We exploit results from the classical Stieltjes moment problem to bring out the totality of all the information regarding phase insensitive nonclassicality of a state as captured by the photon number distribution p_n. Central to our approach is the realization that n !p_n constitutes the sequence of moments of a (quasi) probability distribution, notwithstanding the fact that p_n can by itself be regarded as a probability distribution. This leads to classicality restrictions on p_n that are local in n involving p_n's for only a small number of consecutive n's, enabling a critical examination of the conjecture that oscillation in p_n is a signature of nonclassicality.
Single photon sources are necessary for optical quantum technology. The nonclassicality of emitted single photons manifests itself in diverse experiments and applications. The applications already require different nonclassical aspects of single photons, however, a suitable hierarchy of criteria is missing. We propose variable experimental tests, based on adjustable linear optical networks and single photon detectors, giving a hierarchy of such nonclassicality criteria. The hierarchy goes beyond Hanbury - Brown - Twiss test of photon antibunching and allows us to compare faithfully quality and…
We report the experimental reconstruction of a nonclassicality quasiprobability for a single-photon added thermal state. This quantity has significant negativities, which is necessary and sufficient for the nonclassicality of the quantum state. Our method presents several advantages compared to the reconstruction of the P function, since the nonclassicality filters used in this case can regularize the quasiprobabilities as well as their statistical uncertainties. A-priori assumptions about the quantum state are therefore not necessary. We also demonstrate that, in principle, our method is not …
Nonclassical properties of photon added and photon subtracted squeezed coherent states have been compared with specific focus on the higher order nonclassicalities, such as higher order squeezing, higher order sub-Poissonian photon statistics, higher order antibunching. It is observed that both photon added and photon subtracted squeezed coherent states are highly nonclassical as they satisfy criteria for all of the above mentioned nonclassicalities and a set of other criteria including negativity of Wigner function, Klyshko's criterion and Agarwal's $(A_{3})$ parameter. Further, the amount of…
The effects of von Neumann postselected measurement on nonclassicality of single-photon-added coherent state (SPACS) are studied. Explicit expressions and analytical results for various field properties of SPACS such as the photon number distribution, the Mandel Q_{m} factor and the squeezing parameter of field quadrature after postselected von Neumann measurement are investigated. The results showed that the nonclassicality of SPACS after measurement changed dramatically than initial state. The measurement let SPACS possess more strong sub-Poissonian photon statistics in some definite couplin…
We present a method for the experimental measurement of nonclassicality witnesses and demonstrate its application. Our proposal only requires the coherent displacement of the initial state, which can be achieved by overlapping the latter with a coherent state at a beam splitter, and subsequent photon-number resolved detection. This setup allows a complete test of nonclassicality of an arbitrary quantum state. The role of the quantum efficiency as well as statistical and systematic uncertainties are discussed. Finally, the scheme is demonstrated for a realistic example.
Theoretical analysis is given of nonclassicality and decoherence of the field states generated by adding any number of photons to the squeezed thermal state (STS). Based on the fact that the squeezed number state can be considered as a single-variable Hermite polynomial excited state, the compact expression of the normalization factor is derived, a Legendre polynomial. The nonclassicality is investigated by exploring the sub-Poissonian and negative Wigner function (WF). The results show that the WF of single photon-added STS (PASTS) always has negative values at the phase space center. The dec…
We investigate the nonclassicality of photon-added coherent states in the photon loss channel by exploring the entanglement potential and negative Wigner distribution. The total negative probability defined by the absolute value of the integral of the Wigner function over the negative distribution region reduces with the increase of decay time. The total negative probability and the entanglement potential of pure photon-added coherent states exhibit the similar dependence on the beam intensity. The reduce of the total negative probability is consistent with the behavior of entanglement potenti…
We introduce a kind of entangled state---photon-addition two-mode squeezed thermal state (TMSTS) by adding photons to each mode of the TMSTS. Using the P-representation of thermal state, the compact expression of the normalization factor is derived, a Jacobi polynomial. The nonclassicality is investigated by exploring especially the negativity of Wigner function. The entanglement is discussed by using Shchukin-Vogel criteria. It is shown that the photon-addtion to the TMSTS may be more effective for the entanglement enhancement than the photon-subtraction from the TMSTS. In addition, the quant…
Non-Gaussianity inducing operations are studied in the recent past from different perspectives. Here, we study the role of photon addition, a non-Gaussianity inducing operation, in the enhancement of nonclassicality in a finite dimensional quantum state, namely hypergeometric state with the help of some quantifiers and measures of nonclassicality. We observed that measures to characterize the quality of single photon source and anticlassicality lead to the similar conclusion, i.e., to obtain the desired quantum features one has to choose all the state parameters such that average photon number…
Recently, a non-Gaussian field, which may be a useful basis for entanglement distillation and efficient quantum teleportation, has been experimentally produced by subtracting a photon from a squeezed Gaussian field. We investigate the nonclassicality of such the field using negativity in the Wigner function and the existence of positive well-defined $P$ function. We obtain the condition to see negativity in the Wigner function for the case including the mixed Gaussian incoming field, the threshold photodetection and the inefficient homodyne measurement. We show how similar the photon-subtracte…
We examine nonclassical properties of the field states generated by applying the photon annihilation-then-creation operation (AC) and creation-then-annihilation operation (CA) to the thermal and coherent states. Effects of repeated applications of AC and of CA are also studied. We also discuss experimental schemes to realize AC and CA with a cavity system using atom-field interactions.
Detector stochastic deviations from an ideal response can hamper the measurement of quantum properties of light especially in the mesoscopic regime where photon-number resolution is required. We demonstrate that, by a proper analysis of the output signal, nonclassicality of twin-beam states can be detected and exploited with commercial and cost effective silicon-based photon-number-resolving detectors.
In this work we experimentally demonstrate for the first time a recently proposed criterion adressed to detect nonclassical behavior in the fluorescence emission of ensembles of single-photon emitters. In particular, we apply the method to study clusters of NV centres in diamond observed via single-photon-sensitive confocal microscopy. Theoretical considerations on the behavior of the parameter at any arbitrary order in presence of poissonian noise are presented and, finally, the opportunity of detecting manifold coincidences is discussed.
Higher-order nonclassical properties of r photon added and t photon subtracted qudit states (referred to as rPAQS and tPSQS, respectively) are investigated here to answer: How addition and subtraction of photon can be used engineer higher-order nonclassical properties of qudit states? To obtain the answer higher-order moment of relevant bosonic field operators are first obtained for rPAQS and tPSQS, and subsequently the same is used to study the higher-order nonclassical properties of the corresponding states. A few witnesses of higher-order nonclassicality (e.g. Higher-Order Antibunching, Hig…
We study the nonclassicality of photon-added squeezed vacuum (PASV) and its decoherence in thermal environment in terms of the sub-Poissonian statistics and the negativity of Wigner function (WF). By converting the PASV to a squeezed Hermite polynomial excitation state, we derive a compact expression for the normalization factor of m-PASV, which is an m-order Legendre polynomial of squeezing parameter r. We also derive the explicit expression of WF of m-PASV and find the negative region of WF in phase space. We show that there is an upper bound value of r for this state to exhibit sub-Poissoni…
Rotated quadratures carry the phase-dependent information of the electromagnetic field, so they are somehow conjugate to the photon number. We analyze this noncanonical pair, finding an exact uncertatinty relation, as well as a couple of weaker inequalities obtained by relaxing some restrictions of the problem. We also find the intelligent states saturating that relation and complete their characterization by considering extra constraints on the second-order moments of the variables involved. Using these moments, we construct performance measures tailored to diagnose photon-added and Schröding…
We report the experimental realization and tomographic analysis of novel quantum light states obtained by exciting a classical thermal field by a single photon. Such states, although completely incoherent, possess a tunable degree of quantumness which is here exploited to put to a stringent experimental test some of the criteria proposed for the proof and the measurement of state non-classicality. The quantum character of the states is also given in quantum information terms by evaluating the amount of entanglement that they can produce.
We discuss nonclassical properties of single-photon subtracted squeezed vacuum states in terms of the sub-Poissonian statistics and the negativity of the Wigner function. We derive a compact expression for the Wigner function from which we find the region of phase space where Wigner function is negative. We find an upper bound on the squeezing parameter for the state to exhibit sub-Poissonian statistics. We then study the effect of decoherence on the single-photon subtracted squeezed states. We present results for two different models of decoherence, viz. amplitude decay model and the phase di…
Numerous inequalities involving moments of integrated intensities and revealing nonclassicality and entanglement in bipartite optical fields are derived using the majorization theory, non-negative polynomials, the matrix approach, as well as the Cauchy-Schwarz inequality. Different approaches for deriving these inequalities are compared. Using the experimental photocount histogram generated by a weak noisy twin beam monitored by a photon-number-resolving iCCD camera the performance of the derived inequalities is compared. A basic set of ten inequalities suitable for monitoring the entanglement…
We consider a way to generate operational inequalities to test nonclassicality (or quantumness) of multimode (or multiparty) bosonic fields that unifies the derivation of many known inequalities and allows to propose new ones. The nonclassicality criteria are based on Vogel's criterion corresponding to analyzing the positivity of multimode P functions or, equivalently, the positivity of matrices of expectation values of, e.g., creation and annihilation operators. We analyze not only monomials, but also polynomial functions of such moments, which can sometimes enable simpler derivations of phys…
The concept of photon added two-mode Schrödinger cat states in which both modes are independent is introduced, their non-classical properties and entanglement are studied. The introduced states emerge as the eigenstates of $f_1f_2a_1a_2$, where $f_1, f_2$ are nonlinear functions of the number operator and $a_1, a_2$ are annihilation operators. We study the evolution of these states under the canonical transformation using the parity operator for the case of standard coherent states of the harmonic oscillator. The non-classical properties of these states are evaluated especially by considering …
Non-Gaussian and nonclassical states and processes are already found to be important resources for performing various tasks related to quantum gravity and quantum information processing. The effect of non-Gaussianity inducing operators on the nonclassicality of quantum states has also been studied rigorously. Considering these facts, a quantitative analysis of the nonclassical and non-Gaussian features is performed here for photon added displaced Fock state, as a test case, using a set of measures like entanglement potential, Wigner Yanese skew information, Wigner logarithmic negativity and re…
We study the nonclassicality of the evolution of a superposition of an arbitrary number of photon-added squeezed coherent Schrödinger cat states in a nonlinear Kerr medium. The nonlinearity of the medium gives rise to the periodicities of the quantities such as the Wehrl entropy $S_{Q}$ and the negativity $δ_{W}$ of the $W$-distribution, and a series of local minima of these quantities arise at the rational submultiples of the said period. At these local minima the evolving state coincides with the transient Yurke-Stoler type of photon-added squeezed kitten states, which, for the choice of the…
A method is introduced for the verification of nonclassicality in terms of moments of nonclassicality quasiprobability distributions. The latter are easily obtained from experimental data and will be denoted as nonclassicality moments. Their relation to normally-ordered moments is derived, which enables us to verify nonclassicality by using well established criteria. Alternatively, nonclassicality criteria are directly formulated in terms of nonclassicality moments. The latter converge in proper limits to the usually used criteria, as is illustrated for squeezing and sub-Poissonian photon stat…
{\small We investigate nonclassical properties of the field states generated by subtracting any number photon from the squeezed thermal state (STS). It is found that the normalization factor of photon-subtracted STS (PSSTS) is a Legendre polynomial of squeezing parameter }${\small r}${\small \ and average photon number }$\bar{n}$ {\small of thermal state. Expressions of several quasi-probability distributions of PSSTS are derived analytically. Furthermore, the nonclassicality is discussed in terms of the negativity of Wigner function (WF). It is shown that the WF of single PSSTS always has neg…
Bell nonclassicality of a single photon superposition in two modes, often referred to as `nonlocality of a single photon', is one of the most striking nonclassical phenomena discussed in the context of foundations of quantum physics. Here we show how to robustly violate local realism within the weak-field homodyne measurement scheme for \textit{any} superposition of one photon with vacuum. Our modification of the previously proposed setups involves tunable beamsplitters at the measurement stations, and the local oscillator fields significantly varying between the settings, optimally being {\it…
We present a study of the electromagnetic control of nonclassicality of the outgoing light field in a single atom cavity QED system. By exploring the energy eigenvalues and eigenstates, we show that the eigenstates are similar to the Jaynes-Cummings ladder of eigenstates and can be optically controlled by an external control field. Tuning the control field frequency to the one photon resonance, we show the superbunching behavior in the outgoing light field can be observed at the frequency of one photon resonance. We also show that there exists a magic control field intensity at which two photo…
A perturbative analytic operator solution of a completely quantum mechanical Hamiltonian of multi-photon pump non-degenerate hyper-Raman process is obtained. It is shown that the obtained solution is general in nature as the solutions of non-degenerate hyper-Raman and stimulated Raman processes can be obtained as special cases of the present solution. The analytic solutions obtained here are used to investigate the nonclassical properties of the different modes in the stimulated, spontaneous and partially spontaneous multi-photon pump non-degenerate hyper-Raman processes. The nonclassical natu…
The nonclassicality of photon-added coherent fields in the thermal channel is investigated by exploring the volume of the negative part of the Wigner function which reduces with the dissipative time. The Wigner functions become positive when the decay time exceeds a threshold value. For the case of the single photon-added coherent state, we derive the exact threshold values of decay time in the thermal channel. For arbitrary partial negative Wigner distribution function, a generic analytical relation between the mean photon number of heat bath and the threshold value of decay time is presented…
We calculate exactly the quantum mechanical, temporal characteristic function $χ(η)$ for a single-mode, degenerate parametric amplifier for a system in the Gaussian state, viz., a displaced-squeezed thermal state. Knowledge of $χ(η)$ allows only the determination of the time development of arbitrary functions of equal-time products of creation and annihilation photon operators. We calculate, in particular, the fluctuations in photon number, quadrature operators, and quadrature variance. We contrast the very important difference between the nonclassicality criteria based on the one-time charact…
We propose a definition of nonclassicality for a single-mode quantum-optical process based on its action on coherent states. If a quantum process transforms a coherent state to a nonclassical state, it is verified to be nonclassical. To identify nonclassical processes, we introduce a representation for quantum processes, called the process-nonclassicality quasiprobability distribution, whose negativities indicate nonclassicality of the process. Using this distribution, we derive a relation for predicting nonclassicality of the output states for a given input state. We experimentally demonstrat…
Systems of on-off detectors are well established for measuring radiation fields in the regime of small photon numbers. We propose to combine these detector systems with unbalanced homodyning with a weak local oscillator. This approach yields phase-space functions, which represent the click counterpart of the s parametrized quasiprobabilities of standard photoelectric detection theory. This introduced class of distributions can be directly sampled from the measured click counting statistics. Therefore, our technique visualizes nonclassical effects without further data processing. Surprisingly, …
We devise a new class of criteria to certify the nonclassicality of photon- and phonon-number statistics. Our criteria extend and strengthen the broadly used Klyshko's criteria, which require knowledge of only a finite set of Fock-state probabilities. This makes the criteria well-suited to experimental implementation in realistic conditions. Moreover, we prove the completeness of our method in some scenarios, showing that, when only two or three Fock-state probabilities are known, it detects all finite distributions incompatible with classical states. In particular, we show that our criteria d…
We construct a generalized version of the photon-subtracted squeezed vacuum states (PSSVS), which can be utilized to construct the same for nonlinear, deformed and any usual quantum mechanical models beyond the harmonic oscillator. We apply our general framework to trigonometric Pöschl-Teller potential and show that our method works accurately and produces a proper nonclassical state. We analyze the nonclassicality of the state using three different approaches, namely, quadrature squeezing, photon number squeezing and Wigner function and indicate how the standard definitions of those three tec…
A generalized notion of higher order nonclassicality (in terms of higher order moments) is introduced. Under this generalized framework of higher order nonclassicality, conditions of higher order squeezing and higher order subpoissonian photon statistics are derived. A simpler form of the Hong-Mandel higher order squeezing criterion is derived under this framework by using an operator ordering theorem introduced by us in [J. Phys. A. 33 (2000) 5607]. It is also generalized for multi-photon Bose operators of Brandt and Greenberg. Similarly, condition for higher order subpoissonian photon statis…
The nonclassicality of single photon-added thermal states in the thermal channel is investigated by exploring the volume of the negative part of the Wigner function. The Wigner functions become positive when the decay time exceeds a threshold value $γ{t}_c$, which only depends on the effective temperature or mean thermal photon number of the thermal channel, but not depends on the effective temperature of the initial thermal state. This phenomenon is similar with the case of single quantum excitation of classical coherent states in thermal channel. Furthermore, we firstly demonstrate $γ{t}_c$ …
Nonclassical properties of photon added and subtracted displaced Fock states have been studied using various witnesses of lower- and higher-order nonclassicality. Compact analytic expressions are obtained for the nonclassicality witnesses. Using those expressions, it is established that these states and the states that can be obtained as their limiting cases (except coherent states) are highly nonclassical as they show the existence of lower- and higher-order antibunching and sub-Poissonian photon statistics, in addition to the nonclassical features revealed through the Mandel $Q_M$ parameter,…
Superradiance, i.e., spontaneous emission of coherent radiation by an ensemble of identical two-level atoms in collective states introduced by Dicke in 1954, is one of the enigmatic problems of quantum optics. The startling gist is that even though the atoms have no dipole moment they radiate with increased intensity in particular directions. Following the advances in our understanding of superradiant emission by atoms in entangled $W$ states we examine the quantum statistical properties of superradiance. Such investigations require the system to have at least two excitations as one needs to e…
We introduce a new quantity for describing nonclassicality of an arbitrary optical two-mode Gaussian state which remains invariant under any global photon-number preserving unitary transformation of the covariance matrix of the state. The invariant naturally splits into an entanglement monotone and local nonclassicality quantifiers applied to the reduced states. This shows how entanglement can be converted into local squeezing and vice versa. Twin beams and their transformations at a beam splitter are analyzed as an example providing squeezed light. An extension of this approach to pure three-…
The effect of two quantum state engineering processes that can be used to burn hole at vacuum in the photon number distribution of quantum states of radiation field are compared using various witnesses of lower- and higher-order nonclassicality as well as a measure of nonclassicality. Specifically, the witnesses of nonclassical properties due to the effect of vacuum state filtration and a single photon addition on an even coherent state, binomial state and Kerr state are investigated using the criteria of lower- and higher-order antibunching, squeezing and sub-Poissonian photon statistics. Fur…
We argue that the essence of nonclassicality of a bipartite correlation is a positive signal deficit-- the communication cost excess over the available signaling. By this criterion, while violations of Bell-type and contextuality inequalities are necessarily non-classical, some violations of the Leggett-Garg inequality are classical. Further, signaling tends to diminish nonclassical properties, such as intrinsic randomness, no-cloning, complementarity, etc. Signal deficit is shown to have its ultimate origin in intrinsic randomness. A possible analogy of nonclassicality to the metamathematical…
Driven by single photon detection requirements especially for quantum information sciences, the theory of arrays of off-on detectors has been well developed and applied. However for a comprehensive characterization of nonclassicality one also needs phase sensitive properties. This missing link is fulfilled by the theory of phase sensitive click counting measurements. This theory is presented. It unifies the balanced homodyne detection for high intensities with the click detection in the few photon regime. We formulate and apply a hierarchy of nonlinear squeezing conditions to probe quantum eff…
Two twin beams with a shared signal beam and separated idler beams are used together with the photon-number-resolving postselection in the signal beam to arrive at two coupled beams with anticorrelations in photon-number fluctuations. Moreover, the beams exhibit the sub-Poissonian photon-number statistics in their marginal distributions under suitable conditions. The postselected fields with the increasing mean photon numbers are reconstructed from the experimental photocount histograms by the maximum likelihood approach. Also a suitable Gaussian fit of both original twin beams and simulation …
A bipartite state is classical with respect to party $A$ if and only if party $A$ can perform nondisruptive local state identification (NDLID) by a projective measurement. Motivated by this we introduce a class of quantum correlation measures for an arbitrary bipartite state. The measures utilize the general Schatten $p$-norm to quantify the amount of departure from the necessary and sufficient condition of classicality of correlations provided by the concept of NDLID. We show that for the case of Hilbert-Schmidt norm, i.e. $p=2$, a closed formula is available for an arbitrary bipartite state.…
Multipartite Bell-GHZ nonclassicality from interwoven frustrated down-conversion
International Centre for Theory of Quantum Technologies, University of Gdansk（格但斯克大学国际量子技术理论中心）；Centre for Quantum Technologies, National University of Singapore（新加坡国立大学量子技术中心）；Institute of Theoretical Physics and Astrophysics, University of Gdańsk（格但斯克大学理论与天体物理研究所）；Faculty of Physics, Ludwig Maximilian University（路德维希-马克西米利安大学物理学院）；Institute of Theoretical and Applied Informatics, Polish Academy of Sciences（波兰科学院理论与应用信息学研究所）
We reconsider the all-optical homodyne-measurement based experimental schemes that aim to reveal Bell nonclassicality of a single photon, often termed `nonlocality'. We focus on the schemes put forward by Tan, Walls and Collett (TWC, 1991) and Hardy (1994). In the light of our previous work the Tan, Walls and Collett setup can be described by a precise local hidden variable model, hence the claimed nonclassicality of this proposal is apparent, whereas the nonclassicality proof proposed by Hardy is impeccable. In this work we resolve the following problem: which feature of the Hardy's approach …
