We experimentally examine the nonclassical character of a class of non-Gaussian states known as phase-diffused squeezed states. These states may show no squeezing effect at all, and therefore provide an interesting example to test nonclassicality criteria. The characteristic function of the Glauber-Sudarshan representation (P function) proves to be a powerful tool to detect nonclassicality. Using this criterion we find that phase-diffused squeezed states are always nonclassical, even if the squeezing effect vanishes. Testing other criteria of nonclassicality based on higher-order squeezing and the positive semidefinitness of special matrices of normally ordered moments, it is found that these criteria fail to reveal the nonclassicality for some of the prepared phase-diffused squeezed states.
Single photon sources are necessary for optical quantum technology. The nonclassicality of emitted single photons manifests itself in diverse experiments and applications. The applications already require different nonclassical aspects of single photons, however, a suitable hierarchy of criteria is missing. We propose variable experimental tests, based on adjustable linear optical networks and single photon detectors, giving a hierarchy of such nonclassicality criteria. The hierarchy goes beyond Hanbury - Brown - Twiss test of photon antibunching and allows us to compare faithfully quality and…
A method is introduced for the verification of nonclassicality in terms of moments of nonclassicality quasiprobability distributions. The latter are easily obtained from experimental data and will be denoted as nonclassicality moments. Their relation to normally-ordered moments is derived, which enables us to verify nonclassicality by using well established criteria. Alternatively, nonclassicality criteria are directly formulated in terms of nonclassicality moments. The latter converge in proper limits to the usually used criteria, as is illustrated for squeezing and sub-Poissonian photon stat…
In this work we generalize the Bochner criterion addressing the characteristic function, i.e., the Fourier transform, of the Glauber-Sudarshan phase-space function. For this purpose we extend the Bochner theorem by including derivatives of the characteristic function. The resulting necessary and sufficient nonclassicality criteria unify previously known moment-based criteria with those based on the characteristic function. For applications of the generalized nonclassicality probes, we provide direct sampling formulas for balanced homodyne detection. A squeezed vacuum state is experimentally re…
We use the exact calculation of the quantum mechanical, temporal characteristic function $χ(η)$ and the degree of second-order coherence $g^{(2)}(τ)$ for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state, to study the different criteria for nonclassicality. In particular, we contrast criteria that involve only one-time functions of the dynamical system, for instance, the quasiprobability distribution $P(β)$ of the Glauber-Sudarshan coherent or P-representation of the density of state and the Mandel $Q_{M}(τ)$ parameter, …
We devise a new class of criteria to certify the nonclassicality of photon- and phonon-number statistics. Our criteria extend and strengthen the broadly used Klyshko's criteria, which require knowledge of only a finite set of Fock-state probabilities. This makes the criteria well-suited to experimental implementation in realistic conditions. Moreover, we prove the completeness of our method in some scenarios, showing that, when only two or three Fock-state probabilities are known, it detects all finite distributions incompatible with classical states. In particular, we show that our criteria d…
Nonclassicality criteria based on intensity moments and derived from the usual matrix approach are compared to those provided by the majorization theory. The majorization theory is shown to give a greater number of more suitable nonclassicality criteria. Fifteen experimentally useful criteria of the majorization theory containing the intensity moments up to the fifth order are identified. Their performance is experimentally demonstrated on the set of eleven potentially nonclassical states generated from a twin beam by postselection based on detecting a given number of photocounts in one arm by…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
Driven by single photon detection requirements especially for quantum information sciences, the theory of arrays of off-on detectors has been well developed and applied. However for a comprehensive characterization of nonclassicality one also needs phase sensitive properties. This missing link is fulfilled by the theory of phase sensitive click counting measurements. This theory is presented. It unifies the balanced homodyne detection for high intensities with the click detection in the few photon regime. We formulate and apply a hierarchy of nonlinear squeezing conditions to probe quantum eff…
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode (or multiparty) bosonic fields that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials, but also polynomial functions of such moments, which can sometimes enable simpler derivations of phys…
Nonclassical properties of photon added and photon subtracted squeezed coherent states have been compared with specific focus on the higher order nonclassicalities, such as higher order squeezing, higher order sub-Poissonian photon statistics, higher order antibunching. It is observed that both photon added and photon subtracted squeezed coherent states are highly nonclassical as they satisfy criteria for all of the above mentioned nonclassicalities and a set of other criteria including negativity of Wigner function, Klyshko's criterion and Agarwal's $(A_{3})$ parameter. Further, the amount of…
Mode-entanglement based criteria and measures become insufficient for broadband emission, e.g. from spasers (plasmonic nano-lasers). We introduce criteria and measures for the (i) total entanglement of two wavepackets, (ii) entanglement of a wavepacket with an ensemble and (iii) total nonclassicality of a wavepacket~(WP). We discuss these criteria in the context of (i) entanglement of two WPs emitted from two initially entangled cavities (or two initially entangled atoms) and (ii) entanglement of an emitted WP with the ensemble/atom for the spontaneous emission and the single-photon superradia…
We study different representations of a many-particle system. We reveal the stunning beauty of the connections among the nonclassicalities of a many-particle, a single-mode and a two-mode systems. First, we demonstrate that (separable) atomic coherent states~(ACSs), of a many-particle system, mimic the coherent states of single-mode light. This enables the utilization of a many-particle entanglement~(MPE) criterion as a single-mode nonclassicality~(SMNc) condition via Holstein-Primakoff transformation. As an example, we show that spin-squeezing criterion, for MPE, can be transformed into the q…
We calculate exactly the quantum mechanical, temporal characteristic function $χ(η)$ for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state. Knowledge of $χ(η)$ allows only the determination of the time development of arbitrary functions of equal-time products of creation and annihilation photon operators. We calculate, in particular, the fluctuations in photon number, quadrature operators, and quadrature variance. We contrast the very important difference between the nonclassicality criteria based on the one-time charact…
In a recent paper [R. Alicki and N. Van Ryn, J. Phys. A: Math. Theor., 41, 062001 (2008)] a test of nonclassicality for a single qubit was proposed. Here, we discuss the class of local realistic theories to which this test applies and present an experimental realization.
Interference lies at the heart of the behavior of classical and quantum light. It is thus crucial to understand the boundaries between which interference patterns can be explained by a classical electromagnetic description of light and which, on the other hand, can only be understood with a proper quantum mechanical approach. While the case of two-mode interference has received a lot of attention, the multimode case has not yet been fully explored. Here we study a general scenario of intensity interferometry: we derive a bound on the average correlations between pairs of output intensities for…
We present a method for the experimental measurement of nonclassicality witnesses and demonstrate its application. Our proposal only requires the coherent displacement of the initial state, which can be achieved by overlapping the latter with a coherent state at a beam splitter, and subsequent photon-number resolved detection. This setup allows a complete test of nonclassicality of an arbitrary quantum state. The role of the quantum efficiency as well as statistical and systematic uncertainties are discussed. Finally, the scheme is demonstrated for a realistic example.
We introduce a kind of entangled state---photon-addition two-mode squeezed thermal state (TMSTS) by adding photons to each mode of the TMSTS. Using the P-representation of thermal state, the compact expression of the normalization factor is derived, a Jacobi polynomial. The nonclassicality is investigated by exploring especially the negativity of Wigner function. The entanglement is discussed by using Shchukin-Vogel criteria. It is shown that the photon-addtion to the TMSTS may be more effective for the entanglement enhancement than the photon-subtraction from the TMSTS. In addition, the quant…
Recently a test of nonclassicality for a single qubit was proposed [R. Alicki and N. Van Ryn, J. Phys. A: Math. Theor. 41, 062001 (2008)]. We present an optimized experimental realization of this test leading to a 46 standard deviation violation of classicality. This factor of 5 improvement over our previous result was achieved by moving from the infrared to the visible where we can take advantage of higher efficiency and lower noise photon detectors.
We theoretically introduce and experimentally demonstrate the realization of a nonclassicality test that allows for arbitrarily low detection efficiency without invoking any extra assumptions as independence of the devices. Our test and its implementation is set in a prepare-and-measure scenario with an upper limit on the communication capacity of the channel through which the systems are communicated. The essence for our novel test is the use of two preparation and two measurement devices, which are randomly paired in each round. Our work opens up the possibility of experimental realizations …
Contextuality is an indicator of non-classicality, and a resource for various quantum procedures. In this paper, we use contextuality to evaluate the variational quantum eigensolver (VQE), one of the most promising tools for near-term quantum simulation. We present an efficiently computable test to determine whether or not the objective function for a VQE procedure is contextual. We apply this test to evaluate the contextuality of experimental implementations of VQE, and determine that several, but not all, fail this test of quantumness.
We introduce an experimentally accessible method to measure a unique degree of nonclassicality, based on the quantum superposition principle, for arbitrary quantum states. We formulate witnesses and test a given state for any particular value of this measure. The construction of optimal tests is presented as well as the general numerical implementation. We apply this approach on examples such as squeezed states, and we show how to formulate conditions to certify a particular degree of nonclassicality for single- and multimode radiation fields.
Machine-learning and neural-network approaches have gained huge attention in the context of quantum science and technology in recent years. One of the most essential tasks for the future development of quantum technologies is the verification of nonclassical resources. Here, we present an artificial neural network approach for the identification of nonclassical states of light based on recorded measurement statistics. In particular, we implement and train a network which is capable of recognizing nonclassical states based on the click statistics recorded with multiplexed detectors. We use simu…
The efficient certification of nonclassical effects of light forms the basis for applications in optical quantum technologies. We derive general correlation conditions for the verification of nonclassical light based on multiplexed detection. The obtained nonclassicality criteria are valid for imperfectly-balanced multiplexing scenarios with on-off detectors and do not require any knowledge about the detector system. In this sense they are fully independent of the detector system. In our experiment, we study light emitted by clusters of single-photon emitters, whose photon number may exceed th…
We present Bell-type tests of nonclassicality and non-Gaussianity for single-mode fields employing a generalized quasiprobability function. Our nonclassicality tests are based on the observation that two orthogonal quadratures in phase space (position and momentum) behave as independent realistic variables for a coherent state. Taking four (three) points at the vertices of a rectangle (right triangle) in phase space, our tests detect every pure nonclassical Gaussian state and a range of mixed Gaussian states. These tests also set an upper bound for all Gaussian states and their mixtures, which…
We devise a method to certify nonclassical features via correlations of phase-space distributions by unifying the notions of quasiprobabilities and matrices of correlation functions. Our approach complements and extends recent results that were based on Chebyshev's inequality [Phys. Rev. Lett. 124, 133601 (2020)]. The method developed here correlates arbitrary phase-space functions at arbitrary points in phase space, including multimode scenarios and higher-order correlations. Furthermore, our approach provides necessary and sufficient nonclassicality criteria, applies to phase-space functions…
Random access codes are an intriguing class of communication tasks that reveal an operational and quantitative difference between classical and quantum information processing. We formulate a natural generalization of random access codes and call them random access tests, defined for any finite collection of measurements in an arbitrary finite dimensional general probabilistic theory. These tests can be used to examine collective properties of collections of measurements. We show that the violation of a classical bound in a random access test is a signature of either measurement incompatibility…
We examine whether metrological resolution beyond coherent states is a nonclassical effect. We show that this is true for linear detection schemes but false for nonlinear schemes, and propose a very simple experimental setup to test it. We find a nonclassicality criterion derived from quantum Fisher information.
In a recent paper [arXiv:1301.2887] Ahrens et al. claim that our "(...) experiment on qutrits does not test Klyachko et al.'s inequality, but an inequality with extra correlations" and that the "(...) experiment cannot be considered a proper test of a noncontextuality inequality, since the same observable is measured with different setups in different contexts". We disagree with these claims. In this note we briefly re-state how our test of the non-contextuality inequality was constructed. We explain how we keep the context of measurements when switching between different terms of the tested i…
We report two fundamental experiments on three-level quantum systems (qutrits). The first one tests the simplest task for which quantum mechanics provides an advantage with respect to classical physics. The quantum advantage is certified by the violation of Wright's inequality, the simplest classical inequality violated by quantum mechanics. In the second experiment, we obtain contextual correlations by sequentially measuring pairs of compatible observables on a qutrit, and show the violation of Klyachko et al.'s inequality, the most fundamental noncontextuality inequality violated by qutrits.…
Although nonclassical quantum states are important both conceptually and as a resource for quantum technology, it is often difficult to test whether a given quantum system displays nonclassicality. A simple method to certify nonclassicality is introduced, based on easily accessible collective atomic quadrature measurements, without the need of full state tomography. The statistics is analyzed beyond the ground-state noise level, by direct sampling of a regularized atomic quadrature quasiprobability. Nonclassicality of a squeezed ensemble of 2x10^5 Cesium atoms is demonstrated, with a significa…
We theoretically propose and experimentally demonstrate a nonclassicality test of single-mode field in phase space, which has an analogy with the nonlocality test proposed by Banaszek and Wodkiewicz [Phys. Rev. Lett. 82, 2009 (1999)]. Our approach to deriving the classical bound draws on the fact that the Wigner function of a coherent state is a product of two independent distributions as if the orthogonal quadratures (position and momentum) in phase space behave as local realistic variables. Our method detects every pure nonclassical Gaussian state, which can also be extended to mixed states.…
Various nonclassical and quantum phase properties of photon added then subtracted displaced Fock state have been examined systematically and rigorously. Higher-order moments of the relevant bosonic operators are computed to test the nonclassicality of the state of interest, which reduces to various quantum states (having applications in quantum optics, metrology and information processing) in different limits ranging from the coherent (classical) state to the Fock (most nonclassical) states. The nonclassical features are discussed using Klyshko's, Vogel's, and Agarwal-Tara's criteria as well a…
While negativity in phase space is a well-known signature of nonclassicality, a wide variety of nonclassical states require their characterization beyond negativity. We establish a framework of nonclassicality in phase space that addresses nonclassical states comprehensively with a direct experimental evidence. This includes the negativity of phase-space distribution as a special case and further analyzes quantum states with positive distributions effectively. We prove that it detects all nonclassical Gaussian states and all non-Gaussian states of arbitrary dimension remarkably by examining th…
We study the evolution of higher-order nonclassicality and entanglement criteria in atmospheric fluctuating-loss channels. By formulating input-output relations for the matrix of moments, we investigate the influence of such channels on the corresponding quantumness criteria. This generalization of our previous work on Gaussian entanglement [M. Bohmann et al., Phys. Rev. A 94, 010302(R) (2016)] not only exploits second-order-based scenarios, but it also provides a detailed investigation of nonclassicality and entanglement in non-Gaussian and multimode radiation fields undergoing a fluctuating …
We derive simple practical procedures revealing the quantum behavior of angular momentum variables by the violation of classical upper bounds on the statistics. Data analysis is minimum and definite conclusions are obtained without evaluation of moments, or any other more sophisticated procedures. These nonclassical tests are very general and independent of other typical quantum signatures of nonclassical behavior such as sub-Poissonian statistics, squeezing, or oscillatory statistics, being insensitive to the nonclassical behavior displayed by other variables.
We derive a family of inequalities involving different phase-space distributions of a quantum state which have to be fulfilled by any classical state. The violation of these inequalities is a clear signature of nonclassicality. Our approach combines the characterization of nonclassical effects via negativities in phase-space distributions with inequality conditions usually being formulated for moments of physical observables. Importantly, the obtained criteria certify nonclassicality even when the involved phase-space distributions are non-negative. Moreover, we show how these inequalities are…
Although squeezed states are nonclassical states, so far, their nonclassicality could not be demonstrated by negative quasiprobabilities. In this work we derive pattern functions for the direct experimental determination of so-called nonclassicality quasiprobabilities. The negativities of these quantities turn out to be necessary and sufficient for the nonclassicality of an arbitrary quantum state and are therefore suitable for a direct and general test of nonclassicality. We apply the method to a squeezed vacuum state of light that was generated by parametric down-conversion in a second-order…
We develop a nonclassicality criterion for the interference of three delayed, but otherwise identical, light fields in a three-mode Bell interferometer. We do so by comparing the prediction of quantum mechanics with those of a classical framework in which independent sources emit electric fields with random phases. In particular, we evaluate third-order correlations among output intensities as a function of the delays, and show how the presence of a correlation revival for small delays cannot be explained by the classical model of light. The observation of a revival is thus a nonclassicality s…
In a recent contribution, we introduced and applied a detector-independent method to uncover nonclassicality. Here, we extend those techniques and give more details on the performed analysis. We derive a general theory of the positive-operator-valued measure that describes multiplexing layouts with arbitrary detectors. From the resulting quantum version of a multinomial statistics, we infer nonclassicality probes based on a matrix of normally ordered moments. We discuss these criteria and apply the theory to our data which are measured with superconducting transition-edge sensors. Our experime…
We propose a legitimate and easily computable nonclassicality indicator for the states of electromagnetic fields based on the standard deviation in the measurement of the homodyne rotated quadrature operator. The proposed nonclassicality indicator is the nonclassical area projected by the optical tomogram of the quantum state of light on the optical tomographic plane. If the nonclassical area projected by the optical tomogram of a quantum state is greater than zero, the state is nonclassical, and the area is zero for the pure classical state. It is also noted that the nonclassical area of a qu…
We propose to experimentally test the nonclassicality of quantum states through homodyne tomography. For single-mode states we check violations of inequalities involving the photon-number probability. For two-mode states we test the nonclassicality by reconstructing some suitable number-operator functions. The test can be performed with available quantum efficiency of homodyne detection, by measuring the pertaining quantities on the corresponding noisy states.
The effect of two quantum state engineering processes that can be used to burn hole at vacuum in the photon number distribution of quantum states of radiation field are compared using various witnesses of lower- and higher-order nonclassicality as well as a measure of nonclassicality. Specifically, the witnesses of nonclassical properties due to the effect of vacuum state filtration and a single photon addition on an even coherent state, binomial state and Kerr state are investigated using the criteria of lower- and higher-order antibunching, squeezing and sub-Poissonian photon statistics. Fur…
A standard method to obtain information on a quantum state is to measure marginal distributions along many different axes in phase space, which forms a basis of quantum state tomography. We theoretically propose and experimentally demonstrate a general framework to manifest nonclassicality by observing a single marginal distribution only, which provides a novel insight into nonclassicality and a practical applicability to various quantum systems. Our approach maps the 1-dim marginal distribution into a factorized 2-dim distribution by multiplying the measured distribution or the vacuum-state d…
Maximizing Nonclassicality of Massive Objects via Quantum Zeno Effect
Shiv Nadar Institution of Eminence（希夫纳达尔卓越学院）；S. N. Bose National Centre for Basic Sciences（S.N. 玻色基础科学国家中心）；Faculty of Mathematics and Physics, University of Ljubljana（卢布尔雅那大学数学与物理学院）；School of Physics and Astronomy, University of Southampton（南安普顿大学物理与天文学院）；Raman Research Institute (RRI)（拉曼研究所）；Bose Institute（玻色研究所）；Department of Physics and Astronomy, University College London（伦敦大学学院物理与天文学系）
Practically applicable criteria for the nonclassicality of quantum states are formulated in terms of different types of moments. For this purpose the moments of the creation and annihilation operators, of two quadratures, and of a quadrature and the photon number operator turn out to be useful. It is shown that all the required moments can be determined by homodyne correlation measurements. An example of a nonclassical effect that is easily characterized by our methods is amplitude-squared squeezing.
Quantum features of correlated optical modes define a major aspect of the nonclassicality in quantized radiation fields. However, the phase-sensitive detection of a two-mode light field is restricted to interferometric setups and local intensity measurements. Even the full reconstruction of the quantum state of a single radiation mode relies on such detection layouts and the preparation of a well-defined reference light field. In this work, we establish the notion of the essential quantum correlations of two-mode light fields. It refers to those quantum correlations which are measurable by a g…
In the recent experimental and theoretical literature well-established nonclassicality criteria from the field of quantum optics have been directly applied to the case of excitations in matter-waves. Among these are violations of Cauchy-Schwarz inequalities, Glauber-Sudarshan P-nonclassicality, sub-Poissonian number-difference squeezing (also known as the two-mode variance) and the criterion of nonseparability. We review the strong connection of these criteria and their meaning in quantum optics, and point out differences in the interpretation between light and matter waves. We then calculate …
We show that one single experiment can test simultaneously and independently both the nonclassicality of states and measurements by the violation or fulfillment of classical bounds on the statistics. Nonideal measurements affected by imperfections can be characterized by two bounds depending on whether we test the ideal measurement or the real one.
The interplay between the nonclassical features and the parity-time (PT) symmetry (or its breaking) is studied here by considering a PT symmetric system consisting of two cavities with gain and loss. The conditions for PT invariance is obtained for this system. The behavior of the average photon number corresponding to the gain and loss modes for different initial states (e.g., vacuum, NOON, coherent, and thermal states) has also been obtained. With the help of the number operators, quantum Zeno and anti-Zeno effects are studied, and the observed behavior is compared in PT symmetric (PTS) and …
Negative probability values have been widely employed as an indicator of the nonclassicality of quantum systems. Known as a quasiprobability distribution, they are regarded as a useful tool that provides significant insight into the underlying fundamentals of quantum theory when compared to the classical statistics. However, in this approach, an operational interpretation of these negative values with respect to the definition of probability---the relative frequency of occurred event---is missing. An alternative approach is therefore considered where the quasiprobability operationally reveals …
