Nonclassicality criteria based on intensity moments and derived from the usual matrix approach are compared to those provided by the majorization theory. The majorization theory is shown to give a greater number of more suitable nonclassicality criteria. Fifteen experimentally useful criteria of the majorization theory containing the intensity moments up to the fifth order are identified. Their performance is experimentally demonstrated on the set of eleven potentially nonclassical states generated from a twin beam by postselection based on detecting a given number of photocounts in one arm by using an iCCD camera.
We present an experimental method for complete identification of the nonclassicality of Gaussian states in the whole phase space. Our method relies on nonclassicality witnesses written in terms of measured integrated intensity moments up to the third order, provided that appropriate local coherent displacements are applied to the state under consideration. The introduced approach, thus, only requires linear detectors for measuring intensities of optical fields, that is very convenient and powerful from the experimental point of view. Additionally, we demonstrate that the proposed technique not…
A method is introduced for the verification of nonclassicality in terms of moments of nonclassicality quasiprobability distributions. The latter are easily obtained from experimental data and will be denoted as nonclassicality moments. Their relation to normally-ordered moments is derived, which enables us to verify nonclassicality by using well established criteria. Alternatively, nonclassicality criteria are directly formulated in terms of nonclassicality moments. The latter converge in proper limits to the usually used criteria, as is illustrated for squeezing and sub-Poissonian photon stat…
The interaction between a $\diamondsuit$-type four-level atom and a single-mode field in the presence of Kerr medium with intensity-dependent coupling involving multi-photon processes has been studied. Using the generalized (nonlinear) Jaynes-Cummings model, the exact analytical solution of the wave function for the considered system under particular condition, has been obtained when the atom is initially excited to the topmost level and the field is in a coherent state. Some physical properties of the atom-field entangled state such as linear entropy showing the entanglement degree, Mandel pa…
We present a study of the electromagnetic control of nonclassicality of the outgoing light field in a single atom cavity QED system. By exploring the energy eigenvalues and eigenstates, we show that the eigenstates are similar to the Jaynes-Cummings ladder of eigenstates and can be optically controlled by an external control field. Tuning the control field frequency to the one photon resonance, we show the superbunching behavior in the outgoing light field can be observed at the frequency of one photon resonance. We also show that there exists a magic control field intensity at which two photo…
We develop a nonclassicality criterion for the interference of three delayed, but otherwise identical, light fields in a three-mode Bell interferometer. We do so by comparing the prediction of quantum mechanics with those of a classical framework in which independent sources emit electric fields with random phases. In particular, we evaluate third-order correlations among output intensities as a function of the delays, and show how the presence of a correlation revival for small delays cannot be explained by the classical model of light. The observation of a revival is thus a nonclassicality s…
We investigate the nonclassicality of photon-added coherent states in the photon loss channel by exploring the entanglement potential and negative Wigner distribution. The total negative probability defined by the absolute value of the integral of the Wigner function over the negative distribution region reduces with the increase of decay time. The total negative probability and the entanglement potential of pure photon-added coherent states exhibit the similar dependence on the beam intensity. The reduce of the total negative probability is consistent with the behavior of entanglement potenti…
We investigate the performance of a certain nonclassicality identifier, expressed via integrated second-order intensity moments of optical fields, in revealing bipartite entanglement of quantum-optical frequency combs (QOFCs), which are generated in both spontaneous and stimulated parametric down-conversion processes. We show that, by utilizing that nonclassicality identifier, one can well identify the entanglement of the QOFC directly from the experimentally measured intensity moments without invoking any state reconstruction techniques or homodyne detection. Moreover, we demonstrate that the…
We exploit results from the classical Stieltjes moment problem to bring out the totality of all the information regarding phase insensitive nonclassicality of a state as captured by the photon number distribution p_n. Central to our approach is the realization that n !p_n constitutes the sequence of moments of a (quasi) probability distribution, notwithstanding the fact that p_n can by itself be regarded as a probability distribution. This leads to classicality restrictions on p_n that are local in n involving p_n's for only a small number of consecutive n's, enabling a critical examination of…
Multipartite entanglement and nonclassicality of four-mode Gaussian states generated in two simultaneous nonlinear processes involving parametric down-conversion and frequency up-conversion are analyzed assuming the vacuum as the initial state. Suitable conditions for the generation of highly entangled states are found. Transfer of the entanglement from the down-converted modes into the up-converted ones is also suggested. The analysis of the whole set of states reveals that sub-shot-noise intensity correlations between the equally-populated down-converted modes, as well as the equally-populat…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
We experimentally examine the nonclassical character of a class of non-Gaussian states known as phase-diffused squeezed states. These states may show no squeezing effect at all, and therefore provide an interesting example to test nonclassicality criteria. The characteristic function of the Glauber-Sudarshan representation (P function) proves to be a powerful tool to detect nonclassicality. Using this criterion we find that phase-diffused squeezed states are always nonclassical, even if the squeezing effect vanishes. Testing other criteria of nonclassicality based on higher-order squeezing and…
Rotated quadratures carry the phase-dependent information of the electromagnetic field, so they are somehow conjugate to the photon number. We analyze this noncanonical pair, finding an exact uncertatinty relation, as well as a couple of weaker inequalities obtained by relaxing some restrictions of the problem. We also find the intelligent states saturating that relation and complete their characterization by considering extra constraints on the second-order moments of the variables involved. Using these moments, we construct performance measures tailored to diagnose photon-added and Schröding…
Nonclassicality in the sense of quantum optics is a prerequisite for entanglement in multi-mode radiation states. In this work we bring out the possibilities of passing from the former to the latter, via action of classicality preserving systems like beamsplitters, in a transparent manner. For single mode states, a complete description of nonclassicality is available via the classical theory of moments, as a set of necessary and sufficient conditions on the photon number distribution. We show that when the mode is coupled to an ancilla in any coherent state, and the system is then acted upon b…
In this work we generalize the Bochner criterion addressing the characteristic function, i.e., the Fourier transform, of the Glauber-Sudarshan phase-space function. For this purpose we extend the Bochner theorem by including derivatives of the characteristic function. The resulting necessary and sufficient nonclassicality criteria unify previously known moment-based criteria with those based on the characteristic function. For applications of the generalized nonclassicality probes, we provide direct sampling formulas for balanced homodyne detection. A squeezed vacuum state is experimentally re…
We address the pair of conjugated field modes obtained from parametric-downconversion as a convenient system to analyze the quantum-classical transition in the continuous variable regime. We explicitly evaluate intensity correlations, negativity and entanglement for the system in a thermal state and show that a hierarchy of nonclassicality thresholds naturally emerges in terms of thermal and downconversion photon number. We show that the transition from quantum to classical regime may be tuned by controlling the intensities of the seeds and detected by intensity measurements. Besides, we show …
In this paper, we follow our presented model in J. Opt. Soc. Am. B {\bf 30}, 1109--1117 (2013), in which the interaction between a $Λ$-type three-level atom and a quantized two-mode radiation field in a cavity in the presence of nonlinearities is studied. After giving a brief review on the procedure of obtaining the state vector of the atom-field system, some further interesting and important physical features (which are of particular interest in the quantum optics field of research) of the whole system state, i.e., the number-phase entropic uncertainty relation (based on the two-mode Pegg-Bar…
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode (or multiparty) bosonic fields that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials, but also polynomial functions of such moments, which can sometimes enable simpler derivations of phys…
Distinguishing quantum states that admit a classical counterpart from those that exhibit nonclassicality has long been a central issue in quantum optics. Finding an implementable criterion certifying optical nonclassicality (i.e, the incompatibility with a statistical mixture of coherent states) is of major importance as it often is a prerequisite to quantum information processes. A hierarchy of conditions for detecting whether a quantum state exhibits optical nonclassicality can be written based on some matrices of moments of the optical field [Phys. Rev. A 72, 043808 (2005)]. Here, we design…
We present Bell-type tests of nonclassicality and non-Gaussianity for single-mode fields employing a generalized quasiprobability function. Our nonclassicality tests are based on the observation that two orthogonal quadratures in phase space (position and momentum) behave as independent realistic variables for a coherent state. Taking four (three) points at the vertices of a rectangle (right triangle) in phase space, our tests detect every pure nonclassical Gaussian state and a range of mixed Gaussian states. These tests also set an upper bound for all Gaussian states and their mixtures, which…
Interference lies at the heart of the behavior of classical and quantum light. It is thus crucial to understand the boundaries between which interference patterns can be explained by a classical electromagnetic description of light and which, on the other hand, can only be understood with a proper quantum mechanical approach. While the case of two-mode interference has received a lot of attention, the multimode case has not yet been fully explored. Here we study a general scenario of intensity interferometry: we derive a bound on the average correlations between pairs of output intensities for…
We theoretically propose and experimentally demonstrate a nonclassicality test of single-mode field in phase space, which has an analogy with the nonlocality test proposed by Banaszek and Wodkiewicz [Phys. Rev. Lett. 82, 2009 (1999)]. Our approach to deriving the classical bound draws on the fact that the Wigner function of a coherent state is a product of two independent distributions as if the orthogonal quadratures (position and momentum) in phase space behave as local realistic variables. Our method detects every pure nonclassical Gaussian state, which can also be extended to mixed states.…
Practically applicable criteria for the nonclassicality of quantum states are formulated in terms of different types of moments. For this purpose the moments of the creation and annihilation operators, of two quadratures, and of a quadrature and the photon number operator turn out to be useful. It is shown that all the required moments can be determined by homodyne correlation measurements. An example of a nonclassical effect that is easily characterized by our methods is amplitude-squared squeezing.
In this paper, we study the interaction between a three-level atom and a quantized single-mode field with $` `$intensity-dependent coupling$"$ in a $` `$Kerr medium$"$. The three-level atom is considered to be in a $Λ$-type configuration. Under particular initial conditions, which may be prepared for the atom and the field, the dynamical state vector of the entire system will be explicitly obtained, for arbitrary nonlinearity function $f(n)$ associated to any physical system. Then, after evaluating the variation of the field entropy against time, we will investigate the quantum statistics as w…
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a g…
Using coherent states in optical quantum process tomography is a practically-relevant approach. Here, we develop a framework for complete characterization of quantum-optical processes in terms of normally-ordered moments by using coherent states as probes. We derive the associated superoperator tensors for several optical processes. We also show that our technique can be used to determine nonclassicality features of quantum-optical states and processes. Furthermore, we investigate identification of multi-mode Gaussian processes and show that the number of necessary probe coherent states scales…
We study the evolution of higher-order nonclassicality and entanglement criteria in atmospheric fluctuating-loss channels. By formulating input-output relations for the matrix of moments, we investigate the influence of such channels on the corresponding quantumness criteria. This generalization of our previous work on Gaussian entanglement [M. Bohmann et al., Phys. Rev. A 94, 010302(R) (2016)] not only exploits second-order-based scenarios, but it also provides a detailed investigation of nonclassicality and entanglement in non-Gaussian and multimode radiation fields undergoing a fluctuating …
Characterization of Generalized Coherent States through Intensity-Field Correlations
ANID - Millenium Science Iniciative Program - Millenium Institute for Research in Optics, Chile（智利国家研究与创新发展局-千年科学倡议计划-千年光学研究所）；Departamento de Física, Facultad de Ciencias Físicas y Matemáticas, Universidad de Chile, Santiago, Chile（智利大学物理与数学科学学院物理学系）；Departamento de Física, Facultad de Ciencias Físicas y Matemáticas, Universidad de Concepción, Concepción, Chile（康塞普西翁大学物理与数学科学学院物理学系）
We perform a phase-space analysis of strong-field enhanced ionisation in molecules, with emphasis on quantum-interference effects. Using Wigner quasi-probability distributions and the quantum Liouville equation, we show that the momentum gates reported in a previous publication [N. Takemoto and A. Becker, Phys. Rev. A \textbf{84}, 023401 (2011)] may occur for static driving fields, and even for no external field at all. Their primary cause is an interference-induced bridging mechanism that occurs if both wells in the molecule are populated. In the phase-space regions for which quantum bridges …
The interaction between two $Ξ$-type three-level atoms and a single-mode cavity field in the intensity dependent coupling regime has been studied. Exact analytical solution of the wave function for the considered atoms-field system has been obtained by using the Laplace transform technique when the atoms are initially prepared in the excited state and the field is in a coherent state. The presented structure has the potential ability to generate various new classes of entangled states depending on the chosen nonlinearity function. Two forms of intensity-dependent coupling as well as constant c…
Nonadiabtic dressed states and nonadiabatic induced dipole moment in the leading order of nonadiabaticity is proposed. The nonadiabatic induced dipole moment is studied in the femtosecond time domain.
In this paper, the interaction between a $Λ$-type three-level atom and two-mode cavity field is discussed. The detuning parameters and cross-Kerr nonlinearity are taken into account and it is assumed that atom-field coupling and Kerr medium to be $f$-deformed. Even though the system seems to be complicated, the analytical form of the state vector of the entire system for considered model is exactly obtained. The time evolution of nonclassical properties such as quantum entanglement and position-momentum entropic uncertainty relation (entropy squeezing) of the field are investigated. In each ca…
We exploit results on the classical Stieltjes moment problem to obtain completely explicit necessary and sufficient conditions for the photon number distribution p(n) of a radiation field mode to be classical. These conditions are given in two forms - respectively local and global in the individual photon number probabilities. Central to the first approach is the recognition of the important fact that the quantities n!p(n) are moments of a quasiprobability distribution, notwithstanding the fact that p(n)'s can by themselves be considered as a probability distribution over the nonnegative integ…
The measurement of the position-momentum EPR correlations of a two-photon state is important for many quantum information applications ranging from quantum key distribution to coincidence imaging. However, all the existing techniques for measuring the position-momentum EPR correlations involve coincidence detection and thus suffer from issues that result in less accurate measurements. In this letter, we propose and demonstrate an experimental scheme that does not require coincidence detection for measuring the EPR correlations. Our technique works for two-photon states that are pure, irrespect…
In this paper, we study the interaction between a moving $Λ$-type three-level atom and a single-mode cavity field in the presence of intensity-dependent atom-field coupling. After obtaining the state vector of the entire system explicitly, we study the nonclassical features of the system such as quantum entanglement, position-momentum entropic squeezing, quadrature squeezing and sub-Poissonian statistics. According to the obtained numerical results we illustrate that the squeezed period, the duration of entropy squeezing and the maximal squeezing can be controlled by choosing the appropriate n…
Criteria defining higher-order sub-Poissonian-like fields are given using five different quantities: moments of (I) integrated intensity, (II) photon number, (III) integrated-intensity fluctuation, (IV) photon-number fluctuation, and (V) elements of photocount and photon-number distributions. Relations among the moment criteria are revealed. Performance of the criteria is experimentally investigated using a set of potentially sub-Poissonian fields obtained by post-selection from a twin beam. The criteria based on moments of integrated intensity and photon number and those using the elements of…
Three different noise moments of field strength, intensity, and their correlations are simultaneously measured. For this purpose a homodyne cross-correlation measurement [W. Vogel, Phys. Rev. A 51, 4160 (1995)] is implemented by superimposing the signal field and a weak local oscillator on an unbalanced beam splitter. The relevant information is obtained via the intensity noise correlation of the output modes. Detection details like quantum efficiencies or uncorrelated dark noise are meaningless for our technique. Yet unknown insight in the quantumness of a squeezed signal field is retrieved f…
Identification, and subsequent quantification of quantum correlations, is critical for understanding, controlling, and engineering quantum devices and processes. We derive and implement a general method to quantify various forms of quantum correlations using solely the experimental intensity moments up to the fourth order. This is possible as these moments allow for an exact determination of the global and marginal impurities of two-beam Gaussian fields. This leads to the determination of steering, tight lower and upper bounds for the negativity, and the Kullback-Leibler divergence used as a q…
Generation of an ultra-bright, deterministic, solid-state single photon source with high photon collection rate is an imperative requirement for quantum technologies. In this direction, various nanophotonic systems coupled with single quantum emitters are being implemented, but results in low decay rate enhancement and MHz photon collection rate. Here, we unravel coherent superposition of excited Mie-scattering moments in a dipolar antenna, coupled with a single nitrogen-vacancy (NV-) center, to achieve bright single photon source with GHz collection rate. Such balancing of Mie-scattering mome…
