observable in QND measurements of photon number, and a correlation between measurement induced quantum jumps and quadrature component measuremen…
Considering ultracold atoms traversing a high-Q Fabry-Perot cavity, we theoretically demonstrate a quantum nondemolition measurement of the photon number. This fully quantum mechanical approach may be understood utilizing concepts as effective mass and group velocity of the atom. The various photon numbers induce a splitting of the atomic wave packet, and a time-of-flight measurement of the atom thereby reveals the photon number. While repeated atomic measurements increase the efficiency of the protocol, it is shown that by considering long interaction times only a few atoms are needed to reso…
A polarization preserving quantum nondemolition photodetector is proposed based on nonlinearities obtainable through quantum coherence effects. An atomic level scheme is devised such that in the presence of strong linearly polarized drive field a coherent weak probe field acquires a phase proportional to the number of photons in the signal mode immaterial of its polarization state. It is also shown that the unavoidable phase-kicks resulting due to the measurement process are insensitive to the polarization state of the incoming signal photon. It is envisioned that such a device would have trem…
The ability to nondestructively detect the presence of a single, traveling photon has been a long-standing goal in optics, with applications in quantum information and measurement. Realising such a detector is complicated by the fact that photon-photon interactions are typically very weak. At microwave frequencies, very strong effective photon-photon interactions in a waveguide have recently been demonstrated. Here we show how this type of interaction can be used to realize a quantum nondemolition measurement of a single propagating microwave photon. The scheme we propose uses a chain of solid…
In quantum metrology schemes, one generally needs to prepare $m$ copies of $N$ entangled particles, such as entangled photon states, and then they are detected in a destructive process to estimate an unknown parameter. Here, we present a novel experimental scheme for estimating this parameter by using repeated indirect quantum nondemolition measurements in the setup called "photon box". This interaction-based scheme is able to achieve the phase sensitivity scaling as $1/N$ with a Fock state of $N$ photons. Moreover, we only need to prepare one initial $N$-photon state and it can be used repeti…
Realization of a room-temperature ultra-fast photon-number-resolving (PNR) quantum nondemolition (QND) measurement would have significant implications for photonic quantum information processing (QIP), enabling, e.g., deterministic quantum computation in discrete-variable architectures, but the requirement for strong coupling has hampered the development of scalable implementations. In this work, we propose and analyze a nonlinear-optical route to PNR QND using quadratic (i.e., $χ^{(2)}$) nonlinear interactions. We show that the coherent pump field driving a phase-mismatched optical parametric…
Nonclassical quantum effects gradually reach domains of physics of large systems previously considered as purely classical. We derive a hierarchy of operational criteria suitable for a reliable detection of nonclassicality of light from an arbitrarily large ensemble of independent single-photon emitters. We show, that such large ensemble can always emit nonclassical light without any phase reference and under realistic experimental conditions including incoherent background noise. The nonclassical light from the large ensemble of the emitters can be witnessed much better than light coming from…
We propose a technique for quantum nondemolition (QND) measurement and heralded preparation of Fock states by dynamics of electromagnetically induced transparency (EIT). An atomic ensemble trapped in an optical cavity is driven by two external continuous-wave classical fields to form EIT in steady state. As soon as a weak coherent field is injected into the cavity, the EIT system departs from steady state, falls into transient state dynamics by the dispersive coupling between cavity injected photons and atoms. Because the imaginary part of time-dependent linear susceptibility Im[X(t)] of the a…
Various nonclassical and quantum phase properties of photon added then subtracted displaced Fock state have been examined systematically and rigorously. Higher-order moments of the relevant bosonic operators are computed to test the nonclassicality of the state of interest, which reduces to various quantum states (having applications in quantum optics, metrology and information processing) in different limits ranging from the coherent (classical) state to the Fock (most nonclassical) states. The nonclassical features are discussed using Klyshko's, Vogel's, and Agarwal-Tara's criteria as well a…
The effect of two quantum state engineering processes that can be used to burn hole at vacuum in the photon number distribution of quantum states of radiation field are compared using various witnesses of lower- and higher-order nonclassicality as well as a measure of nonclassicality. Specifically, the witnesses of nonclassical properties due to the effect of vacuum state filtration and a single photon addition on an even coherent state, binomial state and Kerr state are investigated using the criteria of lower- and higher-order antibunching, squeezing and sub-Poissonian photon statistics. Fur…
The Lindblad approach to continuous quantum measurements is applied to a system composed of a two-level atom interacting with a stationary quantized electromagnetic field through a dispersive coupling fulfilling quantum nondemolition criteria. Two schemes of measurements are examined. The first one consists in measuring the atomic electric dipole, which indirectly allows one to infer the photon distribution inside the cavity. The second one schematizes a measurement of photon momentum, which permits to describe the atomic level distribution. Decoherence of the corresponding reduced density mat…
We present a scheme for multipartite entanglement purification of quantum systems in a Greenberger-Horne-Zeilinger state with quantum nondemolition detectors (QNDs). This scheme does not require the controlled-not gates which cannot be implemented perfectly with linear optical elements at present, but QNDs based on cross-Kerr nonlinearities. It works with two steps, i.e., the bit-flipping error correction and the phase-flipping error correction. These two steps can be iterated perfectly with parity checks and simple single-photon measurements. This scheme does not require the parties to posses…
Photon statistics is one of the key properties of the photon state for the study of quantum coherence and quantum information techniques. Here, we discuss the photon indistinguishability induced bunching effect which can significantly change photon statistics. Through the measurement of the second-order degree of coherence of a mixed photon state composed of a single-photon state and a weak coherent state, the statistical transition from a classical behavior to a nonclassical behavior is experimentally demonstrated by modifying the indistinguishability of the two-photon states. The study will …
Dispersive coupling based on the Rabi model with large detuning is widely used for quantum nondemolition (QND) qubit readout in quantum computation. However, the measurement speed and fidelity are usually significantly limited by the Purcell effects, i.e.: Purcell decay, critical photon numbers, and qubit-dependent Kerr nonlinearity. To avoid these effects, we propose how to realize an ideal QND readout of a gradiometric flux qubit with a tunable gap via its non-perturbative dispersive coupling (NPDC) to a frequency-tunable measurement resonator. We show that this NPDC-based readout mechanism …
Nonclassical properties of photon added and photon subtracted squeezed coherent states have been compared with specific focus on the higher order nonclassicalities, such as higher order squeezing, higher order sub-Poissonian photon statistics, higher order antibunching. It is observed that both photon added and photon subtracted squeezed coherent states are highly nonclassical as they satisfy criteria for all of the above mentioned nonclassicalities and a set of other criteria including negativity of Wigner function, Klyshko's criterion and Agarwal's $(A_{3})$ parameter. Further, the amount of…
We observe at record-high speed the nonclassical nature of ultra-broadband bi-photons, reducing the measurement time by four orders of magnitude compared to standard techniques of Hong-Ou-Mandel interference or sum-frequency generation. We measure the quantum state of the broadband bi-photons, amplitude and phase, with a pairwise "Mach-Zehnder" quantum interferometer, where bi-photons that are generated in one nonlinear crystal are enhanced (constructive interference) or diminished (destructive interference) in another crystal, depending on the bi-photon phase. We verify the quantum nature of …
We theoretically consider wave mixing under the irradiation of a single qubit by two photon fields. The first signal is a classical monochromatic drive, while the second one is a nonclassical light. Particularly, we address two examples of a nonclassical light: (i) a broadband squeezed light and (ii) a periodically excited quantum superposition of Fock states with 0 and 1 photons. The mixing of classical and nonclassical photon fields gives rise to side peaks due to the elastic multiphoton scattering. We show that side peaks structure is distinct from the situation when two classical fields ar…
Single photon sources are necessary for optical quantum technology. The nonclassicality of emitted single photons manifests itself in diverse experiments and applications. The applications already require different nonclassical aspects of single photons, however, a suitable hierarchy of criteria is missing. We propose variable experimental tests, based on adjustable linear optical networks and single photon detectors, giving a hierarchy of such nonclassicality criteria. The hierarchy goes beyond Hanbury - Brown - Twiss test of photon antibunching and allows us to compare faithfully quality and…
In cavity optomechanics, single photon detection of Raman scattered photons can be a useful tool for observing nonclassical features of both radiation and motion. While this tool has been employed in experiments with pulsed laser driving of a cavity mode, it has not been readily accessible to experiments with continuous and constant laser driving. To address this, we present a study of a standard optomechanical system where the cavity mode is continuously driven at two different frequencies, and where sideband photons are detected by single photon detectors after frequency filtering the output…
We derive a measurement operator corresponding to a quantum nondemolition (QND) measurement of an atomic ensemble. The quantum measurement operator takes the form of a positive operator valued measure (POVM) and is valid for arbitrary interaction times, initial coherent state amplitudes, and final photon measurement outcomes. We analyze the dependence on various parameters and show that the effect of the QND measurement for short interaction times is to apply a Gaussian modulation of the initial state wavefunction. We derive approximate expressions for the POVM in various limits, such as the s…
We present an experiment of nonclassical interference between a pure heralded single-photon state and a weak coherent state. Our experiment is the first to demonstrate that spectrally pure single photons can have high interference visibility, 89.4 \pm 0.5%, with weak coherent photons. Our scheme lays the groundwork for future experiments requiring quantum interference between photons in nonclassical states and those in coherent states.
Highly nonclassical character of optical quantum detectors, such as single-photon detectors, is essential for preparation of quantum states of light and a vast majority of applications in quantum metrology and quantum information processing. Therefore, it is both fundamentally interesting and practically relevant to investigate the nonclassical features of optical quantum measurements. Here we propose and experimentally demonstrate a procedure for direct certification of quantum non-Gaussianity and Wigner function negativity, two crucial nonclassicality levels, of photonic quantum detectors. R…
We use photon counters to obtain the joint photon counting statistics from twin-beam non-degenerate parametric down conversion, and we demonstrate directly, and with no auxiliary assumptions, that these twin beams are nonclassical.
Manipulating the frequency and bandwidth of nonclassical light is essential for implementing frequency-encoded/multiplexed quantum computation, communication, and networking protocols, and for bridging spectral mismatch among various quantum systems. However, quantum spectral control requires a strong nonlinearity mediated by light, microwave, or acoustics, which is challenging to realize with high efficiency, low noise, and on an integrated chip. Here, we demonstrate both frequency shifting and bandwidth compression of nonclassical light using an integrated thin-film lithium niobate (TFLN) ph…
The nonclassical effect of photon anti-bunching is observed in the mixed field of a narrow band two-photon source and a coherent field under certain condition. A variety of different features in photon statistics are found to be the consequence of a two-photon interference effect with dependence on the relative phase of the fields. Besides the anti-bunching effect, we find another one of the features to be also nonclassical. These features emphasize the importance of quantum entanglement.
Nonclassical properties of photon added and subtracted displaced Fock states have been studied using various witnesses of lower- and higher-order nonclassicality. Compact analytic expressions are obtained for the nonclassicality witnesses. Using those expressions, it is established that these states and the states that can be obtained as their limiting cases (except coherent states) are highly nonclassical as they show the existence of lower- and higher-order antibunching and sub-Poissonian photon statistics, in addition to the nonclassical features revealed through the Mandel $Q_M$ parameter,…
We study nonclassical features of multiphoton light emitted by clusters of single-photon emitters. As signatures of nonclassicality, we use violation of inequalities for normalized correlation functions of different orders or the probabilities of multiphoton detection. In experiment, for clusters of 2 to 14 colloidal CdSe/CdS dot-in-rods we observe nonclassical behavior, which gets even more pronounced for larger clusters.
We report demonstrations of both quadrature squeezed vacuum and photon number difference squeezing generated in an integrated nanophotonic device. Squeezed light is generated via strongly driven spontaneous four-wave mixing below threshold in silicon nitride microring resonators. The generated light is characterized with both homodyne detection and direct measurements of photon statistics using photon number-resolving transition edge sensors. We measure $1.0(1)$~dB of broadband quadrature squeezing (${\sim}4$~dB inferred on-chip) and $1.5(3)$~dB of photon number difference squeezing (${\sim}7$…
Detecting nonclassical properties that do not allow classical interpretation of photoelectric counting events is one of the crucial themes in quantum optics. Observation of individual nonclassical effects for a single-mode field, however, has been so far practically confined to sub-Poissonian statistics and quadrature squeezing. We show that a photon-added classical (coherent or thermal) state exhibits generalized nonclassical features in all orders of creation and annihilation operators, thereby becoming a promising candidate for studying higher-order nonclassical effects. Our analysis demons…
The nonclassical feature of photons in the open finite-size Dicke model is investigated via the two-photon correlation function. The quantum dressed master equation combined with the extended coherent photonic states is applied to analyze the dissipative dynamics of both the photons and qubits. The anti-bunching to bunching transition of photons is clearly observed by tuning the qubit-photon coupling strength. The optimal qubits number is unraveled to enhance the two-photon correlation function. Moreover, the temperature bias of thermal baths induces significant two-photon bunching signature w…
Higher-order nonclassical properties of r photon added and t photon subtracted qudit states (referred to as rPAQS and tPSQS, respectively) are investigated here to answer: How addition and subtraction of photon can be used engineer higher-order nonclassical properties of qudit states? To obtain the answer higher-order moment of relevant bosonic field operators are first obtained for rPAQS and tPSQS, and subsequently the same is used to study the higher-order nonclassical properties of the corresponding states. A few witnesses of higher-order nonclassicality (e.g. Higher-Order Antibunching, Hig…
Single photons and single-photon pairs, inherently nonclassical in their nature, are fundamental elements of quantum sciences and technologies. Here, we propose to realize the nonclassical correlated deterministic photon pairs at the single-photon level for a single atom trapped in bimodal cavities. It is shown that the photon emissions for bimodal cavities exhibit a high single photon purity and relatively large intracavity photon numbers, which are ascribed to the combination of optical Stark shift enhanced energy-spectrum anharmonicity and quantum interference suppressed two-photon excitati…
We report the experimental reconstruction of a nonclassicality quasiprobability for a single-photon added thermal state. This quantity has significant negativities, which is necessary and sufficient for the nonclassicality of the quantum state. Our method presents several advantages compared to the reconstruction of the P function, since the nonclassicality filters used in this case can regularize the quasiprobabilities as well as their statistical uncertainties. A-priori assumptions about the quantum state are therefore not necessary. We also demonstrate that, in principle, our method is not …
The effects of von Neumann postselected measurement on nonclassicality of single-photon-added coherent state (SPACS) are studied. Explicit expressions and analytical results for various field properties of SPACS such as the photon number distribution, the Mandel Q_{m} factor and the squeezing parameter of field quadrature after postselected von Neumann measurement are investigated. The results showed that the nonclassicality of SPACS after measurement changed dramatically than initial state. The measurement let SPACS possess more strong sub-Poissonian photon statistics in some definite couplin…
We report the observation of nonclassical light generated via photon blockade in a photonic crystal cavity with a strongly coupled quantum dot. By tuning the frequency of the probe laser with respect to the cavity and quantum dot resonance we can probe the system in either photon blockade or photon-induced tunneling regime. The transition from one regime to the other is confirmed by the measurement of the second order correlation that changes from anti-bunching to bunching.
Generation of nonclassical light suitable for interaction with atoms corresponds to a crucial goal pursued across the broad quantum optics community. We present the generation of nonclassical photon pairs using the process of spontaneous four-wave mixing in warm atomic vapor with an unprecedentedly high degree of nonclassical photon correlations. We show how the unique combination of excitation of atoms in the proximity of the vapor cell viewport, single excitation laser beam, double-$Λ$ energy level scheme, auxiliary optical pumping, and particular optical filtering setups, allow for the spec…
We investigate the dynamics of nonclassical states of light in coupled optical structures and we demonstrate a number of intriguing features associated with such arrangements. By diagonalizing the system's Hamiltonian, we show that these geometries can support eigenstates having anomalous optical intensity distribution with no classical counterpart. These features may provide new avenues towards manipulating light flow at the quantum level. By projecting the Hamiltonian operator on Hilbert subspaces spanning different numbers of photon excitations, we demonstrate that processes such as coheren…
We demonstrate, theoretically and experimentally, that statistical mixtures of the vacuum state |0> and the single-photon Fock state |1> are nonclassical according to the Vogel criterion (W. Vogel, Phys. Rev. Lett. 84, 1849 (2000)), regardless of the vacuum fraction. The ensembles are synthesized via conditional measurements on biphotons generated by means of parametric downconversion, and their quadrature statistics are measured using balanced homodyne detection. A comparative review of various quantum state nonclassicality criteria is presented.
We present a method for the experimental measurement of nonclassicality witnesses and demonstrate its application. Our proposal only requires the coherent displacement of the initial state, which can be achieved by overlapping the latter with a coherent state at a beam splitter, and subsequent photon-number resolved detection. This setup allows a complete test of nonclassicality of an arbitrary quantum state. The role of the quantum efficiency as well as statistical and systematic uncertainties are discussed. Finally, the scheme is demonstrated for a realistic example.
The measurement of joint signal-idler photon-number distribution of a field obtained from spontaneous parametric downconversion using an intensified CCD camera is presented. It is shown that a classicality criterion is violated directly by the measured data. Characteristic dimensions of the area of correlation are determined in the same experimental setup.
We report experimental generation of non-classically correlated photon pairs from collective emission in a room-temperature atomic vapor cell. The nonclassical feature of the emission is demonstrated by observing a violation of the Cauchy-Schwarz inequality. Each pair of correlated photons are separated by a controllable time delay up to 2 microseconds. This experiment demonstrates an important step towards the realization of the Duan-Lukin-Cirac-Zoller scheme for scalable long-distance quantum communication.
We study the robustness of quantum nondemolition (QND) measurement-induced entanglement between Bose-Einstein Condensates (BECs). We consider an experimental scheme where two BECs are placed in the paths of a Mach-Zehnder interferometer, and a QND interaction creates entanglement between coherent light and the atoms. We analyze the two dominant channels of decoherence, atomic dephasing and photon loss on the entangled states produced by this scheme. We calculate the effect of dephasing on the variance and expectation values of the spin operators, entanglement, and correlation criteria. Our ana…
We experimentally investigate a method of directly characterizing the photon number distribution of nonclassical light beams that is tolerant to losses and makes use only of standard binary detectors. This is achieved in a single measurement by calibrating the detector using some small amount of prior information about the source. We demonstrate the technique on a freely propagating heralded two-photon number state created by conditional detection of a two-mode squeezed state generated by a parametric downconverter.
It is often asserted that quantum effects can be observed in coincidence detection rates or other correlations, but never in the rate of single-photon detection. We observe nonclassical interference in a singles rate, thanks to the intrinsic nonlinearity of photon counters. This is due to a dependence of the effective detection efficiency on the quantum statistics of the light beam. Such measurements of detector response to photon pairs promise to shed light on the microscopic aspects of silicon photodetectors, and on general issues of quantum measurement and decoherence.
With a product state of the form $ρ_{in} = ρ_a\otimes|0>_b_b< 0|$ as input, the output two-mode state $ρ_{\rm out}$, of the beam splitter is shown to be NPT whenever the photon number distribution (PND) statistics $\{p(n_a) \}$ associated with the possibly mixed state $ρ_a$ of the a_mode is antibunched or otherwise nonclassical, i.e., if $\{p(n_a)\}$ fails to respect any one of an infinite of classicality conditions.
We examine nonclassical properties of the field states generated by applying the photon annihilation-then-creation operation (AC) and creation-then-annihilation operation (CA) to the thermal and coherent states. Effects of repeated applications of AC and of CA are also studied. We also discuss experimental schemes to realize AC and CA with a cavity system using atom-field interactions.
