Single photon sources are necessary for optical quantum technology. The nonclassicality of emitted single photons manifests itself in diverse experiments and applications. The applications already require different nonclassical aspects of single photons, however, a suitable hierarchy of criteria is missing. We propose variable experimental tests, based on adjustable linear optical networks and single photon detectors, giving a hierarchy of such nonclassicality criteria. The hierarchy goes beyond Hanbury - Brown - Twiss test of photon antibunching and allows us to compare faithfully quality and performance of single-photon sources via their nonclassical properties.
We experimentally examine the nonclassical character of a class of non-Gaussian states known as phase-diffused squeezed states. These states may show no squeezing effect at all, and therefore provide an interesting example to test nonclassicality criteria. The characteristic function of the Glauber-Sudarshan representation (P function) proves to be a powerful tool to detect nonclassicality. Using this criterion we find that phase-diffused squeezed states are always nonclassical, even if the squeezing effect vanishes. Testing other criteria of nonclassicality based on higher-order squeezing and…
A method is introduced for the verification of nonclassicality in terms of moments of nonclassicality quasiprobability distributions. The latter are easily obtained from experimental data and will be denoted as nonclassicality moments. Their relation to normally-ordered moments is derived, which enables us to verify nonclassicality by using well established criteria. Alternatively, nonclassicality criteria are directly formulated in terms of nonclassicality moments. The latter converge in proper limits to the usually used criteria, as is illustrated for squeezing and sub-Poissonian photon stat…
In this work we generalize the Bochner criterion addressing the characteristic function, i.e., the Fourier transform, of the Glauber-Sudarshan phase-space function. For this purpose we extend the Bochner theorem by including derivatives of the characteristic function. The resulting necessary and sufficient nonclassicality criteria unify previously known moment-based criteria with those based on the characteristic function. For applications of the generalized nonclassicality probes, we provide direct sampling formulas for balanced homodyne detection. A squeezed vacuum state is experimentally re…
We use the exact calculation of the quantum mechanical, temporal characteristic function $χ(η)$ and the degree of second-order coherence $g^{(2)}(τ)$ for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state, to study the different criteria for nonclassicality. In particular, we contrast criteria that involve only one-time functions of the dynamical system, for instance, the quasiprobability distribution $P(β)$ of the Glauber-Sudarshan coherent or P-representation of the density of state and the Mandel $Q_{M}(τ)$ parameter, …
We devise a new class of criteria to certify the nonclassicality of photon- and phonon-number statistics. Our criteria extend and strengthen the broadly used Klyshko's criteria, which require knowledge of only a finite set of Fock-state probabilities. This makes the criteria well-suited to experimental implementation in realistic conditions. Moreover, we prove the completeness of our method in some scenarios, showing that, when only two or three Fock-state probabilities are known, it detects all finite distributions incompatible with classical states. In particular, we show that our criteria d…
Nonclassicality criteria based on intensity moments and derived from the usual matrix approach are compared to those provided by the majorization theory. The majorization theory is shown to give a greater number of more suitable nonclassicality criteria. Fifteen experimentally useful criteria of the majorization theory containing the intensity moments up to the fifth order are identified. Their performance is experimentally demonstrated on the set of eleven potentially nonclassical states generated from a twin beam by postselection based on detecting a given number of photocounts in one arm by…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
Driven by single photon detection requirements especially for quantum information sciences, the theory of arrays of off-on detectors has been well developed and applied. However for a comprehensive characterization of nonclassicality one also needs phase sensitive properties. This missing link is fulfilled by the theory of phase sensitive click counting measurements. This theory is presented. It unifies the balanced homodyne detection for high intensities with the click detection in the few photon regime. We formulate and apply a hierarchy of nonlinear squeezing conditions to probe quantum eff…
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode (or multiparty) bosonic fields that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials, but also polynomial functions of such moments, which can sometimes enable simpler derivations of phys…
Nonclassical properties of photon added and photon subtracted squeezed coherent states have been compared with specific focus on the higher order nonclassicalities, such as higher order squeezing, higher order sub-Poissonian photon statistics, higher order antibunching. It is observed that both photon added and photon subtracted squeezed coherent states are highly nonclassical as they satisfy criteria for all of the above mentioned nonclassicalities and a set of other criteria including negativity of Wigner function, Klyshko's criterion and Agarwal's $(A_{3})$ parameter. Further, the amount of…
Mode-entanglement based criteria and measures become insufficient for broadband emission, e.g. from spasers (plasmonic nano-lasers). We introduce criteria and measures for the (i) total entanglement of two wavepackets, (ii) entanglement of a wavepacket with an ensemble and (iii) total nonclassicality of a wavepacket~(WP). We discuss these criteria in the context of (i) entanglement of two WPs emitted from two initially entangled cavities (or two initially entangled atoms) and (ii) entanglement of an emitted WP with the ensemble/atom for the spontaneous emission and the single-photon superradia…
We study different representations of a many-particle system. We reveal the stunning beauty of the connections among the nonclassicalities of a many-particle, a single-mode and a two-mode systems. First, we demonstrate that (separable) atomic coherent states~(ACSs), of a many-particle system, mimic the coherent states of single-mode light. This enables the utilization of a many-particle entanglement~(MPE) criterion as a single-mode nonclassicality~(SMNc) condition via Holstein-Primakoff transformation. As an example, we show that spin-squeezing criterion, for MPE, can be transformed into the q…
We calculate exactly the quantum mechanical, temporal characteristic function $χ(η)$ for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state. Knowledge of $χ(η)$ allows only the determination of the time development of arbitrary functions of equal-time products of creation and annihilation photon operators. We calculate, in particular, the fluctuations in photon number, quadrature operators, and quadrature variance. We contrast the very important difference between the nonclassicality criteria based on the one-time charact…
The nonclassicality of photon-added coherent fields in the thermal channel is investigated by exploring the volume of the negative part of the Wigner function which reduces with the dissipative time. The Wigner functions become positive when the decay time exceeds a threshold value. For the case of the single photon-added coherent state, we derive the exact threshold values of decay time in the thermal channel. For arbitrary partial negative Wigner distribution function, a generic analytical relation between the mean photon number of heat bath and the threshold value of decay time is presented…
Interference lies at the heart of the behavior of classical and quantum light. It is thus crucial to understand the boundaries between which interference patterns can be explained by a classical electromagnetic description of light and which, on the other hand, can only be understood with a proper quantum mechanical approach. While the case of two-mode interference has received a lot of attention, the multimode case has not yet been fully explored. Here we study a general scenario of intensity interferometry: we derive a bound on the average correlations between pairs of output intensities for…
We report the experimental realization and tomographic analysis of novel quantum light states obtained by exciting a classical thermal field by a single photon. Such states, although completely incoherent, possess a tunable degree of quantumness which is here exploited to put to a stringent experimental test some of the criteria proposed for the proof and the measurement of state non-classicality. The quantum character of the states is also given in quantum information terms by evaluating the amount of entanglement that they can produce.
We introduce a kind of entangled state---photon-addition two-mode squeezed thermal state (TMSTS) by adding photons to each mode of the TMSTS. Using the P-representation of thermal state, the compact expression of the normalization factor is derived, a Jacobi polynomial. The nonclassicality is investigated by exploring especially the negativity of Wigner function. The entanglement is discussed by using Shchukin-Vogel criteria. It is shown that the photon-addtion to the TMSTS may be more effective for the entanglement enhancement than the photon-subtraction from the TMSTS. In addition, the quant…
Recently, a non-Gaussian field, which may be a useful basis for entanglement distillation and efficient quantum teleportation, has been experimentally produced by subtracting a photon from a squeezed Gaussian field. We investigate the nonclassicality of such the field using negativity in the Wigner function and the existence of positive well-defined $P$ function. We obtain the condition to see negativity in the Wigner function for the case including the mixed Gaussian incoming field, the threshold photodetection and the inefficient homodyne measurement. We show how similar the photon-subtracte…
Theoretical analysis is given of nonclassicality and decoherence of the field states generated by adding any number of photons to the squeezed thermal state (STS). Based on the fact that the squeezed number state can be considered as a single-variable Hermite polynomial excited state, the compact expression of the normalization factor is derived, a Legendre polynomial. The nonclassicality is investigated by exploring the sub-Poissonian and negative Wigner function (WF). The results show that the WF of single photon-added STS (PASTS) always has negative values at the phase space center. The dec…
Machine-learning and neural-network approaches have gained huge attention in the context of quantum science and technology in recent years. One of the most essential tasks for the future development of quantum technologies is the verification of nonclassical resources. Here, we present an artificial neural network approach for the identification of nonclassical states of light based on recorded measurement statistics. In particular, we implement and train a network which is capable of recognizing nonclassical states based on the click statistics recorded with multiplexed detectors. We use simu…
The efficient certification of nonclassical effects of light forms the basis for applications in optical quantum technologies. We derive general correlation conditions for the verification of nonclassical light based on multiplexed detection. The obtained nonclassicality criteria are valid for imperfectly-balanced multiplexing scenarios with on-off detectors and do not require any knowledge about the detector system. In this sense they are fully independent of the detector system. In our experiment, we study light emitted by clusters of single-photon emitters, whose photon number may exceed th…
Two twin beams with a shared signal beam and separated idler beams are used together with the photon-number-resolving postselection in the signal beam to arrive at two coupled beams with anticorrelations in photon-number fluctuations. Moreover, the beams exhibit the sub-Poissonian photon-number statistics in their marginal distributions under suitable conditions. The postselected fields with the increasing mean photon numbers are reconstructed from the experimental photocount histograms by the maximum likelihood approach. Also a suitable Gaussian fit of both original twin beams and simulation …
We study the nonclassicality of photon-added squeezed vacuum (PASV) and its decoherence in thermal environment in terms of the sub-Poissonian statistics and the negativity of Wigner function (WF). By converting the PASV to a squeezed Hermite polynomial excitation state, we derive a compact expression for the normalization factor of m-PASV, which is an m-order Legendre polynomial of squeezing parameter r. We also derive the explicit expression of WF of m-PASV and find the negative region of WF in phase space. We show that there is an upper bound value of r for this state to exhibit sub-Poissoni…
The nonclassicality of single photon-added thermal states in the thermal channel is investigated by exploring the volume of the negative part of the Wigner function. The Wigner functions become positive when the decay time exceeds a threshold value $γ{t}_c$, which only depends on the effective temperature or mean thermal photon number of the thermal channel, but not depends on the effective temperature of the initial thermal state. This phenomenon is similar with the case of single quantum excitation of classical coherent states in thermal channel. Furthermore, we firstly demonstrate $γ{t}_c$ …
We present Bell-type tests of nonclassicality and non-Gaussianity for single-mode fields employing a generalized quasiprobability function. Our nonclassicality tests are based on the observation that two orthogonal quadratures in phase space (position and momentum) behave as independent realistic variables for a coherent state. Taking four (three) points at the vertices of a rectangle (right triangle) in phase space, our tests detect every pure nonclassical Gaussian state and a range of mixed Gaussian states. These tests also set an upper bound for all Gaussian states and their mixtures, which…
Various nonclassical and quantum phase properties of photon added then subtracted displaced Fock state have been examined systematically and rigorously. Higher-order moments of the relevant bosonic operators are computed to test the nonclassicality of the state of interest, which reduces to various quantum states (having applications in quantum optics, metrology and information processing) in different limits ranging from the coherent (classical) state to the Fock (most nonclassical) states. The nonclassical features are discussed using Klyshko's, Vogel's, and Agarwal-Tara's criteria as well a…
We study the evolution of higher-order nonclassicality and entanglement criteria in atmospheric fluctuating-loss channels. By formulating input-output relations for the matrix of moments, we investigate the influence of such channels on the corresponding quantumness criteria. This generalization of our previous work on Gaussian entanglement [M. Bohmann et al., Phys. Rev. A 94, 010302(R) (2016)] not only exploits second-order-based scenarios, but it also provides a detailed investigation of nonclassicality and entanglement in non-Gaussian and multimode radiation fields undergoing a fluctuating …
We introduce a quantum-optical notion of nonclassicality that we call as the process output nonclassicality for multimode quantum channels. The motivation comes from an information-theoretic point of view and the emphasis is on the output states of a channel. We deem a channel to be `classical' if its outputs are always classical irrespective of the input, i.e., if the channel is nonclassicality breaking, and nonclassical otherwise. Our condition is stronger than the one considered by Rahimi-Keshari et al. [PRL {\bf 110}, 160401 (2013)] and we compare the two approaches. Using our framework we…
A beam splitter can generate entanglement if the input field is nonclassical, e.g. squeezed. Thus, beam splitter transformation can be utilized for obtaining single-mode nonclassicality conditions from two-mode entanglement criteria. Here, we demonstrate that (i) the generalized quadrature-squeezing condition $\langle\hat{a}^\dagger\hat{a}\rangle < |\langle \hat{a}^2\rangle|$ can be obtained from the two-mode entanglement criterion of Duan-Giedke-Cirac-Zoller~[PRL 84, 2722]. (ii) Single-mode nonclassicality condition, obtained from the two-mode entanglement criterion of Simon~[PRL, 84 2726], c…
In a recent contribution, we introduced and applied a detector-independent method to uncover nonclassicality. Here, we extend those techniques and give more details on the performed analysis. We derive a general theory of the positive-operator-valued measure that describes multiplexing layouts with arbitrary detectors. From the resulting quantum version of a multinomial statistics, we infer nonclassicality probes based on a matrix of normally ordered moments. We discuss these criteria and apply the theory to our data which are measured with superconducting transition-edge sensors. Our experime…
The effect of two quantum state engineering processes that can be used to burn hole at vacuum in the photon number distribution of quantum states of radiation field are compared using various witnesses of lower- and higher-order nonclassicality as well as a measure of nonclassicality. Specifically, the witnesses of nonclassical properties due to the effect of vacuum state filtration and a single photon addition on an even coherent state, binomial state and Kerr state are investigated using the criteria of lower- and higher-order antibunching, squeezing and sub-Poissonian photon statistics. Fur…
The Glauber-Sudarshan diagonal `weight' function provides a natural divide between the quantum-optical notion of classical and nonclassical states of continuous variables systems. Based on this demarcation, a channel is said to be nonclassicality breaking if it outputs only classical states for any input state. We focus on multimode bosonic Gaussian channels and classify those that are nonclassicality breaking by introducing a criterion that needs to be satisfied by the matrices representing these channels. The criterion can be interpreted as a nonclassicality benchmark for these channels sinc…
Practically applicable criteria for the nonclassicality of quantum states are formulated in terms of different types of moments. For this purpose the moments of the creation and annihilation operators, of two quadratures, and of a quadrature and the photon number operator turn out to be useful. It is shown that all the required moments can be determined by homodyne correlation measurements. An example of a nonclassical effect that is easily characterized by our methods is amplitude-squared squeezing.
We demonstrate, theoretically and experimentally, that statistical mixtures of the vacuum state |0> and the single-photon Fock state |1> are nonclassical according to the Vogel criterion (W. Vogel, Phys. Rev. Lett. 84, 1849 (2000)), regardless of the vacuum fraction. The ensembles are synthesized via conditional measurements on biphotons generated by means of parametric downconversion, and their quadrature statistics are measured using balanced homodyne detection. A comparative review of various quantum state nonclassicality criteria is presented.
In the recent experimental and theoretical literature well-established nonclassicality criteria from the field of quantum optics have been directly applied to the case of excitations in matter-waves. Among these are violations of Cauchy-Schwarz inequalities, Glauber-Sudarshan P-nonclassicality, sub-Poissonian number-difference squeezing (also known as the two-mode variance) and the criterion of nonseparability. We review the strong connection of these criteria and their meaning in quantum optics, and point out differences in the interpretation between light and matter waves. We then calculate …
The interplay between the nonclassical features and the parity-time (PT) symmetry (or its breaking) is studied here by considering a PT symmetric system consisting of two cavities with gain and loss. The conditions for PT invariance is obtained for this system. The behavior of the average photon number corresponding to the gain and loss modes for different initial states (e.g., vacuum, NOON, coherent, and thermal states) has also been obtained. With the help of the number operators, quantum Zeno and anti-Zeno effects are studied, and the observed behavior is compared in PT symmetric (PTS) and …
We suggest a method to reconstruct the zero-delay-time second-order correlation function $g^{(2)}(0)$ of Gaussian states using a single homodyne detector. To this purpose, we have found an analytic expression of $g^{(2)}(0)$ for single- and two-mode Gaussian states in terms of the elements of their covariance matrix and the displacement amplitude. In the single-mode case we demonstrate our scheme experimentally, and also show that when the input state is nonclassical, there exist a threshold value of the coherent amplitude, and a range of values of the complex squeezing parameter, above which …
We calculate exactly the quantum mechanical, temporal Wigner quasiprobability density for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state. The Wigner function allows us to calculate the fluctuations in photon number and the quadrature variance. We contrast the difference between the nonclassicality criteria, which is independent of the displacement parameter $α$, based on the Glauber-Sudarshan quasiprobability distribution $P(β)$ and the classical/nonclassical behavior of the Mandel $Q_{M}(τ)$ parameter, which depends …
How much noise can a given quantum state tolerate without losing its entanglement? For qudits of arbitrary dimension, I investigate this question for two noise models: Global white noise, where a depolarizing channel is applied to all qudits simultaneously, and local white noise, where a single qudit depolarizing channel is applied to every qudit individually. Using a unitary generalization of the Pauli group, I derive noise thresholds for stabilizer states, with an emphasis on graph states, and compare different entanglement criteria. The PPT and reduction criteria generally provide high nois…
Nonclassical quantum effects gradually reach domains of physics of large systems previously considered as purely classical. We derive a hierarchy of operational criteria suitable for a reliable detection of nonclassicality of light from an arbitrarily large ensemble of independent single-photon emitters. We show, that such large ensemble can always emit nonclassical light without any phase reference and under realistic experimental conditions including incoherent background noise. The nonclassical light from the large ensemble of the emitters can be witnessed much better than light coming from…
We consider random bipartite quantum states obtained by tracing out one subsystem from a random, uniformly distributed, tripartite pure quantum state. We compute thresholds for the dimension of the system being traced out, so that the resulting bipartite quantum state satisfies the reduction criterion in different asymptotic regimes. We consider as well the basis-independent version of the reduction criterion (the absolute reduction criterion), computing thresholds for the corresponding eigenvalue sets. We do the same for other sets relevant in the study of absolute separability, using techniq…
Entanglement, one of the most intriguing aspects of quantum mechanics, marks itself into different features of quantum states. For this reason different criteria can be used for verifying entanglement. In this paper we review some of the entanglement criteria casted for continuous variable states and link them to peculiar aspects of the original debate on the famous EPR paradox. Moreover, we give a handy expression for valuating Bell-type non-locality on Gaussian states. We also present the experimental measurement of a particular realization of the Bell operator over continuous variable entan…
We calculate the quantum correlations existing among the three output fields (pump, signal, and idler) of a triply resonant non-degenerate Optical Parametric Oscillator operating above threshold. By applying the standard criteria [P. van Loock and A. Furusawa, Phys. Rev. A 67, 052315 (2003)], we show that strong tripartite continuous-variable entanglement is present in this well-known and simple system. Furthermore, since the entanglement is generated directly from a nonlinear process, the three entangled fields can have very different frequencies, opening the way for multicolored quantum info…
Nonclassical states, having no classical analogue, promise advantage in the performance in several fields of technology, such as computation, communication, sensing. This led to an escalated interest in the recent years for the generation and characterization of nonclassical states in various physical systems of interest. Keeping this in mind, we examined generation of various lower- and higher-order nonclassical states in both codirectional and contradirectional asymmetric nonlinear optical couplers operating under second harmonic generation with the help of moments-based criteria. Using anot…
